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Defect engineered nickel hydroxide nanosheets for advanced pseudocapacitor electrodes

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Nano research 2024年第6期17卷 5233-5242页

作者： Yaohang Gu Yuxuan Zhang Xuanyu Wang Ateer Bao Bo Ni haijun Pan Xiaoyan Zhang Xiwei qi School of Materials Science and Engineering Northeastern UniversityShenyang 110189China College of Metallurgy and Energy North China University of Science and TechnologyTangshan 063210China Key Laboratory of Dielectric and Electrolyte Functional Material hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004China School of resources and Materials Northeastern University at QinhuangdaoQinhuangdao 066004China

While the past years have witnessed great achievement in pseudocapacitors,the inauguration of electrode materials of high-performance still remains a formidable ***,the capacity and rate capability of the electrode depends largely on its electrical conductivity,which ensures fast charge transfer kinetics in both the grain bulk and grain ***,nickel hydroxides with oxygen vacancies are facilely fabricated via a hydrothermal *** active materials exhibit a high specific capacitance of 3250 F·g^(−1)and a high areal of capacitance of 14.98 F·cm^(−2)at 4.6 mA·cm^(−2).The asymmetric supercapacitor device based on our material delivers a high energy density of~71.6 Wh·kg^(−1)and a power density of~17,300 W·kg^(−1)and could retain~95%of their initial capacitance even after 30,000 *** addition,the defect-rich hydroxides demonstrate higher electrical conductivity as well as dielectric constant,which is responsible for the superior pseudocapacitive *** new scientific strategy in terms of taking the advantages of oxygen vacancies might open up new opportunities for qualified pseudocapacitive materials of overall high performances not only for nickel hydroxides but also for other metal hydroxides/oxides.

关键词： pseudocapacitors nickel hydroxides oxygen vacancies electrical conductivity

Non-perturbative dynamics of flat-band systems with correlated disorder

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Chinese Physics B 2024年第9期33卷 547-551页

作者： qi Li Junfeng Liu Ke Liu Zi-Xiang hu Zhou Li GBA Branch of Aerospace Information research Institute Chinese Academy of SciencesGuangzhou 510535China Guangdong Provincial Key Laboratory of Terahertz Quantum Electromagnetics Guangzhou 510700China School of Physics and Materials Science Guangzhou UniversityGuangzhou 510006China Department of Physics and Chongqing Key Laboratory for Strongly Coupled Physics Chongqing UniversityChongqing 401331China University of Chinese Academy of Sciences Beijing 100039China

We develop a numerical method for the time evolution of Gaussian wave packets on flat-band lattices in the presence of correlated *** achieve this,we introduce a method to generate random on-site energies with prescribed *** verify this method with a one-dimensional(1D)cross-stitch model,and find good agreement with analytical results obtained from the disorder-dressed evolution *** allows us to reproduce previous findings,that disorder can mobilize 1D flat-band states which would otherwise remain *** explained by the corresponding disorder-dressed evolution equations,such mobilization requires an asymmetric disorder-induced coupling to dispersive bands,a condition that is generically not fulfilled when the flat-band is resonant with the dispersive bands at a Dirac point-like *** exemplify this with the 1D Lieb *** analytical expressions are not available for the two-dimensional(2D)system due to its complexity,we extend the numerical method to the 2D a–T3 model,and find that the initial flat-band wave packet preserves its localization when a=0,regardless of disorder and ***,when a̸=0,the wave packet shifts in real *** interpret this as a Berry phase controlled,disorder-induced wave-packet *** addition,we present density functional theory calculations of candidate materials,specifically hg1−*** flat-band emerges near the G point(α=0)in the Brillouin zone.

关键词： flat-band system dynamics correlated disorder

Evaluating the efficacy of immunotherapy in gastric cancer:Insights from immune checkpoint inhibitors

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World Journal of Gastroenterology 2024年第32期30卷 3726-3729页

作者： Yu-Nuo Yang Li-Sheng Wang Yan-qi Dang Guang Ji Institute of Digestive Diseases Longhua HospitalChina-Canada Center of Research for Digestive DiseasesShanghai University of Traditional Chinese MedicineShanghai 200032China Department of Biochemistry University of OttawaOttawa K1H 8M5ONCanada

The emergence of immunotherapy,particularly immune checkpoint inhibitors(ICIs),represents a groundbreaking approach to treating gastric cancer(GC).however,the prognosis of GC patients receiving ICI treatment is influenced by various *** manuscript identified sarcopenia and myosteatosis as independent prognostic factors impacting the outcomes of GC patients treated with ***,this study introduced a visual predictive model to estimate the prognosis of GC *** confirmed by further studies,this observation could provide valuable insights to propel the advancement of personalized clinical medicine and the integration of precision medicine practices.

