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Amorphous Sb/C composite with isotropic expansion property as an ultra-stable and high-rate anode for lithium-ion batteries

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Rare Metals 2024年第5期43卷 2039-2052页

作者： Ze-Zhou Yang Cheng-Yi Zhang Yu-Qing Ou Zhi-kang Su Yan Zhao Heng-jiang Cong Xin-Ping Ai jiang-Feng Qian Hubei Key Laboratory of Electrochemical Power Sources College of Chemistry and Molecular SciencesWuhan UniversityWuhan430072China Institute of Technological Sciences Wuhan UniversityWuhan 430072China

Antimony(Sb)is an intriguing anode material for Li-ion batteries(LIBs)owing to its high theoretical capacity of 660 m Ah·g^(-1)and appropriate working potential of~0.8 V(***^(+)/Li).However,just like all alloying materials,the Sb anode suffers from huge volume expansion(230%)during repeated insertion/extraction of Li+ions,resulting in structural deterioration and rapid capacity *** this work,a novel amorphous Sb/C composite with atomically dispersed Sb particles in carbon matrix is prepared via a straightforward high-energy ball milling *** intimate intermixing of amorphous Sb with C provides homogeneous element distribution and isotropic volume expansion during cycling,resulting in persistent structural ***,the disordered structure of amorphous material shortens the diffusion distance of lithium ions/electrons,promoting fast reaction kinetics and rate *** from the aforementioned effects,the amorphous Sb/C exhibits a high reversible capacity of537.4 m Ah·g^(-1)at 0.1 A·g^(-1)and retains 201.0 m Ah·g^(-1)at an ultrahigh current rate of 10.0 A·g^(-1).Even after 1500deep cycles at 2.0 A·g^(-1),the amorphous Sb/C electrode still maintains 86.3%of its initial capacity,which outperforms all existing Sb-based anodes reported so *** analysis further reveals a greatly reduced volume variation of merely 34.6%for the amorphous Sb/C electrode,much lower than that of 223.1%for crystalline Sb *** study presents a new approach to stabilizing Sb-based alloy anodes and contributes to the construction of high-performance amorphous anode materials for LIBs,enabling advanced energy storage.

关键词： Amorphous Sb/C anode Homogeneous element distribution Isotropic volume expansion Ultra-long cycle stability High-rate capability Lithium-ion battery

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Recovery and in-situ reduction of precious metals by graphdiyne and graphdiyne oxide for antibacterial use

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Rare Metals 2024年第4期43卷 1747-1757页

作者： Ming-Ji jiang Ya-Na Zhang Ling-Shen Meng Jing kang Yong-Jun Li Alideertu Dong College of Chemistry and Chemical Engineering Inner Mongolia UniversityHohhot010021China Engineering Research Center of Dairy Quality and Safety Control Technology Ministry of EducationInner Mongolia UniversityHohhot010021China Department of Chemistry University of ZurichCH-8057ZurichSwitzerland Laboratory of Organic Solids and Beijing National Laboratory for Molecular Sciences Institute of ChemistryChinese Academy of SciencesBeijing100190China

Based on the in-situ self-reduction and chemical stability,graphdiyne(GDY)and graphdiyne oxide(GDYO)are used as trapping agents to investigate the ability for recovering Au^(3+),Ag^+,and Pd^(2+)under different pH values and interfering *** strong acidity at pH=1,these two agents demonstrate high select recovery towards the three precious metal ions,which could be insitu reduced to nanoparticles(NPs).In addition,superparamagnetic Fe_(3)O_(4)NPs are deposited on the surfaces of GDY and *** magnetic responses enable GDYFe_(3)O_(4)to recover precious metals conveniently and efficiently by the aid of an external magnetic *** study also confirms the antibacterial activity of the as-recovered NPs deposited on GDY and GDYO against Escherichia coli and Staphylococcus aureus(1×10^(5)colony-forming unit(CFU)·mL^(-1)),and the antibacterial rates are 100%.This strategy of recovering precious metals and subsequently reusing to combat pathogens will be of great significance for environmental remediation and biomedical applications.

