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Engineering S-scheme W_(18)O_(49)/ZnIn_(2)S_(4)heterojunction by Co_(x)P nanoclusters for enhanced charge transfer capability and solar hydrogen evolution

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Nano Research 2024年第9期17卷 8095-8103页

作者： Xiaojie Liu Erkang Liu Zixian Wang Wen Zhang Mingyu dou Hua Yang Changhua An Dacheng Li Jianmin dou Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology School of Chemistry and Chemical EngineeringLiaocheng UniversityLiaocheng 252059China Tianjin Key Laboratory of Organic Solar Cell and Photochemical Conversion School of Chemistry and Chemical EngineeringTianjin Key Laboratory of Advanced Functional Porous MaterialsInstitute for New Energy Materials and Low-Carbon TechnologiesTianjin University of TechnologyTianjin 300384China Institute of Powder Metallurgy and Advanced Ceramics School of Materials Science and EngineeringUniversity of Science and Technology BeijingBeijing 100083China

Enhancement of the light-absorption response and utilization of the photogenerated carriers represent a robust strategy for the design of high-performance *** this work,grafting Co_(x)P nanoclusters onto S-scheme heterojunction of W18O49/ZnIn2S4(WO/ZIS-CoxP)with strong response to the ultraviolet-visible-near infrared ray(UV-vis-NIR)region has been achieved,which possesses efficient electron-transfer-channel,and boosts charge-separation and transport *** as-prepared WO/ZIS-Co_(x)P yields an impressive solar-driven hydrogen production rate of 45 mmol·g^(-1)·h^(-1).The increased photocatalytic performance is attributed to the synergistic effect of the composite catalyst:(1)The local surface plasmon resonance-induced“hot electron”injection of W_(18)O_(49)significantly increases the electron density;(2)the engineered S-scheme directional electron transfer promotes charge separation and enhances the reducing capability of photoexcited electrons;and(3)Co_(x)P as electron-trap site for accelerating surface proton reduction *** work provides a platform to impart nonprecious co-catalyst for engineering S-scheme heterojunction,serving a class of efficient solar-driven photocatalyst towards hydrogen production.

关键词： hydrogen cocatalyst photocatalysis S-scheme hot electron

Spatiotemporal Prediction of Urban Traffics Based on Deep GNN

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Computers, Materials & Continua 2024年第1期78卷 265-282页

作者： Ming Luo Huili dou Ning Zheng School of Computer Science Hangzhou Dianzi UniversityHangzhou310018China Zhejiang Institute of Communications Hangzhou310012China School of Cyberspace Security Hangzhou Dianzi UniversityHangzhou310018China

Traffic prediction already plays a significant role in applications like traffic planning and urban management,but it is still difficult to capture the highly non-linear and complicated spatiotemporal correlations of traffic *** well as to fulfil both long-termand short-termprediction objectives,a better representation of the temporal dependency and global spatial correlation of traffic data is *** order to do this,the Spatiotemporal Graph Neural Network(S-GNN)is proposed in this research as amethod for traffic *** S-GNN simultaneously accepts various traffic data as inputs and investigates the non-linear correlations between the *** terms of modelling,the road network is initially represented as a spatiotemporal directed graph,with the features of the samples at the time step being captured by a convolution *** order to assign varying attention weights to various adjacent area nodes of the target node,the adjacent areas information of nodes in the road network is then aggregated using a graph *** data is output using a fully connected layer at the *** findings show that S-GNN can improve short-and long-term traffic prediction accuracy to a greater extent;in comparison to the control model,the RMSE of S-GNN is reduced by about 0.571 to 9.288 and the MAE(Mean Absolute Error)by about 0.314 to *** experimental results on two real datasets,Pe MSD7(M)and PEMS-BAY,also support this claim.

关键词： Urban traffic traffic temporal correlation GNN prediction

Quantized Decoders that Maximize Mutual Information for Polar Codes

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China Communications 2024年第7期21卷 125-134页

作者： Zhu hongfei Cao Zhiwei Zhao Yuping Li dou School of Electronics Engineering and Computer Science Peking UniversityBeijing 100871China

In this paper,we innovatively associate the mutual information with the frame error rate(FER)performance and propose novel quantized decoders for polar *** on the optimal quantizer of binary-input discrete memoryless channels(BDMCs),the proposed decoders quantize the virtual subchannels of polar codes to maximize mutual information(MMI)between source bits and quantized *** nested structure of polar codes ensures that the MMI quantization can be implemented stage by *** results show that the proposed MMI decoders with 4 quantization bits outperform the existing nonuniform quantized decoders that minimize mean-squared error(MMSE)with 4 quantization bits,and yield even better performance than uniform MMI quantized decoders with 5 quantization ***,the proposed 5-bit quantized MMI decoders approach the floating-point decoders with negligible performance loss.

