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Single-atom Rh catalysts for efficiently degrading Rhodamine B with high concentration

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Rare Metals 2024年第5期43卷 2331-2338页

作者： Shou-Yao Hu Jian-Ping Guan Run-Ze Ma Yu Tao dong-hao liu Jia-Xin Gong Yu Xiong Department of Chemistry and Chemical Engineering Central South UniversityChangsha 410083China

Highly concentrated dye wastewater has a serious effect on the quality of natural waters;thus,developing novel catalysts to degrade dyes rapidly and efficiently is of great *** the first time,this study reports an Rh single atom loaded on a nitrogen-doped carbon(SA-Rh/CN)*** catalyst exhibits an excellent processing capacity for high concentrations of Rhodamine B(Rh B),high catalytic activity(95.7% degradation of Rh B in60 min)and excellent stability(93.5% degradation efficiency after 10 stable runs).

关键词： catalyst. catalysts loaded

Review of 2D Bi_(2)X_(3)(X=S,Se,Te):from preparation to photodetector

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Rare Metals 2024年第6期43卷 2349-2370页

作者： Zhi Zeng dong-Bo Wang Xuan Fang Jia-Mu Cao Bing-Ke Zhang Jing-Wen Pan dong-hao liu Si-Hang liu Shu-Jie Jiao Tian-Yuan Chen Gang liu Lian-Cheng Zhao Jin-Zhong Wang Department of Optoelectronic Information Science School of Materials Science and EngineeringHarbin Institute of TechnologyHarbin 150001China Changchun University Science and Technology School of PhysicsThe State Key Laboratory of High Power Semiconductor LasersChangchun 130022China School of Astronautics Harbin Institute of TechnologyHarbin 150001China Center for High Pressure Science and Technology Advanced Research Shanghai 201203China

Detector has become an indispensable part of human *** increasing demand for photodetectors with high performance has promoted the research of novel *** the same time,with the development of rising material system,two-dimensional(2D)materials attract a lot of attention,while the suitable option for fabricating photodetector is still *** prospering of bismuth chalcogenides injected new vitality for material field,thereinto,the unique topological insulator characteristics make the research on bismuth selenide(Bi_(2)X_(3))and bismuth telluride(Bi_(2)X_(3)) intriguing.2D Bi_(2)X_(3) also exhibits unique features among various 2D materials,of which,the adjustable narrow energy band gap and polarization-sensitive photocurrent contribute to the promising application of high performance and broadband *** this review,from a bottom-up perspective,we summarize fundamental properties,synthesis method,photodetector performance of 2D Bi_(2)X_(3) based on the previous study,which provide an overall perspective of 2D Bi_(2)X_(3).Wherein,the section of the photodetector is specifically discu ssed with regard to pure Bi_(2)X_(3) photodetector and heterojunction photodetector.A brief summary and outlook were also explored in the end.

关键词： Bi_(2)X_(3) Preparation 2D Photodetector

Strong-coupling superconductivity with Tc above 70 K in Be-decorated monolayer T-graphene

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Science China(Physics,Mechanics & Astronomy) 2024年第1期67卷 99-105页

作者： liu Yang Peng-Fei liu hao-dong liu Ya-Ping Li Na Jiao Hong-Yan Lu Bao-Tian Wang Ping Zhang School of Physics and Physical Engineering Qufu Normal UniversityQufu 273165China Institute of High Energy Physics Chinese Academy of SciencesBeijing 100049China Spallation Neutron Source Science Center Dongguan 523803China Institute of Applied Physics and Computational Mathematics Beijing 100088China

Using first-principles calculations,we predict a new type of two-dimensional(2D)beryllium(Be)-decorated T-graphene named BeC_(2),where Be atoms are inserted into C–C bonds linking the carbon tetrarings of *** band structure shows that BeC_(2)is metallic,thus,the possible phonon-mediated superconductivity is explored based on the Eliashberg *** calculated electron-phonon coupling(EPC)constantλis up to 4.07,and the corresponding superconducting critical temperature(Tc)is 72.1 K,approaching the liquid nitrogen *** reason for the high Tc is the strong *** it is proved to be an anisotropic single-gap superconductor by analyzing the superconducting gap?kof BeC_(2).The electronic susceptibility calculation shows strong nesting effect in BeC_(2).Since rare 2D superconductors show such a strong EPC constantλwhich originates from the coupling between electrons in C-pzorbital and in-plane vibrations of Be and C atoms,the predicted BeC_(2)provides a new platform for investigating strong EPC 2D superconductor.

