检索结果-南通市图书馆

Elucidating the structure-activity relationship of Cu-Ag bimetallic catalysts for electrochemical CO_(2) reduction

在线全文

学校读者我要写书评

暂无评论

Journal of Energy Chemistry 2024年第6期93卷 345-351,I0009页

作者： Qining Huang Lili Wan Qingxuan ren Jingshan Luo Institute of Photoelectronic Thin Film Devices and Technology State Key Laboratory of Photovoltaic Materials and CellsKey Laboratory of Photoelectronic Thin Film Devices and Technology of TianjinMinistry of Education Engineering Research Center of Thin Film Photoelectronic TechnologyNankai UniversityTianjin 300350China Frontiers Science Center for New Organic Matter Nankai UniversityTianjin 300071China Haihe Laboratory of Sustainable Chemical Transformations Tianjin 300192China

Developing bimetallic catalysts is an effective strategy for enhancing the activity and selectivity of electrochemical CO_(2) reduction reactions,where understanding the structure-activity relationship is essential for catalyst ***,we prepared two Cu-Ag bimetallic catalysts with Ag nanoparticles attached to the top or the bottom of Cu *** tested in a flow cell,the Cu-Ag catalyst with Ag nanoparticles on the bottom achieved a faradaic efficiency of 54%for ethylene production,much higher than the catalyst with Ag nanoparticles on the *** catalysts were further studied in the H-cell and zero-gap MEA *** was found that placing the two metals in the intensified reaction zone is crucial to triggering the tandem reaction of bimetallic *** work elucidates the structure-activity relationship of bimetallic catalysts for CO_(2) reduction and demonstrates the importance of considering both catalyst structures and cell characteristics to achieve high activity and selectivity.

关键词： Electrochemical CO_(2)reduction Bimetallic catalyst Cu-Ag Structure-activity relationship

Two simple memristive maps with adaptive energy regulation and digital signal process verification

在线全文

学校读者我要写书评

暂无评论

Journal of Zhejiang University-Science A(Applied Physics & Engineering) 2024年第5期25卷 382-394页

作者： Feifei YANG Lujie ren Jun MA Zhigang ZHU College of Electrical and Information Engineering Lanzhou University of TechnologyLanzhou 730050China Department of Physics Lanzhou University of TechnologyLanzhou 730050China School of Information Science and Engineering Dalian Polytechnic UniversityDalian 116034China

Mathematical models can produce desired dynamics and statistical properties with the insertion of suitable nonlinear terms,while energy characteristics are crucial for practical application because any hardware realizations of nonlinear systems are relative to energy *** involvement of memristive terms relative to memristors enables multistability and initial-dependent property in memristive *** this study,two kinds of memristors are used to couple a capacitor or an inductor,along with a nonlinear resistor,to build different neural *** corresponding circuit equations are derived to develop two different types of memristive oscillators,which are further converted into two kinds of memristive maps after linear *** Hamilton energy function for memristive oscillators is obtained by applying the Helmholz theorem or by mapping from the field energy of the memristive *** Hamilton energy functions for both memristive maps are obtained by replacing the gains and discrete variables for the memristive oscillator with the corresponding parameters and *** two memristive maps have rich dynamic behaviors including coherence resonance under noisy excitation,and an adaptive growth law for parameters is presented to express the self-adaptive property of the memristive maps.A digital signal process(DSP)platform is used to verify these *** scheme will provide a theoretical basis and experimental guidance for oscillator-to-map transformation and discrete map-energy calculation.

