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Trivalent Ni oxidation controlled through regulating lithium content to minimize perovskite interfacial recombination

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Rare Metals 2022年第1期41卷 96-105页

作者： Jin-Jin Zhao Xiao Su Zhou Mi Ying Zhang Yan-jun Hu hua-jun guo Yi-Nan Jiao Yu-Xia Zhang Yan Shi Wei-Zhong Hao Jing-Wei Wu Yi Wang Cun-Fa Gao guo-Zhong Cao School of Materials Science and Engineering School of Mechanical EngineeringShijiazhuang Tiedao UniversityShijiazhuang 050043China School of Materials Science and Engineering Hebei Key Laboratory of Material Near Net Forming TechnologyHebei University of Science and TechnologyShijiazhuang 050018China State Key Laboratory of Mechanics and Control of Mechanical Structures Nanjing University of Aeronautics and AstronauticsNanjing 210016China Department of Materials Science and Engineering University of WashingtonSeattleWA 98195-2120USA

Organic–inorganic hybrid perovskite solar cells,one of the most promising photovoltaic devices,have made great progress in their efficiency and preparation technology.In this study,uniform,highly conductive Li_(n)NiO... 详细信息

关键词： Lithium ions Ni^(3+) Oxidized defect Photocurrent Perovskite solar cells

A remote sensing system of vehicle emissions based on tunable diode laser technology

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Journal of Environmental Sciences 2006年第1期18卷 154-157页

作者： ZENG jun guo hua-fang HU Yue-ming College of Automation Science and Engineering South China University of Technology Guangzhou 510640 China

As being an effective real-time method of monitoring vehicle emissions on-road, a remote sensing system based on the tunable diode laser （TDL） technology was presented, and the key technologies were discussed. A field test in Guangzhou（Guangdong, China） was performed and was found that the factors, such as slope, instantaneous speed and acceleration, had significant influence on the detectable rate of the system. Based on the results, the proposal choice of testing site was presented.

关键词： remote sensing tunable diode laser vehicle emission detectable rate

Towards fully automatic modelling of the fracture process in quasi-brittle and ductile materials:a unified crack growth criterion

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Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2008年第7期9卷 867-877页

作者： Zhen-jun YANG guo-hua LIU College of Civil Engineering and Architecture Zhejiang University Hangzhou 310027 China

Fully automatic finite element(FE) modelling of the fracture process in quasi-brittle materials such as concrete and rocks and ductile materials such as metals and alloys,is of great significance in assessing structural integrity and presents tre-mendous challenges to the engineering community. One challenge lies in the adoption of an objective and effective crack propagation criterion. This paper proposes a crack propagation criterion based on the principle of energy conservation and the cohesive zone model(CZM) . The virtual crack extension technique is used to calculate the differential terms in the criterion. A fully-automatic discrete crack modelling methodology,integrating the developed criterion,the CZM to model the crack,a simple remeshing procedure to accommodate crack propagation,the J2 flow theory implemented within the incremental plasticity framework to model the ductile materials,and a local arc-length solver to the nonlinear equation system,is developed and im-plemented in an in-house program. Three examples,i.e.,a plain concrete beam with a single shear crack,a reinforced concrete(RC) beam with multiple cracks and a compact-tension steel specimen,are simulated. Good agreement between numerical predictions and experimental data is found,which demonstrates the applicability of the criterion to both quasi-brittle and ductile materials.

关键词：韧性材料易碎材料裂纹发展有限元法

Emergence of SARS and COVID-19 and preparedness for the next emerging disease X

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Frontiers of Medicine 2024年第1期18卷 1-18页

作者： Ben Hu hua guo Haorui Si Zhengli Shi CAS Key Laboratory of Special Pathogens and Biosafety Wuhan Institute of VirologyChinese Academy of SciencesWuhan430071China University of Chinese Academy of Sciences Beijing100049China

Severe acute respiratory syndrome(SARS)and Coronavirus disease 2019(COVID-19)are two human Coronavirus diseases emerging in this century,posing tremendous threats to public health and causing great loss to lives and economy.In this review,we retrospect the studies tracing the molecular evolution of SARS-CoV,and we sort out current research findings about the potential ancestor of SARS-CoV-2.Updated knowledge about SARS-CoV-2-like viruses found in wildlife,the animal susceptibility to SARS-CoV-2,as well as the interspecies transmission risk of SARS-related coronaviruses(SARSr-CoVs)are gathered here.Finally,we discuss the strategies of how to be prepared against future outbreaks of emerging or re-emerging coronaviruses.

