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In situ tracking of the lithiation and sodiation process of disodium terephthalate as anodes for rechargeable batteries by Raman spectroscopy

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Nano Research 2024年第1期17卷 245-252页

作者： Xiu-Mei lin Chong {2. Xin-Tao Yang Jia-Sheng lin wei-Qiang Yang hong-Xu Guo Yao-hui Wang jin-Chao Dong Jian-Feng Li Department of Chemistry and Environment Science Fujian Province University Key Laboratory of Analytical ScienceMinnan Normal UniversityZhangzhou 363000China College of Energy College of Chemistry and Chemical EngineeringCollege of MaterialsState Key Laboratory of Physical Chemistry of Solid SurfacesiChEMXiamen UniversityXiamen 361005China institute of Optical and Electronic Technology China Jiliang UniversityHangzhou 310018China

Organic compounds represent an appealing group of electrode materials for rechargeable batteries due to their merits of biomass,sustainability,environmental friendliness,and *** terephthalate(Na_(2.C_(8)H_(4)O_(4),Na_(2.TP),an organic salt with a theoretical capacity of 2.5 mAh·g^(-1),is electroactive towards both lithium and ***,its electrochemical energy storage(EES)process has not been directly observed via in situ characterization techniques and the underlying mec{2.isms are still under ***,in situ Raman spectroscopy was employed to track the de/lithiation and de/sodiation processes of *** appearance and then disappearance of the–COOLi Raman band at 162. cm^(-1) during the de/lithiation,and the increase and then decrease of the–COONa Raman band at 1615 cm^(-1) during the de/sodiation processes of Na2.P elucidate the one-step with the 2.i+or 2.a+transfer *** also found that the inferior cycling stability of Na2.P as an anode for sodium-ion batteries(SIBs)t{2. lithium-ion batteries(LIBs)could be due to the larger ion radium of Na+t{2. Li+,which results in larger steric resistance and polarization during *** Na2.P,therefore,shows greater c{2.ges in spectra during de/sodiation t{2. de/*** expect that our findings could provide a reference for the rational design of organic compounds for EES.

关键词： disodium terephthalate(Na_(2.C_(8)H_(4)O_(4) Na2.P) in situ Raman spectroscopy de/lithiation de/sodiation mechanisms

A new approach of cascade utilization of the chemical energy of fuel

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Progress in Natural Science:Materials International 2006年第5期16卷 518-523页

作者： han wei, {2. hongguang and lin rumou ( {2. of engineering thermophysics, chinese academy of sciences, beijing 1.0080, china Graduate School of the chinese academy of sciences, beijing 1.0080, china) [a]institute of engineering {2. Chinese Academy of Sciences Beijing China [b]Graduate School of the chinese academy of sciences Beijing China

The indirect release of chemical energy of fuel is investigated, and a new mechanism is proposed to identify the cascade utilization of chemical energy of fuel more clearly. Based on the concept of energy level, the internal phenomenon of the indirect chemical energy release is disclosed, and the equations of energy level describing the utilization of chemical energy and thermal energy during the indirect chemical energy release process are obtained. From theoretical analysis, we find that the superiority of the indirect chemical energy release of fuel comes from the cascade utilization of the fuel's chemical energy. Moreover, the cascade utilization of chemical energy is verified by the investigation of CRGT (chemically recuperated gas turbine). As a result, the thermal exergy obtained from the chemical energy release of fuel increases by 2.% -3 % . The results obtained here may help a deeper understanding of indirect chemical energy release of fuel and provide a theoretical basis for the synthesis of innovative energy systems.

关键词： chemically recuperated gas turbine methane/steam reforming chemical energy level cascade utilization.

