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Significantly Enhanced Energy Storage Performances of PEI-based Composites Utilizing Surface Functionalized ZrO_(2) Nanoparticles for High-Temperature Application

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Chinese Journal of Polymer Science 2024年第3期42卷 322-332,I0006页

作者： Qing-Qing Liu Qiu-Hao Lin Xiao-Dong Qi Nan Zhang Ting Huang jing-hui Yang Yong Wang School of Chemistry Southwest Jiaotong UniversityChengdu 610031China Key Laboratory of Advanced Technologies of Materials Ministry of Education of ChinaSouthwest Jiaotong UniversityChengdu 610031China

Polymer dielectrics with a high energy density and an available energy storage capacity have been playing an important role in advanced electronics and power systems. Nevertheless, the use of polymer dielectrics in harsh environments is limited by their low energy density at high temperatures. Herein, zirconium dioxide(ZrO_(2)) nanoparticles were decorated with amino group utilizing 4,4-methylenebis(phenyl isocyanate)(AMEO) and successfully incorporated into polyetherimide(PEI) matrix. The dielectric properties, breakdown strength, and energy storage performances of PEI/ZrO_(2)-AMEO nanocomposites were investigated from 25 ℃ to 150 ℃. It is found that the combination of moderate bandgap ZrO_(2) with modest dielectric constant and polar groups at interface with deep trap can offer an available strategy to simultaneously increase the dielectric constant and breakdown strength of polymer dielectrics. As a result, the composites containing ZrO_(2)-AMEO exhibit excellent energy storage performance at elevated temperatures. Specially, the PEI-based composites with 3 vol% ZrO_(2)-AMEO display a maximum discharged energy density(U_(d)) of 3.1 J/cm^(3) at 150 ℃, presenting 90% higher than that of neat PEI. This study may help to better develop the polymer-based dielectric composite applied at elevated temperatures.

关键词： Polyetherimide High temperature dielectric ZrO_(2) Interface

Predictive performance of the variation rate of the driving pressure on the outcome of invasive mechanical ventilation in patients with acute respiratory distress syndrome

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Chinese Journal of Traumatology 2024年第2期27卷 107-113页

作者： hui-Dan jing Jun-Ying Tian Wei Li Bing-Ling He Hong-Chao Li Fu-Xia Jian Cui Shang Feng Shen Department of Intensive Care Unit The Affiliated Hospital of Guizhou Medical UniversityGuiyang 550004China Department of Intensive Care Unit Army Medical Center of PLAChongqing400042China College of Foreign Languges Chongqing Medical UniversityChongqing400016China

Purpose:To assess the value of the driving pressure variation rate(ΔP%)in predicting the outcome of weaning from invasive mechanical ventilation in patients with acute respiratory distress syndrome.Methods:In this case-control study,a total of 35 patients with moderate-severe acute respiratory distress syndrome were admitted to the intensive care unit between January 2022 and December 2022 and received invasive mechanical ventilation for at least 48 h were enrolled.Patients were divided into successful weaning group and failed weaning group depending on whether they could be removed from ventilator support within 14 days.Outcome measures including driving pressure,PaO2:FiO2,and positive end-expiratory pressure,etc.were assessed every 24 h from day 0 to day 14 until successful weaning was achieved.The measurement data of non-normal distribution were presented as median(Q1,Q3),and the differences between groups were compared by Wilcoxon rank sum test.And categorical data use the Chi-square test or Fisher's exact test to compare.The predictive value ofΔP%in predicting the outcome of weaning from the ventilator was analyzed using receiver operating characteristic curves.Results:Of the total 35 patients included in the study,17 were successful vs.18 failed in weaning from a ventilator after 14 days of mechanical ventilation.The cut-off values of the medianΔP%measured by Operator 1 vs.Operator 2 in the first 4 days were≥4.17%and 4.55%,respectively(p<0.001),with the area under curve of 0.804(sensitivity of 88.2%,specificity of 64.7%)and 0.770(sensitivity of 88.2%,specificity of 64.7%),respectively.There was a significant difference in mechanical ventilation duration between the successful weaning group and the failure weaning group(8(6,13)vs.12(7.5,17.3),p=0.043).The incidence of ventilator-associated pneumonia in the successful weaning group was significantly lower than in the failed weaning group(0.2‰vs.2.3‰,p=0.001).There was a significant difference noted between these 2 groups in the 28-day mortality(11.8%vs.66.7%,

