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In-situ formation of nitrogen doped microporous carbon nanospheres derived from polystyrene as lubricant additives for anti-wear and friction reduction

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Friction 2024年第3期12卷 439-451页

作者： Yixin WANG qi lu Huijie XIE Shujuan LIU qian YE Feng ZHOU Weimin LIU State Key Laboratory of Solidification Processing Center of Advanced Lubrication and Seal MaterialsSchool of Materials Science and EngineeringNorthwestern Polytechnical UniversityXi'an 710072China State Key Laboratory of Solid lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

This study presents a nitrogen-doped microporous carbon nanospheres(N@MCNs)prepared by a facile polymerization–carbonization process using low-cost *** N element in situ introduces polystyrene(PS)nanospheres via emulsion polymerization of styrene with cyanuric chloride as crosslinking agent,and then carbonization obtains N@*** as-prepared carbon nanospheres possess the complete spherical structure and adjustable nitrogen amount by controlling the relative proportion of tetrachloromethane and cyanuric *** friction performance of N@MCNs as lubricating oil additives was surveyed utilizing the friction experiment of ball-disc *** results showed that N@MCNs exhibit superb reduction performance of friction and *** the addition of N@MCNs was 0.06 wt%,the friction coefficient of PAO-10 decreased from 0.188 to 0.105,and the wear volume reduced by 94.4%.The width and depth of wear marks of N@MCNs decreased by 49.2% and 94.5%,*** carrying capacity of load was rocketed from 100 to 400 N *** the analysis of the lubrication mechanism,the result manifested that the prepared N@MCNs enter clearance of the friction pair,transform the sliding friction into the mixed friction of sliding and rolling,and repair the contact surface through the repair ***,the tribochemical reaction between nanoparticles and friction pairs forms a protective film containing nitride and metal oxides,which can avert direct contact with the matrix and improve the tribological *** experiment showed that nitrogen-doped polystyrene-based carbon nanospheres prepared by in-situ doping are the promising materials for wear resistance and reducing *** preparing method can be ulteriorly expanded to multi-element co-permeable *** and boron co-doped carbon nanospheres(B,N@MCNs)were prepared by mixed carbonization of N-enriched PS and boric acid,and exhibited high load carrying capacity and good tribolog

关键词： lubricant additives hypercrosslinked polystyrene carbon nanospheres friction reduction anti-wear

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Volatile compounds,synergistic effects,precursors and impact factors for odor profiles in Eriocheir sinensis

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Aquaculture and Fisheries 2024年第5期9卷 721-730页

作者： qi lu Lizhi Yu Xueqian Guo Xichang Wang College of Food Science and Technology Shanghai Ocean UniversityShanghai201306China Shanghai Engineering Research Center of Aquaculture Shanghai Ocean UniversityShanghai201306China Shanghai Engineering Research Center of Aquatic-Product Processing and Preservation Shanghai201306China

Flavor,especially odor,is one of the most concerning food qualities for producers and *** odor of *** is a vital quality indicator and highly variable in species,diets,regions and harvest *** differences could diminish consumer acceptance and reduce the economic returns to the *** now,168 volatile compounds have been identified in ***,of which 42 are shared to five edible parts,and the hepatopancreas has 22 specific *** 30 aroma-active compounds may interact to form odor *** compounds are mainly derived from Phosphatidylethanolamine(PE)and free fatty acids(FFA)by a series of biochemical reactions such as thermal degradation,secondary degradation,molecular rearrangement,and Maillard *** odor of crab has a close relationship with *** harvested,the crab also produces odors during processing and storage,which could be controlled by *** work provides information that could support the development of innovative aquaculture strategies to satisfy the needs of the consumer market.

关键词： Volatiles Precursors Impact factors Eriocheir sinensis

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The size effect and analogous boundary states in a circular non-Hermitian chain

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Communications in Theoretical Physics 2024年第2期76卷 157-165页

作者： Xin-Yu Ma Yi-Han Guan qiao-Nan Li Ai-Lei He lu qi School of Physical Science and Technology Yangzhou UniversityYangzhou 225002China

We investigate the size effect and boundary states based on a circular non-Hermitian chain under the nonreciprocal intra-cell coupling and inter-cell coupling *** find that the circular non-Hermitian chain exhibits an even–odd effect on the unit cell corresponding to a large chain,which is different from the open non-Hermitian chain only exhibiting the same effect for a small ***,we find that the originally localized bulk states become totally extended via designing the boundary coupling strength *** extended bulk states reveal the fact of the disappearance of the non-Hermitian skin *** particular,we show that the circular non-Hermitian chain also possesses the analogous edge states under some parameter regimes,which is pretty counterintuitive since the circular chain usually cannot define a *** investigations supply the different non-Hermitian phenomena in a circular non-Hermitian chain.

