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Temperature inversion enables superior stability for low-temperature Zn-ion batteries

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Journal of Energy Chemistry 2024年第4期91卷 245-253页

作者： Fu-Da Yu Zhe-jian Yi Rui-Yang Li Wei-Hao Lin jie Chen Xiao-Yue Chen Yi-Ming Xie ji-huai Wu Zhang Lan Lan-Fang Que Bao-Sheng Liu Hao Luo Zhen-Bo Wang Engineering Research Center of Environment-Friendly Functional Materials Ministry of EducationInstitute of Materials Physical ChemistryHuaqiao UniversityXiamen 361021FujianChina b2 School of Electronic Engineering Guangxi University of Science and TechnologyLiuzhou 545006GuangxiChina School of Materials Science and Engineering Xiamen University of TechnologyXiamen 361024FujianChina School of Materials Science and Engineering Zhengzhou UniversityZhengzhou 450001HenanChina MIIT Key Laboratory of Critical Materials Technology for New Energy Conversion and Storage State Key Laboratory of Space Power-SourcesSchool of Chemistry and Chemical EngineeringHarbin Institute of TechnologyHarbin 150001HeilongjiangChina College of Materials Science and Engineering Shenzhen UniversityShenzhen 518071GuangdongChina

It is challenging for aqueous Zn-ion batteries(ZIBs)to achieve comparable low-temperature(low-T)performance due to the easy-frozen electrolyte and severe Zn ***,an aqueous electrolyte with a low freezing point and high ionic conductivity is *** with molecular dynamics simulation and multi-scale interface analysis(time of flight secondary ion mass spectrometry threedimensional mapping and in-situ electrochemical impedance spectroscopy method),the temperature independence of the V_(2)O_(5)cathode and Zn anode is observed to be ***,dominated by the solvent structure of the designed electrolyte at low temperatures,vanadium dissolution/shuttle is significantly inhibited,and the zinc dendrites caused by this electrochemical crosstalk are greatly relieved,thus showing an abnormal temperature inversion *** the disclosure and improvement of the above phenomena,the designed Zn||V_(2)O_(5)full cell delivers superior low-T performance,maintaining almost 99%capacity retention after 9500 cycles(working more than 2500 h)at-20°*** work proposes a kind of electrolyte suitable for low-T ZIBs and reveals the inverse temperature dependence of the Zn anode,which might offer a novel perspective for the investigation of low-T aqueous battery systems.

关键词： Aqueous Zn-ion batteries Low-temperature performance Opposite temperature dependence Zndendrite growth Vanadium dissolution

交替饥饿下PN1/PN2系统抑制NOB研究

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中国环境科学 2024年第1期44卷 202-210页

作者：李冬任纪元张杰北京工业大学城市建设学部水质科学与水环境恢复工程北京市重点实验室北京100124 哈尔滨工业大学环境学院城市水资源与水环境国家重点实验室黑龙江哈尔滨150090

为了抑制亚硝酸盐氧化菌(NOB)的生长繁殖,采用序批式反应器(SBR)运行PN1/PN2系统,设置4组反应器R1~R4,分别设置连续运行段和交替饥饿/恢复运行段.饥饿期溶解氧(DO)浓度分别设置为(1±0.5),(2±0.5),(3±0.5),(4±0.5)mg/L,探讨交替周期... 详细信息

