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Nanopore design of sulfur doped hollow carbon nanospheres for superior potassium-ion battery anodes

Rare Metals 2024年第5期43卷 2103-2114页

作者： Zhen-Dong Liu Hui-Yan Feng Yu-chen Wang Fei Wang Yue Liu jian-Xiao Yang Yue Gu jun Tan Chong Ye cheng-Zhi Zhang Ji Hua Laboratory Foshan 528000China School of Chemical Engineering and Light Industry Guangdong University of TechnologyGuangzhou 510006China Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology College of Materials Science and EngineeringHunan UniversityChangsha 410082China

Sulfur doped carbonaceous materials are promising anodes for potassium-ion batteries because of their ability to bridge active sites and induce C/S electron coupling,resulting in increased ion storage capacitance However,the large potassium ions could cause significant volume expansion and structure collapse during operation in sulfur doped carbonaceous anodes,which lead to rapidly capacity sacrifice during long-term *** design for anchoring sulfur atom in carbon skeleton is a novel way to alleviate the structure collapse and maintain the cycling ***,this study developed a controlled nanopore and sulfur doped carbon sphere structure(S-NPHCSs).In potassium-ion batteries S-NPHCSs anode demonstrated exceptional performance with a high reversible capacity of 247 mAh·g^(–1)after 50 cycles at 0.2 A·g^(–1)and delivered a long cycle stability of 600 cycles at a high current density of 1.0 A·g^(–1).Interconnected nanopores and doped sulfur structure not only expand the accumulation space and offer ample active sites for diffusion and adsorption of potassium ions,but also build stable channels through nanopore structure to ensure the cyclic *** finding provides a fundamental theory for designing nanopore structures and introducing sulfur doped carbonaceous materials to enhance capacitive potassium storage and long cycle stability.

关键词： Nanopore Carbon materials Sulfur doping Anode Potassium-ionbatteries

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LASPM:the LAMOST stellar parameter pipeline for M-type stars and application to the sixth and seventh data release(DR6 and DR7)

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Research in Astronomy and Astrophysics 2021年第8期21卷 181-192页

作者： Bing Du A-Li Luo Shuo Zhang Xiao Kong Yan-Xin Guo Yin-Bi Li Fang Zuo You-Fen Wang jian-jun chen Yong-Heng Zhao CAS Key Laboratory of Optical Astronomy National Astronomical ObservatoriesBeijing 100101China University of Chinese Academy of Sciences Beijing 100049China Department of Astronomy School of PhysicsPeking UniversityBeijing 100871China

The molecular-rich atmospheres of M type stars complicate our understanding to their atmospheric ***,great progress has been made in atmospheric modeling of M-type stars,and we take advantage of the updated BT-Settl model grid to develop a pipeline LAS PM to measure atmospheric parameters(Teff,log g,[M/H]) of M-type stars from low-resolution *** pipeline was applied to the sixth and seventh data release(DR6 & DR7) of Large Sky Area Multi-Object Fiber Spectroscopic Telescope(LAMOST),which released atmospheric parameters for 610419 and 680 185 Mtype spectra,*** key algorithm is to find the best-matching for templates in the synthetic spectral library for an observed spectrum,and then minimizing χ^(2) through a linear combination of five best-matching *** intrinsic precisions of the parameters were estimated by using the multiple epoch observations for the same stars,which are 118 K,0.20 dex,0.29 dex for Teff,log g,and [M/H]*** Teff and log g are consistent with the spectral and luminosity classifications by LAMOST 1D pipeline,and the loci of giants and dwarfs both on spectral index and color-magnitude diagrams show the *** metallicities of LASPM are also checked with the selected members of four open clusters(NGC 2632,Melotte 22,ASCC16,and ASCC19),which are consistent without any *** the results between LASPM and the APOGEE Stellar Parameter and Chemical Abundance Pipeline(ASPCAP),there is a scatter of 73 K,0.22 dex,0.21 dex for Teff,log g,and [M/H],respectively.

