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Structures and Spectroscopy Properties of One Novel Keggin Type Polyoxomolybdate Compound

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光谱学与光谱分析 2016年第S1期36卷 208-209页

作者： GUO Bing-cui ZHOU meng-xi huang Mei-qing LIN Hui-yun SHI Lin huang meng-meng CHEN Yi-ping College of Chemistry Fuzhou UniversityFuzhou 350108 China Fuzhou No.1High Middle School Fuzhou 350108 China

In this paper,One novel Keggin type polyoxomolybdate compounds have been hydrothermal synthesized:{[(CH3)2NH2]4(SiMo12O40)}[(CH3)2NH]·(DMF)0.5(1).The compound 1have been characterized by infrared spectrum,and the two... 详细信息

关键词： Polyoxomolybdate Keggin type structure 2DIR COS

Enhanced potassium storage of carbon nanofibers as binderfree anodes enabled by coupling ultra-small amorphous Sb_(2)O_(3),graphene modification and sulfur doping

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Rare Metals 2024年第1期43卷 51-64页

作者： Zhao huang Yu-Kang Lou Lin Peng Yuan Peng meng-meng Wang Ming Zhang College of Railway Transportation Hunan University of TechnologyZhuzhou 412007China College of Semiconductors(College of Integrated Circuits) Changsha Semiconductor Technology and Application Innovation Research InstituteHunan UniversityChangsha 410082China Key Laboratory for Micro-Nano Optoelectronic Devices of Ministry of Education College of Semiconductors(College of Integrated Circuits)Hunan UniversityChangsha 410082China

Considering the intrinsic advantages of natural copiousness and cost-effectiveness of potassium resource,potassium-ion batteries(KIBs) are booming as prospective alternatives to lithium-ion batteries(LIBs) in large-scale energy storage scenarios. Nevertheless, lacking desirable electrodes for reversibly hosting the bulky K+hinders the widespread application of KIBs, and it needs to be urgently solved. Hereon, the porous S-doped Sb_(2)O_(3)-graphene-carbon(SAGC) nanofibers are manufactured through an adjustable and facile approach, which involves electrospinning, in situ etching and sulfuration. The synthesized SAGC is featured by the ultra-small amorphous Sb_(2)O_(3) homogeneously wrapped inside the carbon matrix, as well as the co-incorporation of graphene and sulfur. Tentatively,the SAGC nanofiber sheets are applied as binder-free anodes for KIBs, exhibiting a prominent cycling life(256.72 m Ah·g^(-1) over 150 cycles at 100 m A·g^(-1)) and rate·g^(-1) over 100 cycles at 1 A·g^(-1)). The positive synergy among all the active components accounts for the distinguished performances of the SAGC. By reinforcing the tolerability to the swelling stress, producing the valid electrochemical active sites, and promoting the charge transferring for reversible K+uptake, the SAGC finally renders the excellent cyclability, capacity, and rate capability. Moreover, the extrinsic electrochemical pseudocapacitance characteristics induced by the porous carbon substrate elevate the K-storage capacity of the SAGC as well. It is hoped that the conclusions drawn may offer new insights into a direction for the high-performance binderfree KIB anodes.

关键词： S-doped Sb_(2)O_(3)-graphene-carbon Nanofibers Binder-free Anodes Potassium-ion batteries

Integrating Neighborhood Geographic Distribution and Social Structure Influence for Social Media User Geolocation

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Computer Modeling in Engineering & Sciences 2024年第9期140卷 2513-2532页

作者： meng Zhang Xiangyang Luo Ningbo huang Key Laboratory of Cyberspace Situation Awareness of Henan Province Zhengzhou450001China State Key Laboratory of Mathematical Engineering and Advanced Computing Zhengzhou450001China

Geolocating social media users aims to discover the real geographical locations of users from their publicly available data,which can support online location-based applications such as disaster alerts and local content *** relationship-based methods represent a classical approach for geolocating social ***,geographically proximate relationships are sparse and challenging to discern within social networks,thereby affecting the accuracy of user *** address this challenge,we propose user geolocation methods that integrate neighborhood geographical distribution and social structure influence(NGSI)to improve geolocation ***,we propose a method for evaluating the homophily of locations based on the k-order neighbor-hood geographic distribution(k-NGD)similarity among *** are notable differences in the distribution of k-NGD similarity between location-proximate and non-location-proximate *** this distinction,we filter out non-location-proximate social relationships to enhance location homophily in the social *** better utilize the location-proximate relationships in social networks,we propose a graph neural network algorithm based on the social structure *** algorithm enables us to perform a weighted aggregation of the information of users’multi-hop neighborhood,thereby mitigating the over-smoothing problem of user features and improving user geolocation *** results on real social media dataset demonstrate that the neighborhood geographical distribution similarity metric can effectively filter out non-location-proximate social ***,compared with 7 existing social relationship-based user positioning methods,our proposed method can achieve multi-granularity user geolocation and improve the accuracy by 4.84%to 13.28%.

