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Unexpected Li displacement and suppressed phase transition enabling highly stabilized oxygen redox in P3-type Na layered oxide cathode

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Journal of Energy Chemistry 2023年第10期85卷 144-153,I0006页

作者： Myungeun Choi hobin ahn Hyunyoung Park Yongseok Lee Jinho ahn Bonyoung Ku Junseong Kim Wonseok Ko Jungmin Kang Jung-Keun Yoo Duho Kim Jongsoon Kim Department of Energy Science Sungkyunkwan UniversitySuwon 16419Republic of Korea SKKU Institute of Energy Science and Technology(SIEST) Sungkyunkwan UniversitySuwon 16419Republic of Korea Carbon Composites Department Korea Institute of Materials Science(KIMS)Changwon 51508Republic of Korea Department of Mechanical Engineering(Integrated Engineering Program) Kyung Hee University1732Deogyeong-daeroGiheung-guYongin-siGyeonggi-do 17104Republic of Korea Department of KHU-KIST Convergence Science and Technology Kyung Hee University23Kyunghee-daero Dongdaemun-guSeoul 02447Republic of Korea

Oxygen redox is considered a new paradigm for increasing the practical capacity and energy density of the layered oxide cathodes for Na-ion batteries. However, severe local structural changes and phase transitions during anionic redox reactions lead to poor electrochemical performance with sluggish ***, we propose a synergy of Li-Cu cations in harnessing the full potential of oxygen redox, through Li displacement and suppressed phase transition in P3-type layered oxide cathode. P3-type Na_(0.7)[Li_(0.1)Cu_(0.2)Mn_(0.7)]O_(2) cathode delivers a large specific capacity of ~212 mA h g^(-1)at 15 mA g^(-1). The discharge capacity is maintained up to ~90% of the initial capacity after 100 cycles, with stable occurrence of the oxygen redox in the high-voltage region. Through advanced experimental analyses and first-principles calculations, it is confirmed that a stepwise redox reaction based on Cu and O ions occurs for the charge-compensation mechanism upon charging. Based on a concrete understanding of the reaction mechanism, the Li displacement by the synergy of Li-Cu cations plays a crucial role in suppressing the structural change of the P3-type layered material under the oxygen redox reaction, and it is expected to be an effective strategy for stabilizing the oxygen redox in the layered oxides of Na-ion batteries.

关键词： Layered oxide cathode Oxygen redox reaction Structural stability Li displacement No phase transition

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Fibrinogen’s potential role in connecting cerebrovascular abnormalities with glymphatic dysfunction in Alzheimer’s disease

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Neural Regeneration Research 2025年第1期20卷 203-204页

作者： Vishal Singh Arnab Choudhury Hyung Jin ahn Department of Pharmacology Physiology and NeurosciencesRutgers-New Jersey Medical SchoolNewarkNJUSA Brain Health Institute Rutgers UniversityPiscatawayNJUSA

Alzheimer’s disease(AD)stands out as the primary manifestation of age-related dementia,portraying a chronic neurodegenerative disorder distinguished by the accumulation of fibrillar amyloid-β(Aβ)plaques and neurofibrillary tangles of hyperphosphorylated ***,from a clinical standpoint,AD presents itself as a complex condition with a spectrum of dysfunctions rather than a singular pathological *** often-overlooked aspect of the disease is the presence of extensive cerebrovascular abnormalities,given that the majority of AD patients experience altered cerebral blood flow,damaged vasculature,increased microinfarcts and *** models of AD further support this observation,showing cerebrovascular dysfunction such as impaired cerebral blood flow and altered cerebrovascular reactivity(Tataryn et al.,2021;Gareau et al.,2023).

关键词： cerebrovascular dysfunction Alzheimer

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Maximizing biomass utilization: An integrated strategy for coproducing multiple chemicals

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Journal of Energy Chemistry 2025年第1期100卷 180-191页

作者： Byeongchan ahn Sua Jo Jonggeol Na J.Jay Liu Young-Ju Kim Wangyun Won Department of Chemical and Biological Engineering Korea University Department of Chemical Engineering (Integrated process) Kyung Hee University Department of Chemical Engineering and Materials Science Ewha Womans University Department of Chemical Engineering Pukyong National University Resources Engineering Plant Research Department Korea Institute of Geoscience and Mineral Resources