为了抑制亚硝酸盐氧化菌(NOB)的生长繁殖,采用序批式反应器(SBR)运行PN1/PN2系统,设置4组反应器R1~R4,分别设置连续运行段和交替饥饿/恢复运行段.饥饿期溶解氧(DO)浓度分别设置为(1±0.5),(2±0.5),(3±0.5),(4±0.5)mg/L,探讨交替周期的选取、饥饿期DO条件对功能菌活性、污泥浓度、粒径及胞外聚合物(EPS)的影响,以期实现部分硝化段的稳定运行.结果显示,相比于好氧氨氧化菌(AOB),NOB在面对饥饿时表现得更为敏感,活性衰减速率更高,恢复期前3d AOB的活性恢复速率高于NOB,因此3d的交替周期能够有效抑制NOB并保留AOB活性.采用交替周期为3d的交替饥饿/恢复策略进行70d的运行,4组反应器的亚硝酸盐氮积累率(NAR)分别达到73.36%、84.43%、91.21%、95.97%,运行过程中出现了污泥减量化的现象,但经过一段时间的适应后R1~R3的污泥浓度能够保持稳定,而R4则呈下降趋势;交替饥饿/恢复策略使系统逐渐排除沉降性能较差的絮体,而沉降性能好的污泥留在反应器内,第70d 4个反应器的污泥粒径分别达到190.69,197.56,207.69,153.56µm;环境变化刺激微生物分泌更多EPS,因此4组反应器污泥的EPS含量都呈现不同幅度的升高.实验结果表明交替饥饿/恢复策略可以刺激污泥产生有利的变化,实现有效的NOB抑制以及稳定的NO_(2)^(-)-N积累.

关键词：短程硝化饥饿好氧氨氧化菌亚硝酸盐氧化菌活性抑制厌氧氨氧化

肱骨近端锁定钢板或肱骨近端内锁定系统与其他内固定治疗肱骨近端骨折的Meta分析

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中华创伤骨科杂志 2012年第12期14卷 1047-1054页

作者：胡稷杰金丹魏宽海任高宏余斌王钢南方医科大学南方医院创伤骨科广州510515

目的对采用肱骨近端锁定钢板（LPHP）或肱骨近端内锁定系统（PHILOS）与其他内固定治疗肱骨近端骨折（PHFs）的疗效进行Meta分析，为临床治疗提供参考依据。方法通过计算机检索MEDLINE（1966年至2011年12月）、EMbase（1966年至2011年1... 详细信息

目的对采用肱骨近端锁定钢板（LPHP）或肱骨近端内锁定系统（PHILOS）与其他内固定治疗肱骨近端骨折（PHFs）的疗效进行Meta分析，为临床治疗提供参考依据。方法通过计算机检索MEDLINE（1966年至2011年12月）、EMbase（1966年至2011年12月）、Cochrane图书馆（2011年第4期）和中国生物医学文献数据库（2001至2011年）等，搜集有关LPHP／PHILOS和其他内固定治疗PHFs的各种对照研究，对纳入的文献选择Neer评分、Constant-Murley功能评分、肩关节疼痛和功能障碍指数（SPADI）量表和美国肩肘外科医师（ASES）评分、异位骨化发生率、感染率、肱骨头缺血坏死率、骨折延迟愈合率、螺钉松动率、钢板断裂率、肩峰下撞击征发生率、肱骨头半脱位发生率、肩关节活动受限发生率、肩关节疼痛发生率、二次手术率作为Meta分析的评价指标，采用RevMan5．0进行分析。结果共纳入18项研究1133例患者。LPHP／PHILOS与其他内固定治疗PHFs相比，螺钉松动率更低，差异均有统计学意义[OR=0．23，95％CI（0．07，0．74），P=0．01]。LPHP／PHILOS与其他内固定治疗PHFs的Neer评分优良率、异位骨化发生率、感染率、肱骨头缺血坏死率、骨折延迟愈合率、钢板断裂率、肩峰撞击征发生率、肱骨头半脱位发生率、肩关节活动受限发生率比较，差异均无统计学意义（P〉0．05）。结论LPHP／PHILOS与其他内固定在特定条件下各有利弊，不能卣目扩大LPHP／PHILOS的临床适应证，治疗方案要结合患者的病情甚至经济情况综合考虑。

关键词：肱骨骨折近端骨折固定术 Meta分析骨板

Phase I clinical trial of intracerebral injection of lentiviral-ABCD1 for the treatment of cerebral adrenoleukodystrophy

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Science Bulletin 2024年第16期69卷 2596-2603页

