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Exploratory growth and characterization of caNdAl_(3)O_(7) single crystal with nonsymmetric structure in tetragonal family

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journal of Rare Earths 2025年第1期43卷 153-161,I0006页

作者： Xiangkang peng Fapeng Yu State Key Laboratory of crystal Materials Institute of Crystal MaterialsShandong UniversityJinan250100China

The new component of melilite type crystal caNdAl_(3)O_(7)(cNA)was grown by the czochralski pulling *** crystal structure analysis was *** is found that the cNA crystal belongs to the tetragonal system with P-421m space *** cell parameters a=b=0.77461 nm and c=0.51089 *** density and Mohs hardness of cNA crystal are 4.08 g/cm^(3) and 5.45,*** specific heat of the crystal is 0.57-0.77 j/(g·K)in the temperature range of 30-300℃.X-ray photoelectron spectro scopy(XPS)shows that the crystal has stable atomic valence states and chemical *** vibration state of polyhedra groups in the crystal was measured by Raman spectra,and the piezoelectric response was analyzed based on the calculated results for the polyhedra polarization dipole *** relative dielectric permittivity of the cNA crystal at room temperature was determined to be 11.80 and the electrical resistivity was measured to be on the order of 5×10^(6)Ω·cm at 800℃.

关键词： Piezoelectric Melilite crystal growth High-temperature czochralski Rareearths

Anomalous open orbits in Hofstadter spectrum of chern insulator

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Science china(Physics,Mechanics & Astronomy) 2025年第3期Mechanics & Astronomy) .卷 143-148页

作者： Haijiao ji peng Zhou Noah F.Q.Yuan Hua jiang Haiwen Liu X.c.Xie center for Advanced Quantum Studies Department of Physics Beijing Normal University Tsung-Dao Lee Institute Shanghai Jiao Tong University Department of Mathematics UC Berkeley Institute for Nanoelectronic Devices and Quantum computing Fudan University International center for Quantum Materials School of Physics Peking University Hefei National Laboratory

The nontrivial band topology of chern insulator can enrich the content of its Hofstadter butterfly spectra, which is closely related to recent experiments in twisted bilayer graphene and cold atom systems. We investigate the Hofstadter spectrum for various models of chern insulators under a rational flux φ0/q, here φ0=h/e and q being an integer. We find the number of splitting subbands is |q-c| with c denoting the chern number of parent band. Importantly, anomalous open-orbital subbands with chern numbers q-1 and-q-1 emerge unexpectedly, which are beyond the parameter window（-q/2, q/2） of the Diophantine equation studied by Thouless-Kohmoto-Nightingale-den Nijs [Phys. Rev. Lett. 49, 405（1982）]. The emergence of anomalous open orbits can be traced by analyzing the evolution of the Hofstadter spectrum, identifying as a new type of topological phase transition. These novel findings not only pinpoint the peculiar Hofstadter spectrum of chern insulator, but also provide routes to study exotic characteristics beyond the Landau level physics.

关键词： Hofstadter spectrum topological phase transition open orbit

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Analyzing carbon emissions and influencing factors in chengdu-chongqing urban agglomeration counties

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journal of Environmental Sciences 2025年第5期151卷 640-651页

作者： Zhang Heng Lu Wenfu peng Lindan Zhang Key Laboratory of the Evaluation and Monitoring of Southwest Land Resources(Ministry of Education) Sichuan Normal UniversityChengdu 610068China The Institute of Geography and Resources Science Sichuan Normal UniversityChengdu 610068China

Majority of carbon emissions originate from fossil energy consumption,thus necessitating calculation and monitoring of carbon emissions from energy *** this study,we utilized energy consumption data from Sichuan Province and chongqing Municipality for the years 2000 to 2019 to estimate their statistical carbon *** then employed nighttime light data to downscale and infer the spatial distribution of carbon emissions at the county level within the chengdu-chongqing urban ***,we analyzed the spatial pattern of carbon emissions at the county level using the coefficient of variation and spatial autocorrelation,and we used the Geographically and Temporally Weighted Regression(GTWR)model to analyze the influencing factors of carbon emissions at this *** results of this study are as follows:(1)from 2000 to 2019,the overall carbon emissions in the chengdu-chongqing urban agglomeration showed an increasing trend followed by a decrease,with an average annual growth rate of 4.24%.However,in recent years,it has stabilized,and 2012 was the peak year for carbon emissions in the chengdu-chongqing urban agglomeration;(2)carbon emissions exhibited significant spatial clustering,with high-high clustering observed in the core urban areas of chengdu and chongqing and low-low clustering in the southern counties of the chengdu-chongqing urban agglomeration;(3)factors such as GDP,population(Pop),urbanization rate(Ur),and industrialization structure(Ic)all showed a significant influence on carbon emissions;(4)the spatial heterogeneity of each influencing factor was evident.

