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CeO_(2)-clay composites for ultra-long cycle life electrochemical capacitive energy storage application

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Journal of Rare Earths 2023年第5期41卷 728-739,I0004页

作者： Shan-Shan Chai Wei-Bin Zhang jing-lei yang Lun Zhang Xiong-Wei Han Myat Myintzu Theint Xue-jing Ma College of Materials and Chemistry&Chemical Engineering Chengdu University of TechnologyChengdu 610059China Mineral Development Section for the International Relation Department of MinesMinistry of Natural Resources and Environmental ConversationNay Pyi Taw15011Myanmar

The lattice expansion caused by the reduction of Ce(Ⅳ)to Ce(Ⅲ)impeded the development of the CeO_(2)as an effective electrode material for electrochemical ***,we prepared CeO_(2)-clay composites through a one-step hydrothermal *** interlayer structures of clays efficiently accommodate volume changes induced by crystal lattice expansion to achieve ultra-long cycle *** 60000 charge-discharge cycles,the capacitance retention rate of the assembled asymmetric supercapacitors is as high as~-100%.The key findings of this work reveal the potential application of clays in achieving ultralong cycle stability of the CeO_(2)electrode material,paving the way for further application of the CeO_(2)in electrochemical energy storage.

关键词： Cerium dioxide Clay mineral Cycle life Electrochemical supercapacitor Rareearths

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日本红枫育苗技术管理规范研究

园艺与种苗 2024年第7期44卷 8-10页

作者：雷经洋郜文慧陈竹陆小雨黄玉慧任杰安徽省农业科学院农业工程研究所安徽合肥230031 安徽雨田润股份有限公司安徽芜湖242400 中徽生态环境有限公司安徽合肥230088

为提高日本红枫育苗技术水平,从嫁接苗培育、扦插苗培育2种育苗方式,阐述了日本红枫的标准化育苗技术,其中育苗方式、技术规程、容器育苗、经营档案等均采用现有国家或行业标准。另外,简述了日本红枫的主要病虫害及其防治方法,重点介绍... 详细信息

为提高日本红枫育苗技术水平,从嫁接苗培育、扦插苗培育2种育苗方式,阐述了日本红枫的标准化育苗技术,其中育苗方式、技术规程、容器育苗、经营档案等均采用现有国家或行业标准。另外,简述了日本红枫的主要病虫害及其防治方法,重点介绍了天牛类害虫的防治措施。该研究对日本红枫标准化育苗生产具有重要参考价值。

关键词：日本红枫育苗技术天牛防治管理规范化

Increasing ionic conductivity in Li_(0.33)La_(0.56)TiO_(3)thin-films via optimization of processing atmosphere and temperature

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Rare Metals 2022年第1期41卷 179-188页

作者： Shi-Pai Song Cheng yang Chun-Zhi Jiang Yong-Min Wu Rui Guo He Sun jing-lei yang Yong Xiang Xiao-Kun Zhang School of Materials and Energy University of Electronic Science and Technology of ChinaChengdu 611731China School of Materials Science and Engineering Harbin Institute of TechnologyHarbin 150001China State Key Laboratory of Space Power-Sources Technology Shanghai Institute of Space Power-SourcesShanghai 200245China Department of Mechanical and Aerospace Engineering Hong Kong University of Science and TechnologyHong Kong 999077China Advanced Energy Research Institute University of Electronic Science and Technology of ChinaChengdu 611731China Sichuan Provincial Engineering Research Center of Flexible Display Material Genome University of Electronic Science and Technology of ChinaChengdu 611731China

As a promising solid electrolyte for thin-film lithium batteries,the amorphous Li_(0.33)La_(0.56)TiO_(3)(LLTO)thin film has gained great ***,enhancing ionic conductivity remains challenging in the ***,a systematical study was performed to improve the ionic conductivity of sputter-deposited LLTO thin films via the optimization of processing atmosphere and *** combining the optimized oxygen partial pressure(30%),annealing temperature(300℃),and annealing atmosphere(air),an amorphous LLTO thin film with an ionic conductivity of 5.32910^(-5)·S·cm^(-1) at room temperature and activation energy of 0.26 eV was *** results showed that,first,the oxygen partial pressure should be high enough to compensate for the oxygen loss,but low enough to avoid the abusive oxygen scattering effect on lithium precursors that results in a lithium-poor *** oxygen partial pressure needs to achieve a balance between lithium loss and oxygen defects to improve the ionic ***,a proper annealing temperature reduces the oxygen defects of LLTO thin films while maintaining its amorphous state,which improves the ionic ***,the highest ionic conductivity for the LLTO thin films that were annealed in air(a static space without a gas stream)occurs because of the decreased lithium loss and oxygen defects during *** findings show that the lithium-ion concentration and oxygen defects affect the ionic conductivity for amorphous LLTO thin films,which provides insight into the optimization of LLTO thin-film solid electrolytes,and generates new opportunities for their application in thinfilm lithium batteries.

