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Endosulfan residues and farmers’replacement behaviors of endosulfan in the north-west inland cotton region

Frontiers of Environmental Science & Engineering 2024年第4期18卷 35-47页

作者： Shuyan zhou Yang Zhang Jingjing Wang Shikun Cheng Fuyan Zhuo Yun hong School of Energy and Environmental Engineering University of Science and Technology Beijing 100083China Foreign Environmental Cooperation Center Ministry of Ecology and Environment of the People’s Republic of ChinaBeijing 100035China United Nations Development Programme in China Beijing 100600China National Agro-Tech Extension and Service Center Beijing 100125China

We assessed the situation of endosulfan residues in cotton fields after the endosulfan ban came into effect and the current knowledge,attitude,and practice(KAP)of cotton farmers on the phase-out of endosulfan and the application of alternative *** samples(n=91)of cotton fields were collected from the major cotton-producing areas in China,namely the north-west inland cotton region,and the endosulfan residues were analyzed.A KAP survey was carried out for cotton farmers,and 291 questionnaires were *** influences of gender,age,education background,cotton planting years,publicity and training,income sources,and other factors on cotton farmers’KAP were *** results showed that endosulfan sulfate was the main endosulfan residue in the soil,followed byβ-endosulfan andα-endosulfan,the average residual contents were 0.569,0.139,and 0.060μg/kg,*** results of the KAP study showed that cotton farmers scored low on knowledge about the phase-out of endosulfan and the application of alternative technologies but high on attitude and *** number of family members,years of cotton planting,age,and the cottonplanting area had different degrees of influence on KAP *** training could significantly improve the KAP scores of cotton farmers;training should be more targeted and designed reasonably for key groups,such as men and the population under 30,followed by training them to use pesticides *** large-scale cotton growers,training should focus on green prevention and control technologies.

关键词： Cotton fields Endosulfan residues Farmers KAP survey Replacement behaviours

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Multifunctional 2-(2-hydroxyphenyl)benzoxazoles: Ready synthesis,mechanochromism, fluorescence imaging, and OLEDs

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Chinese Chemical Letters 2024年第10期35卷 249-253页

作者： Kangmin Wang Liqiu Wan Jingyu Wang Chunlin zhou Ke Yang liang zhou Bijin Li Chongqing Key Laboratory of Natural Product Synthesis and Drug Research School of Pharmaceutical Sciences Chongqing University State Key Laboratory of Rare Earth Resource Utilization Changchun Institute of Applied Chemistry Chinese Academy of Sciences Jiangsu Key Laboratory of Advanced Catalytic Materials & Technology School of Petrochemical Engineering Changzhou University

Triphenylamine(TPA)-containing 2-(2-hydroxyphenyl)benzoxazoles(2a-2c) have been synthesized via a highly efficient rhodium-catalyzed C–H/C–H cross-coupling reaction. Compound 2a is a novel mechanofluorochromic material with blue-shifted mechanochromic properties. Compounds 2b and 2c presented opposite mechanochromic trends. For 2b, the enol-form emission enhanced, and the ketoform emission blue-shift after grinding. In contrast, 2c exhibited the weak enol-form emission disappeared and the keto-form emission slightly red-shift after grinding treatments. The estrone-containing2b-based water-dispersed nanoparticles(NPs) exhibit apparent dual-emission and were applied for fluorescence images. In addition, bis(TPA)-containing 2c-based devices exhibit dual-emission with good performance and a singlet exciton yield of 92%, which breaks through the theoretical upper limit of 25%in conventional fluorescent OLEDs. This is one of the highest exciton utilization values recorded for the ESIPT molecules with a dual emission system.