关键词： boundary states non-Hermitian chain topological state

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Population genomic data reveal low genetic diversity,divergence and local adaptation among threatened Reeves's Pheasant(Syrmaticus reevesii)

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Avian Research 2024年第1期15卷 1-11页

作者： qi lu Pengcheng Wang Jiang Chang De Chen Shenghan Gao Jacob Hoglund Zhengwang Zhang Ministry of Education Key Laboratory for Biodiversity Science and Ecological Engineering College of Life SciencesBeijing Normal UniversityBeijing100875China Jiangsu Key Laboratory for Biodiversity and Biotechnology College of Life SciencesNanjing Normal UniversityNanjing210023China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing100012China State Key Laboratory of Microbial Resources Institute of MicrobiologyChinese Academy of SciencesBeijing100101China Department of Ecology and Genetics Animal EcologyUppsala UniversityUppsalaSweden

Population genomic data could provide valuable information for conservation efforts;however,limited studies have been conducted to investigate the genetic status of threatened ***’s Pheasant(Syrmaticus reevesii)is facing population decline,attributed to increases in habitat *** is a knowledge gap in understanding the genomic status and genetic basis underlying the local adaptation of this threatened ***,we used population genomic data to assess population structure,genetic diversity,inbreeding patterns,and genetic ***,we identified candidate genes linked with adaptation across the current distribution of Reeves’s *** present study assembled the first de novo genome sequence of Reeves’s Pheasant and annotated 19,458 *** also sequenced 30 individuals from three populations(Dabie Mountain,Shennongjia,qinling Mountain)and found that there was clear population structure among those *** comparing with other threatened species,we found that Reeves’s Pheasants have low genetic *** of homozygosity suggest that the Shennongjia population has experienced serious *** demographic history results indicated that three populations experienced several declines during the glacial *** adaptative analysis among the populations identified 241 candidate genes under directional *** are involved in a large variety of processes,including the immune response and *** results suggest that the three populations should be considered as three different conservation *** current study provides genetic evidence for conserving the threatened Reeves’s Pheasant and provides genomic resources for global biodiversity management.

关键词： Conservation genetics Local adaptation Pheasant Whole-genome sequencing

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Research Progress on the Growth-Promoting Effect of Plant Biostimulants on Crops

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Phyton-International Journal of Experimental Botany 2024年第4期93卷 661-679页

作者： qi lu Longfei Jin Cuiling Tong Feng Liu Bei Huang Dejian Zhang College of Horticulture and Gardening Hubei Key Laboratory of Waterlogging Disaster and Agricultural Use of WetlandYangtze UniversityJingzhou434020China Institute of Citrus Research Zhejiang Academy of Agricultural SciencesTaizhou318026China Jingzhou Institute of Technology Jingzhou434025China

A Plant Biostimulant is any substance or microorganism applied to plants to enhance nutrition efficiency,abioticstress tolerance,and/or crop quality traits,regardless of its nutrient *** application of Plant biostimulants(PBs)in production can reduce the application of traditional pesticides and chemical fertilizers and improvethe quality and yield of crops,which is conducive to the sustainable development of *** in-depthunderstanding of the mechanism and effect of various PBs is very important for how to apply PBs reasonablyand effectively in the practice of crop *** paper summarizes the main classification of PBs;Thegrowth promotion mechanism of PBs was analyzed from four aspects:improving soil physical and chemical properties,enhancing crop nutrient absorption capacity,photosynthesis capacity,and abiotic stress tolerance;At thesame time,the effects of PBs application on seed germination,seedling vigor,crop yield,and quality were summarized;Finally,how to continue to explore and study the use and mechanism of PBs in the future is analyzedand prospected,to better guide the application of PBs in crop production in the future.

