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Energy & Environmental Materials 2024年第4期7卷 404-412页

作者： kang Huang Wenzhuo Wu Song x. Pengfei Yan Zhongming Wei Qun x. Henan Institute of Advanced Technology Zhengzhou University College of Materials Science and Engineering Zhengzhou University State Key Laboratory of Superlattices and Microstructures Institute of Semiconductors Chinese Academy of Sciences

Modulation of Si-O bonds under mild conditions has been a challenging issue in the field of material science,which is critical to manufacture highperformance silica-based optical and photonic ***,we introduce a nondestructive technique to achieve Si-O bond rearrangement,leading to plastic deformation and photoluminescence enhancement of amorphous silica nanoparticles using supercritical carbon diox.des in EtOH/H2O solution under mild temperature.

关键词： amorphous silica anisotropic stress photoluminescence plastic deformation supercritical CO2

Enhancement and Removal of PM_(2.5)by Cold and Warm Air Masses Accompanying Certain Synoptic Weather Systems across Hangzhou,China during 2014-2020

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Journal of Meteorological Research 2024年第3期38卷 620-634页

作者： Bu YU Feng CHEN Hanqing kang Bin ZHU Hongnian LIU Hangzhou Meteorological Bureau Hangzhou310051China Hangzhou International Urbanology Research Center for Urban Governance Studies Hangzhou311121China Zhejiang Institute of Meteorological Sciences Hangzhou310008China Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration Nanjing University of Information Science&TechnologyNanjing210044China School of Atmospheric Sciences Nanjing UniversityNanjing210023China

Local air pollution is strongly affected by synoptic weather systems,such as fronts,troughs,low-altitude vortices,or high-altitude ***,few studies have analyzed the meteorological properties of cold or warm air masses associated to these systems and their impact on local air *** this study,hourly observations of fine particulate matter(diameter of up to 2.5µm,i.e.,PM_(2.5)),wind(V),temperature(T),pressure(P),and precipitation(R),acquired in Hangzhou in 2014-2020,were *** this analysis,weather patterns were categorized into 27 types;89 and 94 cases illustrating the passage of warm and cold air masses over Hangzhou were identified,respectively;the influence of air mass temperature,wind speed,and wind direction on PM_(2.5) concentrations and local accumulation or removal was *** main results are as follows.(1)Pollution events occurred more frequently for cold than for warm air masses,but average pollutant concentration was lower for cold air masses;(2)48%of the cold air mass cases corresponded to PM_(2.5) decreases and 52%to PM_(2.5) increases,with strong cold air masses(ΔT_(24h)>4°C;∣V∣_(average)>4 m s^(−1))markedly reducing local pollution,but weak cold air masses(ΔT24h4°C)reduced the PM_(2.5) concentration whereas weaker winds(∣V∣_(average)<2 m s^(−1))increased it;and(4)PM_(2.5) concentration decreased sharply within 4 h after the passage of strong cold air masses,but more gradually within 14 h after the passage of strong warm air *** results considerably improve the current understanding of the influence of cold and warm air masses on local pollution patterns.

关键词： weather type air mass enhancement removal meteorological condition

Laser‑Induced and MOF‑Derived Metal Ox.de/Carbon Composite for Synergistically Improved Ethanol Sensing at Room temperature

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Nano-Micro Letters 2024年第6期16卷 210-220页

作者： Hyeongtae Lim Hyeokjin Kwon Hongki kang Jae Eun Jang Hyuk‑Jun Kwon Department of Electrical Engineering and Computer Science DGISTDaegu 42988South Korea Convergence Research Advanced Centre for Olfaction DGISTDaegu 42988South Korea

Advancements in sensor technology have significantly enhanced atmospheric ***,metal ox.de and carbon(MO_(x./C)hybrids have gained attention for their ex.eptional sensitivity and room-temperature sensing ***,previous methods of synthesizing MO_(x./C composites suffer from problems,including inhomogeneity,aggregation,and challenges in ***,we introduce a refined method that employs a metal–organic framework(MOF)as a precursor combined with direct laser *** inherent structure of MOFs ensures a uniform distribution of metal ions and organic linkers,yielding homogeneous MO_(x./C *** laser processing facilitates precise micropatterning(x./C *** optimized MOF-derived MO_(x./C sensor rapidly detected ethanol gas even at room temperature(105 and 18 s for response and recovery,respectively),with a broad range of sensing performance from 170 to 3,400 ppm and a high response value of up to 3,500%.Additionally,this sensor ex.ibited enhanced stability and thermal resilience compared to previous MOF-based *** research opens up promising avenues for practical applications in MOF-derived sensing devices.