关键词： carbon emissions chengdu-chongqing urban agglomeration Spatial autocorrelation Geographically and temporally weighted regression

Human activities are intensifying the spatial variation of landslides in the Yellow River Basin

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Science Bulletin 2025年第2期70卷 263-272页

作者： Naiman Tian Hengxing Lan Langping Li jianbing peng Bojie Fu john j.clague State Key Laboratory of Resources and Environmental Information System Institute of Geographic Sciences and Natural Resources ResearchChinese Academy of SciencesBeijing 100101China college of Geological Engineering and Geomatics Chang’an UniversityXi’an 710054China University of chinese Academy of Sciences Beijing 100049China Key Laboratory of Ecological Geology and Disaster Prevention Ministry of Natural ResourcesXi’an 710054China State Key Laboratory of Urban and Regional Ecology Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China State Key Laboratory of Earth Surface Processes and Resource Ecology Faculty of Geographical ScienceBeijing Normal UniversityBeijing 100875China Department of Earth Sciences Simon Fraser UniversityBurnaby BCV5A 1S6Canada

Human activities are a triggering factor for landslides in the Yellow River Basin(YRB,china).However,the extent to which the spatial distribution of landslides is affected by human activities is *** constructed a human activity intensity index(HAII)based on nighttime light data and land cover *** and dominance analyses were used to compare the effects of the HAII,precipitation,distance to river,distance to fault,topographic relief and slope on the landslides spatial density(LSD).The results showed that in the YRB,the HAII,as a dominance influencing factor,had a significant positive influence on the ***,regional differences in the human disturbance of nature intensify the spatial variation of *** quantify the intensity of human disturbance to nature,a human-nature conflict index(HNcI)is constructed by quantifying the difference between the slope distributions of artificial and natural *** results show that in the middle section of the YRB,humans are developing more steep mountainous areas,leading to more dense *** study provides a reference for landslide risk management and land use planning in the YRB.

关键词： Landslide Human activities Spatial variation Human-nature conflict Yellow River Basin

Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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journal of Energy chemistry 2025年第1期100卷 730-738页

作者： peng Zheng Wang Zhou Ying Mo Biao Zheng Miaomiao Han Qin Zhong Wenwen Yang peng Gao Lezhi Yang jilei Liu college of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean EnergyHunan Province Key Laboratory for Advanced Carbon Materials and Applied TechnologyHunan UniversityChangsha 410082HunanChina Greater Bay Area Institute for Innovation Hunan UniversityGuangzhou 511300GuangdongChina changsha Research Institute of Mining&Metallurgy co. LTD.Changsha 410017HunanChina

Hard carbon (Hc) has been considered as promising anode material for sodium-ion batteries (SIBs).The optimization of hard carbon’s microstructure and solid electrolyte interface (SEI) property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectroscopy/electrochemical impedance spectroscopy (FTIR/EIS) and X-ray photoelectron spectroscopy (XPS) analysis demonstrate the presence of more Bc3and less B–c–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping content exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： Hard carbon Sodium-ion batteries Boron doping Pore structure Electrode/electrolyte interphases

Microplastics enhance the adsorption capacity of zinc oxide nanoparticles:Interactive mechanisms and influence factors

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journal of Environmental Sciences 2025年第1期147卷 665-676页

作者： Weiping Xiong Min Hu Siying He Yuhang Ye Yinping Xiang Haihao peng Zhaomeng chen Zhengyong Xu Honglin Zhang Weixiang Li Shudian peng college of Environmental Science and Engineering Hunan University and Key Laboratory of Environmental Biology and Pollution Control(Hunan University)Ministry of EducationChangsha 410082China Hunan Boke Environmental Engineering co.Ltd. Hengyang 421099China college of Environmental Protection and Safety Engineering University of South ChinaHengyang 421001China Hunan Modern Environmental Technology co.Ltd. Changsha 410004China

Microplastics(MPs)are of particular concern due to their ubiquitous occurrence and propensity to interact and concentrate various waterborne contaminants from aqueous *** on the interaction and joint toxicity of MPs on engineered nanoparticles(ENPs)are exhaustive,but limited research on the effect of MPs on the properties of ENPs in multisolute ***,the effect of MPs on adsorption ability of ENPs to antibiotics was investigated for the first *** results demonstrated that MPs enhanced the adsorption affinity of ENPs to antibiotics and MPs before and after aging showed different effects on *** polyamide prevented aggregation of ZnONPs by introducing negative charges,whereas virgin polyamide affected ZnONPs with the help of electrostatic ***-IR and XPS analyses were used to probe the physicochemical interactions between ENPs and *** results showed no chemical interaction and electrostatic interactionwas the dominant force between ***,the adsorption rate of antibiotics positively correlated with pH and humic acid but exhibited a negative correlation with ionic *** study highlights that ENPs are highly capable of accumulating and transporting antibiotics in the presence of MPs,which could result in a widespread distribution of antibiotics and an expansion of their environmental risks and toxic effects on *** also improves our understanding of the mutual interaction of various co-existing contaminants in aqueous environments.

