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Progress in research on metal-based materials in stabilized Zn anodes

Rare Metals 2024年第1期43卷 20-40页

作者： Le Li Shao-Feng jia Ming-Hui Cao Yong-Qiang ji Heng-wei Qiu Dan Zhang Shaanxi Key Laboratory of Industrial Automation School of Mechanical EngineeringShaanxi University of TechnologyHanzhong 723001China School of Electronic and Information Engineering Qingdao UniversityQingdao 266071China State Key Laboratory for Artifcial Microstructure and Mesoscopic Physics School of PhysicsPeking UniversityBeijing 100871China Department of Chemistry Key Laboratory of Bioorganic Phosphorus Chemistry and Chemical BiologyTsinghua UniversityBeijing 100084China Shaanxi Key Laboratory of Catalysis School of Chemistry and Environment ScienceShaanxi University of TechnologyHanzhong 723001China

Aqueous zinc-ion batteries(ZIBs) combine the benefits of metallic Zn anodes with those of aqueous electrolytes and are well suited for large-scale energy storage because of their inherent high safety, cost-effectiveness, and eco-friendliness. Currently, the practical application of such batteries is hindered by the poor cycling performance of Zn anodes due to uncontrolled dendrite formation and severe side reactions, although recent reports suggest that these problems can be mitigated through the modification of Zn anodes with metal-based *** that the mechanisms of improving Zn deposition and the structural evolution of metal-based materials have not been systematically reviewed, we herein systematically overview the metal-based materials used to stabilize Zn anodes, starting with a brief summary of the anode working mechanism and the challenges faced by stabilized Zn anodes. Subsequently, the design principles of Zn anodes stabilized by metal-based materials and the related recent progress are reviewed, and the key challenges and perspectives for the future development of such Zn anodes are proposed.

关键词： Zinc-ion batteries(ZIBs) Zn anode Metalbased materials Alloying metal Stabilized Zn anodes

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Arbitrary skin metallization by pencil-writing inspired solid-ink rubbing for advanced energy storage and harvesting

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Journal of Energy Chemistry 2024年第1期88卷 592-602,I0013页

作者： Yonghan Zhou Zhongfeng ji Wenrui Cai Xuewei He Ruiying Bao Xuewei Fu wei Yang Yu Wang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials EngineeringSichuan UniversityChengdu 610065SichuanChina

The development of a durable metallic coating on diverse substrates is both intriguing and challenging,particularly in the research of metal-conductive materials for applications such as batteries,soft electronics,and ***,by learning from the pencil-writing process,a facile solid-ink rubbing technology(SIR-tech)is invented to address the above *** solid-ink is exampled by rational combination of liquid metal and graphite *** harnessing the synergistic effects between rubbing and adhesion,controllable metallic skin is successfully formed onto metals,woods,ceramics,and plastics without limitation in size and ***,outperforming pure liquid-metal coating,the composite metallic skin by SIR-tech is very robust due to the self-lamination of graphite nanoplate exfoliated by liquid-metal *** critical factors controlling the structures-properties of the composite metallic skin have been systematically investigated as *** applications,the SIR-tech is demonstrated to fabricate high-performance composite current collectors for next-generation batteries without traditional metal ***,advanced skin-electrodes are further demonstrated for stable triboelectricity generation even under temperature fluctuation from-196 to 120℃.This facile and highly-flexible SIR-tech may work as a powerful platform for the studies on functional coatings by liquid metals and beyond.

关键词： Microadhesion guided technology Skin metallization by solid-ink rubbing Liquid metal composites Composite current collector Batteries and triboelectric nanogenerators

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A novel method for calculating broadband electrical performance of high-speed aircraft radome under thermo-mechanical-electrical coupling

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Chinese Journal of Aeronautics 2024年第9期37卷 463-474页

作者： jianmin ji jianhua REN Xunya jiANG wei WANG Huilong YU Kai YIN Bo CHEN Beijing Institute of Remote Sensing Equipment Beijing 100854China Shanghai Dong Jun Information and Technology Co.Ltd Shanghai 200050China

The electrical performance of radomes on high-speed aircraft can be influenced by the thermal and mechanical loads produced during high-speed flight,which can affect the detection dis-tance and accuracy of the guidance *** paper presents a new method that uses the Finite Difference Time Domain(FDTD)method to calculate the electrical performance of radomes under Thermo-Mechanical-Electrical(TME)*** method can accurately characterize the effects of material dielectric temperature drift and structural deformation on the electrical performance of the radome under flight conditions,enabling high-precision full-wave calculations of the broadband electrical performance of the *** method initiates by utilizing a Finite Element Grid Model(FE-GM)of the radome to sequentially acquire the radome's response temperature field and structural deformation field through thermal and mechanical ***,spatial mapping techniques are developed to accurately incorporate the dielectric temperature drift and structural deformation of the radome into its Yee grid Electromagnetic(EM)simulation model.A verification case was designed to test the proposed method,and the results confirmed its high computational ***,the effectiveness and necessity of the method were further demonstrated by analyzing the electrical performance of a fused silica ceramic radome used on a high-speed aircraft.