关键词： Hamilton energy Discrete memristor Self-adaptive regulation Digital signal process(DSP)implementation

Precise phase adjustment and antibacterial property of copper sulfide particles in confined mesoporous silica nanoreactor

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Particuology 2024年第2期85卷 113-121页

作者： Shiyu Xu Jinyong Wu Zhongzhen ren Dechao Niu Low Dimensional Materials Chemistry Laboratory Key Laboratory for Ultrafine Materials of Ministry of EducationFrontier Science Center of the Materials Biology and Dynamic ChemistryShanghai Engineering Research Center of Hierarchical NanomaterialsSchool of Materials Science and EngineeringEast China University of Science and TechnologyShanghai200237China

Bacteria-caused wound infection greatly threatens human health,thus developing an efficient and safe antibacterial agent without drug resistance is still a great ***,a confined vulcanization strategy is proposed to construct copper sulfides-loaded dual-mesoporous silica nanospheres(Cux-Sy@DMSNs)with various crystal phases for reactive oxygen species(ROS)-mediated and photothermal antibacterial *** the pore confinement of DMSNs,the crystal phases of copper sulfides including CuS,Cu_(9)S_(5)and Cui.96S can be easily controlled by changing the vulcanization *** relationships between the crystal phases and photothermal properties as well as peroxidase-like activity of copper sulfides were systematically *** show that the obtained CuS@DMSNs exhibited higher photothermal ability with remarkable photothermal conversion efficiency of 36.86%in the second near-infrared region(NIR-II)and better peroxidase-like activity,compared to those of Cu_(9)S_(5)@DMSNs and Cu_(1.96)S@*** a result,the in vitro experiments showed the good antibacterial effect against both gram-negative *** and gram-positive *** under 1064 nm laser irradiation and the presence of H_(2)O_(2).Besides,the CCK-8 assay indicated that CuS@p-DMSNs have minimal cytotoxicity against normal human umbilical vein endothelial cells at the ranged ***,the resultant CuS@p-DMSNs could act as a promising antibacterial agent for deep wound bacterial infection treatment.

关键词： Copper sulfides Mesoporous silica Photothermal Reactive oxygen species Antibacterial agent

A Cyclic Constitutive Model Based on Crystal Plasticity for Body-Centered Cubic Cyclic Softening Metals

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Acta Mechanica Solida Sinica 2024年第1期37卷 33-42页

作者： Xuehong ren Wenjie Zhao Shaopu Yang Guilin Wen State Key Laboratory of Advanced Design and Manufacturing for Vehicle Body Hunan UniversityChangsha 410082China School of Mechanical Engineering Tianjin Sino-German University of Applied SciencesTianjin 300350China State Key Laboratory of Mechanical Behavior in Traffic Engineering Structure and System Safety Shijiazhuang Tiedao UniversityShijiazhuang 050043China

Under the framework of the small deformation crystal plasticity theory,a crystal plastic cyclic constitutive model for body-centered cubic(BCC)cyclic softening polycrystalline metals is *** constitutive model introduces the isotropic softening rule that includes two different mechanisms:namely softening under monotonic deformation and softening under cyclic deformation on each slip ***,a modified Armstrong-Frederick nonlinear kinematic hardening rule is *** appropriate explicit scale transition rule is selected to extend the single crystal constitutive model to the polycrystalline constitutive *** the model is used to predict the uniaxial and multiaxial ratcheting deformation of BCC axle steel EA4T to verify the rationality of the proposed *** simulation results indicate that the newly established crystal plasticity model can not only describe the cyclic softening characteristics of BCC axle steel EA4T well,but also reasonably describe the evolution laws of uniaxial ratcheting and nonproportional multiaxial ratcheting ***,the established crystal plastic cyclic constitutive model can reasonably predict the ratcheting behavior of BCC single crystal as well.

