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Recent progress in two-dimensional metallenes and their potential application as electrocatalyst

Journal of Energy Chemistry 2024年第7期94卷 577-598页

作者： Umer Shahzad mohsin Saeed muhammad Fazle Rabbee hadi m.marwani Jehan Y.Al-Humaidi muhammad Altaf Raed H.Althomali Kwang-Hyun Baek md.Rabiul Awual mohammed m.Rahman Department of Chemistry Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia Department of Biotechnology Yeungnam UniversityGyeongsanSouth Korea Center of Excellence for Advanced materials Research(CEAmR) King Abdulaziz UniversityJeddah 21589Saudi Arabia Department of Chemistry College of SciencePrincess Nourah Bint Abdulrahman UniversityP.O.BOX 84428Riyadh 11671Saudi Arabia Department of Chemistry Center of Excellence for Innovation in Chemistry(PERCH-CIC)Center of Excellence in Materials Science and TechnologyFaculty of ScienceChiang Mai UniversityChiang Mai 50200Thailand Department of Chemistry College of Art and SciencePrince Sattam Bin Abdulaziz UniversityWadi Al-Dawasir 11991Saudi Arabia Western Australian School of mines:minerals Energy and Chemical EngineeringCurtin UniversityGPO Box U 1987PerthWA 6845Australia

In this article,we looked at metallenes,a novel class of two-dimensional(2D)metals that are attracting interest in the energy and catalysis *** is one area where their exceptional physicochemical and electrical characteristics might be *** are unique because they include several metal atoms that are not in a coordinated *** makes them more active and improves their atomic uti-lization,which in turn increases their catalytic *** article delves into the potential of two-dimensional metals as electrocatalysts for carbon dioxide reduction,fuel oxidation,oxygen evolution,and oxygen reduction reactions in the context of sustainable energy *** to the exception-ally high surface-to-volume ratio,large surface area as well as their optimized atomic use efficiency,2D materials defined by atomic layers are crucial for surface-related sustainable energy *** to its exceptional properties,such as high conductivity and the ability to enhance the exposure of active metal sites,2D metallenes have recently attracted a lot of interest for use in catalysis,electronics,and energy-related *** their highly mobility,adjustable surface states,and electrical struc-tures that can be fine-tuned,2D metallenes are promising nanostructure materials for use in energy con-version with the sustainable applications.

关键词： metallenes Electrocatalysts Electrochemical processes Atomically thin structure

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相位可控的氟钪纳米晶的合成及其上转换发光性能

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无机化学学报 2019年第6期35卷 947-954页

作者：丁玉洁金星刘倩钱桂香 Abdullah m.Asiri hadi m.marwani 安徽工程大学生物与化学工程学院芜湖241000 Chemistry Department Faculty of ScienceKing Abdulaziz UniversityJeddah 21589Saudi Arabia

控制反应条件如表面活性剂的组成、加入量或反应时间,可以制得不同形态、相结构且具有上转换发光(UCL)的氟钪纳米晶(NCs)。改变表面活性剂油酸(OA)/油胺(Om)的比例有利于晶体结构从立方相ScF3∶Yb,Er转变为具有上转换发光性能增强的正交... 详细信息

控制反应条件如表面活性剂的组成、加入量或反应时间,可以制得不同形态、相结构且具有上转换发光(UCL)的氟钪纳米晶(NCs)。改变表面活性剂油酸(OA)/油胺(Om)的比例有利于晶体结构从立方相ScF3∶Yb,Er转变为具有上转换发光性能增强的正交相KSc2F7∶Yb,Er纳米晶,而纳米晶的形态会发生从小到大的转变。改变掺杂元素的种类及含量,在980nm光激发下,KSc2F7纳米晶的上转换发光可以从蓝色变到白色,再到主要发射紫色光。

关键词：上转换氟钪纳米晶相跃迁

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Applying the Protective mn-Co-La_(2)O_(3)Coating on Crofer 22 APU Ferritic Stainless Steel Used as Solid Oxide Fuel Cell Interconnects

