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Advancements and Challenges in Organic–Inorganic Composite Solid Electrolytes for All‑Solid‑State Lithium Batteries

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Nano-Micro Letters 2025年第1期17卷 46-97页

作者： Xueyan Zhang Shichao Cheng Chuankai fu Geping Yin Liguang Wang Yongmin Wu hua Huo State Key Laboratory of Space Power‑Sources School of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001People’s Republic of China College of Chemical and Biological Engineering Zhejiang UniversityHangzhou 310058People’s Republic of China State Key Laboratory of Space Power-Sources 2965 Dongchuan RoadMinhang DistrictShanghai 200240People’s Republic of China

To address the limitations of contemporary lithium-ion batteries,particularly their low energy density and safety concerns,all-solid-state lithium batteries equipped with solid-state electrolytes have been identified as an up-and-coming *** the various SEs,organic–inorganic composite solid electrolytes(OICSEs)that combine the advantages of both polymer and inorganic materials demonstrate promising potential for large-scale ***,OICSEs still face many challenges in practical applications,such as low ionic conductivity and poor interfacial stability,which severely limit their *** review provides a comprehensive overview of recent research advancements in ***,the influence of inorganic fillers on the main functional parameters of OICSEs,including ionic conductivity,Li+transfer number,mechanical strength,electrochemical stability,electronic conductivity,and thermal stability are systematically *** lithium-ion conduction mechanism of OICSE is thoroughly analyzed and concluded from the microscopic ***,the classic inorganic filler types,including both inert and active fillers,are categorized with special emphasis on the relationship between inorganic filler structure design and the electrochemical performance of ***,the advanced characterization techniques relevant to OICSEs are summarized,and the challenges and perspectives on the future development of OICSEs are also highlighted for constructing superior ASSLBs.

关键词： Composite solid electrolytes Inorganic filler Interfacial stability Li-ion conduction mechanism Characterization techniques

Amperometric Glucose Sensor Based on Batch CuO-Modified Screen-Printed Silver-Carbon Electrodes

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Journal of Wuhan University of Technology(Materials Science) 2025年第1期40卷 35-41页

作者： XIA Haiyan huaNG Yin YANG hua WANG Xintian SHI Jianping LIU Lixia fu Yacheng QUAN Changyun LI Suyuan Cofoe Medical Technology Company Limited Changsha 410000China Institute of New Energy Hexi UniversityZhangye 734000China Chemistry and Chemical Engineering Central South UniversityChangsha 410000China

CuO nanoparticles were successfully synthesized via a two-jet electrospun method,and then screen-printed on silver-carbon electrodes,forming CuO-modified Ag-C(CuO/Ag-C)disposable strip *** natural environment condition for glucose detection,the obtained CuO/Ag-C electrodes show a high sensitivity of 540 nA·mM^(-1)·cm^(-2),and a low limit of detection(0.68 mM)in a wide linear response range of 0.68 mM and 3 mM(signal/noise=3),*** addition,the CuO/Ag-C electrodes also exhibit excellent anti-interference,air stability and *** a result,the fabrication of CuO nanoparticles via an electrospun process and the technique of screen-printed electrodes are of great significance for glucose detection.

关键词： electrochemical sensor CuO nanoparticles glucose detection screen-printing technique

A self-adaptive inorganic in-situ separator by particle crosslinking for nonflammable lithium-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 469-480页

作者： Jiarui Yang Jiuzhou Liu Wenrui Cai Ziyu Zhao Shan Wang Lu He Shanshan Lv Zhiwei Zhu Zhongfeng Ji Guojiang Wen hua Li Yuanming Zhai Xuewei fu Wei Yang Yu Wang College of Polymer Science and Engineering State Key Laboratory of Polymer Materials Engineering Sichuan University

