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Nanodiamond/Ti_(3)C_(2) MXene-coated quartz crystal microbalance humidity sensor with high sensitivity and high quality factor

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Rare Metals 2024年第6期43卷 2719-2729页

作者： yao yao Qiao chen Yan-Qi Li Xian-He Huang Wei-Wei Ling Zhe-MiaoXie Jia-QiWang Chang-Ming chen College of Communication Engineering Chengdu University of Information TechnologyChengdu 610225China School of Automation Chongqing University of Posts and TelecommunicationsChongqing 400065China School of Automation Engineering University of Electronic Science and Technology of ChinaChengdu 611731China Advanced Micro-/Nano-Devices Lab Department of Systems Design EngineeringUniversity of WaterlooWaterlooON N2L 3GlCanada

To address the challenge of achieving both high sensitivity and a high quality factor in quartz crystal microbalance(QCM)humidity sensors,a nanodiamond(ND)/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor was *** material characteristics of ND,Ti_(3)C_(2)MXene,and ND/Ti_(3)C_(2)MXene composite were analyzed by transmission electron microscopy(TEM)and Fourier transform infrared(FTIR)*** experimental results demonstrated that the hydrophilic ND nanoparticles coated on Ti_(3)C_(2) MXene nanosheet prevented the self-stacking of Ti_(3)C_(2)MXene and enhanced the sensitivity of Ti_(3)C_(2) MXene-based QCM humidity ***,the high mechanical modulus of Ti_(3)C_(2) MXene material helped ND/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor to achieve a high quality factor(>20,000).ND/Ti_(3)C_(2)MXene compositecoated QCM humidity sensor exhibited a sensitivity of 82.45 Hz/%RH,a humidity hysteresis of 1.1%RH,fast response/recovery times,acceptable repeatability,and good stability from 11.3%RH to 97.3%*** response mechanism of ND/Ti_(3)C_(2) MXene composite-coated QCM humidity sensor was analyzed in combination with a bi-exponential kinetic adsorption ***,the potential application of ND/Ti_(3)C_(2)MXene composite-coated QCM humidity sensor was demonstrated through its frequency response to wooden blocks with different moisture contents.

关键词： Humidity sensor Quartz crystal microbalance Nanodiamond Ti_(3)C_(2)MXene High quality factor

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Design of novel RGO/2D strip-like ZIF-8/DMAOP ternary hybrid structure towards high-efficiency microwave absorption, active and passive anti-corrosion, and synergistic antibacterial performance

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Nano Research 2024年第3期17卷 913-926页

作者： Tanlin chen Yingrui Tian Zihao Guo yao chen Qing Qi Fanbin Meng Key Laboratory of Advanced Technologies of Materials(Ministry of Education) School of Materials Science and EngineeringSouthwest Jiaotong UniversityChengdu 610031China Shenzhen Institute of Southwest Jiaotong University Shenzhen 518000China

In order to meet the requirements of the marine environment for microwave absorption(MA)materials,we put forward the strategy of constructing multi-functional composite materials,which integrate microwave absorption,anti-corrosion,and antibacterial ***,graphene oxide(GO)was used as a template to induce the growth of zeolitic imidazolate framework-8(ZIF-8),simultaneously as a two-dimensional(2D)nanocontainers to load corrosion inhibitors to achieve pH-responsive and self-healing ***,quaternary ammonium salt(dimethyl octadecyl(3-trimethoxylsilyl propyl)ammonium chloride(DMAOP))and sodium ascorbate(VCNa)were introduced to achieve synergistic antibacterial activity and the reduction of *** 2D strip-like structure of ZIF-8 was due to the confined growth induced by the electrostatic attraction between ZIF-8 and GO *** as-obtained reduced GO(RGO)/ZIF-8/DMAOP5 exhibited excellent microwave absorption(MA)properties,with a minimum reflection loss(RL)value of-47.08 dB at 12.73 GHz when the thickness was 2.8 ***,the effective absorption bandwidth reached 6.84 *** soaking in 3.5%NaCl solution for 35 days,the RGO/ZIF-8/DMAOP5-0.7%coating still achieved an impedance value of 4.585×107Ω·cm^(2) and a protective efficiency of 99.994%,providing superior anti-corrosion *** addition,fantastic antibacterial activity was obtained,with the antibacterial rates of RGO/ZIF-8/DMAOP_(10) reaching 99.39%and 100%against Escherichia coli and Staphylococcus *** work could open new avenues towards the development of a new generation of multifunctional MA materials.

