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A study on hydrogen uptake and release of a eutectic mixture of biphenyl and diphenyl ether

Journal of Energy Chemistry 2020年第3期29卷 11-16页

作者： Munjeong Jang Byeong Soo Shin Young suk Jo Jeong Won kang Sang Kyu Kwak Chang Won Yoon Hyangsoo Jeong Center for Hydrogen Fuel Cell Research Korea Institute of Science and Technology(KIST)5 Hwarang-ro 14-gilSeongbuk-guSeoul 02792Republic of Korea Divison of Energy and Environment Technology KIST SchoolKorea University of Science and Technology5 Hwarang-ro 14-gilSeongbuk-guSeoul 02792Republic of Korea Department of Chemical and Biological Engineering Korea UniversityAnam-ro 145Seongbuk-guSeoul 02841Republic of Korea School of Energy and Chemical Engineering Ulsan National Institute of Science and Technology50UNIST-gilUlsan 44919Republic of Korea KHU-kiST Department of Converging Science and Technology Kyung Hee University26 Kyungheedae-roDongdaemun-guSeoul 02447Republic of Korea

Hydrogen storage in Liquid Organic Hydrogen Carrier(LOHC)systems is appealing for the safe storage and distribution of excess renewable energy via existing gasoline infrastructures to *** present the eutectic mixture of biphenyl and diphenyl ether of its first use as a LOHC *** material is hydrogenated with 99%selectivity without the cleavage of C–O bond,with commercial heterogeneous catalysts,which is confirmed by nuclear magnetic spectroscopy and gas chromatography-mass *** concentration,dehydrogenation enthalpy,and thermo-neutral temperature are calculated using a density functional *** results indicate that O-atom-containing material exhibits more favorable dehydrogenation thermodynamics than that of the hydrocarbon *** H2-rich material contains6.8 wt%of gravimetric hydrogen storage capacity.A preliminary study of catalytic dehydrogenation on a continuous reactor is presented to demonstrate a reversibility of this material.

关键词： Hydrogen storage Liquid organic hydrogen carrier Diphenyl ether Dehydrogenation Thermodynamics

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Brain endothelial cell-derived extracellular vesicles with a mitochondria-targeting photosensitizer effectively treat glioblastoma by hijacking the blood-brain barrier

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药学学报:英文版 2023年第9期13卷 3834-3848页

作者： Thuy Giang Nguyen Cao Ji Hee kang Su Jin kang Quan Truong Hoang Han Chang kang Won Jong Rhee Yu Shrike Zhang Young Tag Ko Min suk Shim Division of Bioengineering Incheon National UniversityIncheon 22012Republic of Korea College of Pharmacy Gachon UniversityIncheon 21936Republic of Korea Department of Pharmacy Integrated Research Institute of Pharmaceutical Sciencesand BK21 PLUS Team for Creative Leader Program for Pharmacomics-based Future PharmacyCollege of Pharmacythe Catholic University of KoreaGyeonggi-do 14662Republic of Korea Research Center for Bio Materials&Process Development Incheon National UniversityIncheon 22012Republic of Korea Division of Engineering in Medicine Department of MedicineBrigham and Women’s HospitalHarvard Medical SchoolCambridgeMA 02139USA

Glioblastoma(GBM)is the most aggressive malignant brain tumor and has a high mortality *** therapy(PDT)has emerged as a promising approach for the treatment of malignant brain ***,the use of PDT for the treatment of GBM has been limited by its low blood-brain barrier(BBB)permeability and lack of cancer-targeting ***,brain endothelial cell-derived extracellular vesicles(bEVs)were used as a biocompatible nanoplatform to transport photosensitizers into brain tumors across the *** enhance PDT efficacy,the photosensitizer chlorin e6(Ce6)was linked to mitochondria-targeting triphenylphosphonium(TPP)and entrapped into *** Ce6(TPP-Ce6)selectively accumulated in the mitochondria,which rendered brain tumor cells more susceptible to reactive oxygen species-induced apoptosis under light ***,the encapsulation of TPP-Ce6 into b EVs markedly improved the aqueous stability and cellular internalization of TPP-Ce6,leading to significantly enhanced PDT efficacy in U87MG GBM *** in vivo biodistribution study using orthotopic GBM-xenografted mice showed that b EVs containing TPP-Ce6[b EV(TPP-Ce6)]substantially accumulated in brain tumors after BBB penetration via transferrin receptor-mediated *** such,b EV(TPP-Ce6)-mediated PDT considerably inhibited the growth of GBM without causing adverse systemic toxicity,suggesting that mitochondria are an effective target for photodynamic GBM therapy.

