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First Record of Cyclocarya from the Early Oligocene Qaidam Basin,North Tibet:Implications for the Paleogeography and Paleoecology

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Journal of Earth Science 2024年第1期35卷 201-211页

作者： Yafei hou Bowen Song Xiangchuan li Fang Han Xu zhang Kexin zhang Institute of Geological Survey China University of GeosciencesWuhan 430074China Faculty of Materials Science and Chemistry China University of GeosciencesWuhan 430074China State Key Laboratory of Biogeology and Environmental Geology China University of GeosciencesWuhan 430074China College of Earth Sciences and Resources&Key Laboratory of Western Mineral Resources and Geological Engineering of the Ministry of Education Chang'an UniversityXi'an 710054China State Key Laboratory of Palaeobiology and Stratigraphy Nanjing Institute of Geology and PalaeontologyChinese Academy of SciencesNanjing 210008China School of Earth Sciences East China University of TechnologyNanchang 330013China

As the largest intermontane basin in the northeastern Tibetan Plateau(TP),the Qaidam Basin provides unique insight into paleoclimatic change and its relationship with global change and uplift on the *** this study,based on morphological comparison,fossil fruit of Cyclocarya from the Early Oligocene Shangganchaigou Formation in the Qaidam Basin is assigned as Cyclocarya *** discovery of Cyclocarya *** demonstrates the occurrence of Cyclocarya in the Oligocene sediment in Qaidam *** is the first record of Cyclocarya fossil of Early Oligocene Age in China and indicates that Cyclocarya has existed on the northeastern TP since at least the Early *** living analogues of the current fossil now lives in sub-tropical China,where the East Asian Monsoon is *** the new fossils and previously reported fossil remains of plants and fishes,it can be inferred that the Early Oligocene Qaidam Basin was primarily influenced by westerly circulation and had a relatively warm and humid climate,which was in sharp contrast to the present-day climate in Qaidam Basin.

关键词： biostratigraphy climate change winged-fruit fossil Qaidam Basin Early Oligocene paleoclimate paleogeography

Oxidative Desulfurization of Fuel Oil with H_(3)PO_(4)-based Deep Eutectic Solvents

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China Petroleum Processing & Petrochemical Technology 2024年第2期26卷 178-186页

作者： li Xiuping zhang Jiayin hou liangpei Zhao Rongxiang School of Petrochemical Engineering Liaoning Petrochemical UniversityFushun 113001China

A series of Lewis-acid deep eutectic solvents (DESs) were synthesized by stirring phosphoric acid and zincchloride as raw materials at 80℃ to form H_(3)PO_(4)/nZnCl_(2) (n = 0.1, 0.25, 0.5, 0.75, 1). The DESs were characterized byFourier transform infrared spectrophotometry (FT-IR), thermogravimetry/differential thermogravimetry (TG/DTG), andelectron spray ionization mass spectrometry (ESI-MS). The DESs were used as both extractants and catalysts to removedibenzothiophene from fuels via oxidative desulfurization (ODS). Experiments were performed to investigated the influenceof factors such as composition of DES, temperature, oxidant dosage (molar ratio of O:S), DES dosage (volume ratio ofDES:oil), and number of cycles on desulfurization rate. The results indicated that the removal rate of dibenzothiophene (DBT)was affected by the Lewis acidic DESs, with that of H_(3)PO_(4)/0.25∙ZnCl_(2) reaching 96.4% under optimal conditions (Voil=5 mL,VDES=1 mL, an oxidant dosage of 6, T=50 ℃). After six cycles, the desulfurization rate of H_(3)PO_(4)/0.25∙ZnCl_(2) remained above94.1%. The apparent activation energy of dibenzothiophene (DBT) removal reaction was determined by a pseudo-first orderkinetic equation according to the Arrhenius equation to be 32.34 kJ/mol, as estimated. A reaction mechanism is proposedbased on the experimental data and characterization results.