关键词： Driving pressure Driving pressure variation rate Acute respiratory distress syndrome Mechanical ventilation

Integrated Path‑Following and Fault‑Tolerant Control for Four‑Wheel Independent‑Driving Electric Vehicles

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Automotive Innovation 2022年第3期5卷 311-323页

作者： Yuwei Tong Cong Li Gang Wang hui jing School of Mechanical and Electrical Engineering Guilin University of Electronic TechnologyGuilinChina School of Mechanical Engineering Guilin University of Aerospace TechnologyGuilinChina

Autonomous vehicles are prone to instability when the motors of the four-wheel independent-driving electric vehicles fail at high driving speed on low-adhesion roads.To improve the vehicle tracking performance in the expected path and ensure vehicle stability when the motor fails,this paper designs an integrated path-following and passive fault-tolerant controller.The path-following controller is designed to improve the vehicle path-following performance based on model predictive control(MPC),while the passive fault-tolerant controller is used to ensure vehicle stability when the motor fails.First,a vehicle dynamic model is established and simplified,and an MPC controller based on a state-space equation is designed.Then,taking the motor fault as a fault factor,a first-order sliding mode fault-tolerant controller is developed.The first-order sliding mode fault-tolerant controller takes the vehicle’s yaw rate and sideslip angle into account.Furthermore,to address the chattering problem of the traditional first-order sliding mode fault-tolerant controller,a second-order sliding mode fault-tolerant controller with a disturbance observer is developed.Finally,the developed controller is tested using the Simulink/Carsim platform and applied to a Raspberry Pi 4B for controller hardware-in-the-loop experiment.Simulation and experi-ment results show the practicability and effectiveness of the proposed integrated control strategy.

关键词： Fault-tolerant control Model predictive control Second-order sliding mode control Path following

Competitive assembling strategy to construct carbon nitride homojunctions for boosting photocatalytic performance

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Journal of Materials Science & Technology 2024年第5期172卷 23-32页

作者： Hua-Wei Zhang Yuan-Yuan Li Bo Li jing-hui Shi Tao Huang Gui-Fang Huang Anlian Pan Wangyu Hu Wei-Qing Huang School of Physics&Electronic Engineering Zhengzhou University of Light IndustryZhengzhou 450002China Key Laboratory for Micro/Nano Optoelectronic Devices of Ministry of Education&Hunan Provincial Key Laboratory of Low-Dimensional Structural Physics and Devices School of Physics and ElectronicsHunan UniversityChangsha 410082China College of Materials Science and Engineering Hunan UniversityChangsha 410082China

Both morphology and composition have a great influence on the properties and functions of materials,however,how to rational modulate both of them to achieve their synergistic effects has been a longstanding expectation.Herein,we demonstrate a competitive assembling strategy for the construction of metal-free graphite carbon nitride(CN)homojunctions in which morphology and composition can be easily controlled simultaneously by only changing the ratio of assembly raw materials.These homojunctions are comprised of porous nanotubular S-doped CN(SCN)grafted with CN nanovesicles,which are derived from thermal polycondensation of melamine-thiocyanuric acid(M-T)/melamine-cyanuric acid(M-C)supramolecular hybrid blocks.This unique architecture and component engineering endows the novel SCN-CN homojunction with abundant active sites,enhanced visible trapping ability,and intimate interface contact.As a result,the synthesized SCN-CN homojunctions demonstrate high photocatalytic activity for hydrogen evolution and pollutant degradation.This developed strategy opens up intriguing opportu-nities for the rational construction of intricate metal-free heterostructures with controllable architecture and interfacial contact for applications in energy-related fields.