关键词： 2-(2′-Hydroxyphenyl)benzoxazoles Fluorescence images Mechanochromism OLEDs Rhodium-catalyzed

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The E3 ubiquitin ligase TRAF6 controls CTLA-4 turnover and promotes T-cell-mediated antitumor immunity

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Cellular & Molecular Immunology 2024年第1期21卷 97-99页

作者： Xiao-liang Jie Hua Guo Guang-Biao zhou State Key Laboratory of Molecular Oncology National Cancer Center/National Clinical Research Center for Cancer/Cancer HospitalChinese Academy of Medical Sciences and Peking Union Medical College100021 BejingChina

Yu et al.[1]reported that the tumor necrosis factor(TNF)receptor OX40(CD134)-TNF receptor-associated factor 6(TRAF6)axis mediates Lys63-linked ubiquitination and subsequent lysosomal degradation of cytotoxic T-lymphocyte antigen 4(CTLA-4),leading to the enhancement of CD8^(+)T-cell-mediated antitumor *** findings unveil a previously unknown mechanism in controlling the stability of the immune checkpoint CTLA-4 and provide a potential therapeutic target for the improvement of Tcell-based immunotherapy.

关键词： immunity OX40 ubiquitin

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Effect of unstable resonator stability on laser beam quality

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Optoelectronics Letters 2024年第9期20卷 523-530页

作者： liang Xiaolin BAO Ben'gang zhou Songqing CHEN Huihuang College of Intelligent Manufacturing Hunan University of Science and EngineeringYongzhou 425199China

In order to explore the effect of unstable resonator stability on laser beam quality,the numerical simulation of midinfrared laser and visible laser was carried out in GLAD *** simulation results showed that the existence of defocus aberration,tilt aberration and astigmatic aberration in the unstable resonator can cause the center of the far-field spot of the output annular beam to drift,the number of peripheral diffraction rings to increase,the beam quality to deteriorate,and the degree of effect is different.

关键词： resonator laser beam

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An exo Probe-based Reverse Transcription and Recombinase Polymerase Amplification for Rapid Detection of Feline Calicivirus in Cats

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Biomedical and Environmental Sciences 2024年第3期37卷 325-330页

作者： MU hong Yun zhou hong Lei JING Zheng LU Wei ZHANG Jian Wei Jiangsu Agri-animal Husbandry Vocational College Taizhou 225300JiangsuChina Boehringer Ingelheim Animal Health(Shanghai)Co. LTD.Shanghai 200040China

Feline calicivirus(FCV)was a highly prevalent RNA virus causing upper respiratory tract infections in cats through the mouth and nose around the world,result in the death of cats especially under 1 year old with upper respiratory tract disease(URTD)and virulent systemic disease(FCV-VSD)[1].Infected cats usually presented with mouth ulcers,salivation and ***,both recovered cats and asymptomatic carriers can still carry and spread the FCV virus for extended periods of time,contributing to the potential for *** presented a significant threat to the health and lives of cats,and rare wildlife and took a heavy financial loss on the pet industry,making the prevention and control of the virus ***,rapid identification of FCV in clinical samples was necessary to prevent the spread of FCV and avoid financial loss.

关键词： prevention respiratory Probe

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Differential Game Model of Resource Extraction with Continuous and Dynamic Updating

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Journal of the Operations Research Society of China 2024年第1期12卷 51-75页

作者： Ovanes Petrosian Tihomirov Denis Jiang-Jing zhou hong-Wei Gao School of Mathematics Harbin Institute of TechnologyHarbin150001HeilongjiangChina School of Automation Qingdao UniversityQingdao266071ShandongChina Faculty of Applied Mathematics and Control Processes Saint-Petersburg State UniversitySaint PetersburgRussia National Research University"High School of Economics" Saint-PetersburgRussia School of Mathematics and Statistics Qingdao UniversityQingdao266071ShandongChina

This paper is devoted to a new class of differential games with continuous and dynamic *** direct application of resource extraction in a case of dynamic and continuous updating is *** is proved that the optimal control(cooperative strategies)and feedback Nash equilibrium strategies uniformly converge to the corresponding strategies in the game model with continuous updating as the number of updating instants converges to *** results are presented for an optimal trajectory(cooperative trajectory),equilibrium trajectory and corresponding payoffs.

