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Metal-organic frameworks with dinuclear metal centers for synergistically boosting CO2 photoreduction

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Science China Chemistry 2025年第01期 201-208页

作者： hui-Feng Wang Wen-Jie Shi Yu-Xin Yang Bao-Xia Dong Tong-Bu Lu Di-chang Zhong School of Chemistry and Chemical Engineering Yangzhou University Institute for New Energy Materials and Low Carbon Technologies School of Materials Science and Engineering Tianjin University of Technology

Dinuclear metal synergistic catalysis （DMSC） has been proved powerful in boosting CO2reduction,while this has not been achieved in heterogeneous catalysts with long-range order *** this study,we,by introduction of metal catalytic centers into an indium-based metal-organic framework （MOF）,obtained a series of isostructural In-MOFs,including three MOFs with mononuclear metal catalytic center （M-In）,three MOFs with dinuclear homometallic catalytic centers （MM-In）,and three MOFs with dinuclear heterometallic catalytic centers (MM’-In,M/M’=Co（II）,Ni（II）,Zn（II）).It was found that all these MOFs can serve as catalysts for photochemical CO2reduction to *** with M-In,the catalytic activities of MM-In were obviously enhanced,and that of MM’-In was further significantly *** example,the CO yield of Co Zn-In reaches a record value of 12,700μmol g-1h-1,which is 4.0,8.1,9.4,and 18.6-fold higher than that of Co Co-In,Zn Zn-In,Co-In,and Zn-In,***,the catalytic activities of Co Ni-In and Ni Zn-In also show different fold increase than those of corresponding dinuclear homometallic and mononuclear metallic *** results of control experiments and theoretical calculation reveal that the higher catalytic activities of MM-In over M-In can be ascribed to the DMSC effect,and the higher catalytic activity of MM’-In over MM-In can be ascribed to the strengthened DMSC *** work reveals the relationship between DMSC effect and bimetal centers in CO2reduction,which provides new insights into the DMSC and paves a new way to design highly active catalysts for photochemical CO2reduction.

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Effects of Paper Mill Sludge on Potassium, Sodium, Calcium, and Magnesium Concentrations in Different Soybean Cultivars

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Pedosphere 2005年第1期15卷 84-94页

作者： YANXiang-kui k.W.chang h.L.XU NationalInstituteforAgro-EnvironmentalSciences Tsukuba-shi305-8506Japan／／GansuAgriculturalUniversityLanzhou730070China AgrochemistryDepartment ChungnamNationalUniversityKung-DongTaejon305-764Korea InternationalNatureFarmingResearchCenter 5632HataNagano390-1401（Japan）

A field experiment was conducted on a sandy loam soil at an Experimental Farm in Taejon, South korea, to determine the effects of paper mill sludge compost application rates on k, Na, Ca and Mg concentrations of soybean (Glycine max (L.) Merr.) aboveground tissues and the genotypic effects on the concentrations of these elements. Sludge compost treatments of 0, 75, and 150 t ha-1 were applied to 30 diverse soybean cultivars. Concentrations of k, Na, Ca, and Mg in aboveground tissues harvested 69 days after …

关键词： calcium magnesium paper mill sludge potassium sodium soybean

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Deciphering the molecular mechanisms of Simiaowan in the treatment of hyperuricemia: in vivo and in silico approaches

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Traditional Medicine Research 2025年第2期10卷 37-54页

作者： Yong-chang Zeng Jun-hong Wu Dan-Dan Xu kang he chang-Qing Liu Li-Fei Song Zheng-Zhi Wu Qian-Qian Jiang Shao-Yu Liang Department of Neurology The First Affiliated Hospital of Shenzhen UniversityShenzhen 518020China Pharmaceutical Department The Affiliated TCM Hospital of Guangzhou Medical UniversityGuangzhou 510000China School of Pharmacy Guizhou University of Traditional Chinese MedicineGuiyang 550025China Guangzhou Zeli Medical Technology Co. Ltd.Guangzhou 510700China