作者： Qiu-Hong Wang jing Wanga Zhi-Pei Ling Zhi-Qiang Cui jie Gong Rui Zhang Shi-Jun Li Yang-Yang Wang Rui Yang De-hui huang Wen He jing Gao Chen Feng Pei-Li hu Li-Ying Liu Lung-ji Chang Li-Ping Zou Senior Department of Pediatrics Chinese PLA General HospitalBeijing 100853China Medical School of Chinese PLA Beijing 100853China Department of Neurosurgery Hainan Hospital of PLA General HospitalSanya 572013China Department of Neurosurgery The First Medical Center of Chinese PLA General HospitalBeijing 100853China Chengdu Women’s and Children’s Central Hospital School of MedicineUniversity of Electronic Science and Technology of ChinaChengdu 611731China School of Medicine University of Electronic Science and Technology of ChinaChengdu 610054China Beijing Meikang Biotechnology Co. LTD.Beijing 100085China Department of Radiology The First Medical Center of Chinese PLA General HospitalBeijing 100853China Department of Neurology The First Medical Center of Chinese PLA General HospitalBeijing 100853China Department of Pediatrics Xuanwu HospitalCapital Medical UniversityBeijing 100053China Shenzhen Geno-Immune Medical Institute Shenzhen 518057China Beijing Institute for Brain Disorders Center for Brain Disorders Research Capital Medical UniversityBeijing 100069China

This was a single-arm,multicenter,open-label phase I *** vectors(LV)carrying the ABCD1 gene(LV-ABCD1)was directly injected into the brain of patients with childhood cerebral adrenoleukodystrophy(CCALD),and multi-site injection was *** injection dose increased from 200 to 1600 lL(vector titer:1×10^(9) transduction units per mL(TU/mL)),and the average dose per kilogram body weight ranges from 8 to 63.6 lL/*** primary endpoint was safety,dose-exploration and immunogenicity and the secondary endpoint was initial evaluation of efficacy and the expression of ABCD1 protein.A total of 7 patients participated in this phase I study and were followed for 1 *** injectionrelated serious adverse event or death *** adverse events associated with the injection were irritability(71%,5/7)and fever(37.2-38.5℃,57%,4/7).Adverse events were mild and selflimited,or resolved within 3 d of symptomatic *** maximal tolerable dose is 1600 *** 5 cases(83.3%,5/6),no lentivirus associated antibodies were *** overall survival at 1-year was 100%.The ABCD1 protein expression was detected in neutrophils,monocytes and *** study suggests that the intracerebral injection of LV-ABCD1 for CCALD is safe and can achieve successful LV transduction in vivo;even the maximal dose did not increase the risk of adverse ***,the direct LV-ABCD1 injection displayed low *** addition,the effectiveness of intracerebral LV-ABCD1 injection has been preliminarily demonstrated while further investigation is *** study has been registered in the Chinese Clinical Trial Registry(https://***/,registration number:ChiCTR1900026649).

关键词： Adrenoleukodystrophy Lentiviral vectors ABCD1 Intracerebral injection

Thiol Ligand-Modified Au for Highly Efficient Electroreduction of Nitrate to Ammonia

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Precision Chemistry 2024年第3期2卷 112-119页

作者： Yuheng Wu Xiangdong Kong Yechao Su jiankang Zhao Yiling Ma Tongzheng ji Di Wu Junyang Meng Yan Liu Zhigang Geng jie Zeng Hefei National Research Center for Physical Sciences at the Microscale Key Laboratory of Strongly-Coupled Quantum Matter Physics of Chinese Academy of SciencesKey Laboratory of Surface and Interface Chemistry and Energy Catalysis of Anhui Higher Education InstitutesDepartment of Chemical PhysicsUniversity of Science and Technology of ChinaHefeiAnhui 230026P.R.China School of Chemistry&Chemical Engineering Anhui University of TechnologyMa’anshanAnhui 243002P.R.China

