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Journal of Thermal Science 2024年第1期33卷 207-221页

作者： ZHOU Hao hu liubin Institute for Thermal Power Engineering State Key Laboratory of Clean Energy UtilizationZhejiang UniversityHangzhou 310027China

This paper experimentally studied the effect of CO_(2) opposing multiple jets on the thermoacoustic instability and NO_(x) emissions in a lean-premixed model *** feasibility was verified from three variables:the CO_(2) jet flow rate,hole numbers,and hole diameters of the *** indicate that the control effect of thermoacoustic instability and NO_x emissions show a reverse trend with the increase of open area ratio on the whole,and the optimal jet flow rate range is 1-4 L/min with CO_(2) opposing multiple *** this flow rate range,the amplitude and frequency of the dynamic pressure and heat release signals CH~* basically decrease as the CO_(2) flow rate increases,which avoids high-frequency and high-amplitude thermoacoustic *** amplitude-damped ratio of dynamic pressure and CH*can reach as high as 98.75% and 93.64% with an optimal open area ratio of 3.72%.NO_(x) emissions also decrease as the jet flow rate increases,and the maximum suppression ratio can reach 68.14%.Besides,the flame shape changes from a steep inverted "V" to a more flat "M",and the flame length will become shorter with CO_(2) opposing multiple *** research achieved the synchronous control of thermoacoustic instability and NO_(x) emissions,which could be a design reference for constructing a safer and cleaner combustor.

关键词： thermoacoustic instability lean-premixed model combustor CO_(2)opposing multiple jets open area ratio NO_(x)emissions

Mitigation of Combustion Instability and NO_(x)Emissions by Microjets in Lean Premixed Flames with Different Swirl Numbers

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Journal of Thermal Science 2023年第4期32卷 1697-1709页

作者： ZHOU Hao hu liubin Zhejiang University Institute for Thermal Power EngineeringState Key Laboratory of Clean Energy UtilizationHangzhou310027China

Swirl combustion serves as a helpful flame stabilization method,which also affects the combustion and emission *** article experimentally investigated the effects of CO_(2)microjets on combustion instability and NO_(x)emissions in lean premixed flames with different swirl *** microjets’control feasibility was examined from three variables of CO_(2)jet flow rate,thermal power,and swirl *** indicate that microjets can mitigate the combustion instability and NO_(x)emissions in lean premixed burners with different swirl numbers and thermal ***,the damping effect of microjets in low swirl intensity is better than that in high swirl *** damping ratio of pressure amplitude can reach the maximum of 98%,and NO_(x)emissions can realize the maximum reduction of 10.1×10^(−6)at the swirl angle of 30°.Besides,the flame macrostructure switches from an inverted cone shape to a petal shape,and the flame length reduction at low swirl intensity is higher than that of high swirl *** research clarified the control differences of mitigation of combustion instability and NO_(x)emissions by microjets in lean premixed flames with different swirl numbers,contributing to the optimization of microjets control and the construction of high-performance burners.

关键词： combustion instability swirl numbers thermal power CO_(2)microjets NO_(x)emissions lean premixed flame

Characterization of blueberry exosome-like nanoparticles and miRNAs with potential cross-kingdom human gene targets

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Food Science and human Wellness 2024年第2期13卷 869-878页

作者： Yangfan Leng liubin Yang Siyi Pan Leilei Zhan Fang Yuan College of Food Science and Technology Huazhong Agricultural UniversityWuhan 430070China hubei Key Laboratory of Fruit&Vegetable Processing&Quality Control Huazhong Agricultural UniversityWuhan 430070China Wuhan GeneCreate Biological Engineering Co. Ltd.Wuhan 430070China

Edible plant derived exosome-like nanoparticles(ELNs)have been shown to have multiple nutraceutical ***,the diversity of plant materials makes the plant derived ELN study *** efforts are still needed to explore the feasible isolation methods of edible plant derived ELNs and the possible roles of food-derived ELNs in improving human *** this study,a size exclusion chromatography based method was compared with the traditional ultracentrifugation method to isolate blueberry derived ELNs(B-ELNs),and the miRNA profile of B-ELNs was analyzed by high-throughput sequencing.A total of 36 miRNAs were found to be enriched in B-ELNs compared with berry tissue,and their potential cross-kingdom human gene targets were further *** showed that size exclusion chromatography was effective for B-ELN *** most abundant miRNAs in B-ELNs mainly belonged to the miR166 family and miR396 *** gene prediction indicated that B-ELNs could potentially regulate pathways related to the human digestive system,immune system and infectious diseases.