Possible Energy Network with polygeneration system and CCS for china

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中国科学：技术科学英文版 2010年第1期53卷 33-39页

作者： GAO lin1,LI Sheng1,2.jin hongguang1 & lin Hu1 1 institute of {2. thermophysics,chinese academy of sciences,beijing 100190,china 2.Graduate School of chinese academy of sciences,beijing 100039,china 1. institute of engineering {2. Chinese Academy of Sciences Beijing 100190 China2. Graduate School of Chinese Academy of Sciences Beijing 100039 China

On basis of adopting polygeneration systems for power and alternative fuels,capturing CO2.with near zero energy penalties,and storing CO2.on sites,a new kind of Energy Network can integrate energy utilization,CO2.capture,transportation and storage ***-economic analysis of this solution focusing on Inner Mongolia and the Yangtze River Delta districts had been carried with comparison to the chain method for energy utilization and CO2.*** solution can save 2..5% of energy,and reduce 35% of total *** adoption of advanced polygeneration systems contributes 52.2. of the total saved costs,and the integration of energy utilization and CO2.sequestration in the Energy Network contributes 47.8%.From the aspect of CCS,the CO2.sequestration cost in the Energy Network can be as low as 12.$/t due to the lower energy penalties of capture in polygeneration systems and the combination of CO2.source and *** Energy Network exhibits attractive performance on energy saving,costs reduction for CCS,which may be a promising solution for sustainable development of china.

关键词： CO2 capture and storage Energy Network polygeneration system

Jetting of a near-wall cavitation bubble induced by another tandem bubble

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Journal of Hydrodynamics 2024年第3期36卷 444-456页

作者： hui han {2.g-zhu Wang Jian-lin Huang Peng-bo Bai Yong-gang Chen Yi-wei Wang Key Laboratory for Mechanics in Fluid Solid Coupling Systems Institute of MechanicsChinese Academy of SciencesBeijing100190China School of engineering Science University of Chinese Academy of SciencesBeijing100049China Guangdong Aerospace Research academy Guangzhou511458China School of Future Technology University of Chinese Academy of SciencesBeijing100049China Jianghuai Advance Technology Center Hefei230088China

Double bubbles near a rigid wall surface collapse to produce a significant jet impact,with potential applications in surface cleaning and ultrasonic ***,the dynamic behaviors of near-wall bubbles remain *** this study,we investigate the jetting of a near-wall bubble induced by another tandem *** define two dimensionless standoff distances,γ_(1),γ_(2.,to represent the distances from the center of the near-wall bubble to the rigid wall and the center of controlling bubble to the center of the near-wall bubble,*** observations reveal three distinct jetting regimes for the near-wall bubble:transferred jetting,double jetting,and directed *** further investigate the jetting mechanism,numerical simulations are conducted using the compressibleInterFoam solver in the open-source framework of OpenFOAM.A detailed analysis shows that the transferred jet flow is caused by the pinch-off resulting from the axial contraction velocity at the lower end of the near-wall bubble being greater than the vertical contraction velocity,leading to a maximum jet velocity of 682.58 m/*** the case of double jetting,intense stretching between the controlling bubble and the wall leads to a pinch-off and a double jetting with a maximum velocity of 1096.2. m/*** directed jet flow is caused by the downward movement of the high-pressure region generated by the premature collapse of the controlling bubble,with the maximum jet velocity reaching 444.62.m/s.

关键词： Jetting of near-wall bubble controlling bubble impact velocity

In vivofluorescenceflow cytometry reveals that the nanoparticle tumor vaccine OVA@HA-PEI effectively clears circulating tumor cells

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Journal of Innovative Optical Health sciences 2024年第6期17卷 107-123页

作者： wei jin Yuting Fu Sisi Ge {2. Sun Kai Pang Xunbin wei The Department of Biomedical engineering institute of Advanced C{2.ical Medicine Peking University Beijing 100191P.R.China institute of Medical Technology Peking University Health Science Center beijing 100191 P.R.China Key Laboratory of Carcinogenesis and Translational Research(Ministry of Education/beijing) Peking University Cancer Hospital&InstituteBeijing 100142P.R.China School of Instrument Science and Opto-Electronics engineering beijing Information Science&Technology University beijing 100192 P.R.China

