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Functional decoration on a regenerable bifunctional porous covalent organic framework probe for rapid detection and adsorption of copper ions

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Rare Metals 2024年第2期43卷 758-769页

作者： Yu-Long Li Xi-Lang Jin Yi-Ting Ma jing-rui liu Fazal Raziq Peng-Yuan Zhu Zhi-Feng Deng Hong-Wei Zhou Wei-Xing Chen Wen-Huan Huang School of Materials and Chemical Engineering Xi’an Technological UniversityXi’an710021China Yulin Boyi-jingking Research Institute of Industrial Technology Development Research Yulin719054China KAUST Catalysis Center King Abdullah University of Science and Technology23955-6900ThuwalKingdom of Saudi Arabia Key Laboratory of Chemical Additives for China National Light Industry College of Chemistry and Chemical EngineeringShaanxi University of Science and TechnologyXi’an710021China National and Local Joint Engineering Laboratory for Slag Comprehensive Utilization and Environmental Technology School of Materials Science and EngineeringShaanxi University of TechnologyHanzhong723001China

Developing fluorescence porous probe for detecting and eliminating Cu^(2+) contamination in water or biosystem is an essential research project that has attracted considerable ***,improving the fluorescence detecting efficiency while enhancing the adsorption capacity of the porous probe is of great ***,a bifunctional two-dimensional imine-based porous covalent organic framework(TTP-COF)probe was designed and synthesized from 1,3,5-tris(4-aminophenyl)benzene(TAPB)and 2,4,6-Triformylphloroglucinol(TP)***-COF displayed rapid detection of Cu^(2+)(limit of detection(LOD)=10 nmol·L^(−1) while achieving a high adsorption capacity of 214 mg·g^(−1)(pH=6)at room temperature with high reusability(>5 cycles).The key roles and contributions of highπ-conjugate and delocalized electrons in TABP and functional–OH groups in TP were *** importantly,the fluorescence quenching mechanism of TTP-COF was studied by density functional theory theoretical calculations,revealing the crucial role of intramolecular hydrogen bonds among C=N and–OH groups and the blocking of the excited state intramolecular proton transfer process in detecting process of Cu^(2+).

关键词： Covalent organic framework(COF) Excited-state intramolecular proton transfer(ESIPT) Copper ion detection Copper ion adsorption Renewability

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The Influence of Co Addition on Phase Transformation Behavior and Mechanical Properties of TiNi Alloys

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Chinese Journal of Aeronautics 2007年第2期20卷 153-156页

作者： jing rui-rui liu Fu-shun School of Materials Science and Engineering Beijing University of Aeronautics and Astronautics Beijing 100083 China

The influences of Co-addition on phase transformation behavior and mechanical properties of TiN/alloys were investigated. Resuits indicate that, as a substitute for Ni, Co added to TiNi alloys can dramatically decrease the martensite transformation temperature, and R phase transformation and martensite transformation are accordingly separated. When Co-content reach 10 at.%, the martensite transformation temperature is lower than that of liquid nitrogen. During deformation at room temperature, Ti50Ni48Co2 alloy exhibits good ductility with a lower stress plateau caused by stress-induced martensite and martensite reorientation.

关键词： TiNiCo shape memory alloy martensite transformation mechanical property

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Slowly rotating charges from Weyl double copy for Kerr black hole with Chern-Simons correction

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Communications in Theoretical Physics 2024年第8期76卷 139-146页

作者： Yi-Ran liu jing-rui Zhang Yun-Long Zhang School of Fundamental Physics and Mathematical Sciences Hangzhou Institute for Advanced StudyUCASHangzhou 310024China CAS Key Laboratory of Theoretical Physics Institute of Theoretical PhysicsChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100149China National Astronomy Observatories Chinese Academy of ScienceBeijing 100101China International Center for Theoretical Physics Asia-Pacific Beijing/HangzhouChina

The Weyl double copy builds the relation between gauge theory and gravity theory, in particular the correspondence between gauge solutions and gravity solutions. In this paper, we obtain the slowly rotating charge solutions from the Weyl double copy for the Kerr black hole with small Chern-Simons correction. Based on the Weyl double copy relation, for the Petrov type D solution in Chern-Simons modified gravity, we find the additional correction to the electromagnetic field strength tensor of the rotating charge. For the Petrov type I solution, we find that the additional electromagnetic field strength tensors have external sources, while the total sources vanish at the leading order.

