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Defect engineered nickel hydroxide nanosheets for advanced pseudocapacitor electrodes

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Nano Research 2024年第6期17卷 5233-5242页

作者： Yaohang Gu Yuxuan Zhang Xuanyu wang Ateer Bao Bo Ni haijun pan Xiaoyan Zhang Xiwei Qi School of Materials Science and Engineering Northeastern UniversityShenyang 110189China College of Metallurgy and Energy North China University of Science and TechnologyTangshan 063210China Key Laboratory of Dielectric and Electrolyte Functional Material hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004China School of Resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China

while the past years have witnessed great achievement in pseudocapacitors,the inauguration of electrode materials of high-performance still remains a formidable ***,the capacity and rate capability of the electrode depends largely on its electrical conductivity,which ensures fast charge transfer kinetics in both the grain bulk and grain ***,nickel hydroxides with oxygen vacancies are facilely fabricated via a hydrothermal *** active materials exhibit a high specific capacitance of 3250 F·g^(−1)and a high areal of capacitance of 14.98 F·cm^(−2)at 4.6 mA·cm^(−2).The asymmetric supercapacitor device based on our material delivers a high energy density of~71.6 wh·kg^(−1)and a power density of~17,300 w·kg^(−1)and could retain~95%of their initial capacitance even after 30,000 *** addition,the defect-rich hydroxides demonstrate higher electrical conductivity as well as dielectric constant,which is responsible for the superior pseudocapacitive *** new scientific strategy in terms of taking the advantages of oxygen vacancies might open up new opportunities for qualified pseudocapacitive materials of overall high performances not only for nickel hydroxides but also for other metal hydroxides/oxides.

关键词： pseudocapacitors nickel hydroxides oxygen vacancies electrical conductivity

Pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy for activating water and urea oxidation

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Green Energy & Environment 2024年第4期9卷 684-694页

作者： Guangfu Qian wei Chen Jinli Chen Li Yong Gan Tianqi Yu Miaojing pan Xiaoyan Zhuo Shibin Yin Guangxi Key Laboratory of Electrochemical Energy Materials College of Chemistry and Chemical EngineeringState Key Laboratory of Processing for Non-Ferrous Metal and Featured MaterialsGuangxi University100 Daxue RoadNanning530004China Institute for Structure and Function and Department of Physics Chongqing UniversityChongqing400030China

Exploitation of oxygen evolution reaction(OER)and urea oxidation reaction(UOR)catalysts with high activity and stability at large current density is a major challenge for energy-saving h_(2) production in water ***,we use the pyridinic-N doping carbon layers coupled with tensile strain of FeNi alloy activated by NiFe_(2)O_(4)(FeNi/NiFe_(2)O_(4)@NC)for efficiently increasing the performance of water and urea *** to the tensile strain effect on FeNi/NiFe_(2)O_(4)@NC,it provides a favorable modulation on the electronic properties of the active center,thus enabling amazing OER(η_(100)=196 mV)and UOR(E_(10)=1.32 V)intrinsic ***,the carbon-coated layers can be used as armor to prevent FeNi alloy from being corroded by the electrolyte for enhancing the OER/UOR stability at large current density,showing high industrial *** work thus provides a simple way to prepare high-efficiency catalyst for activating water and urea oxidation.

关键词： Carbon-encapsulated Tensile strain Catalyst Oxygen evolution reaction Urea oxidation reaction

Manipulating photogenerated electron flow in nickel single‐atom catalysts for photocatalytic CO_(2)reduction into tunable syngas

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Carbon Energy 2024年第8期6卷 205-213页

作者： Yida Zhang Qingyu wang Lihui wu haibin pan Chengyuan Liu Yue Lin Gongming wang Xusheng Zheng National Synchrotron Radiation Laboratory University of Science and Technology of ChinaHefeiAnhuiChina College of Chemistry and Materials Science University of Science and Technology of ChinaHefeiAnhuiChina Department of Chemistry Hefei National Research Center for Physical Sciences at the MicroscaleUniversity of Science and Technology of ChinaHefeiAnhuiChina