关键词： Gastric cancer Immune checkpoint inhibitors Sarcopenia Myosteatosis Prediction model

Clinical efficacy of laparoscopic cholecystectomy combined with endoscopic papillary balloon dilation in treatment of gallbladder stones with common bile duct stones: A retrospective study

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World Journal of Gastrointestinal Surgery 2024年第6期16卷 1700-1708页

作者： hong-Dan Liu qi Zhang Wen-Si Xu Shuang Jin Department of Gastroenterology The Third Affiliated Hospital of Qiqihar Medical UniversityQiqihar 161000Heilongjiang ProvinceChina

BACKGrOUND The incidence of cholelithiasis has been on the rise in recent years,but the choice of procedure is *** To investigate the efficacy of laparoscopic cholecystectomy(LC)combined with endoscopic papillary balloon dilation(EPBD)in patients with gallbladder stones(GS)with common bile duct stones(CBDS).METhODS The clinical data of 102 patients with GS combined with CBDS were selected for retrospective analysis and divided into either an LC+EPBD group(n=50)or an LC+endoscopic sphincterotomy(EST)group(n=52)according to surgical ***-related indexes,postoperative recovery,postoperative complications,and expression levels of inflammatory response indexes were compared between the two *** Total surgical time,stone free rate,rate of conversion to laparotomy,and successful stone extraction rate did not differ significantly between the LC+EPBD group and LC+EST *** hemorrhage,time to ambulation,and length of hospitalization in the LC+EPBD group were lower than those of the LC+EST group(Phe rate of total complications of the two groups was 9.80%and 17.65%,respectively,and the difference was not statistically *** serious complications occurred in either *** 48 h postoperatively,the expression levels of interleukin-6,tumor necrosis factor-α,high-sensitivity Creactive protein,and procalcitonin were lower in the LC+EPBD group than in the LC+EST group(Pratively,the expression levels of aspartate transaminase,alanine transaminase,and total bilirubin were lower in the LC+EPBD group than in the LC+EST group(Ph EPBD and LC combined with EST are both effective procedures for the treatment of GS with CBDS,in which LC combined with EPBD is beneficial to shorten the patient’s hospitalization time,reduce the magnitude of elevated inflammatory response indexes,and promote postoperative recovery.

关键词： Gallbladder stone Common bile duct stone Endoscopic papillary balloon dilation Laparoscopic cholecystectomy Endoscopic sphincterotomy

3D-printed MoS_(2)/Ni electrodes with excellent electro-catalytic performance and long-term stability for dechlorination of florfenicol

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Journal of Environmental Sciences 2024年第3期137卷 420-431页

作者： Jianhui Xu Pengxu Wang Shenggui Chen Lei Li Dan Li Yunfei Zhang qi Wu Jinhong Fan LumingMa School of Environment and Civil Engineering Dongguan University of TechnologyDongguan 523808China School of Art and Design Guangzhou Panyu PolytechnicGuangzhou 511483China National Engineering research Center for Urban Pollution Control State Key Laboratory of Pollution Control and Resources ReuseCollege of Environmental Science and EngineeringTongji UniversityShanghai 200092China Dongguan Institute of Science and Technology Innovation Dongguan University of TechnologyDongguan 523808China School of Mechanical Engineering Dongguan University of TechnologyDongguan 523808China

here,we report the production of 3D-printed MoS_(2)/Ni electrodes(3D-MoS_(2)/Ni)with longterm stability and excellent performance by the selective laser melting(SLM)*** a cathode,the obtained 3D-MoS_(2)/Ni could maintain a degradation rate above 94.0%for forfenicol(FLO)when repeatedly used 50 times in *** also found that the removal rate of FLO by 3D-MoS_(2)/Ni was about 12 times higher than that of 3D-printed pure Ni(3D-Ni),attributed to the improved accessibility of h^(*).In addition,the electrochemical characterization results showed that the electrochemically active surface area of the 3D-MoS_(2)/Ni electrode is about 3-fold higher than that of the 3D-Ni electrode while the electrical resistance is 4 times *** on tert-butanol suppression,electron paramagnetic resonance and triple quadrupole mass spectrometer experiments,a“dual path”mechanism and possible degradation pathway for the dechlorination of FLO by 3D-MoS_(2)/Ni were ***,we also investigated the impacts of the cathode potential and the initial ph of the solution on the degradation of ***,this study reveals that the SLM 3D printing technique is a promising approach for the rapid fabrication of high-stability metal electrodes,which could have broad application in the control of water contaminants in the environmental field.