关键词： Metal-organic frameworks Metal ox.de Carbon composite Laser Gas sensor

Effects of long-term fencing on soil microbial community structure and function in the desert steppe,China

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Journal of Arid Land 2024年第3期16卷 431-446页

作者： PAN Yaqing kang Peng QU x.an RAN Yichao LI x.nrong Shapotou Desert Research and Ex.eriment Station Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China School of Biological Science and Engineering North Minzu UniversityYinchuan 750021China

One of the goals of grazing management in the desert steppe is to improve its ***,relatively little is known about soil microbe communities in the desert steppe ecosystem under grazing *** this study,we investigated the diversity and aboveground biomass of Caragana korshinskii *** communities in long-term fencing and grazing areas,combined with an analysis of soil physical-chemical properties and genomics,with the aim of understanding how fence management affects plant-soil-microbial inter-relationships in the desert steppe,*** results showed that fence management(ex.losure)increased plant diversity and aboveground biomass in *** shrub area and effectively enhanced soil organic carbon(233.94%),available nitrogen(87.77%),and available phosphorus(53.67%)*** well,the Shannon indices of soil bacteria and fungi were greater in the fenced ***-soil changes profoundly affected the alpha-and beta-diversity of soil *** management also altered the soil microbial community structure,significantly increasing the relative abundances of Acidobacteriota(5.31%-8.99%),Chloroflex.(3.99%-5.58%),and Glomeromycota(1.37%-3.28%).The soil bacterial-fungal co-occurrence networks under fence management had higher complex.ty and *** on functional predictions,fence management significantly increased the relative abundance of bacteria with nitrification and nitrate reduction functions and decreased the relative abundance of bacteria with nitrate and nitrite respiration *** relative abundances of ecologically functional fungi with arbuscular mycorrhizal fungi,ectomycorrhizal fungi,and saprotrophs also significantly increased under fence *** addition,the differential functional groups of bacteria and fungi were closely related to plant-soil *** results of this study have significant positive implications for the ecological restoration and reconstruction of dry desert steppe and simila

关键词： desert steppe fence management Caragana korshinskii soil physical-chemical property soil microorganism

Numerical modeling of fracture propagation of supercritical CO_(2)compound fracturing

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第7期16卷 2607-2628页

作者： Hao Chen Yong kang Wanchun Jin Changhai Li Can Cai School of Mechanical Engineering Southwest Petroleum UniversityChengdu610500China Laboratory of High-pressure Jet Theory and Application Technology Southwest Petroleum UniversityChengdu610500China Hubei Key Laboratory of Waterjet Theory and New Technology Wuhan UniversityWuhan430072China Sinopec International Petroleum Ex.loration and Production Corporation Beijing 100029China

The ex.loitation of shale gas is promising due to depletion of the conventional energy and intensification of the greenhouse *** this paper,we proposed a heat-fluid-solid coupling damage model of supercritical CO_(2)(SC-CO_(2))compound fracturing which is ex.ected to be an efficient and environmentally friendly way to develop shale *** coupling model is solved by the finite element method,and the results are in good agreement with the analytical solutions and fracturing *** on this model,the fracture propagation characteristics at the two stages of compound fracturing are studied and the influence of pressurization rate,in situ stress,bedding angle,and other factors are *** results show that at the SC-CO_(2)fracturing stage,a lower pressurization rate is conducive to formation of the branches around main fractures,while a higher pressurization rate inhibits formation of the branches around main fractures and promotes formation of the main *** bedding and in situ stress play a dominant role in the fracture *** the in situ stress ratio(δ_(x./δ_(y))is 1,the presence of bedding can reduce the initiation pressure and failure ***,it will cause the fracture to propagate along the bedding direction,reducing the fracture *** rocks without bedding,hydraulic fracturing has the lengthening and widening effects for SC-CO_(2)induced *** shale,fractures induced at the hydraulic fracturing stage are more likely to be dominated by in situ stresses and have a shorter reorientation ***,fracture branches propagating along the max.mum principal stress direction may be generated around the main fractures induced by SC-CO_(2)at the hydraulic fracturing *** the branches converge with the main fractures,fracture zones are easily formed,and thus the fracture complex.ty and damage area can be significantly *** results are instructive for the design and application of SC

关键词： Compound fracturing Fracture propagation Finite element method Damage evolution

Broadband Dual-Input Doherty Power Amplifier Design Based on a Simple Adaptive Power Dividing Ratio Function