The key to designing photocatalysts is to orient the migration of photogenerated electrons to the target active sites rather than dissipate at inert ***,we demonstrate that the doping of phosphorus(P)significantly enriches photogenerated electrons at Ni active sites and enhances the performance for CO_(2)reduction into *** photocatalytic CO_(2)reduction,Ni single‐atom‐anchored P‐modulated carbon nitride showed an impressive syngas yield rate of 85μmol gcat^(−1)h^(−1)and continuously adjustable CO/h_(2)ratios ranging from 5:1 to 1:2,which exceeded those of most of the reported carbon nitride‐based single‐atom *** studies reveal that P doping improves the conductivity of catalysts,which promotes photogenerated electron transfer to the Ni active sites rather than dissipate randomly at low‐activity nonmetallic sites,facilitating the CO_(2)‐to‐syngas photoreduction process.

关键词： carbon nitride CO_(2)photoreduction electron flow Ni single atoms syngas

hybrid-Triggered h∞ sliding mode control for Networked Control System with Deception Attacks

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Hybrid-Triggered H∞ sliding mode control for Networked Cont...

Efficient stabilization of dredged sludge with high water content using an improved bio-carbonation of reactive magnesia cement method

第35届中国过程控制会议

作者： Xiangyang Qu Zhiwen wang pan Zhang Feng wang College of Electrical and Information Engineering Lanzhou University of Technology Gansu Key Laboratory Advanced Control for Industrial Processes

This paper studies the h∞ sliding mode control(SMC) problem for a class of networked control system(NCS) with hybrid event-triggered scheme and deception attacks. To alleviate the communication burden, a hybrid event-triggered mechanism that combines the time-triggered mechanism(TTM) and event-triggered mechanism(ETM) via a Bernoulli random variable is presented. Then, taking into account the influence of deception attacks on system performance, an observer-based output feedback h∞ SMC method is proposed. By using the linear matrix inequality technique and Lyapunov stability theory, the system is asymptotically stable and with given h∞ performance. In addition, an observer-based SMC law is designed to ensure that the system state trajectory reaches a predefined sliding region. Finally, a numerical simulation is used to verify the effectiveness of the proposed method.

关键词： Networked control system sliding mode control hybrid-triggered mechanism deception attacks

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3760-3771页

作者： Rui wang Chaosheng Tang Xiaohua pan Dianlong wang Zhihao Dong Xiying Zhang Xiancai Lu School of Earth Sciences and Engineering Nanjing UniversityNanjing210023China Qinghai Provincial Key Laboratory of Geology and Environment of Salt Lake Qinghai Institute of Salt LakesChinese Academy of SciencesXining810008China

This study proposed an improved bio-carbonation of reactive magnesia cement(RMC)method for dredged sludge stabilization using the urea pre-hydrolysis *** on unconfined compression strength(UCS),pickling-drainage,and scanning electron microscopy(SEM)tests,the effects of prehydrolysis duration(T),urease activity(UA)and curing age(CA)on the mechanical properties and microstructural characteristics of bio-carbonized samples were systematically investigated and *** results demonstrated that the proposed method could significantly enhance urea hydrolysis and RMC bio-carbonation to achieve efficient stabilization of dredged sludge with 80%high water content.A significant strength increment of up to about 1063.36 kPa was obtained for the bio-carbonized samples after just 7 d of curing,which was 2.64 times higher than that of the 28-day cured ordinary Portland cement-reinforced *** elevated T and UA could notably increase urea utilization ratio and carbonate ion yield,but the resulting surge in supersaturation also affected the precipitation patterns of hydrated magnesia carbonates(hMCs),which weakened the cementation effect of hMCs on soil particles and further inhibited strength enhancement of bio-carbonized *** optimum formula was determined to be the case of T?24 h and UA?10 U/mL for dredged sludge stabilization.A 7-day CA was enough for bio-carbonized samples to obtain stable strength,albeit slightly affected by *** benefits of high efficiency and water stability presented the potential of this method in achieving dredged sludge stabilization and resource *** investigation provides informative ideas and valuable insights on implementing advanced bio-geotechnical techniques to achieve efficient stabilization of soft soil,such as dredged sludge.

