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Designing ultrastable P2/O3-type layered oxides for sodium ion batteries by regulating Na distribution and oxygen redox chemistry

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Journal of Energy Chemistry 2024年第7期94卷 466-476页

作者： Jieyou Huang Weiliang Li Debin Ye Lin Xu Wenwei wu Xuehang wu School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004GuangxiChina Guangxi Key Laboratory for High-value Utilization of Manganese Resources Guangxi Normal University for NationalitiesChongzuo 532200GuangxiChina

P2/O3-type Ni/Mn-based layered oxides are promising cathode materials for sodium-ion batteries(SIBs)owing to their high energy ***,exploring effective ways to enhance the synergy between the P2 and 03 phases remains a ***,we design a P2/O3-type Na_(0.76)Ni_(0.31)Zn_(0.07)Mn_(0.50)Ti_(0.12)0_(2)(NNZMT)with high chemical/electrochemical stability by enhancing the coupling between the two *** the first time,a unique Na*extraction is observed from a Na-rich O3 phase by a Na-poor P2 phase and systematically *** process is facilitated by Zn^(2+)/Ti^(4+)dual doping and calcination condition regulation,allowing a higher Na*content in the P2 phase with larger Na^(+)transport channels and enhancing Na transport *** of reduced Na^(+)in the O3 phase,which increases the difficulty of H^(+)/Na^(+) exchange,the hydrostability of the O3 phase in NNZMT is considerably ***,Zn^(2+)/Ti^(4+)presence in NNZMT synergistically regulates oxygen redox chemistry,which effectively suppresses O_(2)/CO_(2) gas release and electrolyte decomposition,and completely inhibits phase transitions above 4.0 *** a result,NNZMT achieves a high discharge capacity of 144.8 mA h g^(-1) with a median voltage of 3.42 V at 20 mA g^(-1) and exhibits excellent cycling performance with a capacity retention of 77.3% for 1000 cycles at 2000 mA g^(-1).This study provides an effective strategy and new insights into the design of high-performance layered-oxide cathode materials with enhanced structure/interface stability forSIBs.

关键词： Sodium-ion batteries P2/O3-type layered oxides Na distribution Oxygen redox chemistry Hydrostability

A fuse-based DC circuit breaker with vacuum interrupter enhanced by an external transverse magnetic field

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High Voltage 2024年第3期9卷 710-720页

作者： Yu Xiao Yi wu Yifei wu Fei Yang Mingzhe Rong Zhuo Yang State Key Laboratory of Electrical Insulation and Power Equipment School of Electric EngineeringXi'an Jiaotong UniversityXi'anChina State Grid Shaanxi Electric Power Company Limited Xi'anChina

Due to the increasing power system capacity,the interruption of large fault currents has gradually become a major challenge in power *** the moment,such currents are interrupted mainly via circuit breakers based on the method of active current ***,these types of circuit breakers tend to be costly and *** possible alternative—a fuse-based circuit breaker with current commutation process enhanced by an external transverse magnetic field(ETMF)—is proposed by the *** main advantage lies in the fast current commutation achieved by an ETMF-enhanced three-stage increase of the vacuum arc *** study of the current commutation process is mainly represented by the authors,and the influencing factors of the current commutation—contact opening speed and ETMF current—are *** last,the proposed circuit breaker is verified by an experiment,whose results show that a short-circuit current of 42 kA can be interrupted within just 2 ms.

关键词： vacuum transverse interrupt

Mechanism Design for Ancillary Service Market Considering Social Welfare and Fairness

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CSEE Journal of Power and Energy Systems 2024年第3期10卷 1000-1010页

作者： Zhi wu Yuanxi wu Wei Gu Zheng Xu Shu Zheng Jingtao Zhao School of Electrical Engineering Southeast UniversityNanjing 210096China NARI Technology Co. Ltd.Nanjing 211106China IEEE CSEE

Increasing penetration of distributed energy resources in the distribution network(DN)is threatening safe operation of the DN,which necessitates setup of the ancillary service market in the *** the ancillary service market,distribution system operator(DSO)is responsible for safety of the DN by procuring available capacities of *** existing studies,this paper proposes a novel market mechanism composed of two parts:choice rule and payment *** proposed choice rule simultaneously considers social welfare and fairness,encouraging risk-averse aggregators to participate in the ancillary service *** is then formulated as a linear programming problem,and a distributed solution using the multi-cut Benders decomposition is ***,successful implementation of the choice rule depends on each aggregator’s truthful adoption of private ***,a payment rule is also designed,which is proved to possess two properties:incentive compatibility and individual *** results demonstrate effectiveness of the proposed choice rule on improving fairness and verify properties of the payment rule.