关键词： Li_(0.33)La_(0.56)TiO_(3) Thin film Ionic conductivity Lithium-ion concentration Oxygen defects

Efficient construction of calcium fluoride nanoaggregates for enhanced water vapor adsorption

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Particuology 2024年第6期89卷 191-197页

作者： Dan-lei yang jing Cao Rong-Kun Liu Jie-Xin Wang School of Life Sciences and Chemical Engineering Jiangsu Second Normal UniversityNanjing210013China State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical TechnologyBeijing 100029China Research Center of the Ministry of Education for High Gravity Engineering and Technology Beijing University of Chemical TechnologyBeijing100029China Petrochemical Research Institute PetroChinaBeijing102206China

Calcium fluoride(CaF_(2))is an ideal adsorbent for the dehydration of gaseous hydrogen fluoride(HF)containing water *** this work,a novel CaF_(2)absorbent,spherical CaF_(2)nanoaggregates(NAs)with a closely packed structure,was proposed and efficiently fabricated by spray drying *** the building blocks of CaF_(2)NAs,the CaF_(2)nanoparticles(NPs)were prepared by the addition of excess calcium ions(Ca^(2+))or fluorine ions(F−)in the *** results indicated that the CaF_(2)NPs synthesized by excess Ca^(2+)and the corresponding NAs exhibited much better water vapor adsorption properties than their counterparts by excess F−,owing to higher zeta *** importantly,whether excess Ca^(2+)or F^(−),CaF_(2)NAs had further enhanced water vapor adsorption capacity compared to primary CaF_(2)NPs,possibly owing to their unique nano-micro secondary structures and higher surface *** work has great potential in the development of high-performance absorbents for separating moisture from corrosive gas HF.

关键词： CaF_(2)nanoaggregates Water vapor adsorption Spray drying

Evolution of inclusions in vacuum induction melting of superalloys containing 70%return material

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Journal of Iron and Steel Research(International) 2024年第3期31卷 719-728页

作者： Jin-guo Gao Shu-lei yang Shu-feng yang jing-she Li Wei Liu Meng-jing Zhao An-ren Wang School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing 100083China State Key Laboratory of Advanced Metallurgy University of Science and Technology BeijingBeijing 100083China Metallurgical and Building Materials Business Department China International Engineering Consulting CorporationBeijing 100048China

The variation law of inclusions type and size in the vacuum induction melting process and ingot of Ni-based superalloy containing 70%return material was studied by industrial test sampling,and the mechanism of inclusions formation was analyzed with thermodynamic *** results show that there are mainly two types of composite inclusions in the vacuum induction melting of Ni-based superalloys,which are nitride-and oxide-based composite inclusions,like Al_(2)O_(3)-SiO_(2)-Cr_(2)O_(3),TiN-(Mo,Nb)C,*** type and proportion of inclusions from the center to the edge of the vacuum induction ingot did not change *** number density of inclusions from the center to the edge of the ingot varied less,and the size of inclusions became smaller from the center to the *** addition,thermodynamic calculations show that oxides(M_(2)O_(3))are present in the liquid phase and mainly contain Al,Ti,Cr,Fe and O *** nitride consists mainly of Ti and N and contains small amounts of Cr,C,Nb,and Mo *** is consistent with the results of industrial *** the temperature decreases,the precipitation phases such as M_(2)O_(3),MN,γ,MC,δ,γ'andμphases are gradually precipitated,where oxides and nitrides are present in the liquid *** contents of O and N elements are the main influencing factors for the inclusions content and precipitation temperature;when the nitrogen content is reduced to below 0.0015%,it can make MN precipitate below the liquid-phase line.

关键词： Ni-based superalloy Vacuum induction melting Return material Inclusion Thermodynamic

Catalytic Reaction Kinetics of Propylene Dimerization to 4-Methyl-1-Pentene Using Cu-K/K_(2)CO_(3) Solid Base Catalyst

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China Petroleum Processing & Petrochemical Technology 2024年第1期26卷 78-87页

作者： Jin Haibo Chai jing yang Suohe He Guangxiang Ma lei Guo Xiaoyan College of New Materials and Chemical Engineering Beijing Institute of Petrochemical Technology/Beijing Key Laboratory of Fuel Cleaning and Efficient Catalytic Emission Reduction TechnologyBeijing102617China