关键词： SARS COVID-19 coronavirus

Insights into photocatalytic mechanism over a novel Cu2WS4/MoS2 S-scheme heterojunction

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Rare Metals 2024年第7期43卷 3118-3133页

作者： Wei Zhao Ji-Hui Cao jun-Jie Liao Yun Liu Xiao-jun Zeng jun-Yu Shen Xue-Kun Hong Yang guo He-hua Zeng Ya-Zi Liu School of Materials Engineering Jiangsu Key Laboratory of Advanced Functional MaterialsSchool of Electronic and Information EngineeringChangshu Institute of Technology School of Chemistry and Chemical Engineering Changji University State Environmental Protection Key Laboratory of Soil Environmental Management and Pollution Control Ministry of Ecology and EnvironmentNanjing Institute of Environmental Sciences School of Environment Jiangsu Engineering Lab of Water and Soil Eco-RemediationNanjing Normal University Department of Chemical Engineering Curtin University

A novel efficient Cu2WS4/MoS2step-scheme（S-scheme） heterojunction photocatalyst was constructed for the first time and applied in the removal of environmental pollutants.Among the as-prepared photocatalysts,the Cu2WS4/MoS2-8 % heterojunc tion photoc atalyst demonstrates the optimal photocatalytic performance,with the catalytic oxidation efficiency of tetracycline（TC） and the catalytic reduction efficiency of Cr6+reaching 93.3%and 82.1 %,respectively.The excellent catalytic properties of Cu2WS4/MoS2heterojunction photocatalysts are attributed to the effective separation pathways of charges and the presence of S-scheme heterojunctions,together with stronger redox capabilities.It is speculated that the photogenerated carrier migration path of the Cu2WS4/MoS2catalyst follows the typical S-scheme photocatalytic mechanism,which is verified by the in-depth experimental study and simulated calculations including the electron paramagnetic resonance（EPR） analysis,free radical quenching experiments,charge density distribution,and simulated built-in electric field formation at the interface,which acts as driving force to promote the separation of photoinduced electrons and holes.Finally,the photocatalytic mechanism of S-scheme photogenerated carrier migration for the Cu2WS4/MoS2catalyst is revealed based on the systematic experimental techniques and simulated calculations,accounting for its superior photocatalytic oxidation and reduction activities.This study provides inspiring implications to develop high-efficient S-scheme photocatalytic systems for versatile applications in solarenergy conversion.

关键词： Cu 2 WS 4 /MoS 2 S-scheme Heterojunction Photocatalysis

Electrochemical anodic oxidation assisted fabrication of memristors

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International Journal of Extreme Manufacturing 2024年第3期6卷 250-272页

作者： Shuai-Bin hua Tian Jin Xin guo School of Materials Science and Engineering State Key Laboratory of Material Processing and Die&Mould TechnologyHuazhong University of Science and TechnologyWuhan 430074People’s Republic of China

Owing to the advantages of simple structure,low power consumption and high-density integration,memristors or memristive devices are attracting increasing attention in the fields such as next generation non-volatile memories,neuromorphic computation and data encryption.However,the deposition of memristive films often requires expensive equipment,strict vacuum conditions,high energy consumption,and extended processing times.In contrast,electrochemical anodizing can produce metal oxide films quickly(e.g.10 s) under ambient conditions.By means of the anodizing technique,oxide films,oxide nanotubes,nanowires and nanodots can be fabricated to prepare memristors.Oxide film thickness,nanostructures,defect concentrations,etc,can be varied to regulate device performances by adjusting oxidation parameters such as voltage,current and time.Thus memristors fabricated by the anodic oxidation technique can achieve high device consistency,low variation,and ultrahigh yield rate.This article provides a comprehensive review of the research progress in the field of anodic oxidation assisted fabrication of memristors.Firstly,the principle of anodic oxidation is introduced;then,different types of memristors produced by anodic oxidation and their applications are presented;finally,features and challenges of anodic oxidation for memristor production are elaborated.

关键词： anodic oxidation anodized aluminium oxide memristor resistive switching electrical properties

Dynamic foraging strategy adaptation to heterogeneous environments contributes to social aggregation in snub-nosed monkeys

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Zoological Research 2024年第1期45卷 39-54页

作者： Lan Zhao Sheng-Nan Ji Xiao-Bing Du Jia-Hui Liu Bo-Lun Zhang Pei-hua Li Yi-jun Yang Bao-guo Li Yan-Qing guo Xiao-Guang Qi College of Life Sciences Northwest UniversityXi’anShaanxi 710069China Chengdu Institute of Biology Chinese Academy of SciencesChengduSichuan 610041China State Key Laboratory of Environmental Criteria and Risk Assessment Chinese Research Academy of Environmental SciencesBeijing 100012China