关键词： two-dimensional(2D)strip-like zeolitic imidazolate framework-8(ZIF-8) microwave absorption active and passive anti-corrosion antibacterial

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A new 4-Ti-added polyoxometalate

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Tungsten 2024年第2期6卷 465-471页

作者： hai-Lou Li chen Lian Guo-Yu Yang MOE Key Laboratory of Cluster Science School of Chemistry and Chemical EngineeringBeijing Institute of TechnologyBeijing 102488China

A new inorganic–organic hybrid 4-Ti-added polyoxometalate:[H_(2)N(CH_(3))_(2)]_(2)Na_(3)H_(5)[{Ti(C_(2)O_(4))(H_(2)O)}_(2){Ti(C_(2)O_(4))}_(2)(B-β-SbW_(9)O_(33))_(2)]·22H_(2)O(1)has been successfully made and further characterized by infrared spectroscopy,thermogravimetric analysis,powder X-ray diff raction and single-crystal X-ray diff *** polyoxoanion of 1 exhibits a Krebs-type structure that is constructed from two[B-β-SbW_(9)O_(33)]^(9)−fragments fused together by a belt of four additional Ti atoms decorated by oxalate ***,1 as a heterogeneous catalyst exhibits high activity for Knoevenagel condensation under mild reaction conditions.

关键词： Polyoxometalate Ti-added POM Krebs-type structure Knoevenagel condensation

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Effect of low-speed waterjet pressure on the rock-breaking performance of unsubmerged cavitating abrasive waterjet

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Petroleum Science 2024年第4期21卷 2638-2649页

作者： chen-Xing Fan Deng Li Yong Kang hai-Tao Zhang Hubei Key Laboratory of Waterjet Theory and New Technology Wuhan University School of Power and Mechanical Engineering Wuhan University

Unsubmerged cavitating abrasive waterjet(UCAWJ) has been shown to artificially create a submerged environment that produces shear cavitation, which effectively enhances rock-breaking performance. The shear cavitation generation and collapse intensity depend on the pressure difference between the intermediate high-speed abrasive waterjet and the coaxial low-speed waterjet. However, the effect of the pressure of the coaxial low-speed waterjet is pending. For this purpose, the effect of low-speed waterjet pressure on rock-breaking performance at different standoff distances was experimentally investigated,and the effects of erosion time and ruby nozzle diameter on erosion performance were discussed. Finally,the micromorphology of the sandstone was observed at different locations. The results show that increased erosion time and ruby nozzle diameter can significantly improve the rock-breaking performance. At different standoff distances, the mass loss increases first and then decreases with the increase of low-speed waterjet pressure, the maximum mass loss is 10.4 g at a low-speed waterjet pressure of0.09 MPa. The surface morphology of cavitation erosion was measured using a 3D profiler, the increase in both erosion depth and surface roughness indicated a significant increase in the intensity of the shear cavitation collapse. At a low-speed waterjet pressure of 0.18 MPa, the cavitation erosion surface depth can reach 600 μm with a roughness of 127 μm.

关键词： Rock-breaking Coaxial low-speed waterjet pressure Abrasive waterjet Cavitation Unsubmerged environment

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Characterizing extreme drought and wetness in Guangdong,China using global navigation satellite system and precipitation data

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Satellite Navigation 2024年第1期5卷 258-274页

作者： hai Zhu Kejie chen haishan Chai Yuanbin Ye Wenjian Liu Department of Earth and Space Sciences Southern University of Science and TechnologyShenzhen518055China Lands and Resource Department of Guangdong Province Surveying and Mapping InstituteGuangzhou510500China