关键词： Crystal plasticity Constitutive model Softening Ratcheting

Vision-Based Adaptive Prescribed-Time Control of UAV for Uncooperative Target Tracking with Performance Constraint

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Systems Science & Complexity 2024年第5期37卷 1956-1977页

作者： SHE Xuehua MA Hui ren Hongru LI Hongyi School of Automation and the Guangdong Provincial Key Laboratory of Intelligent Decision and Cooperative Control Guangdong University of Technology School of Mathematics and Statistics Guangdong University of Technology College of Electronic and Information Engineering and Chongqing Key Laboratory of Generic Technology and System of Service Robots Southwest University

This paper discusses the uncooperative target tracking control problem for the unmanned aerial vehicle(UAV) under the performance constraint and scaled relative velocity constraint, in which the states of the uncooperative target can only be estimated through a vision sensor. Considering the limited detection range, a prescribed performance function is designed to ensure the transient and steady-state performances of the tracking system. Meanwhile, the scaled relative velocity constraint in the dynamic phase is taken into account, and a time-varying nonlinear transformation is used to solve the constraint problem, which not only overcomes the feasibility condition but also fails to violate the constraint boundaries. Finally, the practically prescribed-time stability technique is incorporated into the controller design procedure to guarantee that all signals within the closed-loop system are *** is proved that the UAV can follow the uncooperative target at the desired relative position within a prescribed time, thereby improving the applicability of the vision-based tracking approach. Simulation results have been presented to prove the validity of the proposed control strategy.

关键词： Nonlinear transformation performance constraint prescribed-time tracking uncooperative target vision-based measurement

An interlaminar damage shell model for typical composite structures

在线全文

同方期刊数据库

学校读者我要写书评

暂无评论

Chinese Journal of Aeronautics 2024年第1期37卷 118-137页

作者： Jie ZHOU Zhen WU Zhengliang LIU Xiaohui ren School of Aeronautics Northwestern Polytechnical UniversityXi’an 710072China National Key Laboratory of Strength and Structural Integrity Xi’an 710065China School of Mechanical Engineering Xi’an Aeronautical UniversityXi’an 710065China

Using the plate/shell elements in commercial software,accurate analysis of interlaminar initial damage in typical composite structures is still a challenging *** propose an accurate and efficient model for analysis of interlaminar initial damage,the following work is carried out:(A)A higher-order theory is firstly proposed by introducing the local Legendre polynomials,and then a novel shell element containing initial damage prediction is developed,which can directly predict transverse shear stresses without any postprocessing *** variables at each node are independent of number of layers,so the proposed model is more efficient than the 3D-FEM.(B)Compression experiment is carried out to verify the capability of the proposed *** results obtained from the proposed model are in good agreement with experimental data.(C)Several examples have been analyzed to further assess the capability of the proposed model by comparing to the 3D-FEM ***,accuracy and efficiency have been evaluated in different damage criterion by comparing with the selected *** numerical results show that the proposed model can well predict the initial interlaminar damage as well as other ***,the model is implemented with UEL subroutine,so that the present approach can be readily utilized to analyze the initial damage in typical composite structures.

关键词： Compression experiment Finite element method Initial damage Interlaminar stress Plate/shell element

Optimization Control of Multi-Mode Coupling All-Wheel Drive System for Hybrid Vehicle

在线全文

学校读者我要写书评

暂无评论

Chinese Journal of Mechanical Engineering 2024年第2期37卷 340-355页

作者： Lipeng Zhang Zijian Wang Liandong Wang Changan ren School of Vehicle and Energy Yanshan UniversityQinhuangdao 066004China

The all-wheel drive(AWD)hybrid system is a research focus on high-performance new energy vehicles that can meet the demands of dynamic performance and passing *** optimization of the power and economy of hybrid vehicles becomes an issue.A unique multi-mode coupling(MMC)AWD hybrid system is presented to realize the distributed and centralized driving of the front and rear axles to achieve vectored distribution and full utilization of the system power between the axles of *** on the parameters of the benchmarking model of a hybrid vehicle,the best model-predictive control-based energy management strategy is ***,the drive system model was built after the analysis of the MMC-AWD’s drive ***,three fundamental strategies were established to address power distribution adjustment and battery SOC maintenance when the SOC changed,which was followed by the design of a road driving force ***,the energy consumption rate in the average time domain was processed before designing the minimum fuel consumption controller based on the equivalent fuel consumption ***,the advantage of the MMC-AWD was confirmed by comparison with the dynamic performance and economy of the BYD Song PLUS *** findings indicate that,in comparison to the comparative hybrid system at road adhesion coefficients of 0.8 and 0.6,the MMC-AWD’s capacity to accelerate increases by 5.26%and 7.92%,*** the road adhesion coefficient is 0.8,0.6,and 0.4,the maximum climbing ability increases by 14.22%,12.88%,and 4.55%,*** a result,the dynamic performance is greatly enhanced,and the fuel savings rate per 100 km of mileage reaches 12.06%,which is also very *** proposed control strategies for the new hybrid AWD vehicle can optimize the power and economy simultaneously.