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Acta metallurgica Sinica(English Letters) 2024年第5期37卷 872-888页

作者： Farhad mohsenifar hadi Ebrahimifar Ahmad Irannejad Department of materials Engineering and metallurgy Faculty of EngineeringShahid Bahonar University of KermanKermanIran mechanical Engineering Department Faculty of EngineeringHigher Education Complex of Bam76615-314BamIran Department of materials Engineering Faculty of Mechanical and Materials EngineeringGraduate University of Advanced TechnologyKerman ***Iran

This research studies the effect of mn-Co-La_(2)O_(3) coating synthesized by the electrodeposition method on the oxidation resistance and electrical conductivity of the Crofer 22 APU stainless steel interconnect plates in solid oxide fuel *** test samples were characterized by a field emission scanning electron microscope(FESEm)equipped with energy dispersive spectroscopy(EDS),X-ray diffraction(XRD),and X-ray photoelectron spectroscopy(XPS).The oxidation kinetics of the coated and uncoated samples were studied by tracking their weight changes over time at 800°C,showing that the oxidation mechanism for all samples follows the parabolic *** oxidation rate constant(k_(p))values of the coated sample compared with that of the uncoated one indicated a reduction in the oxidation rate of the steel substrate in the presence of the mn-Co-La_(2)O_(3) *** examination of the cross-section of different samples after the isothermal oxidation for 500 h at 800°C exhibited that applying the composite coating leads to a decrease in the thickness of the chromia layer formed on the steel ***,under these conditions,the area-specific resistance(ASR)of the coated sample(13.11 mΩcm^(2))is significantly lower than that of the uncoated one(41.45 mΩcm^(2)).

关键词： Area specific resistance Oxidation Fuel cell Composite coating

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A novel approach to study generalized coupled cubic Schrödinger-Korteweg-de Vries equations

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Journal of Ocean Engineering and Science 2024年第1期9卷 13-24页

作者： Lanre Akinyemi P.Veeresha m.T.Darvishi hadi Rezazadeh mehmet Senol Udoh Akpan Department of mathematics Lafayette CollegeEastonPAUSA Department of mathematics Christ Deemed to be UniversityBengaluru 560029India Department of mathematics Razi UniversityKermanshah 67149Iran Faculty of Engineering Technology Amol University of Special Modern TechnologiesAmolIran Department of mathematics Nev¸s ehir HacıBekta¸s Veli UniversityNev¸s ehirTurkey Drexel University Department of MathematicsPhiladelphiaPAUSA

The Kortewegde Vries(KdV)equation represents the propagation of long waves in dispersive media,whereas the cubic nonlinear Schrödinger(CNLS)equation depicts the dynamics of narrow-bandwidth wave packets consisting of short dispersive waves.A model that couples these two equations seems in-triguing for simulating the interaction of long and short waves,which is important in many domains of applied sciences and engineering,and such a system has been investigated in recent *** work uses a modified Sardar sub-equation procedure to secure the soliton-type solutions of the generalized cubic nonlinear Schrödinger-Korteweg-de Vries system of *** various selections of arbitrary parameters in these solutions,the dynamic properties of some acquired solutions are represented graph-ically and *** particular,the dynamics of the bright solitons,dark solitons,mixed bright-dark solitons,W-shaped solitons,m-shaped solitons,periodic waves,and other soliton-type *** re-sults demonstrated that the proposed technique is highly efficient and effective for the aforementioned problems,as well as other nonlinear problems that may arise in the fields of mathematical physics and engineering.