关键词： Aggregator ancillary service market distributed mechanism fairness mechanism design

Imide-pillared covalent organic framework protective films as stable zinc ion-conducting interphases for dendrite-free Zn metal anodes

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Journal of Energy Chemistry 2024年第10期97卷 470-477,I0010页

作者： Xiaoman Ye Xuemei Xiao Zhijing wu Xin wu Lin Gu Sheng Liu School of Chemical Engineering and Technology Sun Yat-sen UniversityZhuhai 519082GuangdongChina The Key Lab of Low-Carbon Chemistry&Energy Conservation of Guangdong Province Sun Yat-sen UniversityGuangzhou 510275GuangdongChina

The notorious growth of zinc dendrite and the water-induced corrosion of zinc metal anodes(ZMAs)restrict the practical development of aqueous zinc ion batteries(AZIBs).In this work,a zinc metallized,imide-pillared covalent organic framework(ZPC)protective film has been engineered as a stable Zn^(2+)ion-conducting interphase to modulate interfacial kinetics and suppress side reactions for *** to bare Zn,ZPC@Zn exhibits a higher Zn^(2+)ionic conductivity,a larger Zn^(2+)transference number,a lower electronic conductivity,a smaller desolvation activation energy and correspondingly a significant suppression of corrosion,hydrogen evolution and Zn ***,the ZPC@Zn||ZPC@Zn symmetric cell obtains a cycling lifespan over 3000 h under 5 mA cm^(-2)for 1 mA h cm^(-2).The ZPC@Zn||NH_(4)V_(4)O_(10)coin-type full battery delivers a specific capacity of 195.8 mA h g^(-1)with a retention rate of78.5%at 2 A g^(-1)after 1100 cycles,and the ZPC@Zn||NH_(4)V_(4)O_(10) pouch full cell shows a retention of70.1%in reversible capacity at 3 A g^(-1)after 1100 *** present incorporation of imide-linked covalent organic frameworks in the surface modification of ZMAs will offer fresh perspectives in the search for ideal protective films for the practicality of AZIBs.

关键词： Aqueous zinc ion batteries Zinc metal anodes Surface modification Covalent organic frameworks Imide linkage

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油气成藏动力学模拟评价系统的研制

石油实验地质 2007年第5期29卷 527-530页

作者：何大伟毛小平杨甲明吴景富潘明太中国石油勘探开发研究院中国地质大学北京100083 中海石油研究中心北京100027

在油气成藏动力学模拟评价系统的基础上,进一步考虑各种地质因素,包括快速底层数据建模、模拟数据的透明化、油气初次运移模型、多因数控制的油气运聚模拟、油气最优运移路径的法线追踪等,建立了地质模型,并将地质模型转化成数学模型和... 详细信息

在油气成藏动力学模拟评价系统的基础上,进一步考虑各种地质因素,包括快速底层数据建模、模拟数据的透明化、油气初次运移模型、多因数控制的油气运聚模拟、油气最优运移路径的法线追踪等,建立了地质模型,并将地质模型转化成数学模型和计算机模型,提升了该系统的模拟能力,使该系统成为地质学家的一个油气系统三维可视化分析工具。利用该系统对东海盆地丽水凹陷开展了实际应用,得出丽水凹陷总生烃量为158×108t,其中生油78×108t,生气79×1011m3,从而对该凹陷的油气勘探起到了指导作用。

关键词：三维建模油气成藏动力学模拟评价系统丽水凹陷东海盆地

南海北部深水及超深水区现今地温场及热结构特征研究

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地质科学 2014年第3期49卷 781-790页

作者：杨树春吴景富唐晓音仝志刚王柯郝建荣中海油研究总院北京100027 中国科学院地质与地球物理研究所岩石圈演化国家重点实验室北京100029

依据前人对岩石圈层结构的认识和地震反射界面揭示的沉积充填,本文对南海北部深水及超深水区域的现今地温场特征及岩石圈热结构进行了计算。结果表明:南海北部深水及超深水区具有"热盆"特征,超深水区较深水区更热,但超深水区沉积基底的... 详细信息