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China Communications 2024年第5期21卷 97-112页

作者： Dai Zhijiang Zhong kang Li Mingyu Pang Jingzhou Jin Yi School of Microelectronics and Communication Engineering Chongqing UniversityChongqing 400044China x.’an Branch of China Academy of Space Technology Xi’an 710100China

In this paper,a simple adaptive power dividing function for the design of a dual-input Doherty power amplifier(DPA)is *** the presented approaches,the signal separation function(SSF)at different frequency points can be characterized by a *** in the practical test,the coefficients of SSF can be determined by measuring a small number of data points of input *** as other dualinput DPAs,the proposed approach can also achieve high output power and back-off efficiency in a broadband operation band by adjusting the power distribution ratio ***,a 1.5-2.5 GHz highefficiency dual-input Doherty power amplifier is implemented according to this *** test results show that the peak power is 48.6-49.7d Bm,and the 6-d B back-off efficiency is 51.0-67.0%,and the saturation efficiency is 52.4-74.6%.The digital predistortion correction is carried out at the frequency points of 1.8/2.1GHz,and the adjacent channel power ratio is lower than-54.5d *** and ex.eriment results can verify the effectiveness and correctness of the proposed method.

关键词： broadband doherty power amplifier dualinput efficiency enhancement load modulation

Alterations of soil aggregates and intra-aggregate organic carbon fractions after soil conversion from paddy soils to upland soils:Distribution,mineralization and driving mechanism

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Pedosphere 2024年第1期34卷 121-135页

作者： Longfei kang Jiamei WU Chunfeng ZHANG Baoguo ZHU Guix.n CHU College of Life Science Shaoxing UniversityShaoxing 312000China The Key Laboratory of Oasis Eco-agriculture Xinjiang Production and Construction Group/Department of Resources and Environmental SciencesAgronomy CollegeShihezi UniversityShihezi 832000China Hunan Institute of Agricultural Environment and Ecology Changsha 410000China Jiamusi Branch Heilongjiang Academy of Agricultural SciencesJiamusi 154007China

Investigating the impacts of soil conversion on soil organic carbon(OC) content and its fractions within soil aggregates is essential for defining better strategies to improve soil structure and OC sequestration in terrestrial ecosystems. However, the consequences of soil conversion from paddy soil to upland soil for soil aggregates and intra-aggregate OC pools are poorly understood. Therefore, the objective of this study was to quantify the effects of soil conversion on soil aggregate and intra-aggregate OC pool distributions. Four typical rice-producing areas were chosen in North and South China, paired soil samples(upland soil converted from paddy soil more than ten years ago vs. adjacent paddy soil) were collected(0–20 cm) with three replicates in each area. A set of core parameters(OC preservation capacity, aggregate carbon(C) turnover, and biological activity index. were evaluated to assess the responses of intra-aggregate OC turnover to soil conversion. Results showed that soil conversion from paddy soil to upland soil significantly improved the formation of macro-aggregates and increased aggregate stability. It also notably decreased soil intra-aggregate OC pools, including easily ox.dized OCa(EOCa), particulate OCa(POCa), and mineral-bound(MOCa) OC, and the sensitivity of aggregate-associated OC pools to soil conversion followed the order: EOCa(average reduction of 21.1%) > MOCa(average reduction of 15.4%) > POCa(average reduction of 14.8%). The potentially mineralizable C(C_(0)) was significantly higher in upland soil than in paddy soil, but the corresponding decay constant(k) was lower in upland soil than in paddy soil. Random forest model and partial correlation analysis showed that EOCa and pH were the important nutrient and physicochemical factors impacting k of C mineralization in paddy soil,while MOCa and C-related enzyme(β-D-cellobiohydrolase) were identified as the key factors in upland soil. In conclusion, this study evidenced that soil conversion

关键词： decay constant easily ox.dized organic C macro-aggregate meso-aggregate micro-aggregate mineral-bound organic C particulate organic C potentially mineralizable C

Transfer matrix.method for free and forced vibrations of multi-level functionally graded material stepped beams with different boundary conditions

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Applied Mathematics and Mechanics(English Edition) 2024年第6期45卷 983-1000页

作者： x.aoyang SU Tong HU Wei ZHANG Houjun kang Yunyue CONG Quan YUAN School of Civil Engineering and Architecture Guangxi UniversityNanning 530004China Scientific Research Center of Engineering Mechanics Guangxi UniversityNanning 530004China State Key Laboratory of Featured Metal Materials and Life-Cycle Safety for Composite Structures Guangxi UniversityNanning 530004China