关键词： Plant biostimulants growth promoting effect crop production

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Prognostic Nutritional Index Associates with the Severity of Silicosis:A Study from a Tertiary Class A Prevention and Treatment Institute for Occupational Diseases in China

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Biomedical and Environmental Sciences 2024年第1期37卷 122-126页

作者： HE La Gu LIANG Yun Lai YANG lu qi YUAN Hua Min Medical laboratory Department Hunan Prevention and Treatment Institute for Occupational DiseasesChangsha 410000HunanChina Laboratory Medicine Department Xiangya HospitalCentral South UniversityChangsha 410013HunanChina

Pneumoconiosis is a group of heterogeneous fibrotic lung diseases caused by inorganic mineral dust and includes coal workers’pneumoconiosis and *** involves diffuse or nodular interstitial pulmonary fibrosis caused by exposure to asbestos or silica *** is thought to have the highest number of silicosis cases,with 6,000 new cases reported annually^([1]).Currently,the clinical diagnosis and monitoring of silicosis relies mainly on a history of occupational exposure and radiological abnormalities^([2]).Therefore,determining further indicators is crucial to reflect the severity of silicosis.

关键词： diagnosis lung diseases

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Loneliness,social isolation and incident chronic kidney disease among patients with diabetes

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General Psychiatry 2024年第3期37卷 440-448页

作者： Rui Tang Jian Zhou Xuan Wang Hao Ma Xiang Li Yoriko Heianza lu qi Epidemiology Tulane University School of Public Health and Tropical MedicineNew OrleansLouisianaUSA The Second Xiangya Hospital of Central South University ChangshaHunanChina Nutrition Harvard University T H Chan School of Public HealthBostonMassachusettsUSA

Background Individuals with diabetes have a significantly higher risk of developing chronic kidney disease(CKD)and higher levels of social isolation and loneliness compared with those without ***,the American Heart Association highlighted the importance of considering social determinants of health(SDOH)in conjunction with traditional risk factors in patients with *** To investigate the associations of loneliness and social isolation with incident CKD risk in patients with diabetes in the UK *** A total of 18972 patients with diabetes were included in this prospective *** and Social Isolation Scales were created based on self-reported *** adjusted Cox proportional hazard model was used to investigate the associations of loneliness and social isolation with CKD risk among patients with *** relative importance in predicting CKD was also calculated alongside traditional risk *** During a median follow-up of 10.8 years,1127 incident CKD cases were reported.A higher loneliness scale,but not social isolation,was significantly associated with a 25%higher risk of CKD,independent of traditional risk factors,among patients with *** the individual loneliness factors,the sense of feeling lonely emerged as the primary contributing factor to the elevated risk of *** with individuals not experiencing feelings of loneliness,those who felt lonely exhibited a 22%increased likelihood of developing *** addition,feeling lonely demonstrated greater relative importance of predicting CKD compared with traditional risk factors such as body mass index,smoking,physical activity and *** This study indicates the significant relationship between loneliness and CKD risk among patients with diabetes,highlighting the need to address SDOH in preventing CKD in this population.

关键词： patients diabetes kidney

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Spontaneous anchoring Cl intoα-Co(OH)_(2) as efficient and stable oxygen reduction electrocatalysts for seawater battery

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Rare Metals 2024年第7期43卷 3074-3083页

作者： Wang Zheng Xue-Rong Zheng qi lu Yan-Hui Cao Yang Wang Hai-Peng Fu Jin-Feng Zhang Yi-Da Deng Wen-Bin Hu School of Materials Science and Engineering Key Laboratory of Advanced Ceramics and Machining Technology of Ministry of EducationTianjin UniversityTianjin 300072China State Key Laboratory of Marine Resource Utilization in South China Sea School of Materials Science and EngineeringHainan UniversityHaikou 570228China Key Laboratory of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang 110819China

Seawater battery is an advanced energy storage system that enables conversion of chemical energy to electricity by consuming metals,dissolved oxygen and seawater in anode,cathode and electrolyte,***,the oxygen reduction reaction(ORR)activity and stability of electrocatalysts can be easily deactivated due to the severe Cl~-permeation and corrosion in seawater ***,we developed a structural buffer engineering strategy by spontaneously anchoring Cl~-intoα-Co(OH)_(2) as efficient and stable ORR electrocatalysts,in which the ultrathinα-Co(OH)_(2) nanosheets were synthesized using an ultrafast solution high-temperature shock(SHTS)*** large lattice space(~0.8 nm)of layeredα-Co(OH)_(2) ensured the spontaneously penetration of Cl~-into the lattice structure and replaced part of OH~-to formα-Co(OH)_(2-x)Cl_*** continuous leaching and compensating of saturated Cl inα-Co(OH)_(2-x)Cl_x could enhance the Cl~-corrosion resistance and modulate electronic structure of Co metallic sites,thus improving the ORR electrocatalytic activity and stability in seawater ***α-Co(OH)_(2-x)Cl_x seawater batteries display superior onset and half-wave potentials of 0.71 and 0.66 V,respectively,which are much better than the counterparts ofα-Co(OH)_(2) and ofβ-Co(OH)_(2) with no Cl~-penetrating and no buffer ***α-Co(OH)_(2-x)Cl_x-based seawater batteries display stable open-circuit potential of 1.69 V and outstanding specific capacity of 1345 mAh·g^(-1).

