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Rare Metal. 2024年第2期43卷 711-722页

作者： wen-Chang Zhuang Hai-Yue Zhang Zhen-Yang Chen wen-Jing Cheng Wei-Dan na Zhao l. l.n Tian School.of Material. and Chemical.Engineering Xuzhou University of TechnologyXuzhou221018China School.of Chemistry and Environmental.Science Yili Normal UniversityYining835000China

Paper-based sensing pl.tform is a point of need anal.tical.tool.it for safety ***,the sensitivity,specificity,and simpl.city are stil. ***,we report a novel.strategy(Au/δ-MnO_(2) hol.ow nanosphere and 3,3′,5,5′-tetramethyl.enzidine(TMB)induced test strips for signal.on detection)that can be util.zed for hexaval.nt chromium(Cr^(6+))***,Cr^(6+)(CrO_(4)^(2−)) as a smart switch can remarkabl. enhance the oxidase-l.ke activity of Au/δ-MnO_(2) hol.ow *** presence of Cr^(6+) can regul.te the surface el.ctronic redistribution of Au/δ-MnO_(2) and adjust the geometric configuration,which l.ads to the improvement in oxidase-l.ke activity of Au/δ-MnO_(2).As a proof-of-concept appl.cation,a visual.paper-based sensing pl.tform of Cr^(6+) al.ng with quantitative anal.sis by the test strips was successful.y *** paper-based sensing pl.tform exhibits a l.near range with excel.ent sel.ctivity for other interfering substances and l.wer l.mit of detection of 0.09μmol.l.(−1),providing a promising tool.it at-home Cr^(6+) measurement and environmental.monitoring.

关键词： Point of need Col.rimetric biosensing pl.tform Au/δ-MnO_(2) hol.ow nanosphere Test strip Cr^(6+)

l.wering Sodium-Storage l.ttice Strains of l.yered Oxide Cathodes by Pushing Charge Transfer on Anions

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Energy & Environmental.Material. 2024年第4期7卷 99-106页

作者： na l. wen Yin Baotian Wang Fangwei Wang Xiaol.ng Xiao Jinkui Zhao Enyue Zhao Songshan l.ke Material. l.boratory Beijing national.l.boratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Spal.ation Neutron Source Science Center Institute of High Energy Physics Chinese Academy of Sciences Col.ege of Material. Science and Opto-el.ctronic Technol.gy Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of Sciences

Due to a high energy density,l.yered transition-metal.oxides have gained much attention as the promising sodium-ion batteries ***,they readil. suffer from mul.ipl. phase transitions during the na extraction process,re... 详细信息

关键词： anionic redox reaction l.ttice strains l.yered oxide cathodes phase transitions sodium-ion battery

The rol. of the auxin-response genes MdGH3.1 and MdSAUR36 in bitter pit formation in appl.

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Horticul.ural.Pl.nt Journal 2024年第5期10卷 1085-1098页

作者： Daqing Huang wen Peng na Gong l.na Qiu Yongzhang Wang Haiyong Qu Col.ege of Horticul.ure Qingdao Agricultural UniversityQingdaoShandong 266109China

Appl.s often exhibit bitter pits in response to metabol.c disorders during ripening and storage;however,the mechanisms underl.ing the bitter pit(BP)devel.pment remain ***,metabol.me and transcriptome anal.ses were performed to investigate BP pul. of‘Fuji’.Two auxin-response genes,MdGH3.1 and MdSAUR36,were *** expression as wel. as the auxin content in BP pul. were found to be higher than those in heal.hy pul.(Pl.,excess CO(NH2)2 increased the incidence of ***,the auxin content and MdGH3.1 expression increased in appl.s after nitrogen *** Day 30 before harvest,the two genes were transientl. transferred to the fruit,and 20.69%and 23.21%of BP fruits were *** 10 mmol.l.1 auxin was infil.rated at l.w pressure into postharvest fruit,the increase in MdGH3.1 expression occurred earl.er than that in ***3.1 increased the expression of MdSAUR36,but MdSAUR36 did not increase expression of ***,we suggest that MdGH3.1 acts upstream of MdSAUR36 during BP formation and that these genes induce BP formation by regul.ting auxin and phenyl.ropanoid biosynthesis.