关键词： Reactive magnesia cement(RMC)biocarbonation Urea pre-hydrolysis Dredged sludge Efficient stabilization Unconfined compressive strength Microbially induced carbonate precipitation(MICP)

Efficient guiding and focusing of intense laser pulse using periodic thin slits

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Matter and Radiation at Extremes 2024年第4期9卷 29-39页

作者： L.Xu T.w.huang K.Jiang C.N.wu h.Peng P.C.hen R.Li h.B.Zhuo C.T.Zhou Shenzhen Key Laboratory of Ultraintense Laser and Advanced Material Technology Center for Intense Laser ApplicationTechnologyand College of Engineering PhysicsShenzhen Technology UniversityShenzhen 518118People’s Republic of China

Slits have been widely used in laser-plasma interactions as plasma optical components for generating high-harmonic light and controlling laser-driven particle ***,we propose and demonstrate that periodic thin slits can be regarded as a new breed of optical elements for efficient focusing and guiding of intense laser *** fundamental physics of intense laser interaction with thin slits is studied,and it is revealed that relativistic effects can lead to enhanced laser focusing far beyond the pure diffractive focusing *** addition,the interaction of an intense laser pulse with periodic thin slits makes it feasible to achieve multifold enhancement in both laser intensity and energy transfer efficiency compared with conventional *** results provide a novel method for manipulating ultra-intense laser pulses and should be of interest for many laser-based applications.

关键词： laser pulse intense

Precipitation of multi-type nano-quasicrystals in a Mg-Zn-Y alloy

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Journal of Magnesium and Alloys 2024年第3期12卷 997-1008页

作者： w.Z.wang X.Z.Zhou L.F.Zhang h.Q.Ye Z.Q.Yang Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of ScienceShenyang 110016China Ji hua Laboratory Foshan 528251China Foshan University Foshan 528231China

Mg-6Zn-1Y(at.%)ribbons with strengthening precipitates of multi-type nanoquasicrystals were prepared by melt-spinning followed by aging *** evolution of the rapidly solidified ribbons during isothermal aging was comprehensively studied using various electron microscopy *** new kinds of decagonal quasicrystals were formed in aged ribbons,in addition to precipitation of nanometer icosahedral ***-resolution observations reveal that both decagonal quasicrystals can be modeled by quasiperiodic tiling with decagonal clusters of 2.5 nm in diameter,but overlap of neighboring clusters in both decagonal quasicrystals is different from the Gummelt model observed in other quasicrystals.A shell composed of complex Laves Mg-Zn domains was formed surrounding each decagonal quasicrystal precipitate upon prolonged *** addition,all kinds of nanoprecipitates exhibit excellent structure and size stability at 573 *** findings may have implications for not only fundamental studies about quasicrystals,but also microstructural manipulation of high-performance Mg alloys.

关键词： Quasicrystal Mg alloys Rapid solidification Scanning-transmission electron microscopy.

MiR-30a-5p alleviates LPS-induced hPMEC injury through regulation of autophagy via Beclin-1

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BIOCELL 2024年第3期48卷 431-441页

作者： RAN pan JIAYAN MAO YUELIANG ZhENG wEI ChEN JUNPING GUO LIJUN wANG Rainbowfish Rehabilitation and Nursing School Hangzhou Vocational&Technical CollegeHangzhou310018China Cancer Institute of Integrated Traditional Chinese and western Medicine Key Laboratory of Cancer Prevention and Therapy Combining Traditional Chinese and Western MedicineZhejiang Academy of Traditional Chinese MedicineHangzhou310012China Geriatric Medicine Center Department of EndocrinologyZhejiang Provincial People’s Hospital(Affiliated People’s Hospital)Hangzhou Medical CollegeHangzhou310015China