关键词： maximize mutual information polar codes quantization successive cancellation decoding

Basilic vein variation encountered during surgery for arm vein port:A case report

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World Journal of Clinical Cases 2024年第12期12卷 2086-2091页

作者： Cheng-Da Hu Rui Lv Ya-Xin Zhao Ming-Hao Zhang hong-dou Zeng Yi-Wen Mao Department of Breast Surgery The Second Affiliated Hospital and Yuying Children’s Hospital of Wenzhou Medical UniversityWenzhou 325000Zhejiang ProvinceChina

BACKGROUND Venous variations are uncommon and usually hard to identify,and basilic vein variation is particularly *** vein variation usually presents without any clinical symptoms and is often regarded as a benign *** case was a patient with congenital basilic vein variation encountered during surgery for an infusion *** SUMMARY We documented and analyzed an uncommon anatomical variation in the basilic vein encountered during arm port *** peculiarity has hitherto remained undescribed in the *** offer remedial strategies for addressing this anomaly in the future and precautionary measures to circumvent its *** conducted a comprehensive review of analogous cases in the literature,offering pertinent therapeutic recommendations and solutions,with the aim of enhancing the efficacy and safety of future arm port *** Venous variation is rare and requires detailed intraoperative and postoperative examination to ensure accuracy,so as not to affect subsequent treatment.

关键词： Totally implantable venous access ports Arm ports Venous variation Postoperative breast cancer Systematic review Case report

Parotid metastasis of rare lung adenocarcinoma:A case report

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World Journal of Clinical Cases 2024年第6期12卷 1182-1189页

作者： Ru-Xi Yan Lin-Bo dou Zi-Jia Wang Xue Qiao hong-Hai Ji Yan-Cong Zhang School of Stomatology Weifang Medical UniversityWeifang 261000Shandong ProvinceChina Department of Stomatology Dezhou People’s HospitalDezhou 253000Shandong ProvinceChina Department of Stomatology Dezhou Women and Children's HospitalDezhou 253000Shandong ProvinceChina

BACKGROUND Lung cancer(LC)is the leading cause of malignancy-related deaths *** most common sites of metastasis include the nervous system,bone,liver,respiratory system,and adrenal *** metastasis in the parotid gland is very rare,and its diagnosis presents a ***,we report a case of parotid metastasis in primary *** SUMMARY The patient was a 74-year-old male who was discovered to have bilateral facial asymmetry inadvertently two years *** right earlobe was slightly swollen and without pain or *** tomography(CT)examination showed bilateral lung space-occupying *** biopsy was performed and revealed adenocarcinoma(right-upper-lung nodule tissue).Positron emission tomography-CT examination showed:(1)Two hypermetabolic nodules in the right upper lobe of the lung,enlarged hy-permetabolic lymph nodes in the right hilar and mediastinum,and malignant space-occupying lesion in the right upper lobe of the lung and possible metastasis to the right hilar and mediastinal lymph nodes;and(2)multiple hypermetabolic nodules in bilateral parotid *** puncture biopsy was performed considering lung adenocarcinoma *** detection of lung biopsy specimens revealed an EGFR gene 21 exon L858R *** This case report highlights the challenging diagnosis of parotid metastasis in LC given its rare *** lesions should be differentiated from primary tumors of the parotid *** radiological imaging is unreliable,and puncture biopsy is needed for final diagnosis of this condition.

关键词： Lung cancer Metastasis Parotid gland Pathology Positron emission tomography/computed tomography Case report

Solvent effects on Diels-Alder reaction in ionic liquids:A reaction density functional study

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Chinese Journal of Chemical Engineering 2024年第2期66卷 180-188页

作者： Zijiang dou Weiqiang Tang Peng Xie Shuangliang Zhao Guangxi Key Laboratory of Petrochemical Resource Processing and Process Intensification Technology and School of Chemistry and Chemical Engineering Guangxi UniversityNanning 530004China State Key Laboratory of Chemical Engineering and School of Chemical Engineering East China University of Science and TechnologyShanghai 200237China

Extensive experimental studies have been performed on the Diels-Alder(DA)reactions in ionic liquids(ILs),which demonstrate that the IL environment can significantly influence the reaction rates and ***,the underlying microscopic mechanism remains *** this work,the multiscale reaction density functional theory is applied to explore the effect of 1-butyl-3-methylimidazolium hexafluorophosphate([BMIM][PF_(6)])solvent on the reaction of cyclopentadiene(CP)with acrolein,methyl acrylate,or *** analyzing the free energy landscape during the reaction,it is found that the polarization effect has a relatively small influence,while the solvation effect makes both the activation free energy and reaction free energy *** addition,the rearrangement of local solvent structure shows that the cation spatial distribution responds more evidently to the reaction than the anion,and this indicates that the cation plays a dominant role in the solvation effect and so as to affect the reaction rates and selectivity of the DA reactions.