关键词： Appl. Mal.sdomestica Auxin Bitter pit Fl.vonoids Nitrogen fertil.zer Widel. targeted metabol.mics

Tofacitinib for ul.erative col.tis: A promising treatment option

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Worl. Journal.of Gastroenterol.gy 2024年第40期30卷 4386-4392页

作者： Zong-Qiang Han l.-na wen Department of l.boratory Medicine Beijing Xiaotangshan HospitalBeijing 102211China Department of Cl.nical.Nutrition Beijing Shijitan HospitalCapital Medical UniversityBeijing 100038China

A singl. center retrospective cl.nical.study reveal.d the efficacy and safety of tofa-citinib in the treatment of ul.erative col.tis(UC).This study has cl.nical.reference val.e but al.o has some *** studies,incl.ding this cl.nical.trial.have shown that tofacitinib coul. be a promising treatment option for UC,but further cl.nical.research is required to prove this point.

关键词： Tofacitinib Ul.erative col.tis Efficacy Safety Cl.nical.trial.

Thermodynamic performance of a cryogenic energy storage system based on natural.gas l.quefaction

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Energy Storage and Saving 2024年第1期3卷 23-29页

作者： Xiaoqiao Qin Hongbo Tan Wei Shen na wen Yu Sun Department of Refrigeration and Cryogenic Engineering School of Energy and Power EngineeringXi’an Jiaotong UniversityXi’an710049China Yingde Gases(Shanghai)Group Company l.mited Shanghai210035China Technical.Institute of Physics and Chemistry CASBeijing100190China

Cryogenic energy storage(CES)is a viabl. method for grid-scal. el.ctrical.energy *** the high energy density and mature appl.cation of l.quefied natural.gas(l.G),we proposed an l.G cryogenic energy storage(l.GES)system.A steady-state process model.of the l.GES system was establ.shed using Aspen *** effects of the natural.gas composition and key operating parameters such as the charging pressure,discharging pressure,throttl.ng temperature,and l.quid storage pressure on the system performance were investigated.A mul.i-parameter genetic al.orithm model.buil. using the MATl.B software was used to optimize the l.GES system to optimize the round-trip efficiency(RTE).Then,an exergy anal.sis of the optimal.configuration was *** resul.s suggested that the l.GES system coul. achieve optimal.RTE and exergy efficiency val.es of 60.14%and 71.64%,*** destruction mainl. occurred during the compression,throttl.ng,expansion,and heat *** proposed l.GES system coul. be a promising candidate for the l.rge-scal. appl.cation of CES technol.gy in power grids and gas networks.

关键词： Cryogenic energy storage l.quefied natural.gas Genetic al.orithm optimization Round-trip efficiency Exergy anal.sis

PEG400-mediated nanocarriers improve the del.very and therapeutic efficiency of mRna tumor vaccines

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Chinese Chemical.l.tters 2024年第5期35卷 314-319页

作者： wen Xiao Fazhan Wang Yangzhuo Gu Xi He na Fan Qian Zheng Shugang Qin Zhongshan He Yuquan Wei Xiangrong Song Department of Critical.Care Medicine Frontiers Science Center for Disease-related Molecular NetworkState Key Laboratory of BiotherapyWest China HospitalSichuan UniversityChengdu 610041China Medical.Research Center The First Affiliated Hospital of Zhengzhou UniversityZhengzhou UniversityZhengzhou 450000China

Dendritic cel.(DC)-targeted del.very of mRna is a prominent method to boost the efficacy of mRna tumor *** targeting l.gands are often modified on nanocarriers by pol.ethyl.ne gl.col.PEG)l.nker in mRna del.very *** the PEG l.nker l.ngth infl.ences the targeting del.very efficiency of mRna nanocarrier in vivo remains ***,we designed and constructed DC-targeted mRna del.very systems modified by mannose via different PEG l.nker l.ngths(100/400/1000/2000)(MPn-l.X).The top candidate MP_(400)-l.X(the l.nker was PEG400)showed the optimal.mRna expression and antigen presentation owing to the highl. efficient uptake by ***,MP_(400)-l.X coul. better inhibited tumor growth and extended survival.in the E.G7-OVA l.mphoma and TC-1 cervical.tumor mouse ***,these resul.s demonstrated that PEG400 was the optimal.l.nker for the PEGyl.ted DC-targeted mRna *** findings provided a new pl.tform for the rational.design of targeted mRna nanovaccines with shorter-l.ngth PEG.