Tumor vaccine therapy offers significant advantages over conventional treatments,including reduced toxic side ***,it currently functions primarily as an adjuvant treatment modality in clinical oncology due to limitations in tumor antigen selection and delivery *** vaccines often fail to elicit a su±ciently robust immune response against progressive tumors,thereby limiting their clinical e±*** this study,we developed a nanoparticle-based tumor vaccine,OVA@HA-PEI,utilizing ovalbumin(OVA)as the presenting antigen and hyaluronic acid(HA)and polyethyleneimine(PEI)as adjuvants and *** formulation significantly en{2.ced the proliferation of immune cells and cytokines,such as CD3,CD8,interferon-,and tumor necrosis factor-,in vivo,effectively activating an immune response against B16–F10 *** vivofluorescenceflow cytometry(IVFC)has already become an effective method for monitoring circulating tumor cells(CTCs)due to its direct,noninvasive,and long-term detection *** study utilized a laboratory-constructed IVFC system to monitor the immune processes induced by the OVA@HA-PEI tumor vaccine and an anti-programmed death-1(PD-1)*** results demonstrated that the combined treatment of OVA@HA-PEI and anti-PD-1 antibody significantly improved the survival time of mice compared to anti-PD-1 antibody treatment ***,this combination therapy substantially reduced the number of CTCs in vivo,increased the clearance rate of CTCs by the immune system,and slowed tumor *** greatly en{2.ce the clinical application prospects of IVFC and tumor vaccines.

关键词： Tumor vaccines circulating tumor cells in vivofluorescenceflow cytometry.

Research on intelligent search-and-secure technology in accelerator hazardous areas based on machine vision

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Nuclear Science and Techniques 2024年第4期35卷 96-107页

作者： Ying-lin Ma Yao Wang hong-Mei Shi {2.-Jie Zhang School of Traffic and Transportation Beijing Jiaotong UniversityBeijing 100044China School of Mechanical Electronic and Control EngineeringBeijing Jiaotong UniversityBeijing 100044China institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China

Prompt radiation emitted during accelerator operation poses a significant health risk,necessitating a thorough search and securing of hazardous areas prior to ***,manual sweep methods are ***,the limitations of manual sweeps have become increasingly evident with the implementation of large-scale *** leveraging advancements in machine vision technology,the automatic identification of stranded personnel in controlled areas through camera imagery presents a viable solution for efficient search and *** the criticality of personal safety for stranded individuals,search and security processes must be sufficiently *** ensure comprehensive coverage,180°camera groups were strategically positioned on both sides of the accelerator tunnel to eliminate blind spots within the monitoring *** YOLOV8 network model was modified to enable the detection of small targets,such as hands and feet,as well as larger targets formed by individuals near the ***,the system incorporates a pedestrian recognition model that detects human body parts,and an information fusion strategy is used to integrate the detected head,hands,and feet with the identified pedestrians as a cohesive *** strategy enhanced the capability of the model to identify pedestrians obstructed by equipment,resulting in a notable improvement in the recall ***,recall rates of 0.915 and 0.82.ere obtained for Datasets 1 and 2.*** there was a slight decrease in accuracy,it aligned with the intended purpose of the search-and-secure software *** tests conducted within an accelerator tunnel demonstrated the effectiveness of this approach in achieving reliable recognition outcomes.

关键词： Search and secure Machine vision Camera Human body parts recognition Particle accelerator Hazardous area

Fundamental study of CO_2.control technologies and policies in china

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Science china(Technological sciences) 2008年第7期51卷 857-870页

作者： jin hongguang1, ZhanG XiLiang2. GAO {{2., YUE Li2. HE JianKun2.& CAI RuiXian1 1 institute of {2. thermophysics, chinese academy of sciences, beijing 1.0080, china 2.institute of Nuclear and New Energy Technology, Tsinghua University, beijing 100084, china 1. institute of engineering {2. Chinese Academy of Sciences Beijing 100080 China 2. institute of Nuclear and New Energy Technology Tsinghua University Beijing 100084 China

The technical roadmap and policies for CO2.mitigation suitable for china are a common center of attention in the fields of energy, environment, and management science in the country. Emphasizing interaction between technical research and policy research, this work discovers the potential breakthrough in the integrated field. The technical difficulties of recovering CO2.are pointed out, the mechanism of combining CO2.recovery with energy conversion is investigated, and the basic principle for integrating an environmental-friendly energy system is discussed. Moreover, the formulation of a new energy system that can recover CO2.with very low or even zero energy penalty is proposed, while the assessment methodology and model system for the technical roadmap of CO2.emission control are developed. Finally, a new technical roadmap constructing an energy network suitable for china is proposed, which may provide a new way for the development of sustainable energy and environment technologies.