关键词： Edible plant derived exosomes-like nanoparticles Size exclusion chromatography miRNA Target gene prediction Blueberry

Constructing a fluorinated interface layer enriched with Ge nanoparticles and Li-Ge alloy for stable lithium metal anodes

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Nano Research 2024年第6期17卷 5148-5158页

作者： Fulu Chu Jinwei Zhou Jiamin Liu Fengcheng Tang liubin Song Feixiang Wu School of Metallurgy and Environment Engineering Research Center of the Ministry of Education for Advanced Battery MaterialsHunan Provincial Key Laboratory of Nonferrous Value-added MetallurgyCentral South UniversityChangsha 410083China hunan Provincial Key Laboratory of Materials Protection for Electric Power and Transportation School of Chemistry and Chemical EngineeringChangsha University of Science and TechnologyChangsha 410004China School of Materials Science&Engineering University of JinanJinan 250022China

Lithium metal batteries(LMBs)based on metallic Li exhibit high energy density to be competent for advanced energy storage ***,the unstable solid electrolyte interphase(SEI)layer due to continuous decomposition of electrolytes,and the attendant problem of Li dendrite growth frustrate their commercialization ***,a hybrid SEI comprising abundant LiF,lithiophilic Li-Ge alloy,and Ge nanoparticles is constructed via a simple brush coating *** fluorinated interface layer with embedded Ge-containing components isolates the Li anode from the corrosive electrolyte and facilitates homogenous Li nucleation as well as uniform ***,the modified Li anode exhibits remarkable stability without notorious Li dendrites,delivering stable cycling lives of more than 1000 h for symmetric Li||Li cells and over 600 cycles for Li||Cu cells at 1 mA·cm^(−2).Moreover,the reinforced Li anodes endow multiple full-cell architectures with dramatically improved cyclability under different test *** work provides rational guidance to design an artificial hybrid SEI layer and would stimulate more ideas to solve the dendrite issue and promote the further development of advanced LMBs.

关键词： lithium metal anode artificial solid electrolyte interphase(SEI) dendrite suppression lithium fluoride Li-Ge alloy

High energy density in ultra-thick and flexible electrodes enabled by designed conductive agent/binder composite

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Journal of Energy Chemistry 2024年第3期90卷 133-143,I0005页

作者： Xiaoyu Shen Hailong Yu liubin Ben Wenwu Zhao Qiyu Wang Guanjun Cen Ronghan Qiao Yida Wu Xuejie huang Beijing National Laboratory for Condensed Matter Physics Institute of PhysicsChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China Songshan Lake Materials Laboratory Dongguan 523808Guangdong China

Thick electrodes can increase incorporation of active electrode materials by diminishing the proportion of inactive constituents,improving the overall energy density of ***,thick electrodes fabricated using the conventional slurry casting approach frequently exhibit an exacerbated accumulation of carbon additives and binders on their surfaces,invariably leading to compromised electrochemical *** this study,we introduce a designed conductive agent/binder composite synthesized from carbon nanotube and *** agent/binder composite facilitates production of dry-process-prepared ultra-thick electrodes endowed with a three-dimensional and uniformly distributed percolative architecture,ensuring superior electronic conductivity and remarkable mechanical *** this approach,ultra-thick LiCoO_(2)(LCO) electrodes demonstrated superior cycling performance and rate capabilities,registering an impressive loading capacity of up to 101.4 mg/cm^(2),signifying a 242% increase in battery energy *** another analytical endeavor,time-of-flight secondary ion mass spectroscopy was used to clarify the distribution of cathode electrolyte interphase(CEI) in cycled LCO *** results provide unprecedented evidence explaining the intricate correlation between CEI generation and carbon distribution,highlighting the intrinsic advantages of the proposed dry-process approach in fine-tu ning the CEI,with excellent cycling performance in batteries equipped with ultra-thick electrodes.

关键词： Conductive agent/binder composite Dry process Ultra-thick electrodes High energy density CEI reconstruction ToF-SIMS

正极材料LiNi0.8Co0.1Mn0.1O2的合成工艺优化及电化学性能

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化工学报 2017年第4期68卷 1652-1659页

作者：肖忠良胡超明宋刘斌卢意鹏刘姣曾鹏长沙理工大学化学与生物工程学院电力与交通材料保护湖南省重点实验室湖南长沙410114

采用高温固相法合成锂离子电池富镍三元材料LiNi_(0.8)Co_(0.1)Mn_(0.1)O_2,对其工艺条件进行优化,对产物进行X射线衍射(XRD),扫描电镜(SEM)以及电化学性能分析。结果表明:在氧气气氛下,锂与金属元素摩尔比为1.05:1、烧结时间15 h、烧... 详细信息