关键词： Solvent effect Ionic liquids Diels-Alder reaction Reaction density functional theory

Solvation Engineering via Fluorosurfactant Additive Toward Boosted Lithium-Ion Thermoelectrochemical Cells

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Nano-Micro Letters 2024年第4期16卷 253-268页

作者： Yinghong Xu Zhiwei Li Langyuan Wu Hui dou Xiaogang Zhang Jiangsu Key Laboratory of Electrochemical Energy Storage Technologies College of Material Science and TechnologyNanjing University of Aeronautics and AstronauticsNanjing 211106People’s Republic of China

Lithium-ion thermoelectrochemical cell(LTEC), featuring simultaneous energy conversion and storage, has emerged as promising candidate for low-grade heat harvesting. However, relatively poor thermosensitivity and heat-to-current behavior limit the application of LTECs using LiPF_6 electrolyte. Introducing additives into bulk electrolyte is a reasonable strategy to solve such problem by modifying the solvation structure of electrolyte ions. In this work, we develop a dual-salt electrolyte with fluorosurfactant(FS) additive to achieve high thermopower and durability of LTECs during the conversion of low-grade heat into electricity. The addition of FS induces a unique Li~+ solvation with the aggregated double anions through a crowded electrolyte environment,resulting in an enhanced mobility kinetics of Li~+ as well as boosted thermoelectrochemical performances. By coupling optimized electrolyte with graphite electrode, a high thermopower of 13.8 mV K^(-1) and a normalized output power density of 3.99 mW m^(–2) K^(–2) as well as an outstanding output energy density of 607.96 J m^(-2) can be *** results demonstrate that the optimization of electrolyte by regulating solvation structure will inject new vitality into the construction of thermoelectrochemical devices with attractive properties.

关键词： Solvation engineering Fluorosurfactant Ionic thermoelectric Lithium-ion thermoelectrochemical cell Low-grade heat

Requirements ranking based on crowd-sourcing high-end product USs

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Journal of Systems Engineering and Electronics 2024年第1期35卷 94-104页

作者： MA Yufeng dou Yajie XU Xiangqian JIA Qingyang TAN Yuejin College of Systems Engineering National University of Defense TechnologyChangsha 410003China

Based on the characteristics of high-end products,crowd-sourcing user stories can be seen as an effective means of gathering requirements,involving a large user base and generating a substantial amount of unstructured *** key challenge lies in transforming abstract user needs into specific ones,requiring integration and ***,we propose a topic mining-based approach to categorize,summarize,and rank product requirements from user ***,after determining the number of story categories based on py LDAvis,we initially classify“I want to”phrases within user ***,classic topic models are applied to each category to generate their names,defining each post-classification user story category as a ***,a weighted ranking function is devised to calculate the importance of each ***,we validate the effectiveness and feasibility of the proposed method using 2966 crowd-sourced user stories related to smart home systems.

关键词： high-end product complex system crowd-sourcing user stories topic mining requirements ranking

A review of research progress on continuous cropping obstacles

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Frontiers of Agricultural Science and Engineering 2024年第2期11卷 253-270页

作者： Kunguang WANG Qiaofang LU Zhechao dou Zhiguang CHI Dongming CUI jing MA Guowei WANG Jialing KUANG Nanqi WANG Yuanmei ZUO College of Resources and Environmental Sciences State Key Laboratory of Nutrient Use and ManagementNational Academy of Agriculture Green DevelopmentChina Agricultural UniversityBeijing 100193China College of Resources and Environmental Sciences Southwest UniversityChongqing 400715China Yunnan ICL YTH Phosphate Research and Technology Co. Ltd.Kunming 650228China

Due to the increasing global population and limited land resources, continuous cropping has become common. However, after a few years of continuous cropping, obstacles often arise that cause soil degeneration, decreased crop yield and quality, and increased disease incidence, resulting in significant economic losses. It is essential to understand the causes and mitigation mechanisms of continuous cropping obstacles(CCOs) and then develop appropriate methods to overcome them. This review systematically summarizes the causes and mitigation measures of soil degradation in continuous cropping through a meta-analysis. It was concluded that not all continuous cropping systems are prone to CCOs. Therefore, it is necessary to grasp the principles governing the occurrence of diseases caused by soilborne pathogens in different cropping systems, consider plant–soil-organisms interactions as a system, scientifically regulate the physical and chemical properties of soils from a systems perspective, and then regulate the structure of microbial food webs in the soil to achieve a reduction in diseases caused by soilborne pathogens and increase crop yield ultimately. This review provides reference data and guidance for addressing this fundamental problem.

关键词： Continuous cropping obstacles rhizosphere regulation soil microecological environment