Background:Sepsis,a type of systemic disease,can impact nearly all organs,tissues and *** them,endothelial cells are amongst theﬁrst to be affected and respond to the *** this study,we investigated the protective effects of microRNA-30a-5p(miR-30a-5p)on human pulmonary microvascular endothelial cells(hPMECs)treated with lipolysaccharide(LPS).Methods:An in vitro model of sepsis was established in hPMECs with the use of *** with different tools(mimetic and inhibitor)to modify miR-30a-5p *** viability,proliferation and apoptosis were detected by the CCK-8 assay,the EdU kit andﬂuorescence staining,*** autophagy-related protein and mRNA expression,the number of autophagosomes were separately examined through western blot analysis,qPT-PCR and confocal *** and the luciferase reporter assays were used to probe target genes interacting with ***:LPS caused a reduction in the viability and proliferation of hPMECs,as well as an elevation in the number of apoptotic ***,we observed that miR-30a-5p might play a role in preventing LPS-induced inhibition of cell damage and decreasing hPMEC apoptosis,suggesting the potential function of miR-30a-5p in this injury ***,we conﬁrmed that miR-30a-5p exerts its protective effect by regulating cell autophagy,possibly by targeting ***:Our study provided evidence that autophagy is a crucial aspect in the protective role of miR-30a-5p against LPS-induced hPMEC injury,identifying a promising target for sepsis-related endothelial cell injury.

关键词： Sepsis Endothelial cells MicroRNA Systemic inflammatory response syndrome

FGF4 protects the liver from immune-mediated injury by activating CaMKKβ-PINK1 signal pathway to inhibit hepatocellular apoptosis

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Acta Pharmaceutica Sinica B 2024年第6期14卷 1605-1623页

作者： Zhifeng huang Tongtong pan Liang Xu Lu Shi Xiong Ma Liya Zhou Luyao wang Jiaojiao wang Guoqing Zhu Dazhi Chen Lingtao Song Xiaomin pan Xiaodong wang Xiaokun Li Yongde Luo Yongping Chen hepatology Diagnosis and Treatment Center Zhejiang Provincial Key Laboratory for Accurate Diagnosis and Treatment of Chronic Liver Diseasesthe First Affiliated Hospital of Wenzhou Medical UniversityWenzhou 325035China Oujiang Laboratory(Zhejiang Lab for Regenerative Medicine Vision and Brain Health)&School of Pharmaceutical SciencesWenzhou Medical UniversityWenzhou 325035China School of Laboratory Medicine and Life Sciences Wenzhou Medical University&Key Laboratory of Laboratory MedicineMinistry of EducationWenzhou Medical UniversityWenzhou 325035China Division of Gastroenterology and hepatology Key Laboratory of Gastroenterology and HepatologyMinistry of HealthState Key Laboratory for Oncogenes and Related GenesRenji HospitalSchool of MedicineShanghai Jiao Tong UniversityShanghai 200001China hangzhou Medical College Hangzhou 311300China

Immune-mediated liver injury (ILI) is a condition where an aberrant immune response due to various triggers causes the destruction of hepatocytes. Fibroblast growth factor 4 (FGF4) was recently identified as a hepatoprotective cytokine;however, its role in ILI remains unclear. In patients with autoimmune hepatitis (type of ILI) and mouse models of concanavalin A (ConA)- or S-100-induced ILI, we observed a biphasic pattern in hepatic FGF4 expression, characterized by an initial increase followed by a return to basal levels. hepatic FGF4 deficiency activated the mitochondria-associated intrinsic apoptotic pathway, aggravating hepatocellular apoptosis. This led to intrahepatic immune hyper-reactivity, inflammation accentuation, and subsequent liver injury in both ILI models. Conversely, administration of recombinant FGF4 reduced hepatocellular apoptosis and rectified immune imbalance, thereby mitigating liver damage. The beneficial effects of FGF4 were mediated by hepatocellular FGF receptor 4, which activated the Ca^(2+)/calmodulin-dependent protein kinasekinase 2 (CaMKKβ) and its downstream phosphatase and tensin homologue-induced putative kinase 1 (PINK1)-dependent B-cell lymphoma 2-like protein 1-isoform L (Bcl-XL) signalling axis in the mitochondria. hence, FGF4 serves as an early response factor and plays a protective role against ILI, suggesting a therapeutic potential of FGF4 and its analogue for treating clinical immune disorder-related liver injuries.

关键词： Fibroblast growthfactor 4 Fibroblast growth factor receptor 4 Immune liver injury Ca^(2+)/Calmodulin dependent protein