关键词： Chern-Simons modified gravity Weyl double copy Kerr black hole

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Stretchable multifunctional sensor based on porous silver nanowire/silicone rubber conductive film

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Nano Research 2023年第5期16卷 7618-7626页

作者： Hai-Tao Deng Dan-Liang Wen jing-rui liu Xin-Ran Zhang Yi-Lin Wang Peng Huang Beomjoon Kim Xiao-Sheng Zhang School of Electronic Science and Engineering University of Electronic Science and Technology of ChinaChengdu 611731China CIRMM Institute of Industrial ScienceThe University of TokyoTokyo 153-8505Japan

As one of the promising human–machine interfaces,wearable sensors play an important role in modern society,which advances the development of wearable fields,especially in the promising applications of electronic skin(e-skin),robotics,prosthetics,*** the last decades,wearable sensors tend to be capable of attractive capabilities such as miniaturization,multifunction,smart integration,wearable properties such as lightweight,flexibility,stretchability,conformability for wider *** this work,we developed a stretchable multifunctional sensor based on porous silver nanowire/silicone rubber conductive film(P-AgNW/SR).Its unique structural configuration,i.e.,an assembly of the P-AgNW/SR with good conductivity,stability,resistance response,the insulated silicone rubber layer,provided the feasibility for realizing multiple sensing ***,porous microstructures of the P-AgNW/SR made the device to be used for pressure sensing,exhibiting outstanding dynamic and static resistive responsive behaviors and having a maximum sensitivity of 9.062%∙N^(−1) in a continuous compressive force range of~16 *** the merit of the good piezoresistive property of AgNW/SR networks embedded into the surface of micropores of the P-AgNW/SR,the device was verified to be a temperature sensor for detecting temperature changes in the human body and *** temperature sensor had good sensitivity of 0.844%∙℃^(−1),high linearity of 0.999 in the range of 25–125℃,remarkable dynamic ***,the developed sensor was demonstrated to be a single electrode-triboelectric sensor for active sensing,owing to the unique assembly of the conductive PAgNW/SR electrode and the silicone rubber friction *** on the coupling effect of the triboelectrification and electrostatic induction,the generated electrical signals could be used to sense the human motions,according to the quantitative correlation between the human motions and the features in amplitude and

关键词： wearable electronics porous microstructures multiple sensors pressure sensing temperature sensing triboelectric sensing

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Numerical simulation of melt flow and temperature field during DC casting 2024 aluminium alloy under different casting conditions

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China Foundry 2024年第4期21卷 387-396页

作者： Jin-chuan Wang Yu-bo Zuo Qing-feng Zhu jing Li rui Wang Xu-dong liu Key Laboratory of Electromagnetic Processing of Materials Ministry of EducationNortheastern UniversityShenyang 110819China School of Materials Science and Engineering Northeastern UniversityShenyang 110819China Engineering Research Center of Advanced Materials Preparing Technology Ministry of EducationShenyang 110819China CAS Key Laboratory of Nuclear Materials and Safety Assessment Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China

Casting speed,casting temperature and secondary cooling water flow rate are the main process parameters affecting the DC casting *** parameters significantly influence the flow and temperature fields during casting,which are crucial for the quality of the ingot and can determine the success or failure of the casting *** simulation,with the advantages of low cost,rapid execution,and visualized results,is an important method to study and optimize the DC casting *** the present work,a simulation model of DC casting 2024 aluminum alloy was established,and the reliability of the model was ***,the influence of casting parameters on flow field and temperature field was studied in detail by numerical simulation *** show that with the increase of casting speed,the melt flow becomes faster,the depths of slurry zone and mushy zone increase,and the variation of slurry zone depth is greater than that of mushy *** an increase in casting temperature,the melt flow rate increases,the depth of the slurry zone becomes shallower,and the depth of the mushy zone experiences only minor *** simulation results further indicate that the increase of the flow rate of the secondary cooling water slightly reduces the depths of both slurry and mushy zone.

