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Functionalized Graphene Oxide with Bismuth and Titanium Oxide Nanoparticles for Efficiently Removing Formaldehyde from the Air by Photocatalytic Degradation-Adsorption Process

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Journal of Analysis and Testing 2023年第4期7卷 444-458页

作者： Mohsen Mohammadi Asl hamid shirkhanloo Nabiollah Mansouri Seyed Ali Reza Haji Seyed Mirzahosseini Farideh Atabi Department of Environmental Engineering Faculty of Natural Resource and EnvironmentScience and Research BranchIslamic Azad UniversityTehran 14778-93855Iran Research Institute of Petroleum Industry(RIPI) West BoulevardOlympic VillageTehran 14857-33111Iran

Formaldehyde(HCHO)is formed through the oxidation of volatile organic compounds(VOCs)and can cause human *** oxide and titanium oxide nanoparticles-functionalized nanographene oxide(Bi_(2)O_(3)/TiO_(2)@NGO)were used to rapidly remove the HCHO from the air by a photocatalytic degradation-adsorption process(PC-DAP).The formaldehyde vapor in pure air was generated in a dynamic system within a chamber,and flowed over Bi_(2)O_(3)/TiO_(2)@NGO adsorbent inside a fixed-bed quartz reactor(FBQR)under UV irradiation at optimized conditions(250C).At atmospheric pressure,the flow rate and gas hourly space velocity(GHSV)were adjusted to 300 mL/min and 100-450 L/h,*** radicals of HCHO and nanographene oxide(NGO)were generated through the UV-photochemical process,enhancing the chemical adsorption through the radicals’*** the other hand,the semi-degradation process by catalytic oxidation process converted some HCHO into raw materials of CO_(2)and H_(2)O,while the unconverted HCHO was physically absorbed by ***,the HCHO concentration in the outlet system was measured by gas chromatography with a flame ionization detector(GC-FID)after derivatizing formaldehyde with 2,4-dinitrophenylhydrazine(DNPH)and ***,efficient removal of HCHO from the air,the removal efficiency of more than 95%,was achieved through physical/chemical adsorption and the *** mean removal efficiencies for HCHO with Bi_(2)O_(3)-TiO_(2)@NGO,TiO_(2)@NGO,Bi_(2)O_(3)@NGO,and NGO were 98.7%,73.6%,61.8%,and 11.4%,respectively(n=10,RSD<5%).The methodology was validated by spiking different concentrations of standard HCHO into pure air.

关键词： Formaldehyde removal Air Functionalized graphene oxide UV radiation Photocatalytic degradation-adsorption process

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