采用高温固相法合成锂离子电池富镍三元材料LiNi_(0.8)Co_(0.1)Mn_(0.1)O_2,对其工艺条件进行优化,对产物进行X射线衍射(XRD),扫描电镜(SEM)以及电化学性能分析。结果表明:在氧气气氛下,锂与金属元素摩尔比为1.05:1、烧结时间15 h、烧结温度750℃为最佳合成工艺条件。按最佳工艺合成的样品在1C首次放电容量高达174.9mA·h·g^(-1),50次循环后比容量为158.5 mA·h·g^(-1),容量保持率为90.62%,表现出良好的循环稳定性。XRD和SEM表征表明,在氧气气氛下烧结的样品有良好的层状结构,阳离子混排程度小,具有较好的类球形,粒径均匀分布在10~20μm。循环伏安(CV)和电化学阻抗(EIS)结果表明,工艺条件的优化有助于提高正极材料的电化学性能。

关键词： LiNi0.8Co0.1Mn0.1O2 合成高温固相电化学稳定性锂离子电池

高压水工隧洞BFRP网格增强钢筋混凝土衬砌试验研究

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水利水电技术 2017年第7期48卷 109-115页

作者：鲁和彭立锋苏国韶燕柳斌胡小川秦子华广西大学土木建筑工程学院工程防灾与结构安全教育部重点实验室广西南宁530004

为探究玄武岩纤维增强树脂复合材料网格(简称BFRP网格)对高压水工隧洞钢筋混凝土衬砌结构裂缝控制能力及承载能力的增强作用,进行了高压水工隧洞钢筋混凝土衬砌结构模型对比试验,试验采用真实高压水加载。通过对隧洞模型内壁环向变形监... 详细信息

为探究玄武岩纤维增强树脂复合材料网格(简称BFRP网格)对高压水工隧洞钢筋混凝土衬砌结构裂缝控制能力及承载能力的增强作用,进行了高压水工隧洞钢筋混凝土衬砌结构模型对比试验,试验采用真实高压水加载。通过对隧洞模型内壁环向变形监测,以及通过声发射系统对模型在加载全过程中的声发射信息监测,对比分析了BFRP网格对裂缝产生及扩展的影响。研究结果显示,与常规混凝土衬砌结构模型相比较,BFRP网格增强钢筋混凝土衬砌结构模型的极限承载力提高21%、宏观裂缝最大开度减少了68%、宏观裂缝空间分布更为分散;开裂前内壁环向拉应变增大了81%,开裂时的声发射绝对能量占加载过程中声发射总累积绝对能量的33.78%(前者为99.38%),主要破坏模式表现为韧性破坏。可见,BFRP网格可显著提高高压水工隧洞钢筋混凝土衬砌结构的裂缝控制能力和承载能力。

关键词：水工隧洞高压 BFRP网格衬砌模型试验

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加工条件对亚油酸氧化形成呋喃的影响

中国食品学报 2024年第4期24卷 278-284页

作者：张青李刘滨张梁朱梦婷茶树生物学与资源利用国家重点实验室安徽农业大学茶与食品科技学院合肥230036

呋喃是2B级致癌物(可能使人类致癌),主要形成于食品热加工过程,多不饱和脂肪酸(PUFAs)氧化是形成呋喃的重要途径,然而PUFAs形成呋喃的研究尚处于起步阶段。本研究选用亚油酸为代表性脂肪酸,采用顶空进样-气相色谱-质谱联用法(HS-GC-MS)... 详细信息

呋喃是2B级致癌物(可能使人类致癌),主要形成于食品热加工过程,多不饱和脂肪酸(PUFAs)氧化是形成呋喃的重要途径,然而PUFAs形成呋喃的研究尚处于起步阶段。本研究选用亚油酸为代表性脂肪酸,采用顶空进样-气相色谱-质谱联用法(HS-GC-MS)探究加工条件(温度、时间、pH值、含水量、金属离子、多酚)对亚油酸氧化形成呋喃的影响。结果表明,随着加热温度的升高和加热时间的延长,呋喃含量呈现增长趋势。随着水分添加量的增加(0~100μL),促进效果呈先上升后降低最后趋于稳定的规律。添加Cu^(+)、Cu^(2+)和Fe^(3+)等变价金属离子可显著促进亚油酸氧化形成呋喃(P<0.05),而加入K^(+)、Na^(+)和Ca^(2+)等金属离子对呋喃的形成没有显著影响。与中性条件相比,酸性条件对呋喃形成没有显著影响,而碱性条件可显著抑制呋喃的形成(P<0.05),抑制率达56.64%。此外,添加多酚类物质,如表儿茶素没食子酸酯(ECG)、杨梅素、奎宁酸、对香豆酸、绿原酸可显著抑制呋喃的形成(P<0.05),其中杨梅素抑制效果最好,抑制率最高可达55.54%。本研究结果可为脂质热加工过程中呋喃的调控提供一定的理论参考。