Electroreduction of nitrate(NO_(3)-)to ammonia(NH_(3))is an environmentally friendly route for NH_(3)production,serving as an appealing alternative to the Haber-Bosch ***,various noble metal-based electrocatalysts have been reported for electroreduction of NO_(3)-.However,the application of pure metal electrocatalysts is still limited by unsatisfactory performance,owing to the weak adsorption of nitrogen-containing intermediates on the surface of pure metal *** this work,we report thiol ligand-modified Au nanoparticles as the effective electrocatalysts toward electroreduction of NO_(3)-.Specifically,three mercaptobenzoic acid(MBA)isomers,thiosalicylic acid(ortho-MBA),3-mercaptobenzoic acid(meta-MBA),and 4-mercaptobenzoic acid(para-MBA),were employed to modify the surface of the Au *** the NO_(3)-electroreduction,para-MBA modified Au(denoted as para-Au/C)displayed the highest catalytic activity among these Au-based ***-1.0 V versus reversible hydrogen electrode(vs RHE),para-Au/C exhibited a partial current density for NH_(3)of 472.2 mA cm^(-2),which was 1.7 times that of the pristine Au ***,the Faradaic efficiency(FE)for NH_(3)reached 98.7%at-1.0 V vs RHE for para-Au/*** modification of para-MBA significantly improved the intrinsic activity of the Au/C catalyst,thus accelerating the kinetics of NO_(3)-reduction and giving rise to a high NH_(3)yield rate of para-Au/C.

关键词： Ammonia synthesis NO_(3)-electroreduction Au nanoparticles thiol ligand modification electronic structure

基于虚像相位阵列的光谱检测中角色散均匀性的研究

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光谱学与光谱分析 2024年第7期44卷 1827-1834页

作者：纪文杰谭中伟北京交通大学电子信息工程学院光波技术研究所北京100044

随着光谱学的不断发展,光谱检测作为一种快速无损的检测手段逐渐被应用于越来越多的领域中。而随着对信息精度要求的不断提高,如何得到高分辨率和低波长误差的光谱信息,是设计光谱检测系统时必须解决的问题。传统的色散元件如衍射光栅,... 详细信息

随着光谱学的不断发展,光谱检测作为一种快速无损的检测手段逐渐被应用于越来越多的领域中。而随着对信息精度要求的不断提高,如何得到高分辨率和低波长误差的光谱信息,是设计光谱检测系统时必须解决的问题。传统的色散元件如衍射光栅,虽然有较大的波长响应范围,但是通常只能提供nm量级的分辨率而无法满足当下的高光谱分辨率的要求。虚像相位阵列(VIPA)具有大角度色散特性,可以有效提高系统的光谱分辨率,因而近年来不断被用于精细光谱检测的研究。但其波长和色散角度对应关系存在非线性,而且同一波长易产生多个衍射级次的光斑,从而造成额外的光能损失。因此,本文主要基于VIPA的交叉色散光路就如何降低VIPA色散的非均匀性的问题进行了理论分析和实验验证。首先基于傍轴理论的色散定律展开理论分析探讨了入射光腰尺寸、入射角度等参数对于VIPA色散的非线性程度和衍射级次数量的影响。然后通过进行仿真记录了宽光谱光源在不同VIPA倾斜角度条件下各波长衍射级次的数量,以及各波长对应的光斑质心的坐标值。计算各情况下的质心坐标与拟合曲线之间的距离均差,比较了不同角度条件下线性度的好坏。最后根据理论分析和仿真实验的结果进行实验。实验中记录了VIPA的交叉色散光路在不同的VIPA倾斜条件下出现的衍射级次数量,并利用一个波长可变的激光器得到了不同波长的光源在VIPA倾斜2°的实验条件下各衍射级次光斑的质心坐标。同样通过计算不同衍射级次光斑的质心与拟合曲线之间的距离均差分析不同衍射级次的线性度好坏。实验证明通过控制入射光束参数,可以一定程度上降低VIPA色散的非均匀性。VIPA倾斜角度越大且越靠近探测器中央位置的衍射级次线性度越好。