关键词： Graphdiyne In-situ reduction Recovery Precious metals Antibacterial

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浅析老旧车间工艺改造后的涂装外观提升

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现代涂料与涂装 2024年第2期27卷 52-54页

作者：曹裕清许龙康子江王晓东仲兆婷东风本田汽车有限公司

通过对东风本田汽车一厂各车型腰线部位外观较差问题进行简单分析，从底材、涂料、喷涂参数等方面阐释影响外观的原因，并对涂装老旧设备改造及新工艺导入等影响因素进行相关验证，以期为老旧线体外观提升及老旧设备改造和新工艺导入优... 详细信息

通过对东风本田汽车一厂各车型腰线部位外观较差问题进行简单分析，从底材、涂料、喷涂参数等方面阐释影响外观的原因，并对涂装老旧设备改造及新工艺导入等影响因素进行相关验证，以期为老旧线体外观提升及老旧设备改造和新工艺导入优化提供理论依据及参考。

关键词：外观提升设备改造工艺导入材料改良

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Design of Novel Compact Electromagnetic Bandgap Structures with Enhanced Bandwidth

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Journal of Electronic Science and Technology 2010年第3期8卷 262-266页

作者： Ping jiang kang Xie with School of Optoelectronic Information University of Electronic Science and Technology of China Chengdu 610054 China

Two kinds of compact electromagnetic band gap （EBG） structures are designed. A two layer compact EBG structure configured with cross spiral shape line inductors and interdigital capacitors is first presented. Because of its significantly enlarged equivalent inductor and capacitance, the period of the lattice is approximately 4.5% of the free space wavelength. By insetting several narrow slits in the ground plane, the bandwidth of the main bandgap is enhanced by nearly 19%. Further effort has been made for designing a three layer compact EBG structure. Simulation results show that its period is reduced by about 26% compared to that of proposed two layer EBG structure, and the bandwidth of the main bandgap is about 3 times as that of the proposed two layer EBG structure. The detailed designs including a two layer compact 3×7 EBG array with and without defect ground plane and the three layer EBG array are given and simulation results are presented.

关键词： Defect ground electromagnetic band gap high surface surface wave. structure impedance,

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Discovery of GluN2A subtype-selective N-methyl-d-aspartate(NMDA)receptor ligands

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Acta Pharmaceutica Sinica B 2024年第5期14卷 1987-2005页

作者： Liyang jiang Na Liu Fabao Zhao Boshi Huang Dongwei kang Peng Zhan Xinyong Liu Department of Medicinal Chemistry Key Laboratory of Chemical Biology(Ministry of Education)School of Pharmaceutical SciencesCheeloo College of MedicineShandong UniversityJinan 250012China

The N-methyl-d-aspartate(NMDA)receptors,which belong to the ionotropic Glutamate receptors,constitute a family of ligand-gated ion *** the various subtypes of NMDA receptors,the GluN1/2A subtype plays a significant role in central nervous system(CNS)*** present article aims to provide a comprehensive review of ligands targeting GluN2A-containing NMDA receptors,encompassing negative allosteric modulators(NAMs),positive allosteric modulators(PAMs)and competitive ***,the ligands’structure–activity relationships(SARs)and the binding models of representative ligands are also discussed,providing valuable insights for the clinical rational design of effective drugs targeting CNS diseases.

关键词： NMDA receptors GluN2A subtype Subtype-selective ligands SARs Protein ligand interactions

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Two Monte Carlo-based simulators for imaging-system modeling and projection simulation of flat-panel X-ray source

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Nuclear Science and Techniques 2024年第7期35卷 31-46页

作者： Meng-Ke Qi Ting He Yi-Wen Zhou Jing kang Zeng-Xiang Pan Song kang Wang-jiang Wu Jun Chen Ling-Hong Zhou Yuan Xu School of Biomedical Engineering Southern Medical UniversityGuangzhou510515China State Key Laboratory of Optoelectronic Materials and Technologies Guangdong Province Key Laboratory of Display Material and TechnologySchool of Electronics and Information TechnologySun Yat-sen UniversityGuangzhou510275China Department of Radiotherapy Guangdong Provincial People’s Hospital(Guangdong Academy of Medical Sciences)Southern Medical UniversityGuangzhou510515China

The advantages of a flat-panel X-ray source(FPXS)make it a promising candidate for imaging *** imaging-system modeling and projection simulation are critical for analyzing imaging performance and resolving overlapping projection issues in *** conventional analytical ray-tracing approach is limited by the number of patterns and is not applicable to FPXS-projection ***,the computation time of Monte Carlo(MC)simulation is independent of the size of the patterned arrays in *** study proposes two high-efficiency MC projection simulators for FPXS:a graphics processing unit(GPU)-based phase-space sampling MC(gPSMC)simulator and GPU-based fluence sampling MC(gFSMC)*** two simulators comprise three components:imaging-system modeling,photon initialization,and physical-interaction simulations in the ***-system modeling was performed by modeling the FPXS,imaging geometry,and *** gPSMC simulator samples the initial photons from the phase space,whereas the gFSMC simulator performs photon initialization from the calculated energy spectrum and fluence *** entire process of photon interaction with the geometry and arrival at the detector was simulated in parallel using multiple GPU kernels,and projections based on the two simulators were *** accuracies of the two simulators were evaluated by comparing them with the conventional analytical ray-tracing approach and acquired projections,and the efficiencies were evaluated by comparing the computation *** results of simulated and realistic experiments illustrate the accuracy and efficiency of the proposed gPSMC and gFSMC simulators in the projection calculation of various phantoms.