关键词： User geolocation social media neighborhood geographic distribution structure influence

A Study on Enhancing Chip Detection Efficiency Using the Lightweight Van-YOLOv8 Network

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Computers, Materials & Continua 2024年第4期79卷 531-547页

作者： meng huang Honglei Wei Xianyi Zhai School of Mechanical Engineering and Automation Dalian Polytechnic UniversityDalian116034China

In pursuit of cost-effective manufacturing,enterprises are increasingly adopting the practice of utilizing recycled semiconductor *** ensure consistent chip orientation during packaging,a circular marker on the front side is employed for pin alignment following successful functional ***,recycled chips often exhibit substantial surface wear,and the identification of the relatively small marker proves ***,the complexity of generic target detection algorithms hampers seamless *** these issues,this paper introduces a lightweight YOLOv8s-based network tailored for detecting markings on recycled chips,termed ***,to alleviate the influence of diminutive,low-resolution markings on the precision of deep learning models,we utilize an upscaling approach for enhanced *** technique relies on the Super-Resolution Generative Adversarial Network with Extended Training(SRGANext)network,facilitating the reconstruction of high-fidelity images that align with input ***,we replace the original YOLOv8smodel’s backbone feature extraction network with the lightweight VanillaNetwork(VanillaNet),simplifying the branch structure to reduce network ***,a Hybrid Attention Mechanism(HAM)is implemented to capture essential details from input images,improving feature representation while concurrently expediting model inference *** results demonstrate that the Van-YOLOv8 network outperforms the original YOLOv8s on a recycled chip dataset in various ***,it demonstrates superiority in parameter count,computational intricacy,precision in identifying targets,and speed when compared to certain prevalent algorithms in the current *** proposed approach proves promising for real-time detection of recycled chips in practical factory settings.

关键词： Lightweight neural networks attention mechanisms image super-resolution enhancement feature extraction small object detection

Tailoring sulfur-doped and nitrogen-defective carbon nitride nanosheets for efficient photo-controlled radical polymerizations

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Science China Chemistry 2024年第7期67卷 2325-2334页

作者： Xue Li meng Kai Xu Yuan huang Tao Cai Key Laboratory of Biomedical Polymers of Ministry of Education College of Chemistry and Molecular SciencesWuhan UniversityWuhan 430072China Wuhan University Shenzhen Research Institute Shenzhen 518057China

Despite the challenges that remain,the synergistic adjustment of various microstructures and photochemical parameters of graphitic carbon nitride(g-C_(3)N_(4))in photocatalytic reactions holds promises for improving catalytic efficiency and reducing energy ***,sulfur-doped and nitrogen-defective g-C_(3)N_(4)(n-SC_(3)N_(x))nanosheets were designed and elaborately *** resultant n-SC_(3)N_(x)possessed a precisely defined 2D layer structure with extensive porosity and incremental specific surface *** photoinduced electron transfer-reversible addition-fragmentation chain transfer(PET-RAFT)polymerization of vinyl monomers with low dispersity,excellent temporal control and high chain-end fidelity was achieved under mild blue light irradiation in a nondegassed *** to their ultrathin nanostructures with nitrogen defects and sulfur dopants,n-SC_(3)N_(x)was capable of catalyzing RAFT polymerization in aqueous solutions at significantly accelerated rates,which were nearly 8 times faster compared to bulk g-C_(3)N_(4).The ease of separation and efficient reusability in subsequent polymerizations was enabled by the heterogeneous nature of n-SC_(3)N_(x).The appeal of this approach was illustrated by the fact that utilizing a reusable and metal-free photocatalyst in aqueous environments allowed for the synthesis of polymers with molecular weight up to 300 kg mol^(-1) and a dispersity of 1.32.

关键词： graphitic carbon nitride nitrogen defects sulfur dopants PET-RAFT polymerization recyclability

In situ direct reprogramming of astrocytes to neurons via polypyrimidine tract-binding protein 1 knockdown in a mouse model of ischemic stroke

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Neural Regeneration Research 2024年第10期19卷 2240-2248页

作者： meng Yuan Yao Tang Tianwen huang Lining Ke En huang Key Laboratory of Brain Aging and Neurodegenerative Diseases of Fujian Province Fujian Medical UniversityFuzhouFujian ProvinceChina Department of Human Anatomy School of Basic Medical SciencesFujian Medical UniversityFuzhouFujian ProvinceChina Scientific Research Center School of Basic Medical SciencesFujian Medical UniversityFuzhouFujian ProvinceChina Department of Neurology Fujian Medical University Union HospitalFuzhouFujian ProvinceChina Fujian Key Laboratory of Vascular Aging Fujian Medical UniversityFuzhouFujian ProvinceChina

In situ direct reprogramming technology can directly convert endogenous glial cells into functional neurons in vivo for central nervous system repair. Polypyrimidine tract-binding protein 1(PTB) knockdown has been shown to reprogram astrocytes to functional neurons in situ. In this study, we used AAV-PHP.e B-GFAP-sh PTB to knockdown PTB in a mouse model of ischemic stroke induced by endothelin-1, and investigated the effects of GFAP-sh PTB-mediated direct reprogramming to neurons. Our results showed that in the mouse model of ischemic stroke, PTB knockdown effectively reprogrammed GFAP-positive cells to neurons in ischemic foci, restored neural tissue structure, reduced inflammatory response, and improved behavioral function. These findings validate the effectiveness of in situ transdifferentiation of astrocytes, and suggest that the approach may be a promising strategy for stroke treatment.