关键词： deep eutectic solvents phosphoric acid zinc chloride oxidative desulfurization

Multi-scenario Simulation and Spatial-temporal Analysis of LUCC in China's Coastal Zone Based on Coupled SD-FLUS Model

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Chinese Geographical Science 2024年第4期34卷 579-598页

作者： hou Xiyong SONG Baiyuan zhang Xueying WANG Xiaoli li Dong Yantai Institute of Coastal Zone Research Chinese Academy of SciencesYantai 264003China Shandong Key Laboratory of Coastal Environmental Processes Yantai 264003China CAS Key Laboratory of Coastal Environmental Processes and Ecological Remediation Yantai Institute of Coastal Zone ResearchChinese Academy of SciencesYantai 264003China Shanghai Fuxiong Environmental Technology Corporation Shanghai 200433China

Increased human activities in China's coastal zone have resulted in the depletion of ecological land ***,conducting current and future multi-scenario simulation research on land use and land cover change(LUCC)is crucial for guiding the healthy and sustainable development of coastal *** dynamic(SD)-future land use simulation(FLUS)model,a coupled simulation model,was developed to analyze land use dynamics in China's coastal *** model encompasses five scenarios,namely,SSP1-RCP2.6(A),SSP2-RCP4.5(B),SSP3-RCP4.5(C),SSP4-RCP4.5(D),and SSP5-RCP8.5(E).The SD model simulates land use demand on an annual basis up to the year ***,the FLUS model determines the spatial distribution of land use for the near term(2035),medium term(2050),and long term(2100).Results reveal a slowing trend in land use changes in China's coastal zone from 2000–*** these changes,the expansion rate of construction land was the highest and exhibited an annual *** 2100,land use predictions exhibit high accuracy,and notable differences are observed in trends across *** summary,the expansion of production,living,and ecological spaces toward the sea remains *** A emphasizes reduced land resource dependence,benefiting ecological land *** B witnesses an intensified expansion of artificial *** C sees substantial land needs for living and production,while Scenario D shows coastal forest and grassland ***,in Scenario E,the conflict between humans and land *** study presents pertinent recommendations for the future development,utilization,and management of coastal areas in *** research contributes valuable scientific support for informed,long-term strategic decision making within coastal regions.

关键词： land use and land cover change(LUCC) multi-scenario simulation system dynamic-future land use simulation(SD-FLUS)model SSP-RCP scenarios model coupling China's coastal zone

Experimental validation of adsorption filter model under dynamic VOC concentrations:Prediction of long-term efficiency

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Building Simulation 2024年第7期17卷 1201-1212页

作者： Ruiyan zhang Ziying li Xiangyuan Guan Xin Wang Fei Wang lingjie zeng Zhenhai li School of Environment and Architecture University of Shanghai for Science and TechnologyShanghai 200093China School of Mechanical Engineering Tongji UniversityShanghai 200092China

Indoor volatile organic compound(VOC)concentrations are often dynamic because the ventilation and emission rates of VOC usually *** filters used for air purification may operate with a capacity that fluctuates with unsteady VOC concentrations in *** the dynamic interactions between adsorption filters and indoor air is crucial for predicting their performance under real-world *** study presents a numerical model of partially reversible adsorption equilibrium coupled with a mass transfer model to create a predictive model for adsorption efficiency in environments with dynamic VOC concentrations.A honeycomb adsorption filter for benzene adsorption was simulated and tested,including the breakthrough and purging curve and the long-term efficiency in an experimental chamber with dynamic *** results reveal that the curve generated with the partially reversible adsorption equilibrium model closely aligns with the measured ***,the model was coupled with a chamber model and the simulation results were compared with those calculated using the filter model with a single adsorption *** VOCs were emitted intermittently in the chamber and there was sufficient ventilation,the concentration peaks in the chamber derived from the models with different assumptions on adsorption reversibility were significantly different from each ***,it was observed that the reversible adsorption capacity of the filter was crucial for long-term operation in rooms with dynamic *** the reversible adsorption capacity constituting only 6.7%of the total adsorption capacity of the tested filter,it contributes to a significant“peak shaving and valley filling”effect,even when the irreversible adsorption capacity is *** adsorption reversibility should be taken as an important parameter for selecting adsorbents for dynamic concentration conditions.

