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Full-spectrum bi@SrTiO_(3) for bi-directional promotion effects on photocatalytic redox reaction:Insight into intermediates and mechanism

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journal of Rare Earths 2024年第5期42卷 917-929,I0004页

作者： bin Liu Nanhao Zhou jun Liu Xinglei Wang Peter K.j.Robertson Xiaoyuan Chen Chao Chen jianmin Luo Chuanyi Wang School of Chemistry and Civil Engineering Shaoguan UniversityShaoguan512005China Chengdu Customs Technology Center Chengdu610041China Key Laboratory of Pollutant Chemistry and Environmental Treatment College of Chemistry and Environmental ScienceYili Normal UniversityYining835000China School of Chemistry and Chemical Engineering Queen's University BelfastStranmillis RoadBelfastBT95AGUnited Kingdom Guangzhou Institute of Industrial Intelligence(GIII) Guangzhou511400China

The development of full-spectrum photocatalysts active in the near-infrared(NIR)region has gained increasing attention for deleterious pollutant *** integration of plasmonic metals with semico nductors is an effective way to widen the light re sponse range of photocatalysts due to the strong light absorption and fast plasmonic energy transfer of the localized surface plasmon resonance(LSPR).In this work,the full-spectrum responsive bi@SrTiO_(3) was prepared via facile solvothermal chemical *** optimal bi@SrTiO_(3) achieves exceptional photocatalytic Cr(VI)reduction efficiency and tetracycline degradation,realizing bi-directional promotion effects on redox *** to density functional theory(DFT)simulations,the extraordinary photocatalytic performance is attributed to the tunable builtin electric field(IEF)of the Ohmic *** favorable adaptability in real water and high stability of BSTO-25 were proved by experime ntal *** the po ssible photocatalytic mechanism was proposed based on theoretical calculation and experimental ***,the non-toxicity of the BSTO-25 was evaluated by *** cultivation,which further proves the feasibility of treating wastewater with *** work provides a new perspective on constructing full-spectrum-driven photocatalysts for applications dealing with environmental remediation.

关键词： Full-spectrum photocatalysts Localized surface plasmon resonance Ohmic contact Cr(Ⅵ)reduction Antibiotic degradation Rare earths

5月南极涛动对青藏高原西部夏季气温影响的诊断分析

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气象 2024年第3期50卷 344-356页

作者：张宇李清泉余锦华沈新勇毕淼吴清源南京信息工程大学气象灾害教育部重点实验室/气候与环境变化国际合作联合实验室/气象灾害预报预警与评估协同创新中心南京210044 中国气象局气候预测研究重点开放实验室国家气候中心北京100081 南方海洋科学与工程广东省实验室(珠海) 珠海519082 中国气象局气候资源经济转化重点开放实验室重庆市气象科学研究所重庆401147

青藏高原是全球气候变暖最敏感的地区之一,是北半球夏季最大的热源,其气候响应受到广泛关注。然而,有关南极涛动与青藏高原夏季气温的关系和机理知之甚少。为了研究南极涛动与青藏高原夏季气温的关系,基于1979—2020年英国东安哥拉大学... 详细信息

青藏高原是全球气候变暖最敏感的地区之一,是北半球夏季最大的热源,其气候响应受到广泛关注。然而,有关南极涛动与青藏高原夏季气温的关系和机理知之甚少。为了研究南极涛动与青藏高原夏季气温的关系,基于1979—2020年英国东安哥拉大学气候研究中心(CRU)的逐月气温、美国国家海洋和大气管理局(NOAA)的逐月海表面温度和大气环流再分析数据以及南极涛动指数等数据,采用相关、回归、合成分析等方法进行研究。结果表明,北半球夏季青藏高原西部气温与5月南极涛动存在显著负相关,即当5月南极涛动异常偏弱时,夏季青藏高原西部气温异常偏高。其影响过程为,南极涛动为正位相时,在南印度洋中高纬地区出现“负-正-负”的经向“三极子”海温模态,该模态可持续到夏季,在印度洋形成异常的纬向-垂直环流,相应在热带西印度洋和东印度洋-海洋性大陆之间的降水异常导致热带正“偶极子”降水模态,通过该降水模态在青藏高原西部引起异常反气旋环流和下沉运动,有利于高原西部气温偏高。研究结果显示,海洋的热惯性在“延长”南极涛动影响过程中起着重要的桥梁作用,可为青藏高原夏季气温预测提供科学依据。