关键词： CNLS equation modiﬁed Sardar sub-equation method KdV equation Solitons Long and short waves

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Dysfunction of the adhesion G protein-coupled receptor latrophilin 1(ADGRL1/LPHN1)increases the risk of obesity

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Signal Transduction and Targeted Therapy 2024年第5期9卷 2298-2311页

作者： Heba ZabriTorsten Schöneberg AndréNguyen Dietzsch hadi Al-Hasani Joachim Altschmied Katharina Bottermann Jana Brendler Judith Haendeler Susanne Horn Isabell Kaczmarek Antje Körner Kerstin Krause Kathrin Landgraf Diana Le Duc Laura Lehmann Stefan Lehr Stephanie Pick Albert Ricken Rene Schnorr Angela Schulz martina Strnadová Akhil Velluva Heba Zabri Torsten Schöneberg Doreen Thor Simone Prömel Rudolf Schönheimer Institute of Biochemistry Medical FacultyLeipzig UniversityLeipzigGermany Institute for Clinical Biochemistry and Pathobiochemistry Medical FacultyGerman Diabetes CenterLeibniz Center for Diabetes Research at Heinrich Heine University DüsseldorfDüsseldorfGermany German Center for Diabetes Research(DZD e.V.) Munich-NeuherbergGermany Cardiovascular Degeneration Clinical Chemistry and Laboratory DiagnosticsMedical FacultyUniversity Hospital and Heinrich Heine University DüsseldorfDüsseldorfGermany Cardiovascular Research Institute(CARID) Medical FacultyUniversity Hospital and Heinrich Heine University DüsseldorfDüsseldorfGermany Institute of Pharmacology Medical FacultyUniversity Hospital and Heinrich Heine University DüsseldorfDüsseldorfGermany Institute of Anatomy Medical FacultyLeipzig UniversityLeipzigGermany Center for Pediatric Research Hospital for Children and AdolescentsMedical FacultyLeipzig UniversityLeipzigGermany Helmholtz Institute for metabolic Obesity and Vascular Research(HI-MAG)of the Helmholtz Zentrum München at the University of Leipzig and University Hospital LeipzigLeipzigGermany Department of Endocrinology NephrologyRheumatologyLeipzig University Medical CenterLeipzigGermany Institute of Human Genetics Leipzig University Medical CenterLeipzigGermany Institute of Cell Biology Department of BiologyHeinrich Heine University DüsseldorfDüsseldorfGermany School of medicine University of Global Health EquityKigaliRwanda

Obesity is one of the diseases with severe health consequences and rapidly increasing worldwide *** the complex network of food intake and energy balance regulation is an essential prerequisite for pharmacological intervention with obesity.G protein-coupled receptors(GPCRs)are among the main modulators of metabolism and energy ***,for instance,regulate appetite and satiety in certain hypothalamic neurons,as well as glucose and lipid metabolism and hormone secretion from *** in some GPCRs,such as the melanocortin receptor type 4(mC4R),have been associated with early-onset ***,we identified the adhesion GPCR latrophilin 1(ADGRL1/LPHN1)as a member of the regulating network governing food intake and the maintenance of energy *** of the highly conserved receptor in mice results in increased food consumption and severe obesity,accompanied by dysregulation of glucose ***,we identified a partially inactivating mutation in human ADGRL1/LPHN1 in a patient suffering from ***,we propose that LPHN1 dysfunction is a risk factor for obesity development.

关键词： obesity metabolism intake

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Tensile and tear-type fracture toughness of gypsum material:Direct and indirect testing methods

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Journal of Rock mechanics and Geotechnical Engineering 2023年第7期15卷 1777-1796页

作者： Daniel Pietras m.R.m.Aliha hadi G.Kucheki Tomasz Sadowski Lublin University of Technology Civil Engineering and architecture departmentNadbystrzycka 40 str20-618LublinPoland Welding and Joining Research Center School of Industrial EngineeringIran University of Science and Technology(IUST)Narmak16846-13114TehranIran