关键词：虚像相位阵列光谱检测线性度衍射级次

Clinical feasibility of laparoscopic left lateral segment liver resection with magnetic anchor technique:The first clinical study from China

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World Journal of Gastrointestinal Surgery 2024年第5期16卷 1336-1343页

作者： Miao-Miao Zhang ji-Gang Bai Dong Zhang jie Tao Zhi-Min Geng Zhuo-Qun Li Yu-Xiang Ren Yu-HanZhang Yi Lyu Xiao-Peng Yan Department of Hepatobiliary Surgery The First Affiliated Hospital of Xi’an Jiaotong UniversityXi’an 710061Shaanxi ProvinceChina Shaanxi Provincial Key Laboratory of Magnetic Medicine The First Affiliated Hospital of Xi’an Jiaotong UniversityXi’an 710061Shaanxi ProvinceChina Zonglian College Xi’an Jiaotong UniversityXi’an 710061Shaanxi ProvinceChina Qide College Xi’an Jiaotong UniversityXi’an 710061Shaanxi ProvinceChina

BACKGROUND Magnetic anchor technique(MAT)has been applied in laparoscopic cholecystectomy and laparoscopic appendectomy,but has not been reported in laparoscopic partial *** To evaluate the feasibility of the MAT in laparoscopic left lateral segment liver *** Retrospective analysis was conducted on the clinical data of eight patients who underwent laparoscopic left lateral segment liver resection assisted by MAT in our department from July 2020 to November *** Y-Z magnetic anchor devices(Y-Z MADs)was independently designed and developed by the author of this paper,which consists of the anchor magnet and magnetic grasping *** time,intraoperative blood loss,intraoperative accidents,operator experience,postoperative incision pain score,postoperative complications,and other indicators were evaluated and *** All eight patients underwent a MAT-assisted laparoscopic left lateral segment liver resection,including three patients undertaking conventional 5-port and five patients having a transumbilical single-port *** mean operation time was 138±34.32 min(range 95-185 min)and the mean intraoperative blood loss was 123±88.60 mL(range 20-300 mL).No adverse events occurred during the *** Y-Z MADs showed good workability and maneuverability in both tissue and organ *** particular,the operators did not experience either a“chopstick”or“sword-fight”effect in the single-port laparoscopic *** The results show that the MAT is safe and feasible for laparoscopic left lateral segment liver resection,especially,exhibits its unique abettance for transumbilical single-port laparoscopic left lateral segment liver resection.

关键词： Magnetosurgery/magnetic surgery Magnetic anchor technique Laparoscopic hepatectomy Transumbilical singleport laparoscopy Magnet

Consensus on the clinical diagnosis and treatment of grade 3 pancreatic neuroendocrine tumors

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胰腺病学杂志(英文) 2024年第2期07卷 97-105页

作者： Chen jie Wu Wenming Bai Chunmei Chi Yihebali huo Li jiang Liming ji Yuan Luo jie Li jie Li jingnan Lou Wenhui Shao Chenghao Shen Lin Wang Feng Wang Yu Xue Ling Xu jin Yuan Chunhui Yu Xianjun Yin Xiaoyu Zhao Hong Zhu Xiongzeng Zhao Yupei Centre for Neuroendocrine Tumors Fudan University Shanghai Cancer Center Shanghai China Department of General Surgery State Key Laboratory of Complex Severe and Rare Diseases Peking Union Medical College Hospital Chinese Academy of Medical Science and Peking Union Medical College Beijing China Department of Medical Oncology Peking Union Medical College Hospital Chinese Academy of Medical Science &amp Peking Union Medical College Beijing China Department of Medical Oncology National Cancer Center/ National Clinical Research Center for Cancer/Cancer Hospital Chinese Academy of Medical Sciences and Peking Union Medical College Beijing China Department of Nuclear Medicine State Key Laboratory of Complex Severe and Rare Diseases Beijing Key Laboratory of Molecular Targeted Diagnosis and Therapy in Nuclear Medicine Peking Union Medical College Hospital Chinese Academy of Medical Sciences Beijing China Department of Diagnostic Radiology National Cancer Center/National Clinical Research Center for Cancer/ Cancer Hospital Chinese Academy of Medical Sciences and Peking Union Medical College Beijing China Department of Pathology Zhongshan Hospital Fudan University Shanghai China Department of Pathology China-Japan Friendship Hospital Beijing China Department of Gastroenterological Oncology Beijing Cancer Hospital Peking University Cancer Hospital &amp Institute Beijing China Department of Gastroenterology Peking Union Medical College Hospital Peking Union Medical College Chinese Academy of Medical Sciences Beijing China Department of Pancreatic Surgery Zhongshan Hospital Fudan University Shanghai China Department of Pancreatic-Biliary Surgery Second Affiliated Hospital of Naval Medical University Shanghai China Department of Gastrointestinal Oncology Key Laboratory of Carcinogenesis and Translational Research (Ministry of Education) Peking University Cancer Hospital &amp Department of Nuclear Medicine Nanjing First Hospital Nanjing Medical University Nanjing China Depar