关键词： Competitive assembling strategy Supramolecular hybrid blocks Homojunctions Graphite carbon nitride Photocatalytic

Phase-controlled asymmetric optomechanical entanglement against optical backscattering

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Science China(Physics,Mechanics & Astronomy) 2023年第3期66卷 66-75页

作者： jing-Xue Liu Ya-Feng Jiao Ying Li Xun-Wei Xu Qiong-Yi He hui jing Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Department of Physics and Synergetic Innovation Center for Quantum Efects and ApplicationsHunan Normal UniversityChangsha 410081China Laboratory of Chemical Biology&Traditional Chinese Medicine Research Ministry of Education College of Chemistry and Chemical EngineeringHunan Normal UniversityChangsha 410081China State Key Laboratory for Mesoscopic Physics School of PhysicsFrontiers Science Center for Nano-optoelectronicsCollaborative Innovation Center of Quantum MatterPeking UniversityBeijing 100871China Collaborative Innovation Center of Extreme Optics Shanxi UniversityTaiyuan 030006China Synergetic Innovation Academy for Quantum Science and Technology Zhengzhou University of Light IndustryZhengzhou 450002China

Quantum entanglement plays a key role in both understanding the fundamental aspects of quantum physics and realizing various quantum devices for practical applications. Here we propose how to achieve a coherent switch of optomechanical entanglement in an optical whispering-gallery-mode resonator, by tuning the phase difference of the driving lasers. We find that the optomechanical entanglement and the associated two-mode quantum squeezing can be well tuned in a highly asymmetric way,providing an efficient way to protect and enhance quantum entanglement against optical backscattering, in comparison with conventional symmetric devices. Our findings shed a new light on improving the performance of various quantum devices in the practical noisy environment, which is crucial in such a wide range of applications as noise-tolerant quantum processing and the backscattering-immune quantum metrology.

关键词： quantum entanglement optical backscattering optomechanics

Graphene from microwave-initiated upcycling of waste polyethylene for electrocatalytic reduction of chloramphenicol

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Chinese Chemical Letters 2024年第4期35卷 187-192页

作者： Qiang Cao Xue-Feng Cheng Jia Wang Chang Zhou Liu-Jun Yang Guan Wang Dong-Yun Chen jing-hui He Jian-Mei Lu College of Chemistry Chemical Engineering and Materials ScienceCollaborative Innovation Center of Suzhou Nano Science and TechnologySoochow UniversitySuzhou 215123China

Waste polyolefin plastics, accounting for 50% of all plastic waste, represent a tremendously unexploited carbon source. Efficiently upcycling polyolefin waste into value-added carbon materials for waste water treatment avoiding using noble metals is challenging but economically and environmentally sustainable. In this work, MAX-Ti_(3)AlC_(2) supported Fe selectively catalyzes polyolefin into few-layered graphene in 5 min under microwave treatment. Graphene and MAX supported Fe(Fe@MLC) can completely(99.9%)degrade chloramphenicol(CAP) within 60 min, retain robust after 10 cycles and work efficiently at a wide p H range(3.87–13.03), avoiding the usage of noble metal. Moreover, the electrochemical active surface area(ECSA) of Fe@MLC is 2.7 times higher than that of commercial Pt/C. This work provides a cheap and efficient catalyst that promotes deconstruction of plastic wastes and indirectly degrades antibiotics thereby realizes the treatment of waste water with waste plastic.