关键词： CO2 capture and storage technical roadmap energy policy

Multilevel carbon architecture of subnanoscopic silicon for fast‐charging high‐energy‐density lithium‐ion batteries

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Carbon Energy 2024年第4期6卷 256-268页

作者： Meisheng han Yongbiao Mu Lei wei {2. Zeng Tianshou Zhao Shenzhen Key Laboratory of Advanced Energy Storage Southern University of Science and TechnologyShenzhenChina SUSTech Energy institute for Carbon Neutrality Southern University of Science and TechnologyShenzhenChina Department of Mechanical and Energy engineering Southern University of Science and TechnologyShenzhenChina

Silicon(Si)is widely used as a lithium‐ion‐battery anode owing to its high capacity and abundant crustal ***,large volume change upon cycling and poor conductivity of Si cause rapid capacity decay and poor fast‐charging capability limiting its commercial ***,we propose a multilevel carbon architecture with vertical graphene sheets(VGSs)grown on surfaces of subnanoscopically and homogeneously dispersed Si–C composite nanospheres,which are subsequently embedded into a carbon matrix(C/VGSs@Si–C).Subnanoscopic C in the Si–C nanospheres,VGSs,and carbon matrix form a three‐dimensional conductive and robust network,which significantly improves the conductivity and suppresses the volume expansion of Si,thereby boosting charge transport and improving electrode *** VGSs with vast exposed edges considerably increase the contact area with the carbon matrix and supply directional transport channels through the entire material,which boosts charge *** carbon matrix encapsulates VGSs@Si–C to decrease the specific surface area and increase tap density,thus yielding high first Coulombic efficiency and electrode compaction ***,C/VGSs@Si–C delivers excellent Li‐ion storage performances under industrial electrode *** particular,the full cells show high energy densities of 603.5 Wh kg^(−1)and 1685.5 Wh L^(−1)at 0.1 C and maintain 80.7%of the energy density at 3 C.

关键词： fast charging high energy densities lithium‐ion batteries multilevel carbon architecture subnanoscopic silicon anode

Optimizing near-carbon-free nuclear energy systems:advances in reactor operation digital twin through hybrid machine learning algorithms for parameter identification and state estimation

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Nuclear Science and Techniques 2024年第8期35卷 177-203页

作者： Li‑Zhan hong He‑{2. Gong hong‑Jun Ji Jia‑Liang Lu han Li Qing Li Paris Elite institute of Technology Shanghai Jiao Tong UniversityShanghai 200240China Science and Technology on Reactor System Design Technology Laboratory Nuclear Power Institute of ChinaChengdu 610041China

Accurate and efficient online parameter identification and state estimation are crucial for leveraging digital twin simulations to optimize the operation of near-carbon-free nuclear energy *** previous studies,we developed a reactor operation digital twin(RODT).However,non-differentiabilities and discontinuities arise when employing machine learning-based surrogate forward models,challenging traditional gradient-based inverse methods and their *** study investigated deterministic and metaheuristic algorithms and developed hybrid algorithms to address these *** efficient modular RODT software framework that incorporates these methods into its post-evaluation module is presented for comprehensive *** methods were rigorously assessed based on convergence profiles,stability with respect to noise,and computational *** numerical results show that the hybrid KNNLHS algorithm excels in real-time online applications,balancing accuracy and efficiency with a prediction error rate of only 1%and processing times of less t{2. 0.1 ***,algorithms such as FSA,DE,and ADE,although slightly slower(approximately 1 s),demonstrated higher accuracy with a 0.3%relative L_2.error,which advances RODT methodologies to harness machine learning and system modeling for improved reactor monitoring,systematic diagnosis of off-normal events,and lifetime management *** developed modular software and novel optimization methods presented offer pathways to realize the full potential of RODT for transforming energy engineering practices.

关键词： Parameter identification State estimation Reactor operation digital twin Reduced order model Inverse problem