关键词： two-dimensional carbon-based superconductor electron-phonon coupling strong coupling high superconducting critical temperature

Antenna system characteristics and solar radio burst observations

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Research in Astronomy and Astrophysics 2015年第11期15卷 1917-1930页

作者： Sha Li Yi-Hua Yan Zhi-Jun Chen Wei Wang dong-hao liu Key Laboratory of Solar Activity National Astronomical Observatories Chinese Academy of Sciences Key Laboratory of Radio Astronomy Chinese Academy of Sciences University of Chinese Academy of Sciences

The Chinese Spectral Radio Heliograph（CSRH） is an advanced aperture synthesis solar radio heliograph, independently developed by National Astronomical Observatories, Chinese Academy of Sciences. It consists of 100 reflector antennas,which are grouped into two antenna arrays（CSRH-I and CSRH-II） for low and high frequency bands respectively. The frequency band of CSRH-I is 0.4–2 GHz and that for CSRH-II is 2–15 GHz. In the antenna and feed system, CSRH uses eleven feeds to receive signals coming from the Sun. The radiation pattern has a lower side lobe and the back lobe of the feed is well illuminated. The characteristics of gain G and antenna noise temperature T affect the quality of solar radio imaging. For CSRH, the measured G is larger than 60 d Bi and T is less than 120 K. After CSRH-I was established, we successfully captured a solar radio burst between 1.2–1.6 GHz on 2010 November12 using this instrument and this event was confirmed through observations with the Solar Broadband Radio Spectrometer at 2.84 GHz and the Geostationary Operational Environmental Satellite. In addition, an image obtained from CSRH-I clearly revealed the profile of the solar radio burst. The other observational work involved the imaging the Fengyun-2E geosynchronous satellite which is assumed to be a point *** indicate that the data processing method applied in this study for deleting errors in a noisy image could be used for processing images from other sources.

关键词： captured burst noisy antenna reflector aperture instrument coordinates Solar independently

Quantitative evaluation of the contribution of underground space to urban resilience:A case study in China

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Underground Space 2024年第4期17卷 1-24页

作者： Si-Cong liu Fang-Le Peng Yong-Kang Qiao Yun-hao dong Research Center for Underground Space&Department of Geotechnical Engineering Tongji UniversityShanghai 200092China

Urban underground space(UUS)development has been acknowledged as a positive contribution to urban resilience(UR).Such contribution has been qualitatively addressed in recent years,but only quantitatively discussed in few *** evaluation methods for UR are widely used in China and around the world,but the role of underground space is barely *** paper provides a way to bridge this gap on the city scale.A UR evaluation framework was carefully constructed that covers the basic aspects and elements of *** contributions of UUS to UR were identified and integrated into the UR evaluation framework,and the measurement methods for each indicator related to UUS were determined.A case study of 19 sample cities in China were conducted using the integrated evaluation *** analysis and clustering analysis were further adopted to interpret the evaluation results,mainly with three indicators reflecting the level of UUS development,namely UUS area(m^(2)),UUS density(104 m^(2)/km^(2))and UUS area per capita(m^(2)/person).The results showed a strong correlation between UUS area and *** average proportion of UR provided by UUS in the 19 sample cities was 16.46%,while the maximum figure reached 29.20%.The sample cities were clustered into four categories based on the relationship between the proportion of UR provided by UUS,UUS area,and GDP per capita,where both high and low UUS area tend to provide less proportion of resilience than the medium UUS *** suggestions for UUS utilization were proposed to assist cities in achieving urban resilience.

关键词： Urban underground space(UUS) Urban resilience Resilience evaluation Resilient development

Multi-scale Modeling and Finite Element Analyses of Thermal Conductivity of 3D C/SiC Composites Fabricating by Flexible-Oriented Woven Process

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Chinese Journal of Mechanical Engineering 2024年第3期37卷 275-288页

作者： Zheng Sun Zhongde Shan hao Huang dong Wang Wang Wang Jiale liu Chenchen Tan Chaozhong Chen Nanjing University of Aeronautics and Astronautics Nanjing 210016China School of Mechanical Engineering Beijing Institute of TechnologyBeijing 100081China CRRC Institute Corporation Limited Beijing 100070China

Thermal conductivity is one of the most significant criterion of three-dimensional carbon fiber-reinforced SiC matrix composites(3D C/SiC).Represent volume element(RVE)models of microscale,void/matrix and mesoscale proposed in this work are used to simulate the thermal conductivity behaviors of the 3D C/SiC *** entirely new process is introduced to weave the preform with three-dimensional orthogonal *** 3D steady-state analysis step is created for assessing the thermal conductivity behaviors of the composites by applying periodic temperature boundary *** RVE models of cuboid,hexagonal and fiber random distribution are respectively developed to comparatively study the influence of fiber package pattern on the thermal conductivities at the ***,the effect of void morphology on the thermal conductivity of the matrix is analyzed by the void/matrix *** prediction results at the mesoscale correspond closely to the experimental *** effect of the porosities and fiber volume fractions on the thermal conductivities is also taken into *** multi-scale models mentioned in this paper can be used to predict the thermal conductivity behaviors of other composites with complex structures.

