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MOF-derived Se doped MnS/Ti_(3)C_(2)T_(x) as cathode and Zn-Ti_(3)C_(2)T_(x) membrane as anode for rocking-chair zinc-ion battery

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Nano Research 2024年第4期17卷 2781-2789页

作者： Kaisheng Sun Zemao Xiao Yunfei Shen heng lv Jianpeng Zhu Jianxiang Pang Yang Zheng Wenwen Kong Long Chen School of Chemistry and Chemical Engineering/State Key Laboratory Incubation Base for Green Processing of Chemical Engineering Shihezi UniversityShihezi 832003China CAS Key Laboratory of Functional Materials and Devices for Special Environments Xinjiang Key Laboratory of Electronic Information Materials and DevicesCenter of Materials Science and Optoelectronics EngineeringXinjiang Technical Institute of Physics and Chemistry of CASUrumqi 830011China

Mn-based zinc ion battery has the advantages of low cost and high performance,which makes it the promising energy storage ***,the poor conductivity and the agglomeration in the synthesis process of manganese-based materials restrict the performance of ***,the Se-doped MnS/Ti_(3)C_(2)T_(x)(Se-MnS/Ti_(3)C_(2)T_(x))composite material derived from Mn-based metal-organic framework is *** tests show that Se-doped could generate S defects and enhance the electrochemical activity of *** the same time,the introduction of Ti_(3)C_(2)T_(x) substrate is conducive to exposing more sulfur defects and improving the utilization rate of *** the mechanism study,it is found that Se-MnS/Ti_(3)C_(2)T_(x) is transformed into S/Se co-doped Mn3O_(4) at the first charge,which innovatively elucidated the behavior of S/Se during *** the electrochemical performance test,the specific capacity can reach 74.7 mAh·g^(-1) at 5.0 A·g^(-1).In addition,the Zn-Ti_(3)C_(2)T_(x) membrane electrode is prepared by vacuum filtration as the zinc-poor anode,which is assembled into the rocking chair full battery to avoid dendrite growth and exhibit excellent rate *** addition of Zn2+weakens the electrostatic repulsion between the interlayers of MXene,and the formation of the folded morphology aids the penetration of the *** 1.0 A·g^(-1),the capacity can reach 50.6 mAh·g^(-1).This work is helpful to promote the research and development of the reaction mechanism of manganese based rocking chair batteries.

关键词： rocking-chair zinc-ion battery MnS Zn-Ti_(3)C_(2)T_(x) membrane Se doped Ti_(3)C_(2)T_(x) composite

一种基于时空运动信息交互建模的三维人体姿态估计方法

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图学学报 2024年第1期45卷 159-168页

作者：吕衡杨鸿宇北京航空航天大学计算机学院北京100191 北京航空航天大学人工智能研究院北京100191

三维人体姿态估计在虚拟现实和人机交互等领域具有重要作用。近年来,Transformer已被引入三维人体姿态估计领域,用于捕捉人体关节点的时空运动信息。然而,现有研究通常只关注于人体关节点群的整体运动,或只对单独的人体关节点运动进行建... 详细信息

三维人体姿态估计在虚拟现实和人机交互等领域具有重要作用。近年来,Transformer已被引入三维人体姿态估计领域,用于捕捉人体关节点的时空运动信息。然而,现有研究通常只关注于人体关节点群的整体运动,或只对单独的人体关节点运动进行建模,均没有深入地探讨每个关节点的独特运动模式及不同关节点运动间的相互影响。因此,提出了一种创新的方法,旨在细致地学习每帧中的二维人体关节点的空间信息,并对每个关节点的特定运动模式进行深入分析。通过设计一个基于Transformer编码器的运动信息交互模块,精确地捕捉不同关节点之间的动态运动关系。相较于已有直接对人体关节点的整体运动进行学习的模型,此方法能够使得预测精度提高约3%。与注重单节点运动的最先进MixSTE模型相比,该模型在捕捉关节点的时空特征方面更为高效,推理速度实现了20%以上提升,使其更适合于实时推理的场景。

关键词： 3D人体姿态估计 Transformer编码器关节点间运动时空信息关联实时推理

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超临界水氧化技术中反应器腐蚀问题研究现状

广州化工 2024年第5期52卷 32-34,57页

作者：吕恒侯淼昂高小琦西安特种设备检验检测院陕西西安710065

本研究介绍了超临界水氧化过程中反应器的腐蚀问题以及国内外关于此类问题的研究。目前研究主要使用特殊结构的反应器以降低腐蚀速率,或者利用晶界工程技术提升材料的抗氧化性解决腐蚀问题,但没有对反应器的腐蚀机制进行研究。因此,本... 详细信息

本研究介绍了超临界水氧化过程中反应器的腐蚀问题以及国内外关于此类问题的研究。目前研究主要使用特殊结构的反应器以降低腐蚀速率,或者利用晶界工程技术提升材料的抗氧化性解决腐蚀问题,但没有对反应器的腐蚀机制进行研究。因此,本文提出通过试验研究和数值模拟分析探究反应器的腐蚀机制。这对超临界水氧化技术中的发展和应用具有重要的意义。