关键词： High-speed aircraft Radomes Thermo-Mechanical-Electrical(TME)coupling Finite Difference Time Domain(FDTD)method Spatial mapping

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Multi-UAV Collaborative Edge Computing Algorithm for Joint Task Offloading and Channel Resource Allocation

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Journal of Communications and Information Networks 2024年第2期9卷 137-150页

作者： Yuting wei Sheng Wu Zhe ji Zhigang Yu Chunxiao jiang Linling Kuang School of Information and Communication Engineering Beijing University of Posts and TelecommunicationsBeijing 100876China China Academy of Electronics and Information Technology Beijing 100041China Beijing National Research Center for Information Science and Technology Tsinghua Space CenterTsinghua UniversityBeijing 100084China

Unmanned aerial vehicle (UAV)-based edge computing is an emerging technology that provides fast task processing for a wider area. To address the issues of limited computation resource of a single UAV and finite communication resource in multi-UAV networks, this paper joints consideration of task offloading and wireless channel allocation on a collaborative multi-UAV computing network, where a high altitude platform station (HAPS)is adopted as the relay device for communication between UAV clusters consisting of UAV cluster heads (ch-UAVs) and mission UAVs (m-UAVs). We propose an algorithm, jointing task offloading and wireless channel allocation to maximize the average service success rate (ASSR)of a period time. In particular,the simulated annealing(SA)algorithm with random perturbations is used for optimal channel allocation,aiming to reduce interference and minimize transmission delay.A multi-agent deep deterministic policy gradient (MADDPG) is proposed to get the best task offloading strategy. Simulation results demonstrate the effectiveness of the SA algorithm in channel allocation. Meanwhile,when jointly considering computation and channel resources,the proposed scheme effectively enhances the ASSR in comparison to other benchmark algorithms.

关键词： UAV-based edge computing multi-UAV collaboration joint task offloading and wireless channel allocation simulated annealing(SA)algorithm multi-agent deep deterministic policy gradient(MADDPG)

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A data-driven approach for predicting the fatigue life and failure mode of self-piercing rivet joints

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Advances in Manufacturing 2024年第3期12卷 538-555页

作者： jian Wang Qiu-Ren Chen Li Huang Chen-Di wei chao Tong Xian-Hui Wang Qing Liu Nanjing University of Science and Technology Nanjing210094People’s Republic of China Material Academy JitriSuzhou215100JiangsuPeople’s Republic of China Key Laboratory for Light-weight Materials Nanjing Tech UniversityNanjing210009People’s Republic of China Xi’an jiaotong-Liverpool University Suzhou215123JiangsuPeople’s Republic of China

In lightweight automotive vehicles,the application of self-piercing rivet(SPR)joints is becoming increasingly *** the importance of automotive service performance,the fatigue performance of SPR joints has received considerable ***,this study proposes a data-driven approach to predict the fatigue life and failure modes of SPR *** dataset comprises three specimen types:cross-tensile,cross-peel,and *** ensure data consistency,a finite element analysis was employed to convert the external loads of the different *** selection was implemented using various machine-learning algorithms to determine the model *** Gaussian process regression algorithm was used to predict fatigue life,and its performance was compared with different kernel functions commonly used in the *** results revealed that the Matern kernel exhibited an exceptional predictive capability for fatigue *** the data points,95.9%fell within the 3-fold error band,and the remaining 4.1%exceeded the 3-fold error band owing to inherent dispersion in the fatigue *** predict the failure location,various tree and artificial neural network(ANN)models were *** findings indicated that the ANN models slightly outperformed the tree *** ANN model accurately predicts the failure of joints with varying dimensions and ***,minor deviations were observed for the joints with the same ***,this data-driven approach provided a reliable predictive model for estimating the fatigue life and failure location of SPR joints.