关键词： Differential games Dynamic updating Continuous updating Optimal control Feedback Nash equilibrium

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BSTFNet:An Encrypted Malicious Traffic Classification Method Integrating Global Semantic and Spatiotemporal Features

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Computers, Materials & Continua 2024年第3期78卷 3929-3951页

作者： hong Huang Xingxing Zhang Ye Lu Ze Li Shaohua zhou School of Computer Science and Engineering Sichuan University of Science&EngineeringYibin644002China School of Mathematics and Statistics Sichuan University of Science&EngineeringYibin644002China

While encryption technology safeguards the security of network communications,malicious traffic also uses encryption protocols to obscure its malicious *** address the issues of traditional machine learning methods relying on expert experience and the insufficient representation capabilities of existing deep learning methods for encrypted malicious traffic,we propose an encrypted malicious traffic classification method that integrates global semantic features with local spatiotemporal features,called BERT-based Spatio-Temporal Features Network(BSTFNet).At the packet-level granularity,the model captures the global semantic features of packets through the attention mechanism of the Bidirectional Encoder Representations from Transformers(BERT)*** the byte-level granularity,we initially employ the Bidirectional Gated Recurrent Unit(BiGRU)model to extract temporal features from bytes,followed by the utilization of the Text Convolutional Neural Network(TextCNN)model with multi-sized convolution kernels to extract local multi-receptive field spatial *** fusion of features from both granularities serves as the ultimate multidimensional representation of malicious *** approach achieves accuracy and F1-score of 99.39%and 99.40%,respectively,on the publicly available USTC-TFC2016 dataset,and effectively reduces sample confusion within the Neris and Virut *** experimental results demonstrate that our method has outstanding representation and classification capabilities for encrypted malicious traffic.

关键词： Encrypted malicious traffic classification bidirectional encoder representations from transformers text convolutional neural network bidirectional gated recurrent unit

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Narrowband blue emitter based on fused nitrogen/carbonyl combination with external quantum efficiency approaching 30%

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Science China Chemistry 2024年第1期67卷 351-359页

作者： Long Chen Jia-Heng Cai You-Jun Yu Yang-Kun Qu Sheng-Yi Yang Sheng-Nan Zou Rui-hong Liu Dong-Ying zhou liang-Sheng Liao Zuo-Quan Jiang Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering Macao University of Science and TechnologyMacao 999078China

Multi-resonance thermally activated delayed fluorescence(MR-TADF)emitters can enable narrowband emission with high color purity and electroluminescence ***/carbonyl(N/C=O)system is receiving increasing attention while the nitrogen/boron(N/B)system has been widely *** decoration is an effective approach for N/B type MR-TADF system but always leads to broadening and red-shifting of the emission band in N/C=O MR-TADF *** attribute these unfavorable phenomena to the formation of intramolecular charge transfer between the MR-core and peripheral *** address this issue,we have developed a new strategy by decorating DMQAO(a fused N/C=O MR-core)with a triazine acceptor and a neutral terphenyl group to construct MTDMQAO and MBDMQAO,*** introduction of the triazine acceptor not only realizes efficient narrowband emission in MTDMQAO,but also accelerates the reverse intersystem crossing process through enhanced spin-orbital *** a result,MTDMQAO exhibits a significantly higher external quantum efficiency of 29.4%compared to the referent emitters,validating the rationality of our derivation *** study highlights the potential of the N/C=O system for MR-TADF emitters and provides important insights for understanding the difference between N/B and N/C=O systems.