As global temperature rises,the frequency of extreme climate events,e.g.,severe droughts and floods,has increased significantly and caused severe damage over the past *** this regard,precipitation efficiency,a crucial meteorological parameter,could provide valuable insights for a better understanding of the patterns and characteristics of these extreme *** this study,taking Guangdong province as an exemplary region,we first obtained long-term and high-resolution historical records of precipitation efficiency by integrating the observations from a dense network of Global Navigation Satellite System(GNSS)stations with precipitation data,and then characterized the extreme drought and wetness through climate *** found a distinct seasonal trend in precipitation efficiency in Guangdong,with annual fluctuations ranging from 10 to 25%.Notably,precipitation efficiency is higher in proximity to the Pearl River Delta Plain and gradually decreases towards the east and *** occurrence of anomalous peaks and valleys in precipitation efficiency generally corresponds to dry and wet conditions,respectively.A total of 9 extreme wet events and 6 dry events occurred from January 2007 to May 2022,with durations from 3 to 6 *** results also demonstrated that both wet and dry frequencies exhibit an increasing trend with the expansion of the time scale,and the frequency of extreme events near the Pearl River Delta Plain surpasses that of other ***,the propagation time from meteorological anomalies to agricultural and hydrological anomalies is about 3 *** periodic characteristics of meteorological anomalies are identified as the primary driver for other anomalous periodic *** work unveils the long-term dynamic behavior of precipitation efficiency,as well as the characteristics of extreme drought and wetness events in the regions characterized by intricate land–atmosphere interactions.

关键词： GNSS Precipitation efficiency Extreme drought and wetness

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Parallel Computing Based Solution for Reliability-constrained Distribution Network Planning

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Journal of Modern Power Systems and Clean Energy 2024年第4期12卷 1147-1158页

作者： Yaqi Sun Wenchuan Wu Yi Lin hai Huang Hao chen State Key Laboratory of Power Systems Department of Electrical EngineeringTsinghua UniversityBeijing 100084China Sichuan Energy Internet Research Institute Tsinghua UniversityChengduChina State Grid Fujian Electric Power Co.Ltd. FuzhouChina

The main goal of distribution network(DN)expan-sion planning is essentially to achieve minimal investment con-strained by specified reliability *** reliability-constrained distribution network planning(RcDNP)problem can be cast as an instance of mixed-integer linear programming(MILP)which involves ultra-heavy computation burden espe-cially for large-scale *** this paper,we propose a parallel computing based solution method for the RcDNP *** RcDNP is decomposed into a backbone grid and several lateral grid problems with ***,a parallelizable aug-mented Lagrangian algorithm with acceleration method is devel-oped to solve the coordination planning *** lateral grid problems are solved in parallel through coordinating with the backbone grid planning ***-Seidel iteration is adopted on the subset of the convex hull of the feasible region constructed by *** mild conditions,the opti-mality and convergence of the proposed method are *** tests show that the proposed method can significant-ly reduce the solution time and make the RcDNP applicable for real-worldproblems.

关键词： Distribution network expansion planning reliability parallel computing

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An interpretable graph convolutional neural network based fault diagnosis method for building energy systems

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Building Simulation 2024年第7期17卷 1113-1136页

作者： Guannan Li Zhanpeng yao Liang chen Tao Li chengliang Xu School of Urban Construction Wuhan University of Science and TechnologyWuhan 430065China Anhui Province Key Laboratory of Intelligent Building and Building Energy-saving Anhui Jianzhu UniversityHefei 230601China State Key Laboratory of Green Building in Western China Xi'an University of Architecture&TechnologyXi'an 710055China Key Laboratory of Low-grade Energy Utilization Technologies and Systems(Chongqing University) Ministry of Education of ChinaChongqing UniversityChongqing 400044China Hubei Provincial Engineering Research Centre of Urban Regeneration Wuhan University of Science and TechnologyWuhan 430081China

Due to the fast-modeling speed and high accuracy,deep learning has attracted great interest in the field of fault diagnosis in building energy systems in recent ***,the black-box nature makes deep learning models generally difficult to *** order to compensate for the poor interpretability of deep learning models,this study proposed a fault diagnosis method based on interpretable graph neural network(GNN)suitable for building energy *** method is developed by following three main steps:(1)selecting NC-GNN as a fault diagnosis model for building energy systems and proposing a graph generation method applicable to the model,(2)developing an interpretation method based on InputXGradient for the NC-GNN,which is capable of outputting the importance of the node features and automatically locating the fault related features,(3)visualizing the results of model interpretation and validating by matching with expert knowledge and maintenance *** was performed using the public ASHRAE RP-1043 chiller fault *** diagnosis results show that the proposed method has a diagnosis accuracy of over 96%.The interpretation results show that the method is capable of explaining the decision-making process of the model by identifying fault-discriminative *** almost all seven faults,their fault-discriminative features were correctly identified.