关键词： Self-piercing rivet(SPR)joints Fatigue life prediction Failure mode prediction Machine learning

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Role of bonding filling on HER/OER/ORR multifunctional catalytic activity in transition-metals-doped PdPX(X=S,Se,Te)

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Rare Metals 2024年第10期43卷 5126-5140页

作者： Hai-Hua Huang wei Li Cheng-chao Hu Xue-Qin Sun Lin-Guo Lu Xiao-Feng Fan School of Materials Science and Engineering Laboratory of Sensitive Materials and DevicesShandong Department of EducationLiaocheng University School of Environmental and Material Engineering Yantai University Department of Physics University of Puerto Rico Key Laboratory of Automobile Materials (jilin University) Ministry of EducationCollege of Materials Science and EngineeringJilin University

The development of stable and highly efficien multifunctional electrocatalysts for the hydrogen evolution reaction （HER）,oxygen reduction reaction （ORR） and oxygen evolution reaction （OER） are essential for the efficient conversion and storage of renewable *** significant advantages of single-atom catalysts,such as strong metal slab interactions,unsaturated coordination and efficient atomic utilization,have opened new avenues for designing multifunctional ***,based on density functional theory,a single atom doped PdPX system was designed as a multifunctional electrocatalyst,which demonstrated the synergistic effect between defects and transition metal atoms and led to enhanced catalytic *** results showed that PdPS/PdPSe with P/X vacancy,PdPTe with P/Pd vacancy and Co/Rh/Ir@PdPX exhibited promising HER ***@PdPS（Se）,with an overpotential of 0.56（0.44） V,was predicted to be a promising OER ***,Rh（Ir）@PdPS（Se）catalysts exhibited efficient catalytic properties for ORR Besides,Co@PdPS（Se）,Rh（Ir）@PdPSV（S）,Co@PdP-SeV（Se）and Ir@PdPSV（S）-1exihibited multifunctional catalytic performance with moderate ***,the origin of catalytic activity was revealed by using the crystal orbital Hamilton populations *** a strong adsorption system,proper filling of the anti-bonding state can increase the energy of the system,weaken the adsorption strength,and facilitate the desorption of intermediates Conversely,augmenting bonding states can enhance its adsorption *** findings provide theoretica guidance for the design and fabrication of novel multifunctional electrocatalysts in terms of filling of bondingstate.

关键词： Density functional theory Electrocatalyst Two-dimensional PdPX Water splitting

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Characteristics of the crack tip field in high-speed railway tunnel linings under train-induced aerodynamic shockwaves

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Underground Space 2024年第5期18卷 199-217页

作者： Yi-Kang Liu Yu-Ling Wang E Deng Yi-Qing Ni wei-chao Yang Wai-Kei Ao School of Civil Engineering Central South UniversityChangsha 410075China National Rail Transit Electrification and Automation Engineering Technology Research Center(Hong Kong Branch) The Hong Kong Polytechnic UniversityHong Kong 999077China Department of Civil and Environmental Engineering The Hong Kong Polytechnic UniversityHong Kong 999077China The Hong Kong Polytechnic University Shenzhen Research Institute Shenzhen 518057China National Engineering Research Center of High-speed Railway Construction Technology Changsha 410075China

High-speed railway tunnels in various countries have continuously reported accidents of vault falling concrete *** the concrete block falling occurs,serious consequences follow,and traffic safety may be *** aerodynamic shockwave evolves from the initial compression wave may be an important inducement causing the tunnel lining cracks to grow and form falling concrete blocks.A joint calculation framework is established based on ANSYS Fluent,ABAQUS,and FRANC3D for calculating the crack tip field under the aerodynamic *** intensification effect of aerodynamic shockwaves in the crack is revealed,and the evolution characteristics of the crack tip field and the influence factors of stress intensity factor(SIF)are *** show that(1)the aerodynamic shockwave intensifies after entering the crack,resulting in more significant pressure in the crack than the input *** maximum pressure of the inclined and longitudinal cracks is higher than the corresponding values of the circumferential crack,respectively.(2)The maximum SIF of the circumferential,inclined,and longitudinal crack appears at 0.5,0.68,and 0.78 times the crack front *** maximum SIF of the circumferential crack is higher than that of the inclined and longitudinal *** possibility of crack growth of the circumferential crack is the highest under aerodynamic shockwaves.(3)The influence of train speed on the SIF of the circumferential crack is more than 40%.When the train speed,crack depth,and crack length change,the change of pressure in the crack is the direct cause of the change of SIF.

关键词： Falling concrete blocks Tunnel lining cracks Aerodynamic shockwave Intensification effect Crack tip field Stress intensity factor

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AA6061管锥形模轴压失稳起皱过程建模仿真

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塑性工程学报 2017年第5期24卷 171-177页

作者：郝花蕾孙志超吉卫中国工程物理研究院机械制造工艺研究所四川绵阳621900 西北工业大学材料学院陕西西安710072

管轴压成形省力、高效,但极易发生失稳起皱。通过试验与正交数值模拟相结合,对AA6061铝合金管在锥形模上的轴压失稳起皱进行了研究。在建模过程中建立了AA6061铝合金管材的本构关系,解决了建模过程中的动态加载、求解控制等关键问题,建... 详细信息