关键词： 3D C/SiC composites Finite element analyses Multi-scale modeling Thermal conductivity

Implementation of a particle-in-cell method for the energy solver in 3D spherical geodynamic modeling

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Earth and Planetary Physics 2024年第3期8卷 549-563页

作者： hao dong ZeBin Cao LiJun liu YanChong Li SanZhong Li LiMing Dai XinYu Li Frontiers Science Center for Deep Ocean Multispheres and Earth System Key Laboratory of Submarine Geosciences and Prospecting TechniquesMinistry of Education and College of Marine GeosciencesOcean University of ChinaQingdao 266100China State Key Laboratory of Lithospheric Evolution Institute of Geology and GeophysicsChinese Academy of SciencesBeijing 100029China Laboratory for Marine Geology Laoshan LaboratoryQingdao 266237China Department of Earth Science&Environmental Change University of Illinois at Urbana-ChampaignUrbanaIL 61801USA Laboratory of Seismology and Physics of Earth’s Interior School of Earth and Space SciencesUniversity of Science and Technology of ChinaHefei 230026China

The thermal evolution of the Earth’s interior and its dynamic effects are the focus of Earth ***,the commonly adopted grid-based temperature solver is usually prone to numerical oscillations,especially in the presence of sharp thermal gradients,such as when modeling subducting slabs and rising *** phenomenon prohibits the correct representation of thermal evolution and may cause incorrect implications of geodynamic *** examining several approaches for removing these numerical oscillations,we show that the Lagrangian method provides an ideal way to solve this *** this study,we propose a particle-in-cell method as a strategy for improving the solution to the energy equation and demonstrate its effectiveness in both one-dimensional and three-dimensional thermal problems,as well as in a global spherical simulation with data *** have implemented this method in the open-source finite-element code CitcomS,which features a spherical coordinate system,distributed memory parallel computing,and data assimilation algorithms.

关键词： numerical oscillation overshooting and undershooting particle-in-cell method three-dimensional spherical geodynamic modeling energy solver finite element method

Recent advances in vacancy engineering for reliable lithiumsulfur batteries

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Rare Metals 2024年第2期43卷 455-477页

作者： Wen-dong liu Xiao Tang Jun-An Feng Chao-Yue Zhang hao liu Chuan Shi Xiao-Xian Zhao Jian-Jun Song College of Physics School of Chemistry and Chemical EngineeringQingdao UniversityQingdao266071China Faculty of Science Centre for Clean Energy TechnologySchool of Mathematical and Physical SciencesUniversity of Technology SydneySydneyNSW2007Australia Department of Chemistry College of ScienceHebei Agricultural UniversityBaoding071001China

The high-energy-density and low-cost features endow lithium-sulfur batteries with broad application ***,many drawbacks,especially the detrimental shuttle effect,have hindered the further development of *** response,a lot of new structures have been applied to suppress the shuttle effect and promote the development of ***,vacancy engineering has gained the attention of researchers due to its unique electronic *** review aims to analyze the application of vacancy engineering in ***,the electrochemistry of LSBs has been systematically discussed and the existing challenges as well as improvement tactics of LSBs have also been ***,the preparation methods and characterization technologies of various vacancies are summarized,including oxygen vacancies,sulfur vacancies,selenium vacancies,other anion vacancies,cation vacancies,*** latest applications of vacancy engineering in LSBs are also summarized in this ***,some prospects and insights for further investigation and practical application of vacancy engineering in LSBs are put forward.

关键词： Lithium-sulfur batteries(LSBs) Defects Vacancy engineering Electronic structure Shuttle effect

Texture and Se vacancy optimization induces high thermoelectric performance in Bi_(2)Se_(3) flexible thin films

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Rare Metals 2024年第6期43卷 2796-2804页

作者： dong-Wei Ao Wei-Di liu Yue-Xing Chen Fan Ma Yi-Jie Gu Zhuang-hao Zheng School of Machinery and Automation Weifang UniversityWeifang 261061China Australian Institute for Bioengineering and Nanotechnology The University of QueenslandBrisbane 4072Australia Shenzhen Key Laboratory of Advanced Thin Films and Applications Key Laboratory of Optoelectronic Devices and Systems of Ministry of Education and Guangdong ProvinceCollege of Physics and Optoelectronic EngineeringShenzhen UniversityShenzhen518060China School of Materials Science and Engineering Inner Mongolia University of TechnologyHohhot 010051China

Bi_(2)Se_(3)-based flexible thin film with high thermoelectric performance is promising for the waste heat recovery *** this work,a novel post-selenization method is employed to prepare n-type Bi_(2)Se_(3)flexible thin films with highly textured *** strengthened texture and Se vacancy optimization can be simultaneously achieved by optimizing the selenization *** highly oriented texture leads to the increased carrier mobility and results in a high electric conductivity of~290.47 S·cm^(-1)at 623 ***,a high Seebeck coefficient(>110μW·K-1)is obtained due to the reduced carrier concentration,induced by optimizing vacancy ***,a high power factor of 3.49μW·cm^(-1)·K^(-2)at 623 K has been achieved in asprepared highly-bendable Bi_(2)Se_(3)flexible thin films selenized at 783 *** study introduces an effective post-selenization method to tune the texture structure and vacancies of Bi_(2)Se_(3)flexible thin films,and correspondingly achieves high thermoelectric performance.

关键词： Thermoelectric Bi_(2)Se_(3) Flexible thin film Post-selenization