关键词： Extracellular vesicle Chlorin e6 Triphenylphosphonium Mitochondria-targeting photosensitizer Photodynamic therapy Blood-brain barrier Glioblastoma Transferrin receptor

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Effects of electrochemical synthetic conditions on surface property and photocatalytic performance of copper and iron-mixed p-type oxide electrodes

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Journal of Materials Science & Technology 2018年第9期34卷 1503-1510页

作者： Sun Hee Yoon Dong suk Han Unseock kang Seung Yo Choi Wubulikasimu Yiming Ahmed Abdel-Wahab Hyunwoong Park Chemical Engineering Program Texas A&M University at Qatar School of Energy Engineering Kyungpook National University Department of Mechanical Engineering Texas A&M University at Qatar

Earth-abundant copper and iron-mixed oxide（CuO/CuFeO_2; CFO） film electrodes are synthesized using an electrochemical deposition（ED） technique at two different ED potentials（-0.36 and-0.66 V vs saturated calomel electrode（SCE）; denoted as ED-1 and ED-2, respectively）. Then, their surface morphologies are compared, and the photo（electro）catalytic activities for the reduction of Cr（VI） are examined in aqueous solutions at pH 7 under simulated sunlight（AM 1.5 G; 100 mW cm（-2））. The degree of the electrical potential applied to the ED process significantly affects the thickness of the synthesized electrode film and the intensity ratio of the diffraction peaks of CuO（111） and CuFeO_2（012）. A 200 μm thick ED-2 sample with a distinct stacking of CuO on CuFeO_2 exhibits a larger broadband absorption spectrum than the 50-μm thick ED-1 with less separate stacking. Furthermore, the ED-2 sample has a higher intensity ratio of the diffraction peaks of CuO（111） and CuFe02（012） than ED-1. As-synthesized ED-2 samples produce larger photocurrents, leading to faster Cr（VI） reduction on the surface under given potential bias（-0.5 V vs SCE）or bias-free conditions. The energy levels（i.e., flatband potential） for the two samples are almost the same（only 10 mV difference）, presumably supposing that the enhanced photoactivity of the ED-2 sample for Cr（VI） reduction is due to the facilitated charge transfer. The time-resolved photoluminescence emission spectra analysis reveal that the lifetime（r） of the charge carriers in the ED-1 sample is 0.103 ns, which decreases to 0.0876 ns in the ED-2. The ED-2 sample synthesized at a high negative potential is expected to contribute greatly to the application of other solar-to-fuel energy conversion fields as a highly efficient electrode material.

关键词： Artificial photosynthesis Solar fuel Delafossites Morphology Charge transfer

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A reference-grade genome of the xerophyte Ammopiptanthus mongolicus sheds light on its evolution history in legumes and droughttolerance mechanisms

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Plant Communications 2024年第7期5卷 157-177页

作者： Lei Feng Fei Teng Na Li Jia-Cheng Zhang Bian-Jiang Zhang Sau-Na Tsai Xiu-Le Yue Li-Fei Gu Guang-Hua Meng Tian-Quan Deng suk-Wah Tong Chun-Ming Wang Yan Li Wei Shi Yong-Lun Zeng Yue-Ming Jiang Weichang Yu Sai-Ming Ngai Li-Zhe An Hon-Ming Lam Jun-Xian He School of Life Sciences and State Key Laboratory of Agrobiotechnology The Chinese University of Hong KongSha TinNew TerritoriesHong KongChina Guangdong Provincial Key Laboratory of Biotechnology for Plant Development School of Life SciencesSouth China Normal UniversityGuangzhou 510631China BGI-Shenzhen Tech Co. Ltd.Beishan Industrial ZoneYantian DistrictShenzhen 518083China School of Life Sciences and Ministry of Education Key Laboratory of Cell Activities and Stress Adaptations Lanzhou UniversityLanzhou 730030China State Key Laboratory of Subtropical Silviculture Zhejiang Agriculture and Forestry UniversityHangzhou 311300China State Key Laboratory of Plant Diversity and Specialty Crops South China Botanical GardenChinese Academy of SciencesGuangzhou 510650China Guangdong Provincial Key Laboratory of Applied Botany&Key Laboratory of South China Agricultural Plant Molecular Analysis and Genetic Improvement South China Botanical GardenChinese Academy of SciencesGuangzhou 510650China College of Life Sciences and Oceanography Shenzhen UniversityShenzhen 518060China State Key Laboratory of Efficient Production of Forest Resources Beijing Forestry UniversityBeijing 100083China