关键词： 3D-print Electroreduction MoS_(2)/Ni Antibiotic Florfenicol

A functionalized activated carbon adsorbent prepared from waste amidoxime resin by modifying with h_(3)PO_(4) and ZnCl_(2) and its excellent Cr(Ⅵ)adsorption

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International Journal of Minerals,Metallurgy and Materials 2024年第3期31卷 585-598页

作者： Chunlin he Yun Liu Mingwei qi Zunzhang Liu Yuezhou Wei Toyohisa Fujita Guifang Wang Shaojian Ma Wenchao Yang School of resources Environment and MaterialsGuangxi UniversityNanning 530004China State Key Laboratory of Featured Metal Materials and Life-cycle Safety for Composite Structures Guangxi UniversityNanning 530004China School of Nuclear Science and Technology University of South ChinaHengyang 421000China School of Nuclear Science and Engineering Shanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of New Low-carbon Green Chemical Technology Education Department of Guangxi Zhuang Autonomous RegionNanning 530004China

With the application of resins in various fields, numerous waste resins that are difficult to treat have been produced. The industrial wastewater containing Cr(Ⅵ) has severely polluted soil and groundwater environments, thereby endangering human health. Therefore, in this paper, a novel functionalized mesoporous adsorbent PPr-Z was synthesized from waste amidoxime resin for adsorbing Cr(Ⅵ). The waste amidoxime resin was first modified with h3PO4 and ZnCl_(2), and subsequently, it was carbonized through slow thermal decomposition. The static adsorption of PPr-Z conforms to the pseudo-second-order kinetic model and Langmuir isotherm, indicating that the Cr(Ⅵ) adsorption by PPr-Z is mostly chemical adsorption and exhibits single-layer adsorption. The saturated adsorption capacity of the adsorbent for Cr(Ⅵ) could reach 255.86 mg/g. The adsorbent could effectively reduce Cr(Ⅵ) to Cr(Ⅲ) and decrease the toxicity of Cr(Ⅵ) during adsorption. PPr-Z exhibited Cr(Ⅵ) selectivity in electroplating wastewater. The main mechanisms involved in the Cr(Ⅵ) adsorption are the chemical reduction of Cr(Ⅵ) into Cr(Ⅲ) and electrostatic and coordination interactions. Preparation of PPr-Z not only solves the problem of waste resin treatment but also effectively controls Cr(Ⅵ) pollution and realizes the concept of “treating waste with waste”.

关键词： waste amidoxime resin mesoporous adsorbent h_(3)PO_(4)and ZnCl_(2)processing Cr(VI)adsorption electroplating wastewater

Effects of heat treatment on microstructures and properties of a heterostructured alloy with dissimilar components fabricated by WAAM

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rare Metals 2024年第9期43卷 4441-4461页

作者： Ming-Cai Pan Jun-qiang Xu Yong Peng Ning-Ning Liang Si Lan qi Zhou Ke-hong Wang School of Materials Science and Engineering Nanjing University of Science and TechnologyNanjing 210094China Key Laboratory of Controlled Arc Intelligent Additive Manufacturing Technology Nanjing 210094China

heat treatment significantly influences homogeneous material microstructures and mechanical properties,which can be improved by an optimal heat treatment ***,heat treatment application to heterogeneous materials presents significant challenges due to compositional and microstructural ***,a laminated heterostructured alloy comprising alternating316L stainless steel(SS)and 18Ni300 maraging steel(MS)layers fabricated using wire and arc additive manufacturing was investigated.A solution treatment was applied at900℃for 0.5 ***,the solution-treated and asfabricated(AF)samples were aged at 500℃for 4 h;these samples were denoted SA and AT,*** AT phase compositions and orientations were similar to those of *** SA 316L SS layer resembled that of AF,but the SA 18Ni300 MS layers exhibited a reduced austenite phase fraction and refined grain size,attributable to solid-state *** the AT sample,aging induced the formation of nanoscale acicularωphase and ellipsoidal Ni_(3)Ti,Fe_(2)Mo,and X precipitates in the 18Ni300 MS ***,the SA precipitates contained acicular Fe Ni_(2)and ellipsoidalω,Ni_(3)Ti,and X precipitates,and their fractions were lower than those in AT ***18Ni300 MS layer microhardness in the heat-treated samples increased due to nanoprecipitation,but the 316L SS layer microhardness resembled that of *** AT and SA ultimate tensile strengths increased to(1360±50)and(1473±41)MPa,respectively,attributable to precipitation *** SA 316L SS layer exhibited a high stress-induced martensite fraction,enhancing the ductility of heated samples.