关键词： adsorption filter efficiency model indoor air partially reversible adsorption

Resilience-driven cooperative reconfiguration strategy for unmanned weapon system-of-systems

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Journal of Systems Engineering and Electronics 2024年第4期35卷 932-944页

作者： SUN Qin li Hongxu zeng Yifan zhang Yingchao School of Systems Science and Engineering Sun Yat-sen UniversityGuangzhou 510006China

As the unmanned weap system-of systems(UWSoS)becomes complex,the inevitable uncertain interference gradu-ally increases,which leads to a strong emphasis on the resilience of ***,this paper presents a resilience-driven cooperative reconfiguration strategy to enhance the resilience of ***,a unified resilience-driven coopera-tive reconfiguration strategy framework is designed to guide the UWSoS resilience ***,a cooperative reconfiguration strategy algorithm is proposed to identify the optimal cooperative reconfiguration sequence,combining the cooperative pair resilience contribution index(CPRCI)and coop-erative pair importance index(CPII).At last,the effectiveness and superiority of the proposed algorithm are demonstrated through various attack scenario simulations that include differ-ent attack modes and *** analysis results can pro-vide a reference for decision-makers to manage UWSoS.

关键词： resilience strategy unmanned weapon system-of-systems(UWSoS) cooperative reconfiguration unmanned con-frontation

Nested Saturated Control of Uncertain Complex Cascade Systems Using Mixed Saturation Levels

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IEEE/CAA Journal of Automatica Sinica 2024年第5期11卷 1163-1174页

作者： Meng li Zhigang zeng Wuhan National Laboratory for Optoelectronics Wuhan 430074 School of Artificial Intelligence and Automation Huazhong University of Science and TechnologyWuhan 430074China School of Artificial Intelligence and Automation Huazhong University of Science and TechnologyWuhan 430074 Key Laboratory of Image Processing and Intelligent Control of Education Ministry of China Wuhan 430074China

This study addresses the problem of global asymptotic stability for uncertain complex cascade systems composed of multiple integrator systems and non-strict feedforward nonlinear systems. To tackle the complexity inherent in such structures, a novel nested saturated control design is proposed that incorporates both constant saturation levels and state-dependent saturation levels. Specifically, a modified differentiable saturation function is proposed to facilitate the saturation reduction analysis of the uncertain complex cascade systems under the presence of mixed saturation levels. In addition, the design of modified differentiable saturation function will help to construct a hierarchical global convergence strategy to improve the robustness of control design scheme. Through calculation of relevant inequalities, time derivative of boundary surface and simple Lyapunov function,saturation reduction analysis and convergence analysis are carried out, and then a set of explicit parameter conditions are provided to ensure global asymptotic stability in the closed-loop systems. Finally, a simplified system of the mechanical model is presented to validate the effectiveness of the proposed method.

关键词： method saturation differentiable

Photo-thermal synergistic excitation:Feasible strategy to detect ethanol for wide bandgap ZIF-8at low work temperature

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Journal of Environmental Sciences 2024年第4期138卷 112-120页

作者： Shuhao Shi Qian Du Ming hou Xiaolei Ye li Yang Shenghui Guo Jianhong Yi Ullah Ehsan Hongbo zeng State Key Laboratory of Complex Nonferrous Metal Resources Clean Utilization Faculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming 650093China Department of Chemical and Materials Engineering University of AlbertaEdmonton T6G 2V4Canada FEMTO-ST Institute(UMR CNRS 6174) Universite de Bourgogne Franche-Comte(UBFC)Universite de technologie de Belfort Montbéliard(UTBM)Site de MontbeliardBelfort F-90010France Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming 650093China

Zeolitic Imidazolate Framework-8(ZIF-8)material was prepared by chemical precipitation *** microstructure and physical properties of the as-prepared samples were characterized by XRD,BET,FESEM and UV *** self-made four-channel measurement device was used to test the gas sensitivity of ZIF-8 material toward ethanol gas under photo-thermal synergistic *** results showed that the sample was typical ZIF-8(E_(g)=4.96 eV)with a regular dodecahedron shape and the specific surface is up to 1793 m^(2)/*** as-prepared ZIF-8 has a gas response value of 55.04 to 100 ppm ethanol at 75℃ and it shows good gas sensing selectivity and repeated *** excellent gas sensitivity can be attributed to the increase of free electron concentration in the ZIF-8 conduction band by photo-thermal synergistic excitation,and the large specific surface area of ZIF-8 material provides more active sites for gas-solid surface *** reaction mechanism of ZIF-8 material under multi-field excitation was also discussed.