关键词： aluminium DC casting flow field temperature field numerical simulation

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Thermal stability improvement and microstructure optimization of high cobalt content Nd-Fe-B magnets via terbium grain boundary diffusion

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Journal of Rare Earths 2024年第8期42卷 1531-1538,I0004页

作者： Jiyuan Xu ruiyang Meng jing liu Jiateng Zhang rui Han Yikun Fang Shengzhi Dong Wei Li Division of Functional Materials Research Central Iron and Steel Research InstituteBeijing100081China

The substitution of Fe by Co in the 2:14:1 phase is an effective method to increase the Curie temperature and enhance the thermal stability of the Nd-Fe-B ***,the accumulation of Co ele ment at the grain boundaries(GBs) changes the GBs from nonmagnetic to ferromagnetic and causes the thinlayer GBs to become rare,In this paper,the method of diffusing Tb element was chosen to improve the microstructure and temperature stability of high-Co *** original sintered Nd_(28.5)Dy_(3)-CO_(x)e_(bal)M_(0.6)B_(i)(x=0,6 wt%,12 wt%;M = Cu,Al,Zr) magnets with different Co contents were diffused with Tb by grain boundary diffusion(GBD).After GBD,high-Co magnets exhibit more continuously distributed thin-layer GBs,and their thermal stability is significantly *** high-Co magnets(x=6 wt%),the absolute value of the temperature coefficient of coercivity decreases from 0.603%/K to0.508%/K in the temperature range of 293-413 K,that of remanence decreases from 0.099%/K to 0.091%/K,and the coercivity increases from 18.44 to 25.04 *** electron microscopy(TEM)characterization reveals that there are both the 1:2 phase and the amorphous phase in the high-Co magnet before and after GBD,EDS elemental analysis shows that Tb element is more likely to preferentially replace the rare earth elements in the 2:14:1 main phase than in the 1:2 phase and the amorphous *** concentration of Tb at the edge of the main phase is much higher than that in the 1:2phase and amorphous phase,which is beneficial to the improvement of the *** preferential replacement of Tb elements at the edge of the 2:14:1 phase and thin-layer GBs with a more continuous distribution are synergistically responsible for improving the thermal stability of high-Co *** study indicates that GBD is an effective method to improve the microstructure and thermal stability of high-Co magnets.

关键词： Nd-Fe-B magnets Coercivity Grain boundary diffusion Thermal stability Micro structure Rare earths

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Inhibiting HMGCR represses stemness and metastasis of hepatocellular carcinoma via Hedgehog signaling

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Genes & Diseases 2024年第5期11卷 470-483页

作者： Zhirong Zhang Jiayao Yang rui liu jing Ma Kai Wang Xiaojun Wang Ni Tang Key Laboratory of Molecular Biology for Infectious Diseases(Ministry of Education) Institute for Viral HepatitisDepartment of Infectious DiseasesThe Second Affiliated HospitalChongqing Medical UniversityChongqing 400016China Institute of Hepatobiliary Surgery Southwest HospitalThird Military Medical University(Army Medical University)Chongqing 400038China

Cancer stem cells(CSCs)play a crucial role in tumor initiation,recurrence,metastasis,and drug ***,the current understanding of CSCs in hepatocellular carcinoma(HCC)remains *** a comprehensive analysis of the database,it has been observed that 3-hydroxy-3-methylglutaryl-coenzyme A reductase(HMGCR),a critical enzyme involved in cholesterol synthesis,is up-regulated in HCC tissues and liver ***,high expression of HMGCR is associated with a poor prognosis in patients with ***,HMGCR promotes the stemness and metastasis of HCC both in vitro and in *** screening various signaling pathway inhibitors,we have determined that HMGCR regulates stemness and metastasis by activating the Hedgehog signaling in ***,HMGCR positively correlates with the expression of the Smoothened receptor and facilitates the nuclear translocation of the transcriptional activator GLI family zinc finger *** of the Hedgehog pathway can reverse the stimulatory effects of HMGCR on stemness and metastasis in ***,simvastatin,an FDA-approved cholesterol-lowering drug,has been shown to inhibit stemness and metastasis of HCC by targeting *** together,our findings suggest that HMGCR promotes the regeneration and metastasis of HCC through the activation of Hedgehog signaling,and simvastatin holds the potential for clinical suppression of HCC metastasis.