关键词： Microplastics Engineered nanoparticles Adsorption Tetracycline

correlation between the rock mass properties and maximum horizontal stress:A case study of overcoring stress measurements

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International journal of Minerals,Metallurgy and Materials 2025年第1期32卷 39-48页

作者： peng Li Meifeng cai Shengjun Miao Yuan Li Yu Wang Key Laboratory of Ministry of Education for Efficient Mining and Safety of Metal Mines University of Science and Technology BeijingBeijing 100083China State Key Laboratory of coal Resources and Safe Mining China University of Mining and TechnologyXuzhou 221116China

Understanding the mechanical properties of the lithologies is crucial to accurately determine the horizontal stress *** investigate the correlation between the rock mass properties and maximum horizontal stress,the three-dimensional(3D)stress tensors at 89 measuring points determined using an improved overcoring technique in nine mines in china were adopted,a newly defined characteristic parameter c_(ERP)was proposed as an indicator for evaluating the structural properties of rock masses,and a fuzzy relation matrix was established using the information distribution *** results indicate that both the vertical stress and horizontal stress exhibit a good linear growth relationship with *** is no remarkable correlation between the elastic modulus,Poisson's ratio and depth,and the distribution of data points is scattered and ***,there is no obvious relationship between the rock quality designation(RQD)and *** maximum horizontal stress σ_(H) is a function of rock properties,showing a certain linear relationship with the c_(ERP)at the same *** addition,the overall change trend of σ_(H) determined by the established fuzzy identification method is to increase with the increase of c_(ERP).The fuzzy identification method also demonstrates a relatively detailed local relationship betweenσ_H and c_(ERP),and the predicted curve rises in a fluctuating way,which is in accord well with the measured stress data.

关键词： overcoring stress measurements elastic modulus Poisson's ratio rock quality designation maximum horizontal stress fuzzy identification

The influence mechanism of environmental factors on DGT adsorbing sulfonamides and the migration between water and sediment

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journal of Environmental Sciences 2025年第5期151卷 347-359页

作者： peng Zhang jingfeng Yan Hao ji Linke Ge Yanying Li School of Environmental Science and Technology Shaanxi University of Science&TechnologyXi’an 710021China college of Environmental Sciences and Engineering Dalian Maritime UniversityDalian 116026China

Obtaining the sulfonamides(SAs)concentrations in the water body and sediment bulk was a prerequisite to reveal their transport and partitioning behavior in sediment-water environments and accurately assess their ecological *** the present study,the influences of multifactor interactions on the performance of o-DGTs with XAD-18 binding gels were analyzed by central combination experiments and response surfaces analysis,in which the target compounds were 9 *** results indicated that dissolved organic matter(DOM),pH,and suspended particulate matter(SS)had significant effects on the o-DGT sampling,whereas this o-DGT was independent of the ionic strength(IS).concentning the composite influence of the four factors,the interaction between DOM and SS posed the most significant effect on all 9 SAs ***,an o-DGT and DIFSmodel was applied to explore the SAs migration between the water-sediments *** difference between desorption rate(k_(b))and adsorption rates(k_(f))values suggested that the kinetics of SAs was dominated by ***,the short-term sediment-water partitioning of SAs was clarified on the basis of distribution coefficient(K_(dl))for the labile SAs,among which the sulfadiazine(SDZ)had the largest labile *** ability of sediments to release SAs to the liquid phase as a sink was determined by response time(T_(c)).Among the 9 SAs,the longterm release of soseulfamethoxypyridazine(SMP)from the solid phase of sediments would have a potential risk to the aquatic environment,to which more attention should be paid in the future.

关键词： Sulfonamides O-DGT Water-sediments interface DIFS Distribution

critical new insights into the interactions of hexafluoropropylene oxide-dimer acid(GenX or HFPO-DA)with albumin at molecular and cellular levels

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journal of Environmental Sciences 2025年第3期149卷 88-98页

作者： Shi-Ya peng Ya-Di Yang Rong Tian Naihao Lu jiangxi Key Laboratory of Green chemistry College of Chemistry and Chemical EngineeringJiangxi Normal UniversityNanchang 330022China

A key characteristic to be elucidated,to address the harmful health risks of environmental perfluorinated alkyl substances(PFAS),is their binding modes to serum albumin,the most abundant protein in *** oxide-dimer acid(GenX or HFPO-DA)is a new industrial replacement for the widespread linear long-chain ***,the detailed interaction of new-generation short-chain PFAS with albumin is still ***,the binding characteristics of bovine serum albumin(BSA)to GenX were explored at the molecular and cellular *** found that this branched short-chain GenX could bind to BSA with affinity lower than that of legacy linear long-chain perfluorooctanoic acid(PFOA).Site marker competitive study and molecular docking simulation revealed that GenX interacted with subdomain IIIA to form BSA-GenX *** with its weaker affinity to albumin protein,the cytotoxicity of branched short-chain GenX was less susceptible to BSA binding compared with that of the linear long-chain *** contrast to the significant effects of strong BSA-PFOA interaction,the weak affinity of BSA-GenX binding did not influence the structure of protein and the cytotoxicity of *** detailed characterization and direct comparisons of serum albumin interaction with new generation short-chain GenX will provide a better understanding for the toxicological properties of this new alternative.

关键词： GenX Protein binding Albumin cytotoxicity Risk assessment