Plants that grow in extreme environments represent unique sources of stress-resistance genes and *** mongolicus(Leguminosae)is a xerophytic evergreen broadleaf shrub native to semi-arid and desert regions;however,its drought-tolerance mechanisms remain poorly ***,we report the assembly of a reference-grade genome for ***,describe its evolutionary history within the legume family,and examine its drought-tolerance *** assembled genome is 843.07 Mb in length,with 98.7%of the sequences successfully anchored to the nine chromosomes of *** genome is predicted to contain 47611 protein-coding genes,and 70.71%of the genome is composed of repetitive sequences;these are dominated by transposable elements,particularly longterminal-repeat *** analyses revealed two whole-genome duplication(WGD)events at 130 and 58 million years ago(mya)that are shared by the genus Ammopiptanthus and other legumes,but no species-specific WGDs were found within this *** genome reconstruction revealed that the *** genome has undergone fewer rearrangements than other genomes in the legume family,confirming its status as a"relict plant".Transcriptomic analyses demonstrated that genes involved in cuticular wax biosynthesis and transport are highly expressed,both under normal conditions and in response to polyethylene glycol-induced *** induction of genes related to ethylene biosynthesis and signaling was also observed in leaves under dehydration stress,suggesting that enhanced ethylene response and formation of thick waxy cuticles are two major mechanisms of drought tolerance in *** expression of AmERF2,an ethylene response factor unique to ***,can markedly increase the drought tolerance of transgenic Arabidopsis thaliana plants,demonstrating the potential for application of *** genes in crop improvement.

关键词： Ammopiptanthus mongolicus genome sequencing genome evolution drought tolerance cuticular wax ethylene

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Fabrication, microstructure and properties of SiCp/Cu heat sink materials

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Rare Metals 2006年第Z2期25卷 232-236页

作者： kang suk-bong Korea Institute of Machinery and Materials 66 Sangnam-dong Changwon 641-010 Korea

Cu-coated powder was fabricated by electroless plating process, and the composition and morphology of coated powder were studied. Moreover, Cu-30, 40, 50 vol.%SiCp heat sink materials were fabricated by hot pressing using coated and uncoated powder. And the microstructure and thermophysical properties of the heat sink materials were also studied. The results show that SiCp particles distribute uniformly in heat sink materials and the interface between SiCp particles and Cu matrix is clear and well bonded. On the condition of same volume fraction of SiCp, the thermal conductivity of the material using coated powder is larger than that of the material using uncoated powder. Under experiment conditions, the thermal conductivity and coefficient of thermal expansion of Cu-30 vol.%SiCp heat sink material is 236.2 W·m-1·K-1 and 9.9×10-6/K (30-200 ℃) respectively. It provides important reference data for future experiments.

关键词： heat sink material electroless copper plating coefficient of thermal expansion thermal conductivity

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Does the discrepancy in histologic differentiation between a forceps biopsy and an endoscopic specimen necessitate additional surgery in early gastric cancer?

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World Journal of Gastrointestinal Oncology 2017年第8期9卷 319-326页

作者： Jae Seung Soh Hyun Lim Ho suk kang Jong Hyeok kim Kab Choong kim Department of Internal Medicine University of Hallym College of Medicine Hallym University Sacred Heart Hospital Department of Surgery University of Hallym College of Medicine Hallym University Sacred Heart Hospital