关键词： atmospheric parameters data analysis spectrographs

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Capturing carbon dioxide from air by using amine-functionalized metal-organic frameworks

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Chinese Journal of Structural Chemistry 2024年第5期43卷 3-4页

作者： jian Yang Guang Yang Zhijie chen Stoddart Institute of Molecular Science Department of ChemistryState Key Laboratory of Silicon and Advanced Semiconductor MaterialsZhejiang UniversityHangzhou310058PR China Zhejiang-Israel Joint Laboratory of Self-Assembling Functional Materials ZJU-Hangzhou Global Scientific and Technological Innovation CenterZhejiang UniversityHangzhou311215PR China

Along with the rapid rise of industry and technology,carbon dioxide(CO_(2))is released as a major by-product of fossil fuels *** continuous CO_(2)emission results in a steep increase of atmospheric CO_(2)concentrations and precipitated severe environmental and climatic ***,it is of great importance to reduce CO_(2)emission and atmospheric CO_(2)*** CO_(2)directly from air is one of the most straightforward strategies to mitigate atmospheric CO_(2)concentrations[1].

关键词： dioxide straight carbon

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An Update of the Catalog of Radial Velocity Standard Stars from the APOGEE DR17

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Research in Astronomy and Astrophysics 2023年第11期23卷 243-251页

作者： Qing-Zheng Li Yang Huang Xiao-Bo Dong jian-jun chen A-Li Luo Yunnan Observatories Chinese Academy of SciencesKunmingYunnan 650011China School of Astronomy and Space Science University of Chinese Academy of SciencesBeijing 100049China CSA Key Laboratory of Optical Astronomy National Astronomical ObservatoriesChinese Academy of SciencesBeijing 100101China Key Laboratory of Space Astronomy and Technology National Astronomical ObservatoriesChinese Academy of SciencesBeijing 100101China

We present an updated catalog of 46,753 radial velocity(RV)standard stars selected from the APOGEE *** stars cover the Northern and Southern Hemispheres almost evenly,with 62%being red giants and 38%being main sequence *** RV standard stars are stable on a baseline longer than 200 days(with 54%longer than one year and 10%longer than five years)with a median stability better than 215 m s~(-1).The average number of observations of those stars is 5 and each observation is required to have signal-to-noise ratio greater than50 and RV measurement error smaller than 500 m s~(-1).Based on the new APOGEE RV standard star catalog,we have checked the RV zero-points(RVZPs)for current large-scale stellar spectroscopic surveys including RAVE,LAMOST,GALAH and *** careful analysis,we estimate their mean RVZP to be+0.149 kms~(-1),+4.574 km s~(-1)(for LRS),-0.031 km s~(-1)and+0.014 kms~(-1),respectively,for the four *** the RAVE,LAMOST(for MRS),GALAH and Gaia surveys,RVZP exhibits a systematic trend with stellar parameters(mainly[Fe/H],T_(eff),log g,G_(BP)-G_(RP)and G_(RVS)).The corrections to those small but clear RVZPs are of vital importance for these massive spectroscopic surveys in various studies that require extremely high RV accuracies.

关键词： stars:fundamental parameters (stars:)binaries:general stars:general catalogs

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Molecular Mechanism of Polysaccharides Extracted from Chinese Medicine Targeting Gut Microbiota for Promoting Health

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Chinese Journal of Integrative Medicine 2024年第2期30卷 171-180页

作者： ZHAO Wen-xiao WANG Tong ZHANG Ya-nan chen Qian WANG Yuan XING Yan-qing ZHENG jun DUAN chen-chen chen Lijun ZHAO Hai-jun WANG Shijun School of Nursing Shandong University of Traditional Chinese MedicineShandong University of Traditional Chinese MedicineJi'nan(250355)China Shandong Co-innovation Center of Classic Traditional Chinese Medicine Formula Shandong University of Traditional Chinese MedicineJi'nan(250355)China College of Traditional Chinese Medicine Shandong University of Traditional Chinese MedicineJinan(250355)China

The accumulating evidence revealed that gut microbiota plays an important role in pathological process of disease including obesity,type 2 diabetes mellitus,heart failure,and non-alcoholic fatty liver *** extracted from Chinese medicine(CM)can not only alleviate pathological status but also promote health by anti-inflammatory,regulating immunity,lowering blood glucose and lipids,anti-cancer,and *** alterations of gut microbiota composition and metabolism pathways are the potential mechanisms of CM polysaccharides *** addition,they exert functions through gut-organ axis or play an indirect role by synergistic actions with other drugs or components mediated by gut *** review summarizes the molecular mechanisms of CM polysaccharides interacted with intestinal microbial inhabitants as potential prebiotics forpromoting health.