关键词： astrocyte in situ direct reprogramming ischemic stroke miR-30 based shRNA neuron polypyrimidine tract-binding protein 1 transdifferentiation

High Dynamic Bounding and Jumping Motion of Quadruped Robot Based on Stable Optimization Control

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Journal of Bionic Engineering 2024年第1期21卷 101-111页

作者： Sai Gu Fei meng Botao Liu Junyao Gao Qiang huang School of Mechatronical Engineering Beijing Institute of Technology100081 BeijingChina Key Laboratory of Biomimetic Robots and Systems Ministry of EducationBeijing 100081China

Aiming at the environment such as ravines and obstacles that may be encountered in the actual movement,this paper proposes a method for optimizing the bounding and jumping motion based on the ground touching force trajectory and the air motion trajectory of the quadruped *** method of optimizing the ground reaction force according to the speed of the demand and the height of the jump,and adjusting the stance and swing time according to the relationship of dynamics and momentum *** the same time,under the constraints of dynamics and energy consumption of the robot system,considering the jumping distance and height,a method for optimizing the air trajectory of bounding and jumping is *** switching and landing stability control are also ***,the experimental results show that the quadruped robot has strong bounding and jumping ability,and has achieved stable bounding movement and forward jump movement of 0.8 m.

关键词： Quadruped robot High dynamic motion control-Periodic limit cycle Trajectory optimization

A LiDAR Point Clouds Dataset of Ships in a Maritime Environment

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IEEE/CAA Journal of Automatica Sinica 2024年第7期11卷 1681-1694页

作者： Qiuyu Zhang Lipeng Wang Hao meng Wen Zhang Genghua huang the College of Intelligent Systems Science and Engineering Harbin Engineering UniversityHarbin 150001China Key Laboratory of Space Active Opto-Electronics Technology Shanghai Institute of Technical PhysicsChinese Academy of SciencesShanghai 200083China

For the first time, this article introduces a LiDAR Point Clouds Dataset of Ships composed of both collected and simulated data to address the scarcity of LiDAR data in maritime applications. The collected data are acquired using specialized maritime LiDAR sensors in both inland waterways and wide-open ocean environments. The simulated data is generated by placing a ship in the LiDAR coordinate system and scanning it with a redeveloped Blensor that emulates the operation of a LiDAR sensor equipped with various laser beams. Furthermore,we also render point clouds for foggy and rainy weather conditions. To describe a realistic shipping environment, a dynamic tail wave is modeled by iterating the wave elevation of each point in a time series. Finally, networks serving small objects are migrated to ship applications by feeding our dataset. The positive effect of simulated data is described in object detection experiments, and the negative impact of tail waves as noise is verified in single-object tracking experiments. The Dataset is available at https://***/zqy411470859/ship_dataset.

关键词： 3D point clouds dataset dynamic tail wave fog simulation rainy simulation simulated data

Non-equilibrium kinetic separation of thulium,yttrium and erbium on the surface of freely rising oil droplets

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Journal of Rare Earths 2024年第1期42卷 200-209,I0007页

作者： Na Sui Shukai Miao Kaihui Cui Fancheng meng Kun huang School of Metallurgical and Ecological Engineering University of Science and Technology BeijingBeijing100083China Beijing Key Laboratory of Green Recovery and Extraction of Rare and Precious Metals University of Science and Technology BeijingBeijing100083China Key Laboratory of Green Process and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing100190China

It is difficult to achieve selective separation and enrichment of different rare earths from high abundance yttrium ores efficiently only dependent on their discrepancy in thermodynamic *** present work suggests a new strategy based on non-equilibrium kinetic separation of Er and Tm on the surface of freely rising oil droplets to control the separation order of *** is revealed that the mutual separation of Er/Tm is significantly promoted with the separation coefficient of 2.89 during the non-equilibrium extraction with the addition of diethylenetriaminepentaacetic acid(DTPA).The extraction sequence of Tm,Er and Y can be controlled as Tm>Y>Er,thus Y can be selectively enriched during the process of separation of Er and Tm,Such a sequence is subject to the controllable dissociation rates of RE(Ⅲ)-DTPA complexes and extraction abilities of P507 with the three RE(Ⅲ)*** dissociation rate is dependent on the stabilities of RE(Ⅲ)-DTPA complexes and follows the sequence ofY(Ⅲ)—DTPA Er>Y to Tm>Y>Er.

关键词： DTPA Interface interaction Non-equilibrium kinetic separation Rare earths P507