All-safe liquid-state lithium-ion batteries(ASLS-LIBs) is of great interest as they can potentially combine the safety of all-solid-state batteries with the high performance and low manufacturing cost of traditional liquid-state LIBs. However, the practical success of ASLS-LIBs is bottlenecked by the lack of advanced separator technology that can simultaneously realize high performances in puncturing-tolerability,fire-resistance, and importantly, wetting-capability with non-flammable liquid-electrolytes. Here, we propose a concept of inorganic in-situ separator(IISS) by hybrid-sol physical crosslinking directly onto the electrode surface to address the above challenges. Particularly, the hybrid-sol is designed with silica nanoparticles as the building block and poly(vinylidene difluoride) nanoparticles as the crosslinking agent. The critical factors for controlling the IISS microstructures and properties have been systematically investigated. The advantages of the IISS have been confirmed by its fast wetting with various fireresistant liquid-electrolytes, customizable thickness and porous structures, robust interface with planar or three-dimensional(3D)-structured electrodes, and importantly, unexpected self-adaptability against puncturing. Enabled by the above merits, a fire-resistant ASLS-LIB is successfully assembled and demonstrated with stable electrochemical performance. This sol-crosslinked IISS may open an avenue for the studies on the next-generation separator technology, cell assembling, solid electrolyte processing as well as non-flammable secondary batteries.

关键词： Silica nanoparticles

光通过散射介质聚焦的空间位相逐个单元调节方法

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生物化学与生物物理进展 2018年第3期45卷 336-350页

作者：方龙杰张熙程张诚左浩毅朱建华高福华庞霖四川大学物理科学与技术学院成都610064

本研究在分析现有散射介质聚焦方法的基础上,提出一种利用单元裂解进行波前位相调制,将经过强散射介质的散射光聚焦的快速收敛方法.文中详细地描述了这一新方法的原理,并同现有逐个单元调节方法进行运行对比.单元裂解方法的物理本质,即... 详细信息

本研究在分析现有散射介质聚焦方法的基础上,提出一种利用单元裂解进行波前位相调制,将经过强散射介质的散射光聚焦的快速收敛方法.文中详细地描述了这一新方法的原理,并同现有逐个单元调节方法进行运行对比.单元裂解方法的物理本质,即为实现空间光调制器的调制各单元光波之间同位相干涉.本方法具有更高的信噪比,并且聚焦收敛的速度快.这一新方法为进一步开展生物成像的光学理论研究提供了新思路.

关键词：空间光调制器聚焦干涉散射介质

Positive effect of Mo on mechanical properties of a Ni-42W-10Co-x Mo medium heavy alloy

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China Foundry 2025年

作者： Guo-xin Cao Jian-xin Dong Yong-sheng He He Jiang Fang Hao Zhi-hua Nie Teng-fei Ma Bao-quan fu School of Materials Science and Engineering University of Science and Technology Beijing Xi'an Superalloy Technology Co. Ltd. School of Materials Science and Engineering Beijing Institute of Technology Key Laboratory of Air-driven Equipment Technology of Zhejiang Province Quzhou University

In this study,a novel Ni-W-Co-Mo medium heavy alloy (MHA) was designed to improve its mechanical strength via Mo *** the Ni-42W-10Co-xM o alloy series,where x represents the weight percent of Mo and varies between 0,1,2,5,and 10,the microstructure transitions from a dendritic structure to a hypoeutectic structure as the Mo content increases from 0 to 5wt.%.Moreover,as the Mo content increases from 0to 10wt.%,the distribution of theμ-phase shifts from being individually dispersed to forming aggregates,and its volume fraction rises from 0.5%to 7.9%.Notably,theμ-phase evolves into an eutectic microstructure,which helps in minimizing the segregation of *** change is accompanied by a substantial enhancement in mechanical properties;specifically,the compressive yield strength at room temperature increases from 350 MPa to 646 MPa,indicating a significant 85%***,the microhardness increases from 230 HV to 304 *** dynamics simulations further reveal that the strengthening mechanism of Ni-42W-10Co-xM o alloys is Mo-induced solid solution strengthening and precipitation strengthening.