Lignocellulosic biomass is one of the viable solutions to alleviate the global warming. However, the limited utilization of biomass majorly focused on cellulose and hemicellulose restricts the economic and environmental feasibilities. To cope with this issue, we proposed an integrated process of co-producing 1,6-hexanediol（1,6-HDO） with tetrahydrofuran and adipic acid from biomass, referred to as Strategy A. To compare the impacts of lignin upgrading and feedstock, Strategy B, which co-produces tetrahydrofuran alone, and Strategy C, which is the traditional route to produce 1,6-HDO from fossil fuels, were used. Heat networks are also designed to reduce operating costs and indirect carbon emissions due to energy consumption, saving 87% and 83% of the heat and cooling requirements, respectively, in Strategy A. The market competitiveness of Strategy A was evaluated by determining the minimum selling price through techno-economic analysis, and sustainability was thoroughly investigated by quantifying the environmental impacts through both midpoint and endpoint life-cycle assessments（LCAs）.Strategy A was found to be the most favorable both economically（USRDSCHARDOLLAR3,402/ton） and environmentally（-26.9 kg CO2eq.）. This indicates that lignin valorization is not only economically but also environmentally preferred. Finally, changes in economic and environmental feasibilities depending on economic, process, and environmental parameters were investigated using sensitivity and uncertainty analyses. The results of these analyses provide valuable insight into bio-based chemical production.

关键词： Biorefinery Carbon mitigation Climate change Global warming Lignin utilization Bioeconomy

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Prominent cycling reversibility and kinetics enabled by CaTiO3 protective layer on Zn metal for aqueous Zn-ion batteries

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Journal of Energy Chemistry 2025年第1期100卷 245-258页

作者： Gaeun Lee Yong Nam ahn Seongjoon So Chanwoo Park Jong-Seong Bae Taehyun Park Il Tae Kim Jaehyun Hur School of Chemical Biological and Battery Engineering Gachon University Seongnam Busan Center Korea Basic Science Institute

Aqueous Zn-ion batteries （AZIBs） have received considerable attention owing to their various advantages such as safety,low cost,simple battery assembly conditions,and high ionic ***,they still suffer from serious problems,including uncontrollable dendrite growth,corrosion,hydrogen evolution reaction （HER） from water decomposition,electrode passivation,and unexpected *** creation of a uniform artificial nanocrystal layer on the Zn anode surface is a promising strategy for resolving these ***,we propose the use of a perovskite CaTiO3（CTO） protective layer on Zn（CTO@Zn） as a promising approach for improving the performance of *** CTO artificial layer provides an efficient pathway for Zn ion diffusion towards the Zn metal because of the high dielectric constant （εr=180） and ferroelectric characteristics that enable the alignment of dipole moments and redistribute the Zn2+ions in the CTO *** avoiding the direct contact of the Zn anode with the electrolyte solution,the uneven dendrite growth,corrosion,parasitic side reactions,and HER are mitigated,while CTO retains its mechanical and chemical robustness during ***,CTO@Zn demonstrates an improved lifespan in a symmetric cell configuration compared with bare ***@Zn shows steady overpotential （～68 m V） for 1500 h at 1 mA cm-2/0.5 mA h cm-2,excelling bare ***,when paired with the V2O5-C cathode,the CTO@Zn//V2O5-C full battery delivers 148.4 mA h g-1（based on the mass of the cathode） after 300 *** study provides new insights into Zn metal anodes and the development of high-performance AZIBs.

关键词： Artificial layer Dielectric constant Zn metal anode Zinc aqueous battery

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The IOSS Chaos Synchronization Method

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Chinese Physics Letters 2011年第1期28卷 32-35页

作者： Choon Ki ahn Faculty of the Department of Automotive Engineering Seoul National University of Science&Technology172 Gongneung 2-dongNowon-guSeoul 139-743Korea

A new synchronization method, called the input/output-to-state stable synchronization (IOSSS) method, is proposed for a general class of chaotic systems with external disturbance. By introducing Lyapunov stability theory and linear matrix inequality (LMI) for the first time, the IOSSS controller is shown to not only guarantee the synchronization of the chaotic systems, but also reduce the effect of external disturbance. The proposed IOSSS controller can be obtained by solving the LMI, which can easily be done using standard numerical packages. A numerical example is given to demonstrate the availability of the proposed method.

关键词： method chaotic inequality

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Design and Analysis of Osmosis-based Artificial Muscle

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Journal of Bionic Engineering 2019年第1期16卷 56-65页

作者： Juhui Gim Changsun ahn School of Mechanical Engineering Pusan National UniversityBusan 46241Korea

This paper presents the design and analysis of an osmosis-based artificial muscle inspired by the leaf movements of Mimosa ***'s leaves quickly contract using osmosis pressure in the pulvinus when they are *** analyzed and simulated an osmosis system to identify the factors for fast osmosis reactions and designed a prototype artificial muscle based on the *** osmosis phenomenon was mathematically modeled,analyzed,and verified through several *** analysis shows that fast osmosis responses require a large diffusion coefficient with a high-flux membrane or small ratio of the cross-sectional area to the volume of the osmosis *** designed a micro-scale system to achieve the required *** contraction and relaxation of the artificial muscle are realized by changes of the local concentration of potassium ions,which can be aggregated by a controllable electric *** a result,the artificial muscle shows controllable behavior with fast reactions.