关键词： Cancer stem cells Hedgehog Hepatocellular carcinoma Metastasis Statin

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Accelerating the evaluation of operational lifetimes of perovskite solar cells and modules

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Journal of Energy Chemistry 2024年第7期94卷 1-9页

作者： Fumeng Ren Qian Lu Xin Meng jing Zhou rui Chen Jianan Wang Haixin Wang Sanwan liu Zonghao liu Wei Chen Wuhan National Laboratory for Optoelectronics Huazhong University of Science and TechnologyWuhan 430074HubeiChina China-EU Institute for Clean and Renewable Energy Huazhong University of Science and TechnologyWuhan 430073HubeiChina Powerchina Huadong Engineering Corporation Limited Hangzhou 311122ZhejiangChina Optics Valley Laboratory Wuhan 430074HubeiChina

Compared with the power conversion efficicency,the operational stability of perovskite solar cells(PsCs)remains a major challenge hampering its ***,conducting a light soaking test under 1 sun illumination to get a long lifetime is time-consuming and experimentally ***,we report an accelerated stability test protocol by aging PsCs under high-intensity light illumination to accelerate the evaluation of their operation *** is found that the efficiency degradation rate of a typical inverted PsC is almost linearly dependent on the light intensity within the range of 1 to 4 suns regardless of the *** results prove that it can save the light-soaking time by at least 4 times to predict the operation lifetime on the basis of the equivalent light irradiation dose.

关键词： Perovskite Light-soaking Stability

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Construction of multifunctional lanthanum manganese mixed nanoparticles mediated by ionic liquids for selective aerobic oxidation of cyclohexane

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Rare Metals 2024年第5期43卷 2205-2221页

作者： Hao Li rui-rui Zhang Ke-Xin Li Shuang Wei Yu-Mei liu rui-Xia liu Beijing Key Laboratory of Ionic Liquids Clean Process CAS Key Laboratory of Green Process and EngineeringState Key Laboratory of Multiphase Complex SystemsInstitute of Process EngineeringChinese Academy of SciencesBeijing 100190China University of Chinese Academy of Sciences Beijing 100049China

Selective oxidation of alkanes to produce highvalue chemicals is an essential strategy and means to realize efficient utilization of *** this work,a strategy of lanthanum manganese mixed metal oxides(LMMO)regulated via a facile ionic liquid(IL)-assisted hydrothermal method was proposed to construct the multifunctional catalysts,which exhibited excellent catalytic performance in the selective aerobic oxidation of *** 8.9%cyclohexane conversion with 90%KA oi(cyclohexanol and cyclohexanone)selectivity was achieved over the optimal LMMO catalyst under mild *** effects of anion type,carbon chain length and concentration of ILs on the structure and properties of catalysts were investigated through various characterizations,indicating the structure-directing and template effect of ILs on the multifunctional *** formation of self-assembled spherical nanoparticles followed the"dissolution-nucleation-proliferation"mechanism with the introduction of 1-butyl-3-methylimidazolium hydrogen sulfate,ascribing the synergistic effect between the microenvironment of ILs and the hydrothermal ***,the high reactive oxygen concentration redox capacity,and suitable basic sites of LMMO catalysts mediated by ILs enhance the activation of C-H bonds and molecular oxygen,simultaneously influencing the adsorption and desorption of the substrate.A comprehensive understanding of the high KA oil selectivity and radical reaction mechanism was elucidated based on in situ diffuse reflectance infrared Fourier transform spectroscopy(DRIFTS)and radical trapping *** recycling and regeneration experiments further illuminated that the removal of adsorbed cyclohexanone acting on the LMMO catalyst was the key to achieve high KA oil selectivity.

关键词： Ionic liquids Nanoparticle Multifunctional catalyst Cyclohexane oxidation

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Clinical practice guidelines for neoadjuvant therapy in patients with early-stage breast cancer:Chinese Society of Breast Surgery practice guidelines 2022

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Chinese Medical Journal 2024年第12期137卷 1387-1388页

作者： Juliang Zhang Ting Wang Zhe Wang jing Fan Xiaolong Xu jing Kong Xinxin Wen rui Ling Yinhua liu Department of Thyroid Breast and Vascular SurgeryXijing HospitalThe Fourth Military Medical UniversityXi’anShaanxi 710032China Breast Disease Center Peking University First HospitalBeijing 100034China.

Neoadjuvant therapy can yield clinical benefits in earlystage breast cancer with *** indications,treatment regimens,and efficacy of neoadjuvant therapy have been investigated,which have contributed valuable clinical evidence.[1,2]The Chinese Society of Breast Surgery convened a panel of breast disease experts to review and discuss the literature on neoadjuvant therapy for breast cancer and evaluate relevant evidence by referring to the Grading of Recommendations,Assessment,Development,and Evaluations(GRADE)*** into account China’s specific circumstances,the society and participating experts developed the Clinical Practice Guidelines for Neoadjuvant Therapy for Early-stage Breast Cancer(Version 2022)to serve as a reference for breast surgeons in China.

关键词： Surgery Breast breast

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