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沙角衣藻转化难溶性磷的研究

四川大学学报（自然科学版） 2003年第1期40卷 127-130页

作者：卿人韦兰利琼刘英华陈儒牛培叶华勋傅华龙四川大学生命科学学院成都610064

以磷矿石粉为沙角衣藻(ChlamydomonassajaoLewin)的唯一生长磷源,研究沙角衣藻对难溶性磷源(矿石磷)的转化利用作用.结果表明:沙角衣藻对矿石磷的转化强度可达40.56%～63.49%,以有效磷mg/g磷源为单位可达41～64,是一般溶磷细菌溶磷强度... 详细信息

以磷矿石粉为沙角衣藻(ChlamydomonassajaoLewin)的唯一生长磷源,研究沙角衣藻对难溶性磷源(矿石磷)的转化利用作用.结果表明:沙角衣藻对矿石磷的转化强度可达40.56%～63.49%,以有效磷mg/g磷源为单位可达41～64,是一般溶磷细菌溶磷强度的2～4倍,相当于每产1g鲜藻体可得磷酸1.52g.该藻不仅能快速地转化利用磷矿石粉中的难溶性磷源以满足其自身的生理需要,而且能迅速提高介质中的有效磷浓度,为环境中其它生物的生活提供磷源;而且这种转化作用的强度与其对磷的需要相协调.可确保体系供磷和需磷的和谐同步进行.

关键词：难溶性磷沙角衣藻矿石磷转化强度生态磷肥农业生态系统生长磷源

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城市垃圾堆肥的生态效应与对策研究

土壤 2004年第5期36卷 498-505页

作者：范海荣华珞傅桦王学江首都师范大学资源环境与地理信息系统北京重点实验室北京100037

本文分析了城市垃圾堆肥的生态效应,其中包括肥力效应:提高土壤养分,改善土壤的理化性质;生物效应:改善土壤的微生物特性,提高植物的产量和品质;环境负效应:造成土壤的沙化、盐渍化、重金属积累等;环境正效应:修复被污染的土壤,防止水... 详细信息

本文分析了城市垃圾堆肥的生态效应,其中包括肥力效应:提高土壤养分,改善土壤的理化性质;生物效应:改善土壤的微生物特性,提高植物的产量和品质;环境负效应:造成土壤的沙化、盐渍化、重金属积累等;环境正效应:修复被污染的土壤,防止水土流失;并阐述了垃圾堆肥环境效应的预防措施。最后提出了城市垃圾堆肥的发展对策:提高垃圾堆肥的质量,发展有机无机复合肥。

关键词：垃圾堆肥生态效应肥力效应生物效应环境效应有机无机复合肥

Reducing the measurement errors in nonadiabatic holonomic quantum computers

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Science China(Physics,Mechanics & Astronomy) 2025年第1期Mechanics & Astronomy) .卷 64-70页

作者： Guo-fu Xu Department of Physics Shandong University

Nonadiabatic holonomic quantum computers serve as the physical platform for nonadiabatic holonomic quantum *** quantum computation has entered the noisy intermediate-scale era, building accurate intermediate-scale nonadiabatic holonomic quantum computers is clearly necessary. Given that measurements are the sole means of extracting information, they play an indispensable role in nonadiabatic holonomic quantum computers. Accordingly, developing methods to reduce measurement errors in nonadiabatic holonomic quantum computers is of great importance. However, while much attention has been given to the research on nonadiabatic holonomic gates, the research on reducing measurement errors in nonadiabatic holonomic quantum computers is severely lacking. In this study, we propose a measurement error reduction method tailored for intermediate-scale nonadiabatic holonomic quantum computers. The reason we say this is because our method can not only reduce the measurement errors in the computer but also be useful in mitigating errors originating from nonadiabatic holonomic gates. Given these features,our method significantly advances the construction of accurate intermediate-scale nonadiabatic holonomic quantum computers.

关键词： quantum holonomy quantum computation measurement errors

基于地域特点、景观生态、土壤性质的土地利用模式研究进展

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首都师范大学学报（自然科学版） 2003年第4期24卷 76-81页

作者：赵红华珞傅桦首都师范大学资源环境与旅游学院北京100037

首先简要介绍国内外土地利用研究的概况 ;然后着重阐述基于地域特点、景观生态学、土壤性质三个方面的土地利用模式的研究进展 ,旨在综合已有研究经验和成果 ,促进今后相关研究的发展 ;最后提出有待进一步研究的问题 .

关键词：地域特点景观生态土壤性质土地利用模式