关键词： Seawater battery Oxygen reduction electrocatalyst Solution high-temperature shock Structural buffer engineering

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基于衍生搜索政治优化算法解决含可再生能源的多区域经济调度问题

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电网技术 2024年第4期48卷 1583-1592,I0055,I0056-I0059页

作者：陈旭鲁启江苏大学电气信息工程学院江苏省镇江市212013

随着可再生能源并入多区域电力系统,其不确定性大大增加了电力系统多区域经济调度的复杂度。如何高效求解含有风力和太阳能的多区域经济调度(multi-areaeconomic dispatch containing wind and solar energy,MAEDWS)问题面临着严峻的挑... 详细信息

随着可再生能源并入多区域电力系统,其不确定性大大增加了电力系统多区域经济调度的复杂度。如何高效求解含有风力和太阳能的多区域经济调度(multi-areaeconomic dispatch containing wind and solar energy,MAEDWS)问题面临着严峻的挑战。针对现有优化算法在处理MAEDWS问题时存在收敛速度慢和求解精度低等不足,该文提出一种基于衍生搜索的政治优化(derivative search-based political optimizer,DSPO)算法。在政治优化算法的基础上,引入首脑引领策略和衍生搜索机制。前者引领候选解前往更有希望的区域,加快收敛速度;后者在区域获胜者周围衍生邻域解,丰富多样性。该文将DSPO算法和其他6种代表性算法应用于MAEDWS问题,并进行对比分析。收敛曲线和性能指标的结果表明DSPO算法在收敛效率、求解精确度、稳定性方面取得了整体最优。

关键词：多区域经济调度风力和太阳能政治优化算法衍生搜索

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Ultraclean transfer of graphene by mechanically exfoliating polymer with modified crosslink density

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Nano Research 2024年第8期17卷 6795-6802页

作者： qi lu Jiawei Yang Chaofan Zhou Zhaoning Hu Saiyu Bu Bingbing Guo Yixuan Zhao Junhao Liao Mingpeng Shang Ge Chen Kaicheng Jia Jianbo Yin qiang Zeng Li Lin Zhongfan Liu College of Science China University of Petroleum(Beijing)Beijing 102249China School of Materials Science and Engineering Peking UniversityBeijing 100871China Center for Nanochemistry Beijing Science and Engineering Center for NanocarbonsBeijing National Laboratory for Molecular ScienceCollege of Chemistry and Molecular EngineeringPeking UniversityBeijing 100871China Beijing Graphene Institute Beijing 100095China Faculty of Information Technology Beijing University of TechnologyBeijing 100124China Academy for Advanced Interdisciplinary Studies Peking UniversityBeijing 100871China Department of Electronics Peking UniversityBeijing 100871China Second Clinical Division National Engineering Laboratory for Digital and Material Technology of StomatologyPeking University School and Hospital of StomatologyBeijing 100081China

The transfer of graphene from metallic substrates onto application-specific substrates is usually inevitable for the applications of high-quality graphene films derived from chemical vapour deposition(CVD)*** used to support the graphene films during the transfer,the coating of the polymer would produce the surface contaminations and hinder the industrially compatible *** this work,through the thermal imidization of polyamide acid(PAA)to polyimide(PI)and tuning of the concentration of dangling chains,we achieved the ultraclean and crack-free transfer of graphene wafers with high electronic *** resulting contamination-free and hydrophilic surface also enabled the observed improved cell viability in a biomedical *** avoiding aqueous etching or the usage of strong bases,our proposed transfer method is industrially compatible for batch transfer of graphene films towards the real applications.

关键词： chemical vapour deposition(CVD)graphene films graphene transfer ultraclean transfer transfer medium crosslink density cell viability assay

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