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Chemical modification of ordered/disordered carbon nanostructures for metal hosts and electrocatalysts of lithium-air batteries

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InfoMat 2022年第1期4卷 105-129页

作者： jeongyeon lee Tae Hyung lee Ho Won Jang Ho Seok Park School of Chemical Engineering Convergence Research Center for Energy and Environmental SciencesDepartment of Health Sciences and TechnologySamsung Advanced Institute for Health Sciences and Technology(SAIHST)Sungkyunkwan University(SKKU)SuwonRepublic of Korea Institute of Textiles Clothing The Hong Kong Polytechnic UniversityHung HomHong Kong SARChina Department of Materials Science and Engineering Research Institute of Advanced MaterialsSeoul National UniversitySeoulRepublic of Korea

Although lithium-air batteries(LABs)are considered the promising alternative of existing lithium–ion batteries owing to their high energy density of 11680 W h kg^(-1),their practical applications are limited by the technical issues,such as unstable solid electrolyte interface and dendrite formation from metal anode and insufficient bifunctional activities and durability from cathode *** order to resolve these bottlenecks,carbon nanostructures have been investigated owing to their high surface area,excellent electrical conductivity,electrochemical stability,and various modification ***,we comprehensively review a recent progress on the design of carbon nanostructures for their applications into metal hosts,protection layers,and bifunctional electrocatalysts of *** correlation between the crystalline,electronic,porous,and chemical structures and the electrochemical properties of carbon nanomaterials are discussed depending on their classification and *** chemical modifications,such as morphological control,hierarchical architecturing,heteroatom incorporation,and the formation of composites,for the improved electrochemical performances of anode and cathode will be also ***,we deal with the perspectives for the ongoing obstruction and future guidance.

关键词： bifunctional catalysts carbon nanostructures lithium-air batteries metal anodes surface modification

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Wearable and stretchable conductive polymer composites for strain sensors:How to design a superior one?

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Nano Materials Science 2023年第4期5卷 392-403页

作者： Liwei Lin Sumin Park Yuri Kim Minjun Bae jeongyeon lee Wang Zhang Jiefeng Gao Sun Ha Paek Yuanzhe Piao Department of Applied Bioengineering Graduate School of Convergence Science and TechnologySeoul National UniversitySeoul08826South Korea Department of Neurosurgery Movement Disorder CenterSeoul National University HospitalHypoxia/Ischemia Disease InstituteCancer Research InstituteSeoul National University College of MedicineSeoul03080South Korea School of Chemistry and Chemical Engineering Yangzhou UniversityYangzhouJiangsu225002China Institute of Textiles and Clothing The Hong Kong Polytechnic UniversityHung HomHong Kong SAR999077China Advanced Institutes of Convergence Technology 145 Gwanggyo-roYeongtong-guSuwon-siGyeonggi-do443-270South Korea

Wearable and stretchable strain sensors have potential values in the fields of human motion and health monitoring,flexible electronics,and soft robotic *** wearable and stretchable strain sensors can be directly attached to human skin,providing visualized detection for human motions and personal *** polymer composites(CPC)composed of conductive fillers and flexible polymers have the advantages of high stretchability,good flexibility,superior durability,which can be used to prepare flexible strain sensors with large working strain and outstanding *** review has put forward a comprehensive summary on the fabrication methods,advanced mechanisms and strain sensing abilities of CPC strain sensors reported in recent years,especially the sensors with superior ***,the structural design,bionic function,integration technology and further application of CPC strain sensors are prospected.

关键词： Wearable strain sensors Conductive polymer composites Mechanism Sensing performance

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Sodium-Coordinated Polymeric Phthalocyanines as Stable High-Capacity Organic Anodes for Sodium-Ion Batteries

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Energy & Environmental Materials 2023年第4期6卷 22-30页

作者： jeongyeon lee Yoonbin Kim Soyong Park Kang Ho Shin Gun Jang Min Jun Hwang Daekyu Kim Kyung-Ah Min Ho Seok Park Byungchan Han Dennis K.P.Ng Lawrence Yoon Suk lee Department of Applied Biology and Chemical Technology and Research Institute for Smart Energy The Hong Kong Polytechnic UniversityHung HomKowloon Hong Kong SAR China Department of Chemistry The Chinese University of Hong KongShatinNew Territories Hong Kong SAR China Convergence Research Center for Energy and Environmental Sciences Sungkyunkwan UniversitySuwon Korea Department of Chemical and Biomolecular Engineering Yonsei UniversitySeoul Korea School of Chemical Engineering Sungkyunkwan UniversitySuwon Korea

Sodium-ion batteries(SIBs)have attracted considerable interest as an alternative to lithium-ion batteries owing to their similar electrochemical performance and superior long-term cycle *** materials are regarded as promising anode materials for constructing SIBs with high capacity and good ***,utilization of organic materials is rather limited by their low energy density and poor stability at high current *** overcome these limitations,we utilized a novel polymeric disodium phthalocyanines(pNaPc)as SIB anodes to provide stable coordination sites for Na ions as well as to enhance the stability at high current *** varying the linker type during a one-pot cyclization and polymerization process,two pNaPc anodes with O-(O-pNaPc)and S-linkers(S-pNaPc)were prepared,and their structural and electrochemical properties were *** O-pNaPc binds Na ions with a lower binding energy compared with S-pNaPc,which leads to more facile Na-ion coordination/dissociation when engaged as SIB *** use of O-pNaPc significantly improves the redox kinetics and cycle stability and allows the fabrication of a full cell against Na_(3)V_(2)(PO_(4))_(2)F_(3)/C cathode,which demonstrates its practical application with high energy density(288 Wh kg^(-1))and high power density(149 W kg^(-1)).

关键词： coordination chemistry organic anode phthalocyanine polymerization sodium ion battery

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