关键词： carbonyl group narrowband acceptor decoration thermally activated delayed fluorescence OLEDs

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Decoupled water electrolysis:Flexible strategy for pure hydrogen production with small voltage inputs

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Journal of Energy Chemistry 2024年第7期94卷 340-356页

作者： Kexin zhou Jiahui Huang Daili Xiang Aijiao Deng Jialei Du hong Liu Institute for Advanced Interdisciplinary Research(iAIR) Collaborative Innovation Center of Technology and Equipment for Biological Diagnosis and Therapy in Universities of ShandongUniversity of JinanJinan 250022ShandongChina State Key Laboratory of Crystal Materials Shandong UniversityJinan 250100ShandongChina Zhengzhou Vocational College of Industrial Safety Zhengzhou 451192HenanChina

Hydrogen gas is widely regarded as an ideal green energy carrier and a potential alternative to fossil fuels for coping with the aggravating energy crisis and environmental ***,the vast majority of the world's hydrogen is produced by reforming fossil fuels;however,this hydrogen-making technology is not sustainable or environmentally friendly because ofits high energy consumption and large carbon ***-driven water splitting(2H_(2)0-2H_(2)+0_(2))becomes an extensively studied scheme for sustain-able hydrogen *** water electrolysis requires an input voltage higher than 1.23 V and forms a gas mixture of H_(2)/O_(2),which results in high electricity consumption,potential safety hazards,and harmful reactive oxygen *** virtue of the auxiliary redox mediators(RMs)as the robust H^(+)/e^(-)reservoir,decoupled electrolysis splits water at a much lower potential and evolves O_(2)(H_(2)O+RMS_(ox)-O_(2)+H-RMS_(red))and H_(2)(H-RMS_(red)-H_(2)+RMS_(ox))at separate times,rates,and spaces,thus pro-ducing the puretarget hydrogen gas *** electrolysis has accelerated the development ofwater electrolysis technology for H_(2) ***,itis still lack of a comprehensive and in-depth review in this field based on different types of *** review highlights the basic principles and critical progress of this emerging water electrolysis mode over the past *** representative examples are then dis-played in detail according to the differences in the *** rational choice and design of RMs have also been ***,novel applications of decoupled water splitting are briefly discussed,including the manufacture of valuable chemicals,Cl_(2) production,pollutant degradation,and other half-reactions in artificial ***,thekey characteristics and disadvantages of each type of mediator are sum-marized in *** addition,we present an outlook for future directions in decoupled

关键词： Hydrogen production Conventional water splitting Decoupled water splitting Redox mediators Biomimetics

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Waste acid recovery utilizing monovalent cation permselective membranes through selective electrodialysis

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Chinese Journal of Chemical Engineering 2024年第7期71卷 45-57页

作者： Yanran Zhu Yue zhou Qian Chen Rongqiang Fu Zhaoming Liu liang Ge Tongwen Xu Anhui Provincial Engineering Laboratory of Functional Membrane Materials and Technology Department of Applied ChemistrySchool of Chemistry and Materials ScienceUniversity of Science and Technology of ChinaHefei 230026China Key Laboratory of Charged Polymeric Membrane Materials of Shandong Province Shandong Tianwei Membrane Technology Co.Ltd.Weifang 261000China

Selective electrodialysis(SED)has surfaced as a highly promising membrane separation technique in the realm of acid recovery owing to its ability to effectively separate monovalent ions through the utilization of a potential ***,the current SED process is limited by conventional commercial monovalent cation permselective membranes(MCPMs).This study systematically investigates the use of an independently developed MCPM in the SED process for acid *** factors such as current density,volume ratio,initial ion concentration,and waste acid systems are *** independently developed MCPM offers several advantages over the commercial monovalent selective cation-exchange membrane(CIMS),including higher recovered acid concentration,better ion flux ratio,improved acid recovery efficiency,increased recovered acid purity,and higher current *** SED process with the MCPM achieves a recovered acid of 95.9%and a concentration of 2.3 mol·L^(–1) in the HCl/FeCl_(2) system,when a current density of 20 mA·cm^(-2) and a volume ratio of 1:2 are ***,in the H_(2)SO_(4)/FeSO_(4) system,a purity of over 99%and a concentration of 2.1 mol·L^(–1) can be achieved in the recovered *** study thoroughly examines the impact of operation conditions on acid recovery performance in the SED *** independently developed MCPM demonstrates outstanding acid recovery performance,highlighting its potential for future commercial utilization.

关键词： Selective electrodialysis Wastewater Monovalent cation permselective membranes Separation Recovery

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