关键词： Flat-panel X-ray source(FPXS) Imaging-system modeling Projection simulation Monte Carlo-based simulators

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新疆天山南北两侧大型叠合盆地石炭纪的连通性

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中南大学学报（自然科学版） 2009年第4期40卷 1139-1145页

作者：康德江大庆油田有限责任公司勘探开发研究院黑龙江大庆163712

对新疆天山南北两侧的大型复杂叠合盆地经过综合整理、分析地化、地球物理和古生物等发现,由于双峰式岩系、含强不相容元素的玄武岩存在,以及航磁异常,推测准噶尔盆地的基底性质应该属于陆壳或以陆壳为主体,其年代应该至少不晚于前寒武... 详细信息

对新疆天山南北两侧的大型复杂叠合盆地经过综合整理、分析地化、地球物理和古生物等发现,由于双峰式岩系、含强不相容元素的玄武岩存在,以及航磁异常,推测准噶尔盆地的基底性质应该属于陆壳或以陆壳为主体,其年代应该至少不晚于前寒武纪。结合巨厚的中石炭统沉积、深水耕作迹的存在以及古地貌的变迁等证据,推测准噶尔盆地在石炭纪应该是与塔里木等周边盆地大体相连,两者至少在石炭纪时期是相互联通的,具有相似的沉积环境,应该具有较类似的沉积物质基础。综合考虑油气成藏要素可知,噶尔盆地石炭系地层能够具有与塔里木盆地石炭系相近的生烃能力,具有较强的生排烃及储集能力,油气蕴藏潜力巨大,可以作为深层油气勘探的潜在接替层位。

关键词：叠合盆地石炭系连通性基底准噶尔盆地

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Lignin‐derived carbon with pyridine N‐B doping and a nanosandwich structure for high and stable lithium storage

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Carbon Energy 2024年第8期6卷 232-247页

作者： Dichao Wu Jiayuan Li Yuying Zhao Ao Wang Gaoyue Zhang Jianchun jiang Mengmeng Fan kang Sun Key Lab of Biomass Energy and Material Jiangsu ProvinceNational Engineering Lab for Biomass Chemical UtilizationKey and Open Lab on Forest Chemical EngineeringSFAInstitute of Chemical Industry of Forest ProductsChinese Academy of ForestryNanjingChina jiangsu Co‐Innovation Center of Efficient Processing and Utilization of Forest Resources International Innovation Center for Forest Chemicals and MaterialsCollege of Chemical EngineeringNanjing Forestry UniversityNanjingChina School of Energy and Environment Southeast UniversityNanjingChina Department of Chemistry Tsinghua UniversityBeijingChina Fujian Provincial Key Laboratory of Biomass Low‐Carbon Conversion Academy of Advanced Carbon Conversion TechnologyHuaqiao UniversityXiamenChina Chinese Academy of Sciences Xinjiang Lihua Institute of Technology UrumqiChina

Biomass‐derived carbon is a promising electrode material in energy storage ***,how to improve its low capacity and stability,and slow diffusion kinetics during lithium storage remains a *** this research,we propose a“self‐assembly‐template”method to prepare B,N codoped porous carbon(BN‐C)with a nanosandwich structure and abundant pyridinic N‐B *** nanosandwich structure can increase powder density and cycle stability by constructing a stable solid electrolyte interphase film,shortening the Li^(+)diffusion pathway,and accommodating volume expansion during repeated charging/*** abundant pyridinic N‐B species can simultaneously promote the adsorption/desorption of Li^(+)/PF_(6)^(−)and reduce the diffusion *** BN‐C electrode showed a high lithium‐ion storage capacity of above 1140 mAh g^(−1)at 0.05 A g^(−1)and superior stability(96.5%retained after 2000 cycles).Moreover,owing to the synergistic effect of the nanosandwich structure and pyridinic N‐B species,the assembled symmetrical BN‐C//BN‐C full cell shows a high energy density of 234.7Wh kg^(−1),high power density of 39.38 kW kg−1,and excellent cycling stability,superior to most of the other cells reported in the *** the density functional theory simulation demonstrated,pyridinic N‐B shows enhanced adsorption activity for Li^(+)and PF_(6)^(−),which promotes an increase in the capacity of the anode and cathode,***,the relatively lower diffusion barrier of pyridinic N‐B promotes Li^(+)migration,resulting in good rate ***,this study provides a new approach for the synergistic modulation of a nanostructure and an active site simultaneously to fabricate the carbon electrode material in energy storage devices.