关键词： fault diagnosis graph neural network building energy system InputXGradient feature interpretation

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Layer Hall effect induced by hidden Berry curvature in antiferromagnetic insulators

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National Science Review 2024年第2期11卷 15-23页

作者： Rui chen hai-Peng Sun Mingqiang Gu Chun-Bo Hua Qihang Liu hai-Zhou Lu X.C.Xie Shenzhen Institute for Quantum Science and Engineering and Department of Physics Southern University of Science and Technology(SUSTech) International Quantum Academy Institute for Theoretical Physics and Astrophysics University of Würzburg School of Electronic and Information Engineering Hubei University of Science and Technology Guangdong Provincial Key Laboratory of Computational Science and Material Design Southern University of Science and Technology Shenzhen Key Laboratory of Quantum Science and Engineering International Center for Quantum Materials School of PhysicsPeking University Collaborative Innovation Center of Quantum Matter CAS Center for Excellence in Topological Quantum Computation University of Chinese Academy of Sciences

The layer Hall effect describes electrons spontaneously deflected to opposite sides at different layers, which has been experimentally reported in the MnBi2Te4thin films under perpendicular electric fields. Here, we reveal a universal origin of the layer Hall effect in terms of the so-called hidden Berry curvature, as well as material design principles. Hence, it gives rise to zero Berry curvature in momentum space but non-zero layer-locked hidden Berry curvature in real space. We show that, compared to that of a trivial insulator, the layer Hall effect is significantly enhanced in antiferromagnetic topological insulators. Our universal picture provides a paradigm for revealing the hidden physics as a result of the interplay between the global and local symmetries, and can be generalized in various scenarios.

关键词： layerHall effect hidden Berry curvature antiferromagnetic insulator axion insulator, quantum transport

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Nanomedicine Disrupts Stromal Barriers to Augment Drug Penetration for Improved Cancer Therapy

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Chinese Journal of Chemistry 2024年第10期42卷 1175-1189页

作者： Guo-Feng Luo Wei-hai chen Xian-Zheng Zhang state Key Laboratory of Oral&Maxillofacial Reconstruction and Regeneration Key Laboratory of Oral Biomedicine Ministry of EducationHubei KeyLaboratory of StomatologySchool&Hospital of StomatologyWuhan UniversityWuhanHubei 430079China Key Laboratoryof Biomedical Polymers of Ministry of Education&Departmentof Chemistry Wuhan UniversityWuhanHubei 430072China

Tumor stroma composing diverse extracellular matrixes(ECM)and stromal cells shapes a condensed physical barrier,which severely hampers the efficient accessibility of nanomedicine to tumor cells,especially these deep-seated in the core of *** barrier significantly compromises the antitumor effects of drug-loaded nanomedicine,revealing the remarkable importance of disrupting stromal barrier for improved tumor therapy with deep penetration *** achieve this goal,various nanoparticle-based strategies have been developed,including direct depleting ECM components via delivering anti-fibrotic agents or targeting stromal cells to suppress ECM expression,dynamic regulation of nanoparticles’physicochemical properties(i.e.,size,surface charge,and morphology),mechanical force-driven deep penetration,natural/biomimetic self-driven nanomedicine,and transcytosis-inducing *** these nanostrategies were systemically summarized in this review,and the design principles for obtaining admirable nanomedicine were *** the rapid development of nanotechnology,elaborate design of multifunctional nanomedicine provides new opportunities for overcoming the critical stromal barriers to maximize the therapeutic index of various therapies,such as chemotherapy,photodynamic therapy,and immunotherapy.

关键词： Nanomedicine Tumor stroma Deep penetration Enhanced drug perfusion Cancer therapy Drug carriers Biomaterials Nanotechnology

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Non-cooperative Game Based Optimal Dispatch Model for Integrated Energy Systems

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CSEE Journal of Power and Energy Systems 2024年第3期10卷 1195-1207页

作者： Jiandong Duan Qian Sun chen Wu yao Yang Siyu Tu School of Electrical Engineering Xi’an University of TechnologyXi’an710056China IEEE CSEE

In order to improve the efficiency of energy utilization,the integrated energy system(IES)has *** IES typically acts as a whole system during operations,the subsystems are separated,and the interests of each system are *** this paper,considering the relationship between the various energy systems,non-cooperative game theory is used to establish the optimal dispatch *** proposed model mainly relies on the relationship between the cooperation and competition among various subsystems to obtain the maximum benefit they can ***,the basic definition is combined with the particle swarm optimization algorithm to solve the *** results show that the optimization strategy proposed in this paper can operate safely and reliably,and effectively distribute the benefits of each energy system.

关键词： Integrated energy system multi-energy complimentarily non-cooperative game theory

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