关键词：南极涛动青藏高原印度洋气温

Nuclear receptors and non-alcoholic fatty liver disease:An update

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Liver Research 2020年第2期4卷 88-93页

作者： Xiao Yang Frank j.Gonzalez Min Huang Huichang bi Guangdong Provincial Key Laboratory of New Drug Design and Evaluation School of Pharmaceutical SciencesSun Yat-sen UniversityGuangzhouChina Laboratory of Metabolism Center for Cancer ResearchNational Cancer InstituteNIHBethesdaMDUSA

Non-alcoholic fatty liver disease(NAFLD)has become the leading cause of chronic liver disease in adults and children *** symptoms of NAFLD range from simple steatosis and non-alcoholic stea-tohepatitis(NASH)to hepatic fibrosis or cirrhosis,even ultimately develops to hepatocellular *** receptors(NRs)are a superfamily of ligand-activated transcription factors,most of which are ligand-activated that control cellular homeostasis in the liver and other tissues.A growing number of studies demonstrated the important role of NRs in *** this review,the current findings on the role of NRs in NAFLD are summarized and future perspectives to target NRs for NAFLD are discussed.

关键词： Nuclear receptors(NRs) Non-alcoholic fatty liver disease(NAFLD) Pregnane X receptor(PXR) Constitutive androstane receptor(CAR) Farnesoid X receptor(FXR) Peroxisome proliferator activated receptor (PPAR) Liver X receptor(LXR)

bionic Flapping Pectoral Fin with Controllable Spatial Deformation

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journal of bionic Engineering 2019年第5期16卷 916-930页

作者： Yueri Cai Lingkun Chen Shusheng bi Guoyuan Li Houxiang Zhang Robotics Institute Beihang UniversityBeijing 100191China Department of Ocean Operations and Civil Engineering Norwegian University of Science and TechnologyAalesund 6025Norway

This paper presents the design of a bionic pectoral fin with fin rays driven by multi-joint *** by the cownose ray,the bionic pectoral fin is modeled and simplified based on the key structure and movement parameters of the cownose ray's pectoral fin.A novel bionic propulsion fin ray composed of a synchronous belt mechanism and a slider-rocker mechanism is designed and optimized in order to minimize the movement errors between the designed fin rays and the spanwise curves observed from the cownose ray,and thereby reproducing an actively controllable flapping deformation.A bionic flapping pectoral fin prototype is developed *** verify that the bionic pectoral fin flaps consistently with the design rule extracted from the cownose *** in a towing tank are set up to test its capability of generating the lift force and the propulsion *** movement parameters within the usual propulsion capabilities of the bionic pectoral fm are utilized:The flapping frequency of 0.2 Hz-0.6 Hz,the flapping amplitude of 3°-18°,and the phase di^rence of 10°-60°.The results show that the bionic pectoral fin with actively controllable spatial deformation has expected propulsion performance,which supports that the natural features of the cownose ray play an important role in designing and developing a bionic prototype.

关键词： cownose ray bionic pectoral fin controllable deformation multiple fin rays propulsion perfonnance

Corrosion and aging of organic aviation coatings:A review

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Chinese journal of Aeronautics 2023年第4期36卷 1-35页

作者： Tianyu ZHANG Teng ZHANG Yuting HE Yuchen WANG Yaping bi Air Force Engineering University Xi’an 710038China

Organic anticorrosive aviation coatings are an effective guarantee for aviation structure,since aircraft corrosion can lead to great economic *** it is during ground parking or air cruises,organic aviation coatings are important barriers to the corrosion of aviation *** the vigorous development of the aviation industry,organic aviation coatings continue to meet the challenges of diverse,complex,and harsh service *** review analyzes and summarizes the research status of the types and development of organic aviation coatings,influencing factors and mechanisms,experimental methods,calendar life research methods,and modification *** also summarizes the research results that have been achieved to *** current research deficiencies in the equivalence relationship between atmospheric exposure and artificial acceleration,failure criteria and life prediction were pointed out,and nano-modification technology,and future research strategies and directions that need breakthroughs are discussed.