To investigate the clinicopathological variables in early gastric cancer (EGC) patients in relation to differentiation discrepancy. METHODSThe data of 265 specimens from 240 patients with EGC, who had undergone radical operation at Hallym University Sacred Heart Hospital from 2010 to 2015, were retrospectively analyzed. We evaluated clinical, endoscopic, and histopathological data according to histological discrepancy. RESULTSClinically significant discrepancy rate showed the difference in differentiated type (well and moderately differentiated) and undifferentiated type (poorly differentiated and signet ring cell) between endoscopic biopsies and postoperative specimens was 9.4% (25/265). There were no differences in tumor location, size, gross pattern, and number of biopsies. Specimens having histological discrepancy showed more submucosal invasion (72.0% vs 49.6%, P = 0.033) and lymph node involvement (24.0% vs 7.9%, P = 0.009) than specimens having non-discrepancy. The rate of a positive epidermal growth factor receptor status was higher in specimens having discrepancy than in specimens having non-discrepancy (81.0% vs 55.4%, P = 0.035). CONCLUSIONThe discordance of histologic differentiation is associated with higher submucosal invasion and lymph node metastases in EGC. Patients have histological discrepancy may require additional surgical treatments.

关键词： Early gastric cancer Histological discrepancy Differentiation Clinicopathological factor Endoscopic treatment Surgical treatment

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AZ451镁合金薄带的组织和力学性能研究

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金属学报 2008年第4期44卷 397-402页

作者：陈洪美 kang suk-Bong 于化顺闵光辉山东大学材料科学与工程学院济南250061 韩国材料研究所韩国昌原

利用OM,SEM,TEM,数字显微硬度计和电子万能试验机,对常规轧制与铸轧法制备的AZ451镁合金薄带的显微组织和力学性能进行了分析.常规铸锭轧制后仍为等轴晶组织,晶粒尺寸明显细化.铸轧条带在350℃多道次轧制后显微组织由树枝晶转变为纤维... 详细信息

利用OM,SEM,TEM,数字显微硬度计和电子万能试验机,对常规轧制与铸轧法制备的AZ451镁合金薄带的显微组织和力学性能进行了分析.常规铸锭轧制后仍为等轴晶组织,晶粒尺寸明显细化.铸轧条带在350℃多道次轧制后显微组织由树枝晶转变为纤维状变形组织,350℃/10 min热处理后合金发生再结晶,得到等轴晶组织.轧制后两种合金均具有良好的力学性能,双辊铸轧合金的强度和延伸率均明显高于传统铸造合金的强度和延伸率,两种合金1 mm厚薄带经350℃/10 min均匀化退火后的抗拉强度、屈服强度和延伸率分别为334.4 MPa,229.3 MPa,23.8%和270.8 MPa,174.4 MPa,10.8%.两种合金的断口形貌均呈现河流花样,撕裂棱和韧窝共存,是明显的韧性断裂,铸轧合金的韧窝更明显,尺寸更小一些,这与铸轧合金的组织更细小有关.

关键词： AZ451镁合金双辊铸轧热轧显微组织力学性能

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A356/SiC_P与列车实用中的有机闸片的滑动摩擦磨损特性

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稀有金属材料与工程 2008年第11期37卷 1956-1960页

作者：金云学 Jung-Moo Lee suk-Bong kang 江苏科技大学先进焊接技术省级重点实验室江苏镇江212003 Advanced Materials Division Korea Institute of Machinery and Materials

以铝基复合材料作为列车制动盘材料的实用化为目的，选用A356／SIC 20％（体积分数，下同）复合材料和AISI D2工具钢为摩擦材料，以中速列车实用中的有机闸片为对偶材料，进行对比干摩擦磨损试验，并分析比较了磨损特性。结果表明：铝... 详细信息

以铝基复合材料作为列车制动盘材料的实用化为目的，选用A356／SIC 20％（体积分数，下同）复合材料和AISI D2工具钢为摩擦材料，以中速列车实用中的有机闸片为对偶材料，进行对比干摩擦磨损试验，并分析比较了磨损特性。结果表明：铝基复合材料在小于200Y（3．98MPa）的低载荷下，只存在轻微的氧化磨损，耐磨性比实用中的铁合金材料更好；而超过该载荷时。开始发生磨削磨损，磨损量逐步超过铁合金材料，当载荷达到400N（7．96MPa）时，由于严重的磨削磨损，磨损量剧增。而铁合金材料则随载荷和滑动速度增加，磨损率缓慢增加；磨损过程中的复合材料的摩擦系数平均值与载荷、滑动速度无关，始终保持0．3～0．4，同时随磨损距离的波动也非常小，而工具钢的摩擦系数平均值则对试验参数的敏感度相对大些，且摩擦系数平均值也比复合材料略小，即摩擦系数方面复合材料具有更好的特性。