Functionally graded materials(FGMs)are a novel class of composite materials that have attracted significant attention in the field of engineering due to their unique mechanical *** study aims to ex.lore the dynamic behaviors of an FGM stepped beam with different boundary conditions based on an efficient solving *** the assumptions of the Euler-Bernoulli beam theory,the governing differential equations of an individual FGM beam are derived with Hamilton’s principle and decoupled via the separation-of-variable ***,the free and forced vibrations of the FGM stepped beam are solved with the transfer matrix.method(TMM).Two models,i.e.,a three-level FGM stepped beam and a five-level FGM stepped beam,are considered,and their natural frequencies and mode shapes are *** demonstrate the validity of the method in this paper,the simulation results by ABAQUS are also *** this basis,the detailed parametric analyses on the frequencies and dynamic responses of the three-level FGM stepped beam are carried *** results show the accuracy and efficiency of the TMM.

关键词： transfer matrix.method(TMM) free vibration forced vibration functionally graded material(FGM) stepped beam

Enhancing leaching efficiency of ion adsorption rare earths by ameliorating mass transfer effect of rare earth ions by applying an electric field

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Journal of Rare Earths 2024年第1期42卷 172-180,I0006页

作者： Lingbo Zhou Jie Yang Shijie kang x.aojun Wang Hongdong Yu Yinhua Wan Rare Earth Institute University of Science and Technology of ChinaHefei230000China Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou341000China Jiangx. Institute of Rare Earths Chinese Academy of SciencesGanzhou341000China School of Resources and Environment Engineering Jiangxi University of Science and TechnologyGanzhou341000China

Improving the seepage of leaching solution in the ore body and strengthening the mass transfer process of rare earth ions during in-situ leaching are two critical methods to improve the leaching efficiency of rare *** this study,2 wt%MgSO_(4)solution was used for the indoor simulated column leaching ex.eriment on rare earth samples and an electric field was applied at both ends of the *** the effects of different intensities,initial application time and duration of the electric field on the rare earth leaching system and its mechanism were *** results show that compared with the single MgSO_(4)solution leaching,applying an electric field with a strength of 6 V/cm can save the leaching time of 30 min and increase the flow velocity of the rare earth leachate by 26.98%.Under the optimal conditions of applying an electric field with a strength of 6 V/cm for 20 min to the leaching system after10 min of the rare earth leachate flowing out,the leaching efficiency of sample increases from 81.20% to 86.05% with the increase of 4.85%.The mechanism analysis shows that when a direct current electric field is applied to the rare earth leaching system,rare earth ions rapidly change from disorderly movement with the seepage into faster and directional *** addition,the seepage of the leaching solution is also improved due to the increase of the cross-sectional area of the seepage channel,the polarized water molecules migrate directionally by force from the negative pole,and the movement of the hydrogen is generated by the electrolytic *** impo rtantly,based on the principle of in-situ leaching process,the layout of injection holes and deflector holes in this process provides a natural site for the electrode layout of the electric *** the simple equipme nt and the ope ration,the rare earth leaching process with the applied electric field has high feasibility in industrial application.

关键词： Ion adsorption rare earths Leaching system Electric field Mass transfer process Seepage

On-surface synthesis and characterization of polyynic carbon chains

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National Science Review 2024年第3期11卷 192-199页

作者： Wenze Gao Wei Zheng Luye Sun Faming kang Zheng Zhou Wei x. Interdisciplinary Materials Research Center School of Materials Science and Engineering Tongji University

Carbyne, an elusive sp-hybridized linear carbon allotrope, has fascinated chemists and physicists for decades. Due to its high chemical reactivity and ex.reme instability, carbyne was much less ex.lored in contrast to the sp2-hybridized carbon allotropes such as graphene. Herein, we report the on-surface synthesis of polyynic carbon chains by demetallization of organometallic polyynes on the Au（111） surface;the longest one observed consists of ～60 alkyne units（120 carbon atoms）. The polyynic structure of carbon chains with alternating triple and single bonds was unambiguously revealed by bond-resolved atomic force microscopy. Moreover, an atomically precise polyyne, C14, was successfully produced via tip-induced dehalogenation and ring-opening of the decachloroanthracene molecule(C14Cl10) on a bilayer NaCl/Au（111） surface at 4.7 K, and a band gap of 5.8 eV was measured by scanning tunnelling spectroscopy,in a good agreement with the theoretical HOMO–LUMO gap（5.48 eV）.

关键词： polyyne scanning probe microscopy carbon allotrope on-surface synthesis organometallic polyyne