关键词： high cycling stability high energy density lithium‐ion batteries pyridinic N‐B species sandwich structure carbon nanosheet

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Investigation of pore structure alteration and permeability enhancement of shale matrix by supercritical water treatment after hydraulic fracturing

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Petroleum 2024年第2期10卷 265-274页

作者： Yili kang Peisong Li Wangkun Cao Mingjun Chen Lijun You jiang Liu Zhehan Lai State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum University Institute of Engineering Technology PetroChina Coalbed Methane Company Limited Chemical and Petroleum Engineering University of Calgary

Shale gas reservoirs are unconventional tight gas reservoirs, in which horizontal wells and hydraulic fracturing are required to achieve commercial development. The fracture networks created by hydraulic fracturing can increase the drainage area extensively to enhance shale gas recovery. However, large volumes of fracturing fluid that is difficult to flow back to the surface and remained in the shale formation, will inevitably lead to damages of the shale formations and limit the effectiveness of *** water(SCW) treatment after hydraulic fracturing is a new method to enhance shale gas recovery by using appropriate heat treatment methods to the specific formation to convert the retained fracturing fluid into a supercritical state(at temperatures in excess of 373.946°C and pressures in excess of 22.064 MPa). An experiment was conducted to simulate the reaction between shale and SCW, and the capacity of SCW treatment to enhance the permeability of the shale was evaluated by measuring the response of the shale porosity and permeability on SCW treatment. The experimental results show that the shale porosity and permeability increase by 213.43% and 2198.37%, respectively. The pore structure alteration and permeability enhancement of the shale matrix were determined by analyzing the changes in pore structure and mineral composition after SCW treatment. The mechanisms that affect pore structure and mineral composition include oxidative catalysis decomposition of organic matters and reducing minerals, acid-catalyzed decomposition of carbonate minerals and feldspar minerals, hydrothermal catalysis induced fracture extension and cementation weakening induced fracture *** treatment converts harm into a benefit by reducing the intrusion of harmful substances into the shale formation, which will broaden the scope and scale of shale formation stimulation.

关键词： Shale gas Formation damage control Formation heat treatment Supercritical water

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Spatiotemporal variations in glacier area and surface velocity of the northern Antarctic Peninsula during 2018-2022

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Advances in Climate Change Research 2024年第2期15卷 297-311页

作者： Yu-Long kang Shi-Chang kang Wan-Qin GUO Tao CHE Zong-Li jiang Zhen-Feng WANG Qiang-Qiang XU Cheng-De YANG State Key Laboratory of Cryospheric Science Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China University of Chinese Academy of Sciences Beijing 100083China Key Laboratory of Remote Sensing of Gansu Province Northwest Institute of Eco-Environment and ResourcesChinese Academy of SciencesLanzhou 730000China School of Earth Sciences and Spatial Information Engineering Hunan University of Science and TechnologyXiangtan 411201China

Ice sheet serves as a crucial indicator for assessing climate *** loss in recent remote sensing-based studies indicated that the Antarctic Peninsula has rapid rates of glacier retreat and speed up of surface ***,observations of seasonal variability of ice speed are limited,and glacier-area changes require multi-temporal *** study investigated the changes in area and surface velocities of∼375 glaciers on the northern Antarctic Peninsula(NAP)utilizing satellite images acquired by the Sentinel 1&2 satellites during *** results indicate that the glacier area reduced by approximately 166.1±44.2 km^(2)(-0.2%±0.1%per year)during the study period,with an acceleration after 2020(-0.4%±0.3%per year),and the most dramatic reduction happened on the eastern *** maximum annual ice speeds on the NAP generally exceeded 3500 m per year,while the ice speeds in 2021 were the highest(exceeded 4210 m per year).The ice speed variability in austral autumn was higher than in other seasons,meanwhile the summer ice speeds showed an increasing *** glacier G012158E47018N,McNeile Glacier,glacier G299637E64094S and Drygalski Glacier showed the most remarkable ice speed variations represented by high daily velocities and strong fluctuations on their *** results demonstrated that the variations in glacier area and seasonal ice speed on the NAP were responsive to the ice-ocean-atmosphere ***,seasonal velocity and area variations should be considered when conducting accurate mass balance calculations,model validations and change mechanism analyses under climate warming scenarios.

关键词： Glacier area Seasonal ice speed Sentinel 1&2 Northern Antarctic Peninsula Ice-ocean-atmosphere processes

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