关键词： Aging Calendar life Classification Corrosion Experimental methods Modification Organic aviation coatings

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纳米纤维素/聚己内酯的等温结晶动力学

塑料 2024年第3期53卷 184-188页

作者：刘枫吴鹏张宇柯洋陈绪煌毕斯雯湖北工业大学材料与化学工程学院湖北武汉430068

利用差示扫描量热仪(DSC)研究了聚己内酯(PCL)与纳米纤维素复合材料的等温结晶动力学,采用了Avrami理论来解析结晶过程中成核和生长的动力学。研究结果表明,纳米纤维素(CNC)诱导PCL异相成核能有效提高PCL基体的结晶速率。在等温结晶过程... 详细信息

利用差示扫描量热仪(DSC)研究了聚己内酯(PCL)与纳米纤维素复合材料的等温结晶动力学,采用了Avrami理论来解析结晶过程中成核和生长的动力学。研究结果表明,纳米纤维素(CNC)诱导PCL异相成核能有效提高PCL基体的结晶速率。在等温结晶过程中,相对分子质量为300和3000的聚乙烯亚胺(PEI)修饰的CNC(CNC-P1、CNC-P2)能够将PCL的半结晶时间由5.19 s降低至1.70和2.07 s。为研究修饰后CNC对PCL结晶结构的影响,结合Thomson-Gibbs方程和Lauritzen-Hoffman方程计算了PCL的折叠表面自由能和片晶厚度,结果表明,加入修饰后的CNC导致PCL的折叠表面自由能显著降低,分别由0.024 j/m^(2)降低至0.179 j/m^(2)和0.020 j/m^(2),片晶厚度由18.6 nm增大至20.2 nm和18.9 nm。修饰后的CNC对于PCL的等温结晶动力学及结晶特性均有显著的影响。

关键词：聚己内酯纳米纤维素成核剂等温结晶动力学片晶厚度

Covalent triazine-based frameworks confining cobalt single atoms for photocatalytic CO_(2) reduction and hydrogen production

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journal of Materials Science & Technology 2022年第21期116卷 41-49页

作者： Guocheng Huang Guiyun Lin Qing Niu jinhong bi Ling Wu Department of Environmental Science and Engineering Fuzhou UniversityMinhouFujian 350108China State Key Laboratory of Photocatalysis on Energy and Environment Fuzhou UniversityMinhouFujian 350108China

Single-atom catalysts(SACs)have emerged as an advanced frontier in heterogeneous catalysis due to their potential to maximize the atomic ***,covalent triazine-based frameworks(CTFs)confining cobalt single atoms(Co-SA/CTF)photocatalysts have been synthesized and used for efficient CO_(2) reduction and hydrogen production under visible light *** resulted Co-SA/CTF demonstrate excellent photocatalytic activity,with the CO and H2 evolution rates reaching 1665.74μmol g^(−1) h^(−1) and 1293.18μmol g^(−1) h^(−1),respectively,far surpassing those of Co nanoparticles anchored CTF and pure CTF.A variety of instrumental analyses collectively indicated that Co single atoms sites served as the reaction center for activating the adsorbed CO_(2) molecules,which significantly improved the CO_(2) reduction ***,the introduction of Co single atoms could accelerate the separation/transfer of photogenerated charge carriers,thus boosting the photocatalytic *** study envisions a novel strategy for designing efficient photocatalysts for energy conversion and showcases the application of CTFs as attractive support for confining metal single atoms.

关键词： Covalent triazine-based frameworks Co single atoms Photocatalysis CO_(2)reduction Hydrogen evolution

空穴效应对连杆小头轴承润滑及动力学特性的影响

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内燃机工程 2024年第5期45卷 47-56页

作者：毕玉华段磊磊马雄张国强唐明超昆明理工大学云南省内燃机重点实验室昆明650500 昆明云内动力股份有限公司昆明650217

将热弹流理论与活塞连杆组柔性多体动力学分析结合,利用AVL EXCITE软件建立连杆小头轴承润滑模型,并以油膜压力、轴心轨迹及润滑油填充率确定连杆小头轴承空穴位置,研究空穴效应对连杆小头轴承润滑及动力学特性产生的影响。结果表明,在... 详细信息