The catalysis technology of propylene dimerization to form 4-methyl-1-pentene(4MP1)using a Cu-K/K_(2)CO_(3) solid base catalyst is a well-known heterogeneous catalytic *** this study,the intrinsic kinetics of propylene dimerization were studied in a fixed-bed continuous *** and external diffusion during the dimerization reaction experiments were eliminated by adjusting the flow rate of the carrier gas and the particle size of the catalyst ***,the concentration changes of each substance at the outlet of the catalyst bed under different residence times were ***,the suitable reaction kinetics equations was derived using the Langmuir Hinshelwood-Hougen-Watson kinetic ***,the activation energy for each reaction involved in the dimerization reaction was *** activation energies of 4MP1,branched by-products,and 1-hexene were 115.0,150.8,and 177.4 kJ/mol,*** effect of process conditions on propylene dimerization with solid base catalysts was studied through kinetic model *** comparing the theoretical values obtained from the simulation with the experimental results,the applicability and accuracy of the kinetic model were verified.

关键词： propylene dimerization 4-methyl-1-pentene intrinsic kinetics surface reaction

Epidermal visualized health monitoring system based on stretchable and washable TPU hybrid conductive microtextiles

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Rare Metals 2024年第7期43卷 3185-3193页

作者： jing-Bo Yuan Zhi-Hong Feng Dong-Chan Li yang Luo Yun-lei Zhou School of Chemical Engineering Hebei University of Technology Engineering Research Center of Chemical Technology for Efficient Utilization of Seawater ResourcesMinistry of Education National Key Laboratory of Application Specific Integrated Circuit Department of Materials ETH Zürich Hangzhou Institute of Technology Xidian University

Electronic textiles,an emerging class of electronic technology,offer exciting opportunities for seamless integration with the human *** applications have been developed based on electronic ***,researches on integrating multiple electronic textilebased devices are still *** this study,we present a system integrated with an electrocardiogram monitoring sensor and an electroluminescence device based on stretchable and washable conductive micro *** signal is acquired by an electrocardiograph amplifier and displayed by a dual-color electroluminescence device based on the processed *** integrated electronic device has excellent moisture permeability and comfort for long-term *** system reported in this study opens a new avenue for the application of electronic textiles in health monitoring,robotic prosthetics,and competitive sports.

关键词： Conductive microtextile Textile composite Electronic textile Electroluminescent displays

Atomic tailoring-induced deficiency in tungsten oxides for high-performance energy-related devices

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Tungsten 2024年第2期6卷 269-277页

作者： jing-Huang Lin Yao-Tian Yan Jun-lei Qi Chen-yang Zha Institute of Applied Physics and Materials Engineering Zhuhai UM Science and Technology Research InstituteUniversity of MacaoTaipaMacao SAR 999078China State Key Laboratory of Advanced Welding and Joining Harbin Institute of TechnologyHarbin 150001China Jiangmen Laboratory of Carbon Science and Technology Hong Kong University of Science and Technology(Guangzhou)Jiangmen 529199China Key Laboratory of Flexible Electronics School of Flexible Electronics(Future Technologies)Institute of Advanced MaterialsNanjing Tech UniversityNanjing 211816China

Nowadays,tungsten oxides,as a typical transition metal oxide,are widely and intensively investigated owing to their excellent material properties and device *** oxygen defi ciency in tungsten oxides is typically the key to enhance their performances for a variety of critical technological *** a gradual increase of oxygen defi ciency,various non-stoichiometric tungsten oxides can be formed by re-adjustment of the atomic arrangement,which exhibits superior performances than their traditional stoichiometric *** review mainly focuses on the recent advances in oxygen-defi cient tungsten oxides from the point of atomic structures,including the forming mechanism of non-stoichiometric tungsten oxides and the superiority of these oxygen-defi cient tungsten oxides in energy-related ***,the challenge and perspective of oxygen-defi cient tungsten oxides are also discussed.

关键词： Oxygen defi ciency Tungsten oxide Atomic structures Catalyst Storage

Design and preparation of highly crystalline K-intercalated W@PCN:an efficient material for aniline elimination

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Rare Metals 2024年第3期43卷 1337-1342页

作者： Hao-Fei Li Kai-Wen Yu Xiao-Bi jing lei Duan Yi-yang Zhang School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhou225002China School of Mechanical Engineering Yangzhou UniversityYangzhou225127China School of Material Science and Engineering Huazhong University of Science and TechnologyWuhan430071China School of Chemical Engineering and Materials Changzhou Institute of TechnologyChangzhou213032China Department of Basic Courses Army Engineering University of PLANanjing211101China

In this paper,we designed and prepared the polymeric carbon nitride-supported tungsten(W@PCN)*** were employed as the catalysts for photocatalytic oxidation of aniline in *** the process,H_(2)O_(2)was initially generated via the PCN-catalyzed *** by supported tungsten,aniline was oxidized by the in situ generated H_(2)O_(2)to obtain less toxicpoly aniline.

关键词： materials aniline crystalline