关键词： Hybrid vehicle All-wheel drive Multi-mode coupling Energy management Model predictive control

Effects of Co-Firing Biomass and Pulverized Coal on NO Reduction in Cement Precalciner

在线全文

学校读者我要写书评

暂无评论

Journal of Thermal Science 2024年第2期33卷 751-760页

作者： LI Pengpeng ren Qiangqiang LYU Qinggang WANG Mingyue School of Energy Power and Mechanical Engineering North China Electric Power UniversityBeijing102206China Institute of Engineering Thermophysics Chinese Academy of SciencesBeijing100190China University of Chinese Academy of Sciences Beijing100049China

With increased awareness of the large-scale CO_(2) emissions from the cement industry,there has been growing focus on greenhouse gas reduction *** all these strategies,fuel substitution using biomass fuel is extensively used to achieve CO_(2) zero-emission in cement *** to the avoidable high-temperature-generated thermal nitrogen oxides during cement production,research on the impact of biomass application on nitrogen oxide emissions shall be carried *** types of biomass fuel and bituminous coal were used to investigate the NO reduction characteristics under different O_(2) concentrations on experimental *** was found that the change in oxygen concentration from 9% to 1% increased the reaction time in the reactor from 555 s to 1425 s,which means the increase in oxygen concentration can lead to shorter reaction time,and correspondingly,the existing time of nitric oxide in the flue gas is also shortened,but the peak value of nitric oxide rises,during the process of O_(2) concentration changing from 1% to 9%,the peak NO concentration in the flue gas increased from 5.4×10^(-5) to 1.05×10^(-4).An increase in O_(2) concentration greatly reduces the total reduction of NO and the minimum change in NO *** peak NO concentration during the combustion process of corn stalk is 4.56×10^(-4),which is approximately 7 times higher than that of coal,and it is caused by the high amount of N in corn *** addition of raw meal has an inhibitory effect on the reduction of NO:after adding raw meal,the effective reduction time of NO by fuel decreased by about 20%,but adding raw meal raises CO_(2) concentration of fuel gas in the early stage of reaction.

关键词： cement precalciner biomass fuel coal NO reduction co-firing

Commentary:The central lymphatic drainage in pharmacological,surgical and physical therapies of Alzheimer’s disease

在线全文

学校读者我要写书评

暂无评论

Acta Pharmaceutica Sinica B 2024年第7期14卷 3291-3293页

作者： Lixuan ren Jianping Ye Metabolic Disease Research Center Zhengzhou Central Hospital Affiliated to Zhengzhou UniversityZhengzhou 450000China Tianjian Laboratory of Advanced Biomedical Sciences Academy of Medical SciencesZhengzhou UniversityZhengzhou 450001China

Alzheimer’s disease(AD)is a prevalent neurodegenerative disease in the aged *** of AD remains largely unknown and no effective drugs are available in clinical settings to reverse or delay the disease *** recent years,the brain’s lymphatic systems,including glymphatic3 that exists in the brain interstitial space and meningeal lymphatic vessels4 that presents within the dural sinuses,have been found to play an important role in the AD pathogenesis.

关键词： Ab Central lymphatic drainage Surgery NPLP AD