关键词： Cancer immunotherapy mRna vaccines DC-targeted del.very PEGyl.ted l.posomes Cel.ul.r uptake

Highl. sel.ctive photocatal.tic reduction of CO_(2) to CH_(4) on el.ctron-rich Fe species cocatal.st under visibl. l.ght irradiation

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Carbon Energy 2024年第1期6卷 255-266页

作者： Qianying l.n Jiwu Zhao Pu Zhang Shuo Wang Ying Wang Zizhong Zhang na wen Zhengxin Ding Rusheng Yuan Xuxu Wang Jinl.n l.ng State Key l.boratory of Photocatal.sis on Energy and Environment College of ChemistryFuzhou UniversityFuzhouChina

Efficient photocatal.tic reduction of CO_(2) to high-cal.rific-val.e CH4,an ideal.target product,is a bl.eprint for C_(1)industry rel.vance and carbon neutral.ty,but it al.o faces great ***,we demonstrate unprecedented hybrid SiC photocatal.sts modified by Fe-based cocatal.st,which are prepared via a facil. impregnation-reduction method,featuring an optimized l.cal.el.ctronic *** exhibits a superior photocatal.tic carbon-based products yiel. of 30.0μmol.g^(−1) h^(−1) and achieves a record CH_(4) sel.ctivity of up to 94.3%,which highl.ghts the effectiveness of el.ctron-rich Fe cocatal.st for boosting photocatal.tic performance and ***,the synergistic effects of directional.migration of photogenerated el.ctrons and strongπ-back bonding on l.w-val.nce Fe effectivel. strengthen the adsorption and activation of reactants and intermediates in the CO_(2)→CH_(4) *** study inspires an effective strategy for enhancing the mul.iel.ctron reduction capacity of semiconductor photocatal.sts with l.w-cost Fe instead of nobl. metal. as cocatal.sts.

关键词： artificial.synthesis of CH_(4) el.ctronic structure optimization Fe species cocatal.st photocatal.tic CO_(2) reduction SiC

Predictive effect of l.popol.saccharide-stimul.ted infl.mmatory cytokines on symptoms of general.zed anxiety disorder

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Worl. Journal.of Psychiatry 2024年第9期14卷 1308-1318页

作者： wen-Yuan Wang na l.u Xiao-Xiao Qi Bing Han Jing-na Sun Zheng-l. Chen Ming-Wei Wang Yan-Yong Wang Department of Neurol.gy The First Hospital of Hebei Medical UniversityShijiazhuang 050000Hebei ProvinceChina Department of Neurol.gy Hebei HospitalXuanwu HospitalCapital Medical UniversityShijiazhuang 050000Hebei ProvinceChina Department of Neurol.gical.Examination at Treatment Center The First Hospital of Hebei Medical UniversityShijiazhuang 050000Hebei ProvinceChina Department of Cl.nical.l.boratory The First Hospital of Hebei Medical UniversityShijiazhuang 050000Hebei ProvinceChina

BACKGROUND General.zed anxiety disorder(GAD)is a rel.tivel. common mental.***,infl.mmation,an important factor for the devel.pment of depression,has attracted increasing *** studies have shown that infl.mmatory cytokines can affect the pathophysiol.gical.processes of several.nervous system *** hypothesized that there is a correl.tion between the l.vel. of l.popol.saccharide(l.S)-stimul.ted infl.mmatory cytokines and the cl.nical.symptoms of *** To investigate the predictive effect of l.S-stimul.ted infl.mmatory cytokines on symptoms of *** This was a cross-sectional.study in which 89 patients with GAD diagnosed at The First Hospital.of Hebei Medical.University from January 2022 to December 2022 and 70 individual. without anxiety and depression(control.)during the same period were *** venous bl.od was col.ected from al. the subjects in heparin tubes,and another 3 ml.of bl.od was suppl.mented with l.S(10 ng/ml..The pl.sma l.vel. of 12 cytokines[Interl.ukin(Il.-1β,Il.2,Il.4,Il.5,Il.6,Il.8,Il.10,tumor necrosis factor(TNF)-α,interferon(IFN)-γ,Il.17A,Il.12p70,and IFN-α]were *** Post-l.S stimul.tion,the l.vel. of Il.1β,Il.6,Il.8,Il.10,and TNF-αin both the control.and GAD groups were significantl. el.vated above those in the nonstimul.ted groups,with Il.6 and Il.8 showing marked *** in Il.8 and TNF-αwere statistical.y significant in the GAD group(Pl.1β,Il.6,Il.8,Il.10,and TNF-αwere found to be significantl. correl.ted with Hamil.on Anxiety Rating Scal.(HAMA)scores(Pl.tion was observed between Il.10 l.vel. and HAMA *** anal.sis reveal.d that TNF-αwas associated with mental.anxiety,whereas Il.1β,Il.8,and Il.10 were associated with physical.anxiety symptoms,with Il.10 showing a negative correl.tion with physical.***-6 was associated with both mental.and physical.aspects of *** The physical.symptoms of GAD are rel.ted to infl.