关键词：超临界水氧化技术反应器腐蚀晶界工程数值模拟腐蚀机制

2006—2020年中国丙型病毒性肝炎发病趋势及年龄-时期-队列分析

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现代预防医学 2024年第14期51卷 2497-2500+2534页

作者：白峻竹游姝萌张馨吕恒梁王勇徐元勇张文义中国医科大学公共卫生学院中国人民解放军疾病预防控制中心安徽医科大学公共卫生学院

目的分析2006—2020年间中国丙型病毒性肝炎(丙肝)发病趋势，探索年龄、时期、出生队列对丙肝发病率产生的影响。方法收集2006—2020年间中国丙肝病例数据和人口学资料。应用Joinpoint回归模型分析全人群及分年龄组人群丙肝发病率的... 详细信息

目的分析2006—2020年间中国丙型病毒性肝炎(丙肝)发病趋势，探索年龄、时期、出生队列对丙肝发病率产生的影响。方法收集2006—2020年间中国丙肝病例数据和人口学资料。应用Joinpoint回归模型分析全人群及分年龄组人群丙肝发病率的变化趋势，应用年龄-时期-队列模型探讨年龄、时期和出生队列对发病率的影响。结果 2006—2020年间丙肝发病率整体呈现上升趋势，平均发病率为12.82/10万。与其他年龄组不同的是，60岁及以上年龄组人群丙肝发病在2010—2018年间仍呈现上升趋势(APC=3.40)。丙肝发病时期效应从2006—2010年期间的0.63(95%CI:0.57～0.70)升至2016—2020年间的0.92(95%CI:0.84～1.00);出生队列效应以1926—1930年出生人群最低，1991—1995年间出生的人群中达到峰值(RR=1.41,95%CI:1.01～1.97)。结论丙肝研究期间内发病率整体呈现上升趋势，疾病负担随年龄增长而增加。对于高危人群应当进行定期筛查，加强监测。

关键词：丙型病毒性肝炎发病率 Joinpoint回归模型年龄-时期-队列模型

Thermodynamic and Economic Analysis of a Conceptual System Combining Sludge Gasification,SOFC,Supercritical CO_(2)Cycle,and Organic Rankine Cycle

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Journal of Thermal Science 2024年第4期33卷 1491-1508页

作者： lv Jiayang WANG Chizhong CHEN heng PAN Peiyuan XU Gang ZHANG Guoqiang School of Energy Power and Mechanical EngineeringNorth China Electric Power UniversityBeijing102206China

In order to reduce the environmental impact of conventional sludge treatment methods and to utilize the energy in sludge more effectively,a coupled system based on sewage sludge gasifier(SSG),solid oxide fuel cells(SOFC),supercritical CO_(2)cycle(S-CO_(2)),and organic Rankine cycle(ORC)is *** clean syngas obtained from sludge gasification is mixed with CH4 and then first utilized by the fuel *** exhaust gas from the fuel cell is fully combusted in the afterburning chamber and then enters the bottom cycle system consisting of S-CO_(2)&ORC to generate *** understand the performance of the system,thermodynamic and economic analyses were conducted to examine the project's *** thermodynamics as well as the economics of the coupled system were analyzed to arrive at the following conclusions,the power production of the system is 37.34 MW;the exergy efficiency is 55.62%,and the net electrical efficiency is 61.48%.The main exergy destruction is the gasifier and SOFC,accounting for 62.45%of the total exergy *** takes only6.13 years to repay the construction investment in the novel system,and the project obtains a NPV of 17723820USD during 20 years *** above findings indicate that the new coupled system has a better performance in terms of energy utilization and economy.

关键词： sewage sludge gasifier SOFC supercritical CO_(2)cycle organic Rankine cycle multi-system coupling

Reversible on-off switching of spin-crossover behavior via photochemical [2+2] cycloaddition reaction

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Science China Chemistry 2022年第1期65卷 120-127页

作者： Long-Fei Wang Bang-heng lv Feng-Tai Wu Guo-Zhang Huang Ze-Yu Ruan Yan-Cong Chen Min Liu Zhao-Ping Ni Ming-Liang Tong Key Laboratory of Bioinorganic and Synthetic Chemistry of Ministry of Education School of ChemistrySun Yat-Sen UniversityGuangzhou 510006China School of Nuclear Science and Technology University of South ChinaHengyang 421001China