依据前人对岩石圈层结构的认识和地震反射界面揭示的沉积充填,本文对南海北部深水及超深水区域的现今地温场特征及岩石圈热结构进行了计算。结果表明:南海北部深水及超深水区具有"热盆"特征,超深水区较深水区更热,但超深水区沉积基底的现今温度较深水区低。大地热流值的总体变化趋势表现为从深水区向超深水区逐渐增高,与地壳和岩石圈向南减薄趋势一致。南海北部深水及超深水区具有"冷壳热幔"的岩石圈热结构特征。地壳热流主要由基底的构造形态和地壳减薄程度控制,地幔热流则只受控于岩石圈基底埋深。

关键词：南海北部超深水区地温梯度大地热流岩石圈热结构

RecBERT:Semantic recommendation engine with large language model enhanced query segmentation for k-nearest neighbors ranking retrieval

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Intelligent and Converged Networks 2024年第1期5卷 42-52页

作者： Richard wu the Dublin Unified School District and the SF Artificial Intelligence Club DublinCA 94568USA

The increasing amount of user traffic on Internet discussion forums has led to a huge amount of unstructured natural language data in the form of user *** modern recommendation systems rely on manual tagging,relying on administrators to label the features of a class,or story,which a user comment corresponds *** common approach is to use pre-trained word embeddings to compare class descriptions for textual similarity,then use a distance metric such as cosine similarity or Euclidean distance to find top k ***,neither approach is able to fully utilize this user-generated unstructured natural language data,reducing the scope of these recommendation *** paper studies the application of domain adaptation on a transformer for the set of user comments to be indexed,and the use of simple contrastive learning for the sentence transformer fine-tuning process to generate meaningful semantic embeddings for the various user comments that apply to each *** order to match a query containing content from multiple user comments belonging to the same class,the construction of a subquery channel for computing class-level similarity is *** channel uses query segmentation of the aggregate query into subqueries,performing k-nearest neighbors(KNN)search on each individual *** achieves state-of-the-art performance,outperforming other state-of-the-art models in accuracy,precision,recall,and F1 score for classifying comments between four and eight classes,*** outperforms the most precise state-of-the-art model(distilRoBERTa)in precision by 6.97%for matching comments between eight classes.

关键词： sentence transformer simple contrastive learning large language models query segmentation k-nearest neighbors

Principal components of nuclear mass models

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Science China(Physics,Mechanics & Astronomy) 2024年第7期67卷 65-71页

作者： Xin-Hui wu Pengwei Zhao Department of Physics Fuzhou UniversityFuzhou 350108China State Key Laboratory of Nuclear Physics and Technology School of PhysicsPeking UniversityBeijing 100871China

Principal component analysis(PCA)is employed to extract the principal components(PCs)present in nuclear mass models for the first *** effects from different nuclear mass models are reintegrated and reorganized in the extracted *** PCs are recombined to build new mass models,which achieve better accuracy than the original theoretical mass *** comparison indicates that using the PCA approach,the effects contained in different mass models can be collaborated to improve nuclear mass predictions.

关键词： nuclear mass principal component analysis nuclear models statistical methods

Sonoafterglow luminescence for in vivo deep-tissue imaging

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Chinese Chemical Letters 2024年第10期35卷 9-10页

作者： Shihong wu Ronghui Zhou Hang Zhao Peng wu State Key Laboratory of Oral Diseases West China Hospital of StomatologySichuan UniversityChengdu 610041China Analytical&Testing Center Sichuan UniversityChengdu 610064China School of Chemistry and Chemical Engineering Henan Normal UniversityXinxiang 453007China

Optical imaging is a key technique to study the pathological process and disease diagnosis,but there is still a great challenge to achieve highly sensitive in vivo deep-tissue *** interferences from the intrinsic autofluorescence and light scattering and re-absorption are typically observed in biological tissues,which severely impair target signal sensing and *** address the above issues,using of afterglow luminescence for imaging has been *** to its long lifetime,the images can be collected after ceasing the excitation,thus could eliminate the ***,the current afterglow luminescence still requires photoexcitation(mainly ultraviolet or visible light),the penetration depth of which is still limited for deeptissue imaging.

关键词： scattering luminescence excitation