关键词： Chinese medicine polysaccharides gut microbiota short-chain fatty acids lipopolysaccharides gut-organaxis synergistic actions

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Attention,neighbors:Methyl salicylate mediates plant airborne defense

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Plant Communications 2024年第1期5卷 1-3页

作者： Shan Liu Faisal Islam jianping chen Zongtao Sun jian chen International Genome Center Jiangsu UniversityZhenjiang 212013China State Key Laboratory for Managing Biotic and Chemical Threats to the Quality and Safety of Agro-products Key Laboratory of Biotechnology in Plant Protection of Ministry of Agriculture and Zhejiang ProvinceInstitute of Plant VirologyNingbo UniversityNingboChina

Plants have evolved to generate and release a wide array of volatile organic compounds(VOCs)when challenged by environmental stimuli such as biotic and abiotic stresses,which facilitate their reproduction,defense responses,and plant-plant communication(Karban,2021).Once emitted,some VOCs can elicit defense signaling in neighboring plants by interacting with specific receptor(s),a phenomenon referred to as airborne defense(AD)(Loreto and D’Auria,2022).

关键词： neighboring neighbor media

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Metal-to-insulator transition in platinum group compounds

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Rare Metals 2024年第8期43卷 3460-3474页

作者： Yu-Xuan Xia jian-Gang He Nuo-Fu chen Ji-Kun chen School of New Energy North China Electric Power UniversityBeijing102206China School of Mathematics and Physics University of Science and Technology BeijingBeijing 100083China Key Laboratory of Advanced Materials and Devices for PostMoore Chips(Ministry of Education) School of Materials Science and EngineeringJniversity of Science and Technology BeijingBeijing 100083China

The metal-to-insulator transition(MIT) as usually achieved in 3d-orbital transitional metal(TM) compounds opens up a new paradigm in correlated electronics via triggering abrupt variations in their transportation *** to such 3d-orbital TM compounds,the MIT within the platinum group(Pg) element compounds based on the 4d-and 5d-orbital configurations is more complicated,owing to their elevation in the spinorbit coupling and meanwhile weakened intra-atomic Coulomb *** brings in a new freedom to regulate the balance in their metallic or semiconductive orbital configurations,while their MIT properties can be potentially combined with their spintronic properties to enable new electronic ***,we review the electronic transport and MIT behaviors within the existing family of Pg-containing compounds,particularly those showing first-order MIT behaviors that can be useful in correlated *** is also hoped that summarizing the presently reported Pg-containing MIT compounds will lead to the discovery of more new material families and/or new mechanisms associated with the Pg-containing compounds showing MIT properties.

关键词： Metal-to-insulator transition Platinum group compounds Electron correlation Spin-orbital coupling

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Skin-inspired interface modification strategy toward a structurefunction integrated hybrid smart fabric system with self-powered sensing property for versatile applications

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Nano Research 2024年第9期17卷 8200-8208页

作者： Xiang cheng Teng chen De Gong Pengcheng Ma Bo chen jun Cai Aerospace Information Research Institute Chinese Academy of SciencesBeijing 100190China School of Mechanical Engineering and Automation Beihang UniversityBeijing 100191China Beijing U-Precision Tech Co. Ltd.Beijing 100176China University of Chinese Academy of Sciences Beijing 100049China

Fabric-based composites with superior mechanical properties and excellent perceptive function are highly ***,it remains a huge challenge to attain structure-function integration,especially for hybrid fabric ***,a skin-inspired interface modification strategy is proposed toward this target by constructing a hybrid smart fabric system consisting of two types of smart fabrics:carbon nanotube(CNT)/MXene-modified aramid fabrics and zinc oxide nanorod(ZnO NR)-modified carbon *** on that,flexible piezoelectric pressure sensors with skin-like hierarchical perception interfaces are fabricated,which demonstrate superb sensitivity of 2.39 V·kPa^(-1)and are capable of various wearable monitoring ***,the interface-modified hybrid fabric reinforced plastics can also be fabricated,which are proven to possess 13.6%higher tensile strength,10.1%elastic *** impressively,their average energy absorption can be improved by 111.9%,accompanied with inherent damage alert *** offers a paradigm to fabricate structure-function integrated hybrid smart fabric composites for the smart clothing and intelligent aerial vehicles.