The World Health Organization (WHO) 2017 classifications for neuroendocrine neoplasms (NENs) subdivided grade 3 pancreatic neuroendocrine neoplasms (pNENs) into G3 well-differentiated pancreatic neuroendocrine tumors (G3 pNETs) and poorly differentiated pancreatic neuroendocrine carcinomas (pNECs), according to the mitotic count, Ki-67 index, and cell differentiation. As a new category, G3 pNETs remain a challenging group of tumors to manage by lacking large randomized trials and consensus to support its clinical practice. Therefore, the Chinese Pancreatic Surgery Association, Chinese Society of Surgery, Chinese Medical Association gathered experts in this field to formulate this consensus for the diagnosis and treatment of G3 pNETs.

关键词： Clinical diagnosis Grade 3 Pancreatic neuroendocrine tumors Treatment

负载BMP的新型组织工程骨的构建及骨缺损修复实验

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第一军医大学学报 2005年第11期25卷 1369-1374页

作者：胡稷杰金丹全大萍钟世镇陈炅昊魏宽海赵洁裴国献南方医科大学南方医院创伤骨科广东广州510515 中山大学高分子研究所广东广州510275 南方医科大学临床解剖研究所广东广州510515

目的探讨以聚乳乙醇酸(poly-(D,L-lactide-co-glycolide),PLGA)、骨形态发生蛋白(BMP)、骨髓基质干细胞(BM-SCs)构建成新型组织工程骨并观察其在动物体内的成骨能力。方法制作新西兰大白兔右桡骨中段15mm骨缺损实验模型,随机分为实验组... 详细信息

目的探讨以聚乳乙醇酸(poly-(D,L-lactide-co-glycolide),PLGA)、骨形态发生蛋白(BMP)、骨髓基质干细胞(BM-SCs)构建成新型组织工程骨并观察其在动物体内的成骨能力。方法制作新西兰大白兔右桡骨中段15mm骨缺损实验模型,随机分为实验组、对照组和空白组,实验组植入同时负载5mgBMP及1×106个已向成骨细胞诱导的BMSCs的PLGA、对照组植入负载1×106个已向成骨细胞诱导的BMSCs的PLGA、空白组仅植入PLGA。术后对动物进行大体观察、摄X线片观察各组不同时相骨缺损修复情况、比较不同时相的骨缺损区X线阻射密度、并于术后第4、8、12周取出骨缺损区标本进行大体观察和组织学切片观察,图像分析骨小梁的生成数量。结果实验组在12周内骨缺损完全修复,且同时期内新生骨的数量和质量显著优于对照组,空白材料组骨缺损主要由纤维结缔组织填充。结论利用含BMP的PLGA支架与BMSCs复合构建的新型组织工程骨具有良好的骨缺损修复能力。

关键词：骨形态发生蛋白聚乳乙醇酸骨髓基质干细胞组织工程