关键词：亚油酸呋喃热加工抑制顶空进样-气相色谱-质谱联用法

鄂尔多斯盆地东部边界的构造学分析:以石楼北地区为例

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古地理学报 2024年第1期26卷 150-164页

作者：石婧何登发包洪平魏柳斌中国地质大学(北京)能源学院北京100083 中国石油长庆油田公司勘探开发研究院陕西西安710018

通常认为鄂尔多斯东部边界带由晋西挠褶带和离石断裂组成,但这一边界为残余边界,并非原始的沉积边界。文中以石楼北区域为例,过该区域构建了1条鄂尔多斯盆地东部盆-山尺度的区域地质大剖面,运用2D-Move软件进行构造演化的反演与正演模拟... 详细信息

通常认为鄂尔多斯东部边界带由晋西挠褶带和离石断裂组成,但这一边界为残余边界,并非原始的沉积边界。文中以石楼北区域为例,过该区域构建了1条鄂尔多斯盆地东部盆-山尺度的区域地质大剖面,运用2D-Move软件进行构造演化的反演与正演模拟,对其构造变形进行定量分析,并根据研究结果对鄂尔多斯盆地东部边界进行重新厘定。研究认为:(1)石楼北地区在加里东晚期受深部基底断裂活动影响,奥陶系膏盐岩层中形成盐滑脱褶皱,之后沉积石炭系—白垩系,至燕山期受到东西向的挤压应力,地层整体发生掀斜,最终在新生代吕梁隆起加速隆升,遭受差异风化剥蚀形成现今构造格局。(2)构建的区域地质大剖面现今长度为263.76 km,海拔最高可达2000 m,从加里东晚期到白垩纪地层缩短量为3.14 km,缩短率为1.18%,地层抬升高度为3.82 km。(3)根据地层、构造、演化特征对燕山运动期鄂尔多斯盆地的东部边界进行重新厘定,认为东部边界应向东延伸至吕梁隆起东侧。该成果可为鄂尔多斯盆地东缘范围、构造变形研究以及晋西挠褶带煤层气勘探开发提供参考与新思路。

关键词：鄂尔多斯盆地构造特征构造演化断层相关褶皱东部边界

鄂尔多斯盆地奥陶系马家沟组四段优质白云岩储层发育特征及成因机制

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天然气工业 2024年第2期44卷 30-39页

作者：于洲罗晓容周进高胡子见魏柳斌李靖师平平曹斌风吕玉珍中国石油杭州地质研究院国家能源碳酸盐岩油气重点实验室西北大学中国石油长庆油田公司勘探事业部中国石油长庆油田公司勘探开发研究院

鄂尔多斯盆地米探1井在奥陶系马家沟组四段(以下简称马四段)白云岩获得天然气勘探新发现,展示出马四段良好的天然气勘探前景,但马四段白云岩储层发育特征及其分布规律不清,制约了该层系下一步的天然气勘探部署。为此,基于岩心、薄片、工... 详细信息

鄂尔多斯盆地米探1井在奥陶系马家沟组四段(以下简称马四段)白云岩获得天然气勘探新发现,展示出马四段良好的天然气勘探前景,但马四段白云岩储层发育特征及其分布规律不清,制约了该层系下一步的天然气勘探部署。为此,基于岩心、薄片、工业CT、U-Pb定年、物性分析及地球化学特征等资料,系统研究了马四段白云岩储层发育特征及成因机制,并预测了该盆地白云岩储层分布和天然气有利勘探区带。研究结果表明:(1)马四段主要发育丘滩相白云岩储层和斑状白云岩储层,其中丘滩相白云岩储层岩性为砂砾屑白云岩、细—中晶白云岩、粉—细晶白云岩和叠层石白云岩,斑状白云岩储层岩性为斑状粉—细晶白云岩、斑状粉晶白云岩和斑状灰质白云岩。(2)丘滩相白云岩储层储集空间主要为晶间(溶)孔,含少量溶蚀孔洞、残余粒间孔和微裂缝,平均孔隙度为5.06%;斑状白云岩储层储集空间以晶间孔为主,含少量晶间溶孔和微裂缝,平均孔隙度为2.46%。(3)丘滩相白云岩储层发育主要受微生物丘和颗粒滩控制,并经历了准同生白云石化作用和埋藏白云石化作用的改造,斑状白云岩储层发育主要受生物扰动作用、准同生白云石化作用和埋藏白云石化作用控制。(4)构造古地理格局和海平面升降变化共同控制了丘滩体发育、生物扰动作用程度和白云石化流体的形成。结论认为,马四段优质白云岩储层主要沿中央古隆起和神木—志丹低隆起规模分布,其中神木—志丹低隆起马四段白云岩储层位于岩性相变带上,其储盖配置关系好,是天然气富集区,预测有利区储层面积18 000 km^(2)。

关键词：鄂尔多斯盆地奥陶系马家沟组四段白云岩储层构造古地理格局海平面升降变化