关键词： ZIF-8 material Photo-thermal synergistic excitation UV-light irradiation Photon-generated electron and hole Gas-sensitive property

Boosting li-ion storage kinetics via constructing layered TiO_(2) anode

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Particuology 2024年第10期93卷 22-29页

作者： Jiyue hou Fei Wang Enfeng zhang Ying Wang Peng Dong Yunxiao Wang Yiyong zhang Xue li Yingjie zhang National and Local Joint Engineering Research Center of lithium-ion Batteries and Materials Preparation Technology Faculty of Metallurgical and Energy EngineeringKunming University of Science and TechnologyKunming650093China College of Electrical Information Engineering Panzhihua UniversityPanzhihua617000China University Wollongong Australian Inst Innovat MatInst Superconducting&Elect MatInnovat Campus Squires WayWollongongNSW2500Australia

Due to the typical intercalation-deintercalation mechanism,TiO_(2) holds great promise as a sustainable anode for next-generation lithium-ion batteries(liBs).However,commercial TiO_(2)(C–TiO_(2))is granular and shows slow ionic conductivity,which greatly hinders its development due to sluggish kinetics,leading to low reversible capacity and inferior rate *** this study,a two-dimensional layered TiO_(2)(L-TiO_(2))anode is prepared via a one-step calcination process,which can effectively shorten the lithium ions diffusion path and improve its lithium ions *** elucidated the enhanced electrochemical performance of L-TiO_(2) as an anode in liBs through pseudocapacitive acceleration of lithium ions intercalation and deintercalation using various characterization techniques,including different scan rate cyclic voltammetry tests,in situ electrochemical impedance spectroscopy,in situ Raman spectroscopy,and in situ X-ray *** comparison to C–TiO_(2) material,L-TiO_(2) material showcases remarkable electrochemical performance,achieving a capacity of 166 mAh/g after 100 cycles at 0.1 ***,the lithium-ion diffusion coefficient calculated for the L-TiO_(2) is two orders of magnitude greater,underscoring its potential as a negative electrode material for liBs.

关键词： lithium-ionbatteries Anode MXene Layered TiO_(2)

High-performance self-powered GaN/PEDOT:PSS hybrid heterojunction UV photodetector for optical communication

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Science China(Technological Sciences) 2024年第2期67卷 608-615页

作者： li Shan liU zeng zhang Maolin YANG lili GUO YuFeng TANG WeiHua College of Integrated Circuit Science and Engineering&National and Local Joint Engineering Laboratory for RF Integration and Micro-Packing Technologies Nanjing University of Posts and TelecommunicationsNanjing 210023China

Self-powered ultraviolet photodetectors(UVPDs)provide great possibility for the next-generation energy conservation optical communication technology;while the high photodetection performance at zero bias is still a tremendous ***,ntype GaN film with Si-doping concentration of~1018cm^(-3)and p-type organic PEDOT:PSS were adopted to construct a planar hybrid heterojunction via the simple spin-coating *** from typical type-Ⅱenergy band alignment and giant photovoltaic effect at GaN/PEDOT:PSS inorganic-organic interface,the fabricated UVPD achieved excellent self-powered photoelectrical properties in dual-band with large R of 0.96 A/W(2.8 A/W),superior D*of 5.7×1012Jones(1.7×10^(13)Jones),prominent EQE of 325%(1371%),high on/off ratio of 9.65×10^(3)(6.15×10^(3))and fast rise/decay time of 60.7/124.5 ms(30.9/26.7 ms)for UVA(UVC)band,as well as outstanding UV/visible rejection ratio and great detection *** as an optical signal receiver,this designed self-powered UVPD decoded a message of“NJUPT”from a simple optical communication *** results open a new avenue for GaN/PEDOT:PSS heterojunction in UV communications and related applications.

关键词： GaN UV photodetector self-powered heterojunction optical communication