关键词： Microwave Ti_(3)AlC_(2) Electrochemistry Dechlorination Chloramphenicol

Anti-parity-time symmetry hidden in a damping linear resonator

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Science China(Physics,Mechanics & Astronomy) 2023年第10期66卷 22-32页

作者： Xun-Wei Xu Jie-Qiao Liao hui jing Le-Man Kuang Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Key Laboratory for Matter Microstructure and Function of Hunan ProvinceDepartment of Physics and Synergetic Innovation Center for Quantum Effects and ApplicationsHunan Normal UniversityChangsha 410081China

Phase transition from the over-damping to under-damping states is a ubiquitous phenomenon in physical systems. However, what kind of symmetry is broken associated with this phase transition remains unclear. Here, we discover that this phase transition is determined by an anti-parity-time(anti-PT) symmetry hidden in a single damping linear resonator, which is significantly different from the conventional anti-PT-symmetric systems with two or more modes. We show that the breaking of the anti-PT symmetry yields the phase transition from the over-damping to under-damping states, with an exceptional point(EP) corresponding to the critical-damping state. Moreover, we propose an optomechanical scheme to show this anti-PT symmetry breaking by using the optical spring effect in a quadratic optomechanical system. We also suggest an optomechanical sensor with the sensitivity enhanced significantly around the EPs for the anti-PT symmetry breaking. Our work unveils the anti-PT symmetry hidden in damping oscillations and hence opens up new possibilities for exploiting wide anti-PT symmetry applications in single damping linear resonators.

关键词： anti-parity-time symmetry exceptional points damping linear resonator optomechanics

Research progress of rare earth composite shielding materials

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Journal of Rare Earths 2023年第1期41卷 32-41页

作者： hui jing Laiyao Geng Shaoyu Qiu Huawei Zou Mei Liang Dan Deng The State Key Laboratory of Polymer Materials Engineering Polymer Research Institute of Sichuan UniversityChengdu 610065China Science and Technology on Reactor Fuel and Materials Laboratory Nuclear Power Institute of ChinaChengdu 610213China

With the rapid development of nuclear technology,nuclear protection has received extensive attention.As an important strategic resource,rare earth plays an important role in the field of nuclear shielding materials.In this review,the shielding principles of rare earth materials are first introduced.According to the type of matrix,the characteristics and current research status of metal-based,inorganic nonmetallic-based and polymer-based rare earth shielding materials are reviewed.Meanwhile,the future development trend of rare earth shielding materials is discussed.

关键词： Rare earths Nuclear radiation Shielding composites

Bioinformatics comprehensive analysis confirmed the potential involvement of SLC22A1 in lower-grade glioma progression and prognosis

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BIOCELL 2024年第5期48卷 803-815页

作者： jing hui NANA SUN YONG LIU CHUNBO YU YONG KE YONG CAO ANXIAO YU QINGHONG KONG YUN LIU Guizhou Provincial College-Based Key Lab for Tumor Prevention and Treatment with DistinctiveMedicines Zunyi Medical UniversityZunyi563000China College of Basic Medicine Zunyi Medical UniversityZunyi563000China Department of Dermatology Guizhou Province Cosmetic Plastic Surgery HospitalAffiliated Hospital of Zunyi Medical UniversityZunyi563000China School of Forensic Medicine Zunyi Medical UniversityZunyi563000China

Background:Although it has been established that the human Solute Carrier Family 22(SLC22)functions as a cationic transporter,influencing cellular biological metabolism by modulating the uptake of various cations,its impact on cancer prognosis remains unclear.Methods:We conducted a comprehensive analysis utilizing data from The Cancer Genome Atlas(TCGA)and other databases to assess the prognostic value and functional implications across various tumors.Silence of SLC22A1 RNA in glioma U251 cells was performed to access the impact of SLC22A1 on lowergrade glioma(LGG)progression.Results:Our findings demonstrated a significant correlation between SLC22A1 expression and the survival time of patients with various cancers(p0.8).Cell proliferation and clone formation experiment proved that decreased expression of SLC22A1 in glioma U251 cells inhibited glioma cell growth.Conclusion:Our findings suggest SLC22A1 has huge prospects as a promising biomarker and therapeutic target for LGG prognosis.SLC22A1 has only been proved to support cellular function previously.Our findings demonstrated a robust connection between the tumor microenvironment and functional proteins that maintain basal cell metabolism,which gifts unique tumor immune characteristics of gliomas.Additionally,we provide a highly practical prediction model for estimating the survival rate of LGG patients.

关键词： SLC22A1 LGG prognosis immune nomogram