In this context,four specimens,i.e.(i)circumferentially notched cylindrical torsion(CNCT),(ii)circum-ferentially notched cylindrical direct tension(CNCDT),(iii)edge notch disc bend(ENDB)and(iv)three-point bend beam(3PBB),were utilized to measure the modesⅠandⅢfracture toughness values of *** the CNCT specimen provides pure modeⅢloading in a direct manner,this pure mode condition is indirectly produced by the ENDB *** ENDB specimen provided lower KⅢc and a non-coplanar(***)fracture surface compared with the CNCT specimen,which showed a planar modeⅢfracture *** ENDB specimen is also employed for conducting pure modeⅠ(with different crack depths)and mixed modeⅠ/Ⅲ*** value was independent of the notch depth,and it was consistent with the RILEm and ASTm standard *** the modeⅢfracture results were highly sensitive to the notch *** the fracture resistance against modeⅢwas significantly lower than that of modeⅠ,the greater work of fracture under modeⅢwas noticeable.

关键词： Gypsum Pure modesⅠandⅢfracture toughness mixed modeⅠ/Ⅲ Circumferentially notched cylindrical torsion(CNCT)specimen Circumferentially notched cylindrical direct tension(CNCDT)specimen Edge notch disc bend(ENDB)specimen Experimental measurement Geometry and loading type effects

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Silica Gel Supported Hydrophobic Ionic Liquid for Selective Extraction and Determination of Coumarin

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American Journal of Analytical Chemistry 2013年第1期4卷 8-16页

作者： hadi m. marwani Esraa m. Bakhsh Center of Excellence for Advanced materials Research King Abdulaziz University Jeddah Saudi Arabia Department of Chemistry Faculty of Science King Abdulaziz University Jeddah Saudi Arabia

In this study, a modified silica gel surface with a hydrophobic ionic liquid (SG-1,10-PhenanNTf2) was used as an adsorbent for a selective extraction of coumarin prior to its determination by use of high performance liquid chromatography. Results demonstrated that SG-1,10-PhenanNTf2 phase had a good adsorption capacity up to 85.29 mg?g?1, high selectivity, good site accessibility and fast binding kinetics toward coumarin. The adsorption capacity for coumarin was improved by 62.33% with the SG-1,10-PhenanNTf2 phase as compared to activated silica gel. Adsorption isotherm data displayed that the adsorption process was mainly monolayer on a homogeneous adsorbent surface, confirming the validity of Langmuir adsorption isotherm model. The adsorption of coumarin on the SG-1,10-PhenanNTf2 phase was accomplished after only 60 min contact time. Results of kinetic models showed that the adsorption of coumarin on the SG-1,10-PhenanNTf2 phase obeyed a pseudo second-order kinetic model. Finally, the efficiency of this methodology was confirmed by applying it to real water samples.

关键词： Coumarin Silica Gel Uptake Capacity Ionic Liquid Batch method

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New ordered mAX phase mo_2 TiAlC_2: Elastic and electronic properties from first-principles

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Chinese Physics B 2016年第10期25卷 323-329页

作者： m A hadi m S Ali Department of Physics University of Rajshahi Department of Physics Pabna University of Science and Technology

First-principles computation on the basis of density functional theory(DFT) is executed with the CASTEP code to explore the structural, elastic, and electronic properties along with Debye temperature and theoretical Vickers’ hardness of newly discovered ordered mAX phase carbide mo2TiAlC2. The computed structural parameters are very reasonable compared with the experimental results. The mechanical stability is verified by using the computed elastic constants. The brittleness of the compound is indicated by both the Poisson’s and Pugh’s ratios. The new mAX phase is capable of resisting the pressure and tension and also has the clear directional bonding between atoms. The compound shows significant elastic anisotropy. The Debye temperature estimated from elastic moduli(B, G) is found to be 413.6 K. The electronic structure indicates that the bonding nature of mo2TiAlC2is a mixture of covalent and metallic with few ionic characters. The electron charge density map shows a strong directional mo–C–mo covalent bonding associated with a relatively weak Ti–C *** calculated Fermi surface is due to the low-dispersive mo 4d-like bands, which makes the compound a conductive *** hardness of the compound is also evaluated and a high value of 9.01 GPa is an indication of its strong covalent bonding.