The dynamics of animal social structures are heavily influenced by environmental patterns of competition and cooperation.In folivorous colobine primates,prevailing theories suggest that larger group sizes should be favored in rainforests with a year-round abundance of food,thereby reducing feeding competition.Yet,paradoxically,larger groups are frequently found in high-altitude or high-latitude montane ecosystems characterized by a seasonal scarcity of leaves.This contradiction is posited to arise from cooperative benefits in heterogeneous environments.To investigate this hypothesis,we carried out a six-year field study on two neighboring groups of golden snub-nosed monkey(Rhinopithecus roxellana),a species representing the northernmost distribution of colobine primates.Results showed that the groups adjusted their movement and habitat selection in response to fluctuating climates and spatiotemporal variability of resources,indicative of a dynamic foraging strategy.Notably,during the cold,resource-scarce conditions in winter,the large group occupied food-rich habitats but did not exhibit significantly longer daily travel distances than the smaller neighboring group.Subsequently,we compiled an eco-behavioral dataset of 52 colobine species to explore their evolutionary trajectories.Analysis of this dataset suggested that the increase in group size may have evolved via home range expansion in response to the cold and heterogeneous climates found at higher altitudes or latitudes.Hence,we developed a multi-benefits framework to interpret the formation of larger groups by integrating environmental heterogeneity.In cold and diverse environments,even smaller groups require larger home ranges to meet their dynamic survival needs.The spatiotemporal distribution of high-quality resources within these expanded home ranges facilitates more frequent interactions between groups,thereby encouraging social aggregation into larger groups.This process enhances the benefits of collaborative actions and reproductive opportunities,whi

关键词： Social evolution Folivore paradox MLS Rhinopithecus roxellana Multi-benefits framework

Carbon dots-derived three-dimensional-ordered macroporous host with high penetrability and catalytic activity for LSBs under lean electrolyte

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Rare Metals 2024年第6期43卷 2560-2573页

作者： Jiao-Zi Duan hua-Yu Pei Quan Yang Xue Li Xin Ba Xue Yong jun-Ling guo Si-Yu Lu Green Catalysis Center College of ChemistryZhengzhou University Country State Center for International Cooperation On Designer Low-Carbon & Environmental Materials School of Materials Science and EngineeringZhengzhou University Hubei Institute of Quality Supervision Inspection Department of Chemistry University of Sheffield

The practical energy density of lithium-sulfur batteries（LSBs） is seriously limited by the high electrolyte-to-sulfur ratios（E/S）.The E/S can be reduced by employing hosts with easy-to-infiltrate structure that ensures the uniform distribution of a lean electrolyte and high catalytic activity that can suppress "shuttle effect" via accelerating the slow conversion of soluble poly sulfides to insoluble sulfides.Among the easy-to-infiltrate structures,the three-dimensional-ordered macroporous（3DOM）structure is easier to scale preparation and more suitable for the existing industrial processes.However,it is difficult to obtain the 3DOM with（1） high penetrability due to the high viscosity of frequently-used organic polymer precursors and（2） high catalytic activity due to the low confinement effect,meaning that uniformly dispersed small-sized catalytic materials are difficult to load on 3DOM.Herein,using carbon dots（CDs） with both organic and inorganic properties as a precursor and aggregation limiting agent,a 3DOM host with high penetrability and homodispersed Ni particles of small sizes（Ni-CDs-3DOM）was synthesized.In this host:（1） CDs precursor with suitable viscosity can improve the penetrability.（2） CDs can effectively inhibit the agglomeration of Ni particles.（3） Uniformly dispersed small-size Ni particles offer high-efficiency catalytic activity toward sulfur reactions.Consequently,the Ni-CDs-3DOM/sulfur cathode exhibits high sulfur utilization and stable cycling performance even under high sulfur loading(5.5 mg·cm-1) and low E/S(6.5 μl·mg-1).This work indicates the usefulness of CDs in constructing hosts for LSBs with high energy density.

关键词： Lithium–sulfur batteries Carbon dots Catalytic action Easy-to-infiltrate structure Lean electrolyte

Preface:special topic on rechargeable battery technology

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Science China Chemistry 2024年第1期67卷 1-3页

作者： Yu-guo guo Qiang Zhang jun Chen Li-jun Wan CAS Key Laboratory of Molecular Nanostructure and Nanotechnology CAS Research/Education Center for Excellence in Molecular SciencesBeijing National Laboratory for Molecular Sciences(BNLMS)Institute of ChemistryChinese Academy of Sciences(CAS)Beijing 100190China University of Chinese Academy of Sciences Beijing 100049China Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing 100084China Frontiers Science Center for New Organic Matter Renewable Energy Conversion and Storage Center(RECAST)Haihe Laboratory of Sustainable Chemical TransformationsKey Laboratory of Advanced Energy Materials Chemistry(Ministry of Education)College of ChemistryNankai UniversityTianjin 300071China

Rechargeable batteries play a major role in the transition from fossil energy to renewable energy and are considered the key-enabling decarbonization technology for several industries,including electronics,transportat... 详细信息

关键词： battery artificial technology