关键词： hybrid fabrics interface modification piezoelectric pressure sensors self-diagnostic composites structure-function integration

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Remarkable Wear Resistance in a Complex Concentrated Alloy with Nanohierarchical Architecture and Composition Undulation

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Research 2024年第1期2023卷 403-416页

作者： Yushan Geng Wenyuan chen Hui Tan jun cheng Shengyu Zhu jun Yang Weimin Liu State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000PR China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049PR China Shandong Laboratory of Yantai Advanced Materials and Green Manufacturing Yantai 264000PR China

Sustained wear damages on the sliding surfaces of alloys are generally the culprit responsible for the failure of various mechanical *** by high-entropy effects,here we deliberately deploy nanohierarchical architecture with composition undulation in a Ni50(AlNbTiV)_(50) complex concentrated alloy,which yields ultralow wear rate within the order of 10^(−7) to 10^(−6) mm^(3)/Nm between room temperature and 800℃.Such remarkable wear resistance heretofore represents one of the highest wear resistance reported for the bulk alloys or composites,and originates from the multi-type adaptive friction interface protection governed by intrinsically nano-coupled grains and *** cooperative heterostructure releases gradient frictional stress in stages upon wear at room temperature through the coexistence of multiple deformation pathways while activating a dense nanocrystalline glaze layer upon wear at 800℃ to minimize adhesive and oxidative *** work uncovers a practical avenue for tailoring wear properties with multicomponent heterostructures over a wide temperature range.

关键词： wear alloys friction

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The Bright Single Pulse Emission from PSR B1133+16

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Research in Astronomy and Astrophysics 2024年第4期24卷 253-261页

作者： jun Tan Zhi-Gang Wen Zhen Wang Xue-Feng Duan Hong-Guang Wang Na Wang Vishal Gajjar jian-Ping Yuan Rai Yuen Wen-Ming Yan jian-Ling chen Wei Han Hui Wang cheng-Bing Lyu Ai-jun Dong Maths and Information Technology School Yuncheng UniversityYuncheng 044000China Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China Xinjiang Key Laboratory of Radio Astrophysics Urumqi 830011China School of Physics and Materials Science Guangzhou UniversityGuangzhou 510006China Space Science Laboratory University of CaliforniaBerkeley 94710USA Department of Physics and Electronic Engineering Yuncheng UniversityYuncheng 044000China School of Physics and Electronic Science Guizhou Normal UniversityGuiyang 550025China

We have conducted a comprehensive investigation into the bright single pulse emission from PSR B1133+16using the Giant Metrewave Radio *** time resolution data(61μs)were obtained at a center frequency of 322 MHz with a bandwidth of 32 MHz over a continuous observation period of 7.45 hr.A total of 1082 bright pulses were sporadically detected with peak flux densities ranging from 10 to 23 times stronger than the average pulse ***,no giant pulse-like emission with a relative pulse energy larger than 10 and extremely short duration was detected,indicating that these bright pulses cannot be categorized as giant pulse *** majority of these bright pulses are concentrated in pulse phases at both the leading and trailing windows of the average pulse profile,with an occurrence ratio of approximately *** pulse energy distribution for all individual pulses can be described by a combination of two Gaussian components and a cutoff power-law with an index of α=-*** updated nulling fraction of 15.35%±0.45% was determined from the energy *** emission of individual pulses follows a log-normal distribution in peak flux density *** is imperative that regular phase drifting in bright pulse sequence is identified in both the leading and trailing components for the first *** physical mechanisms are discussed in detail to provide insights into these observations.

关键词： (stars:)pulsars:general (stars:)pulsars:individual(PSR B1133+16) methods:observational methods:data analysis

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