管轴压成形省力、高效,但极易发生失稳起皱。通过试验与正交数值模拟相结合,对AA6061铝合金管在锥形模上的轴压失稳起皱进行了研究。在建模过程中建立了AA6061铝合金管材的本构关系,解决了建模过程中的动态加载、求解控制等关键问题,建立并验证了管轴压失稳起皱的有限元模型。通过有限元模拟与试验相结合,分析了模具半锥角对管轴压失稳起皱过程的影响。结果发现,模具半锥角对管轴压失稳过程中的变形方式及位置、管壁应力状态、临界失稳力等均产生重要影响。

关键词： AA6061铝合金管轴压失稳起皱本构关系数值模拟模具半锥角

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Experimental Study on Consolidation Properties of Hydrate-Bearing Fine-Grained Sediments Collected from the Shenhu Area of the Northern South China Sea

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Journal of Ocean University of China 2024年第4期23卷 981-990页

作者： wei Ruchun LIU Lele jiA chao DONG Xiao BU Qingtao ZHANG Yongchao LIU Changling WU Nengyou School of Water Conservancy and Environment University of JinanJinan 250022China Shandong Engineering Research Center of Marine Exploration and Conservation Ocean University of ChinaQingdao 266100China Key Laboratory of Gas Hydrate Ministry of Natural ResourcesQingdao Institute of Marine GeologyQingdao 266237China Institute of Marine Science and Technology Shandong UniversityQingdao 266232China

Mechanical properties of hydrate-bearing fine-grained sediments are crucial to effectively mitigate environmental risks caused by artificial and natural decomposition of natural gas hydrates,and the decomposition can induce laterally confined *** explore the effect of natural gas hydrates on laterally confined compression properties,consolidation tests are conducted on remolded hydrate-free and hydrate-bearing samples by using natural fine-grained sediments collected from the northern South China Sea as the host sediments,and empirical equations are developed based on the analyses of consolidation *** results show that vertical loading induces a reduction in void ratio,and the reduction increases with decreasing hydrate saturation when samples are subjected to the same vertical stress *** compression index of samples is about 0.53 whether there is hydrate or not,but the yield stress of samples increases sharply with increasing hydrate saturation once beyond the critical *** coefficient of volume compression and the coefficient of consolidation of hydrate-bearing samples both increase firstly and then decrease to a relative stable level with increasing vertical stress,and the transition occurs at 200 *** average consolidation degree with elapsed time increases rapidly under low vertical stresses,slowly under median vertical stresses,and under high vertical stresses,the consolidation increases a little faster but still slower than those under low vertical stresses.

关键词： natural gas hydrate stiffness compression index hydraulic permeability geohazard

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Four New Terpyridine Complexes Based Polyoxometalates with[W_(10)O_(32)]^(4-) Anions as High-Efficiency Dual-Site Catalysis for Thioether Oxidation Reaction

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Chinese Journal of Chemistry 2024年第6期42卷 592-598页

作者： Yin Zhang wei-Dong Yu Fang-Qian Wang Xiangnan Wang jiawan Zhou chao Liu Jun Yan Junior Education Department Changsha Normal UniversityChangshaHunan410100 China School of Science Hunan University of Technology and BusinessChangshaHunan410000 China College of Chemistry and Chemical Engineering Central South UniversityChangshaHunan410000 China

Polyoxometalates modified with complex cations have attracted increasing attention because of the fascinating properties and the controllable *** adjusting the synthesis conditions,four new terpyridine complexes based hybrid POMs,[(TPY-H)CuCl]_(4)[W_(10)O_(32)]·2DMF·2H_(2)O(1),[(TPY-H)Cu(DMSO)(H_(2)O)]_(2)[W_(10)O_(32)]·2H_(2)O(2),[(TPY-H)_(2)Cu]_(2)[W_(10)O_(32)]·6DMSO·8H_(2)O(3) and[(TPY-Br)CuCl(DMSO)(H_(2)O)]_(2)[(TPY-Br)CuCl]_(2)[W_(10)O_(32)]·2DMSO·4H_(2)O(4),were prepared by using‘one-pot’***-crystal X-ray diffraction analyses,infrared radiation,etc.,revealed the structural composition of compounds 1—4,which indicates that synthesis conditions have a directional regulatory effect on the compounds *** oxidation catalytic reactions show 1—4 have good catalytic activities,and powder X-ray diffraction and thermogravimetry analysis show 1—4 have superduper catalytic ***,4 has better catalytic activity because of the different structure of terpyridine ***,a possible mechanism of dual-site catalysis by both cations and anions is proposed.

关键词： Polyoxometalates Terpyridine complexes Thioether oxidation Dual-site catalysis Clusters

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