Herein,we report the first example showing the reversible on-off switching of spin-crossover(SCO)property by solid state photochemical[2+2]*** ultraviolet(UV)light-induced[2+2]cycloaddition reaction of 3-spy ligands in a twodimensional(2D)Hofmann-type framework[Fe(3-spy)_(2){Pd(CN)_(4)}](1,3-spy=3-styrylpyridine),which shows a hysteretic twostep SCO behavior,gives a 3D Hofmann-type framework[Fe(rctt-3-ppcb){Pd(CN)_(4)}](2,rctt-3-ppcb=rctt-1,3-bis(3-pyridyl)-2,4-bis(phenyl)cyclobutane,r=reference group,c=cis and t=trans)accompanied with the disappearing of SCO ***,upon heating at 250℃ for 12 h,the rctt-3-ppcb ligand in 2 could be partially dedimerized to 3-spy with 68%completion through single-crystal-to-single-crystal(SCSC)transformation,giving the annealing complexes[Fe(3-spy)1.36(rctt-3-ppcb)0.32{Pd(CN)_(4)}](3)which display an incomplete SCO *** 2■3 interconversion is successfully achieved via continuous UV irradiation and thermal annealing,demonstrating the effectiveness of photochemical[2+2]reaction on switching on-off SCO properties.

关键词： reversible photo cycloaddition spin-crossover Hofmann-type frameworks photomagnetism

A Noteof CP_(2) Groups

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Communications in Mathematics and Statistics 2017年第4期5卷 447-451页

作者： Wujie Shi heng lv Department of Mathematics Chongqing University of Arts and SciencesChongqing 402160People’s Republic of China School of Mathematics and Statistics Southwest UniversityChongqing 400715People’s Republic of China

A new class CP_(2) groups of finite groups was characterized by using an inequality of the orders of *** this short paper we give a note of CP_(2) groups since CP_(2) groups is a subclass of CP(EPPO)***,we discuss the... 详细信息

关键词： Finite groups Element orders CP groups Frobenius groups·2-Frobenius groups

Room-temperature phonon-coupled single-photon emission in hexagonal boron nitride

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Science China(Physics,Mechanics & Astronomy) 2024年第5期67卷 109-114页

作者： Jia-Min Lai Qing-Hai Tan Feilong Song Haonan Chang Yanpei lv Xue-Lu Liu Jinghua Teng Weibo Gao Ping-heng Tan Jun Zhang State Key Laboratory of Superlattices and Microstructures Institute of SemiconductorsChinese Academy of SciencesBeijing100083China Key Laboratory of Magnetic Molecules and Magnetic Information Materials of Ministry of Education&Research Institute of Materials Science Shanxi Normal UniversityTaiyuan 030000China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Division of Physics and Applied Physics School of Physical and Mathematical SciencesNanyang Technological UniversitySingapore 637371Singapore Institute of Materials Research and Engineering(IMRE) Agency for ScienceTechnology and Research(A*STAR)Singapore 138634Singapore

Photon-lattice(phonon)coupling is fundamental to light-matter interaction,particularly when it reaches the quantum limit of the phonon-coupled single-photon emission,which holds great potential for quantum manipulation and quantum information ***,we report single defect state-phonon coupling in hexagonal boron nitride(h BN)at room *** ultrabroad spectrum of single-photon emissions can be achieved by selecting the excitation *** photoluminescence excitation spectroscopy,we observe single-phonon-assisted resonance-enhanced single-photon emission,along with multiple phonon replicas that herald the creation of phonon Fock *** also develop a transition model to gain insight into the physical process behind the single defect state-phonon *** work sets the stage for manipulating electron-phonon coupling state with single quantum-level precision at room temperature.

关键词： temperature phonon hexagonal

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Damage and deterioration mechanism and curing technique of concrete structure in main coal cleaning plants

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Mining Science and Technology 2009年第6期19卷 750-755页

作者： lv heng-lin ZHAO Cheng-ming SONG Lei MA Ying XU Chun-hua School of Architecture and Civil Engineering China University of Mining ＆ Technology Xuzhou Jiangsu 221116 China State Key Laboratory for Geomechanics and Deep Underground Engineering Xuzhou Jiangsu 221008 China Wuhan Design ＆ Research Institute of Sinocoal International Engineering Group Wuhan Hubei 430064 China

Concrete structures in main coal cleaning plants have been rebuilt and reinforced in the coal mines of the Shanghai Datun Energy Sources Co. Ltd., the first colliery of the Pingdingshan Coal Co. Ltd. and the Sanhejian mine of the Xuzhou Mining Group Co. Ltd. In these projects, the operating environment and reliability of concrete structures in the main plants of the three companies were investigated and the safety of the structures inspected. Qualitative and quantitative analyses were made on the special natural, technological and mechanical environments around the structures. On the basis of these analyses, we discuss the long-term, combined actions of the harsh natural (corrosive gases, liquids and solids) and mechanical environments on concrete structures and further investigated the damage and deteriorating mechanisms and curing techniques of concrete structures in the main coal cleaning plants. Our study can provide a theoretical basis for ensuring the reliability of concrete structures in main coal cleaning plants.

关键词：混凝土结构净化装置固化技术退化机制煤炭三河尖煤矿徐州矿务集团作业环境