关键词： Laminated heterostructured alloy heat treatment Wire and arc additive manufacturing Microstructure Mechanical property

Chiral quantum heating and cooling with an optically controlled ion

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Light(Science & Applications) 2024年第7期13卷 1393-1400页

作者： Jin-Tao Bu Jian-qi Zhang Ge-Yi Ding Jia-Chong Li Jia-Wei Zhang Bin Wang Wen-qiang Ding Wen-Fei Yuan Liang Chen qi Zhong Ali Keçebaş Şahin KÖzdemir Fei Zhou hui Jing Mang Feng State Key Laboratory of Magnetic resonance and Atomic and Molecular Physics Wuhan Institute of Physics and MathematicsInnovation Academy of Precision Measurement Science and TechnologyChinese Academy of Sciences430071 WuhanChina. University of the Chinese Academy of Sciences 100049 BeijingChina. research Center for Quantum Precision Measurement Guangzhou Institute of Industry Technology511458 GuangzhouChina. Department of Engineering Science and Mechanics and Materials Research InstitutePennsylvania State UniversityUniversity ParkState CollegePA 16802USA. Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education Department of Physics and Synergetic Innovation Center for Quantum Effects and ApplicationsHunan Normal University410081 ChangshaChina. Department of Physics Zhejiang Normal University321004 JinhuaChina

Quantum heat engines and refrigerators are open quantum systems,whose dynamics can be well understood using a non-hermitian formalism.A prominent feature of non-hermiticity is the existence of exceptional points(EPs),which has no counterpart in closed quantum *** has been shown in classical systems that dynamical encirclement in the vicinity of an EP,whether the loop includes the EP or not,could lead to chiral mode ***,we show that this is valid also for quantum systems when dynamical encircling is performed in the vicinity of their Liouvillian EPs(LEPs),which include the effects of quantum jumps and associated noise—an important quantum feature not present in previous *** demonstrate,using a Paul-trapped ultracold ion,the first chiral quantum heating and refrigeration by dynamically encircling a closed loop in the vicinity of an *** witness the cycling direction to be associated with the chirality and heat release(absorption)of the quantum heat engine(quantum refrigerator).Our experiments have revealed that not only the adiabaticity breakdown but also the Landau–Zener–Stückelberg process play an essential role during dynamic encircling,resulting in chiral thermodynamic *** observations contribute to further understanding of chiral and topological features in non-hermitian systems and pave a way to exploring the relation between chirality and quantum thermodynamics.

关键词： quantum chiral dynamical

Precipitating thermally reinforcement phase in aluminum alloys for enhanced strength at 400℃

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Journal of Materials Science & Technology 2024年第5期172卷 71-82页

作者： Xiang Su Yuan Lei Yang Chen hongjie Qu Zhixiang qi Gong Zheng Xu Liu henggao Xiang Guang Chen National Key Laboratory of Advanced Casting Technologies MIIT Key Laboratory of Advanced Metallic and Intermetallic Materials TechnologyEngineering Research Center of Materials Behavior and DesignMinistry of EducationNanjing University of Science and TechnologyNanjing 210094China School of Aviation and Mechanical Engineering Changzhou Institute of TechnologyChangzhou 213032China

heat-resistant aluminum alloys are widely used in aerospace and automotive fields for manufacturing hot components due to their advantages in lightweight design and energy ***,the high-temperature strength of existing cast aluminum alloys is always limited to about 100 MPa at 350℃due to coarsening and transformation of strengthening ***,we reveal that the yield strength and ultimate tensile strength of the T6 state Al-8.4Cu-2.3Ce-1.0Mn-0.5Ni-0.2Zr alloy at 400◦C increase by 34%and 44%after re-aging at 300℃for 100 h,and its thermal strength exhibits distinguished ad-vantage over traditional heat-resistant aluminum *** enhanced elevated-temperature strength is attributed to the reprecipitation of the Ni-bearing T-Al_(20)Cu_(2)Mn_(3)phase,whose number density increases over one *** significant segregation of Ni,Ce,and Zr elements at the interfaces helps improve the thermal stability of the T *** thermostable T phase effectively strengthens the matrix by in-hibiting dislocation ***,a highly interconnected 3D intermetallic network along the grain boundaries can still remain after long-term re-aging at 300℃,which is conducive to imposing a drag on the grain boundaries at high *** finding offers a viable route for enhancing the elevated-temperature strength of heat-resistant aluminum alloys,which could provide expanded opportunities for higher-temperature applications.

关键词： Aluminum alloys Precipitation Thermally reinforcement phase re-aging treatment high-temperature strength