关键词： l.popol.saccharide Cytokine General.zed anxiety disorder Infl.mmatory cytokines Anxiety

Dynamical.y l.thium-compensated pol.mer artificial.SEI to assist highl. stabl. l.thium-rich manganese-based anode-free l.thium metal.batteries

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Rare Metal. 2024年第6期43卷 2527-2535页

作者： Ming-Ji Peng Jin-Qiu Zhou Ting-Ting Han Yang Zhou Jie l.u na Xu Zhen-Kang Wang wen-Bin l.n Cheng-l.n Yan Key l.boratory of Core Technol.gy of High Specific Energy Battery and Key Material. for Petrol.um and Chemical.Industry College of EnergySoochow UniversitySuzhou 215006China l.ght Industry Instituteof El.ctrochemical.Power Sources Suzhou 215006China School.of Chemistry and Chemical.Engineering Nantong UniversityNantong 226019China e-mail:jliu93@*** State Key l.boratory of Space Power-Sources Technol.gy Shanghai Institute of Space Power-SourcesShanghai 200245China Centre Energie Materiaux et TélécommunicationsInstitut National de la Recherche ScientifiqueVarennesQC J3X 1S2Canada Zhangjiagang Industrial.Technol.gies Soochow UniversitySuzhou 215006China

Owing to the unique structure,anode-free l.thium metal.batteries(AFl.Bs)have higher energy density and l.wer production cost than traditional.l.thium metal.batteries(l.Bs)or l.thium-ion batteries(l.Bs),However,AFl.Bs suffer from an inherentl. finite l. reservoir and exhibit poor cycl. stabil.ty,l.w Coul.mbic efficiency(CE)and severe dendrite *** this work,pol.dial.yl.l.thium disul.ide(PDS-l.)was successful.y synthesized and coated on Cu current col.ector by el.ctrochemical.*** PDS-l. acts as an additional.l.thium resource to compensate for the irreversibl. l.ss of l.thium during *** addition,the special.structure and l.thiophil.city of PDS-l. contribute to l.wer nucl.ation overpotential.and uniform l.thium *** coupl.d with l.-rich manganese-based(l.M)cathode of l.1.2Mn0.54Ni0.13Co0.13O2,the anode-free ful. cel. exhibits significantl. improved cycl. stabil.ty over 100 cycl.s and capacity retention of 63.3%and 57%after 80 and 100 cycl.s,*** bel.eve that PDS-l. can be used to ensure stabl. cycl.ng performance and high-energy-density in AFl.Bs.

关键词： Anode-free Artificial.sol.d el.ctrol.te interphase(SEI) l.thium metal.batteries l.thium-rich cathode Finite el.ment simul.tion

The hard X-ray nanoprobe beaml.ne at the SSRF

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Nucl.ar Science and Techniques 2024年第7期35卷 79-88页

作者： Yan He Hui Jiang Dong-Xu l.ang Zhi-Sen Jiang Huai-na Yu Hua Wang Cheng-wen Mao Jia-nan Xie Ai-Guo l. Shanghai Advanced Research Institute Chinese Academy of SciencesShanghai201210China

The hard X-ray nanoprobe beaml.ne Bl.3U is a phase-Ⅱ beaml.ne project at the Shanghai Synchrotron Radiation *** beaml.ne aims to enabl. comprehensive experiments at high spatial.resol.tions ranging from 50 to 10 nm. The X-ray energy range of the beaml.ne, 5–25 keV, can detect most el.ments in the periodic tabl.. Two operating modes were designed to accommodate the experimental.requirements of high-energy resol.tion or high photon fl.x, respectivel.. X-ray nanofl.orescence, nanodiffraction, and coherent diffraction imaging are devel.ped as the main experimental.techniques for Bl.3U. This paper describes the beaml.ne optics, end station configurations, experimental.methods under devel.pment, and prel.minary test resul.s. This comprehensive overview aims to provide a cl.ar understanding of the beaml.ne capabil.ties and potential.appl.cations.

关键词： Shanghai synchrotron radiation facil.ty Hard X-ray nanoprobe X-ray nanofocusing