将热弹流理论与活塞连杆组柔性多体动力学分析结合,利用AVL EXCITE软件建立连杆小头轴承润滑模型,并以油膜压力、轴心轨迹及润滑油填充率确定连杆小头轴承空穴位置,研究空穴效应对连杆小头轴承润滑及动力学特性产生的影响。结果表明,在发动机整个循环工况中连杆小头轴承一直存在空穴现象。考虑空穴后平均峰值油膜压力降低了6.5 MPa,平均油膜厚度降低了1.35μm,活塞销相对连杆小头轴承的速度及加速度分别增大了1.57μm/s和0.25μm/s^(2),连杆小头轴承润滑性能减弱,所受冲击增大。

关键词：空穴效应连杆小头轴承润滑

Further investigation on the fusion of ^(6)Li with ^(209)bi target at near-barrier energies

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Chinese Physics C 2024年第7期48卷 106-117页

作者：张高龙焦振威张广鑫 M.R.Cortes 胡世鹏钱建强 D.Mengoni 屈卫卫李聪博郑云张焕乔孙慧斌王楠张春雷 j.j.Valiente-Dobón D.Testov M.Mazzocco A.Gozzelino C.Parascandolo D.Pierroutsakou M.La Commara A.Goasduff D.Bazzacco D.R.Napoli F.Galtarossa F.Recchia A.Illana S.Bakes I.Zanon S.Aydin G.de Angelis M.Siciliano R.Menegazzo S.M.Lenzi j.L.Ferreira j.Rangel Serkan Akkoyun L.F.Canto j.Lubian School of Physics Beihang UniversityBeijing 100191China Sino-French Institute of Nuclear Engineering and Technology Sun Yat-Sen UniversityZhuhai 519082China Instituto de Física Universidade Federal Fluminense24210-340NiteróiRio de JaneiroBrazil Institute for Advanced Study in Nuclear Energy&Safety Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Research and Manufacture of High Purity Germanium Materials and Fetectors Shenzhen UniversityShenzhen 518060China INFN Sezione di PadovaPadovaItaly Dipartimento di fisica Astronomia dell'Universita di padova PadovaItaly State Key Laboratory of Radiation Medicine and Protection School of Radiation Medicine and ProtectionSoochow UniversitySuzhou 215123China China Institute of Atomic Energy Beijing 102413China The Key Laboratory of Beam Technology and Material Modification of Ministry of Education College of Nuclear Science and TechnologyBeijing Normal UniversityBeijing 100875China INFN Laboratori Nazionali di LegnaroI-35020 LegnaroItaly INFN Sezione di NapoliI-80126 NapoliItaly Dipartimento di Farmacia Universitàdi Napoli"Federico II"I-80131 NapoliItaly Department of Natural and Mathematical Sciences Faculty of EngineeringTarsus University33480 MersinTurkiye Physics Division Argonne National LaboratoryLemont-ILUSA Departamento de Matemaética Física e Computaç˜ao Universidade do Estado do Rio de JaneiroFaculdade de Tecnologia27537-000ResendeRio de JaneiroBrazil Department of Physics Sivas Cumhuriyet UniversitySivasTurkey Instituto de Física Universidade Federal do Rio de JaneiroCP 6852821941-972Rio de JaneiroBrazil

The complete and incomplete fusion cross sections for ^(6)Li+^(209)bi were measured using the in-beamγ-ray method around the Coulomb *** cross sections of(deuteron captured)incomplete fusion(ICF)products were re-quantified experimentally for this reaction *** results reveal that the ICF cross section is equivalent to that of complete fusion(CF)above the Coulomb barrier and dominant near or below the Coulomb barrier.A theoretical calculation based on the continuum discretized coupled channel(CDCC)method was performed for the aforementioned CF and ICF cross sections;the result is consistent with the *** universal fusion function(UFF)was also compared with the measured CF cross section for different barrier parameters,demonstrating that the CF suppression factor is significantly influenced by the choice of potential,which can reflect both dynamic and static effects of breakup on the fusion process.

关键词： cross section incomplete fusion suppression factor weakly bound nuclei