关键词：列车制动盘铝基复合材料摩擦磨损

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T6态A356/SiC与Semi-Metallic Pad的干滑动摩擦磨损特性

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稀有金属材料与工程 2008年第12期37卷 2147-2151页

作者：金云学 Jung-Moo Lee suk-Bong kang 江苏科技大学先进焊接技术省级重点实验室江苏镇江212003 Korea Institute of Machinery and Materials Changwon 641-010Korea

选用A356/SiC复合材料与Semi-metallic pad材料进行干滑动摩擦磨损试验,并采用SEM、XRD、EDS等手段分析了复合材料的摩擦磨损特点及磨损机制。铝基复合材料与该pad间表现出非常出色的耐摩擦磨损特性,在1m/s的低滑动速度下,即使载荷增加... 详细信息

选用A356/SiC复合材料与Semi-metallic pad材料进行干滑动摩擦磨损试验,并采用SEM、XRD、EDS等手段分析了复合材料的摩擦磨损特点及磨损机制。铝基复合材料与该pad间表现出非常出色的耐摩擦磨损特性,在1m/s的低滑动速度下,即使载荷增加到700N也几乎不发生磨损;载荷不大于500N时,磨损率与滑动速度无关,保持非常小的范围。只有在高载荷、高滑动速度下才会有较为明显的磨损。摩擦系数则随载荷增大产生无规则变化,而随滑动速度的增加而减少,但变化幅度在0.1之内。复合材料耐磨特性好的主要原因是,磨损过程中磨损面上迅速形成以氧化物和石墨为主的润滑膜,减少磨损。高载荷、高滑动速度下磨损的主要特点为,复合材料表层形成塑性流动层,大的塑性流动变形使得较软的铝合金基体沿磨损方向以片状形式挤出,形成特殊的磨屑。而不易变形的SiC颗粒则留在磨损面上形成SiC聚集区,该区域又能在一定程度上减少进一步的磨损。

关键词： SiC 铝合金滑动磨损机制摩擦磨损

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Multimodal imaging evaluation in staging of rectal cancer

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World Journal of Gastroenterology 2014年第15期20卷 4244-4255页

作者： suk Hee Heo Jin Woong kim Sang Soo Shin Yong Yeon Jeong Heoung-Keun kang Department of Radiology Chonnam National University Hwasun HospitalChonnam National University Medical SchoolJeollanam-do 519-763South Korea Department of Radiology Chonnam National University HospitalChonnam National University Medical SchoolGwang-ju 501-757South Korea

Rectal cancer is a common cancer and a major cause of mortality in Western countries. Accurate staging is essential for determining the optimal treatment strategies and planning appropriate surgical procedures to control rectal cancer. Endorectal ultrasonography (EUS) is suitable for assessing the extent of tumor invasion, particularly in early-stage or superficial rectal cancer cases. In advanced cases with distant metastases, computed tomography (CT) is the primary approach used to evaluate the disease. Magnetic resonance imaging (MRI) is often used to assess preoperative staging and the circumferential resection margin involvement, which assists in evaluating a patient’s risk of recurrence and their optimal therapeutic strategy. Positron emission tomography (PET)-CT may be useful in detecting occult synchronous tumors or metastases at the time of initial presentation. Restaging after neoadjuvant chemoradiotherapy (CRT) remains a challenge with all modalities because it is difficult to reliably differentiate between the tumor mass and other radiation-induced changes in the images. EUS does not appear to have a useful role in post-therapeutic response assessments. Although CT is most commonly used to evaluate treatment responses, its utility for identifying and following-up metastatic lesions is limited. Preoperative high-resolution MRI in combination with diffusion-weighted imaging, and/or PET-CT could provide valuable prognostic information for rectal cancer patients with locally advanced disease receiving preoperative CRT. Based on these results, we conclude that a combination of multimodal imaging methods should be used to precisely assess the restaging of rectal cancer following CRT.

关键词： Rectal cancer Multimodality Imaging Staging Restaging

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