关键词： Mimosa pudica osmosis artificial muscle cross-sectional area to volume ratio micro-scale

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Architecture for mobile group communication in campus environment

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Frontiers of Computer Science 2013年第4期7卷 505-513页

作者： Yujin LIM Sanghyun ahn Department of Information Media University of Suwon Hwaseong 445-743 Korea School of Computer Science University of Seoul Seoul 130-743 Korea

The demand for group communication using smart devices in campus environment is increasing rapidly. In this paper, we design an architecture for a mobile group communication system （MGCS） on campus by using Wi-Fi networks and smart devices. The architecture is composed of a web-based system and a smart device based mobile system. Through the systems, users on campus create community/mobile group, maintain dynamic group membership, and reliably deliver the message to other users. We use the common features of many smart devices to develop a prototype that works on off-the-shelf hardware. In the experimental section, we demonstrate our system using various real scenarios which can occur in university campuses.

关键词： smart campus smartphone location tracking,mobile community

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Regression tree ensemble learning-based prediction of the heating and cooling loads of residential buildings

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Building Simulation 2022年第11期15卷 2003-2017页

作者： Nikhil Pachauri Chang Wook ahn Al Graduate School Gwangju Institute of Science and Technology123 Cheomdangwagi-roBuk-guGwangju 61005R.O.Korea

Building energy consumption is heavily dependent on its heating load(HL)and cooling load(CL).Therefore,an efficient building demand forecast is critical for ensuring energy savings and improving the operating efficacy of the heating,ventilation,and air conditioning(HVAC)*** and specialized energy-efficient building modeling technologies may offer a fair estimate of the influence of different construction ***,deploying these tools could be time-consuming and complex for the ***,in this article,an ensemble model based on decision trees and the least square-boosting(LS-boosting)algorithm known as the regression tree ensemble(RTE)is proposed for the accurate prediction of HL and *** hyper parameters of the RTE are optimized by shuffled frog leaping optimization(SFLA),which leads to *** regression(STR)and Gaussian process regression(GPR)based on different kernel functions are also designed for comparison *** demonstrate that the value of root mean squared error is reduced by 37%–68%and 30%–41%for HL and CL of residential buildings,respectively,by the proposed SRTE in comparison to other ***,the findings from the real dataset support the proposed model’s effectiveness in predicting HVAC energy *** can be concluded that the proposed SRTE is more effective and accurate than other methods for predicting the energy consumption of HVAC systems.

关键词： energy heating load cooling load decision tree LS-boosting shuffled frog leaping optimization

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L_2-L_∞ learning of dynamic neural networks

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Chinese Physics B 2010年第10期19卷 1-6页

作者： Choon Ki ahn Department of Automotive Engineering Seoul National University of Technology 172 Gongneung 2-dong Nowon-gu Seoul 139-743 Korea

This paper proposes an y2-y∞ learning law as a new learning method for dynamic neural networks with external disturbance. Based on linear matrix inequality （LMI） formulation, the y2-y∞ learning law is presented to not only guarantee asymptotical stability of dynamic neural networks but also reduce the effect of external disturbance to an y2-y∞ induced norm constraint. It is shown that the design of the y2-y∞ learning law for such neural networks can be achieved by solving LMIs, which can be easily facilitated by using some standard numerical packages. A numerical example is presented to demonstrate the validity of the proposed learning law.

关键词： y2-y∞ learning law dynamic neural networks linear matrix inequality Lyapunovstability theory

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Item Response Theory Based Ensemble in Machine Learning

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International Journal of Automation and computing 2020年第5期17卷 621-636页

作者： Ziheng Chen Hongshik ahn Department of Applied Mathematics and Statistics Stony Brook UniversityNew York 11794−3600USA

In this article,we propose a novel probabilistic framework to improve the accuracy of a weighted majority voting *** order to assign higher weights to the classifiers which can correctly classify hard-to-classify instances,we introduce the item response theory(IRT)framework to evaluate the samples′difficulty and classifiers′ability *** assigned the weights to classifiers based on their *** models are created with different assumptions suitable for different *** making an inference,we keep a balance between the accuracy and *** our experiment,all the base models are constructed by single trees via *** explain the models,we illustrate how the IRT ensemble model constructs the classifying *** also compare their performance with other widely used methods and show that our model performs well on 19 datasets.

关键词： Classification ensemble learning item response theory machine learning expectation maximization(EM)algorithm

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