关键词： new ordered mAX phase density functional theory calculations Debye temperature Vickers hardness

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Influence of Recycling Waste Glass as Fine Aggregate on the Concrete Properties

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Journal of Renewable materials 2023年第6期11卷 2925-2940页

作者： Rafal A.hadi Suhad m.Abd Hadee mohammed Najm Shaker Qaidi moutaz mustafa A.Eldirderi Khaled mohamed Khedher Department of Civil Engineering Bilad Alrafidain University CollegeDiyala32001Iraq Department of Civil Engineering College of EngineeringUniversity of DiyalaDiyala32001Iraq Department of Civil Engineering Zakir Husain Engineering CollegeAligarh Muslim UniversityAligarh202002India Department of Civil Engineering College of EngineeringUniversity of DuhokDuhok42001Iraq Department of Civil Engineering College of EngineeringNawroz UniversityDuhok42001Iraq Department of Chemical Engineering College of EngineeringKing Khalid UniversityAbha61421Saudi Arabia Department of Civil Engineering College of EngineeringKing Khalid UniversityAbha61421Saudi Arabia Department of Civil Engineering High Institute of Technological StudiesMrezgua University CampusNabeul8000Tunisia

Recent years have witnessed an increase in the quantity of waste glass(WG)across the *** the fine aggregate with WG is one of the steps toward preserving the natural resources of the environment and creating low-cost *** present study is concerned with replacing fine aggregates with glass powder(GP)at(0%,15%,30%,and 50%).It has studied the fresh and hardened properties(compressive strength,tensile strength,hardened density,and slump)for all the mentioned percent *** findings have shown that all mixtures containing GP gave acceptable slump results within the design limits(2–5 cm)according to ACI standard *** has been observed that increasing the proportion of GP led to a decrease in the weight of ***,replacing GP with sand by 30%has led to an increase in the compressive strength by about 2.4%and 12.45%,and the tensile strength by about 2.5%and 26.54%at 7-and 28-d,respectively in comparison to normal concrete.

关键词： Sustainable concrete glass powder fine aggregate partial replacement

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Structural and biological engineering of 3D hydrogels for wound healing

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生物活性材料(英文) 2023年第6期24卷 197-235页

作者： mohammad hadi Norahan Sara Cristina Pedroza-González mónica Gabriela Sánchez-Salazar mario moisés Álvarez Grissel Trujillo de Santiago Escuela de Ingeniería y Ciencias Tecnológico de MonterreyMonterreyNL64849Mexico Centro de Biotecnología-FEmSA Tecnológico de MonterreyMonterreyNuevo LeónCP64849Mexico Departamento de Bioingeniería Tecnológico de MonterreyMonterreyNuevo LeónCP64849Mexico

Chronic wounds have become one of the most important issues for healthcare systems and are a leading cause of death *** dressings are necessary to facilitate wound *** wound dressings may substantially reduce healing time,reduce the risk of recurrent infections,and reduce the disability and costs *** the path of engineering of an ideal wound dressing,hydrogels have played a leading *** are 3D hydrophilic polymeric structures that can provide a protective barrier,mimic the native extracellular matrix(ECm),and provide a humid *** to their advantages,hydrogels(with different architectural,physical,mechanical,and biological properties)have been extensively explored as wound dressing *** we describe recent studies on hydrogels for wound healing applications with a strong focus on the interplay between the fabrication method used and the architectural,mechanical,and biological performance ***,we review different categories of additives which can enhance wound regeneration using 3D hydrogel *** engineering for wound healing applications promises the generation of smart solutions to solve this pressing problem,enabling key functionalities such as bacterial growth inhibition,enhanced re-epithelialization,vascularization,improved recovery of the tissue functionality,and overall,accelerated and effective wound healing.

关键词： Wound healing Wound dressing Hydrogel Tissue engineering 3D culture

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