Background:Simiaowan(SMW),a well-known traditional Chinese medicine,has been employed to treat hyperuricemia(hUA)and gout for ***,the bioactive components and underlying mechanisms have not been *** objective of this study was to identify the active components and potential mechanisms of SMW by integrating pharmacological experimentation,serum pharmacochemistry,network pharmacology and molecular ***:hUA rats modelling by high-fat/high-sugar diet and potassium oxonate/adenine oral administration were used to evaluate the pharmacodynamic effects of ***-Q-Exactive-MS/MS was employed to detect the bioactive components present in SMW-containing *** pharmacology and molecular docking were utilized to elucidate the potential targets and underlying ***:SMW effectively ameliorated hUA rats via the inhibition of uric acid(UA)production,promotion of UA excretion,improvement of lipid and glucose metabolic abnormalities,antioxidant,anti-inflammatory and anti-insulin resistance effects.A total of 73 compounds detected in SMW-containing serum were identified as potential active components,with alkaloids,flavonoids,organic acids,and terpenoids emerging as the primary active *** 203 corresponding targets were obtained as SMW anti-hUA/gout targets,which mainly participated in apoptosis,insulin resistance,TNF,PI3k-Akt,hIF-1,NF-κB,MAPk,IL-17 and TLR signaling *** docking indicated that active compounds(***,phellodendrine,quercetin,formononetin,ferulic acid)had superior binding abilities to the key targets(*** carrier family 22 member 12(URAT1),solute carrier family 22 member 6(OAT1),ATP-binding cassette sub-family G member 2(ABCG2),solute carrier family 2,facilitated glucose transporter member 9(GLUT9),xanthine dehydrogenase/oxidase(XDh),transcription factor p65(RELA),toll-like receptor 4(TLR4),prostaglandin G/h synthase 2(PTGS2),caspase-3(CASP3),insulin(INS)).Conclusion:S

关键词： hyperuricemia network pharmacology serum pharmacochemistry Simiaowan UPLC-Q-Exactive-MS/MS

Microbiota or short-chain fatty acids: which regulates diabetes?

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Cellular & Molecular Immunology 2018年第2期15卷 88-91页

作者： chang h kim Department of Comparative Pathobiology and Biological Sciences Laboratory of Immunology and HematopoiesisWeldon School of Biomedical EngineeringPurdue Institute of InflammationImmunology and Infectious DiseasesPurdue Center for Cancer ResearchPurdue UniversityWest Lafayette47907INUSA

Diabetes mellitus,with sustained high-sugar levels in the blood,has been steadily rising in prevalence *** 12–14%of the US population has been diagnosed with diabetes in recent years.1 One major reason for the rise of diabetes is dietary *** consumption of processed carbohydrates with inadequate consumption of dietary fiber(DF)has been recognized as a major risk factor for diabetes,as hypothesized several decades ago by Trowell.

关键词： diabetes sustained dietary

Complex regulatory effects of gut microbial short-chain fatty acids on immune tolerance and autoimmunity

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Cellular & Molecular Immunology 2023年第4期20卷 341-350页

作者： chang h.kim Department of Pathology University of Michigan School of MedicineAnn ArborMI48109USA Mary h.Weiser Food Allergy Center Center for Gastrointestinal Researchand Rogel Center for Can

Immune tolerance deletes or suppresses autoreactive lymphocytes and is established at multiple levels during the development,activation and effector phases of T and B *** mechanisms are cell-intrinsically programmed and critical in preventing autoimmune *** have witnessed the existence of another type of immune tolerance mechanism that is shaped by lifestyle choices,such as diet,microbiome and microbial ***-chain fatty acids(SCFAs)are the most abundant microbial metabolites in the colonic lumen and are mainly produced by the microbial fermentation of prebiotics,such as dietary *** review focuses on the preventive and immunomodulatory effects of SCFAs on *** tissue-and disease-specific effects of dietary fiber,SCFAs and SCFA-producing microbes on major types of autoimmune diseases,including type I diabetes,multiple sclerosis,rheumatoid arthritis and lupus,are ***,their key regulatory mechanisms for lymphocyte development,tissue barrier function,host metabolism,immunity,autoantibody production,and inflammatory effector and regulatory lymphocytes are *** shared and differential effects of SCFAs on different types and stages of autoimmune diseases are discussed.

关键词： Short-chain fatty acids Immune tolerance Diabetes mellitus Rheumatoid arthritis Lupus Multiple sclerosis

Control of lymphocyte functions by gut microbiota-derived short-chain fatty acids

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Cellular & Molecular Immunology 2021年第5期18卷 1161-1171页

作者： chang h.kim Department of Pathology and Mary h.Weiser Food Allergy Center University of Michigan School of MedicineAnn ArborMIUSA

A mounting body of evidence indicates that dietary fiber(DF)metabolites produced by commensal bacteria play essential roles in balancing the immune ***,considered nonessential nutrients in the past,is now considered to be necessary to maintain adequate levels of immunity and suppress inflammatory and allergic ***-chain fatty acids(SCFAs),such as acetate,propionate,and butyrate,are the major DF metabolites and mostly produced by specialized commensal bacteria that are capable of breaking down DF into simpler saccharides and further metabolizing the saccharides into *** act on many cell types to regulate a number of important biological processes,including host metabolism,intestinal functions,and immunity *** review specifically highlights the regulatory functions of DF and SCFAs in the immune system with a focus on major innate and adaptive *** information regarding how SCFAs regulate innate lymphoid cells,T helper cells,cytotoxic T cells,and B cells and how these functions impact immunity,inflammation,and allergic responses are discussed.

关键词： Microbiota Dietary fiber Short-chain fatty acids Innate lymphoid cells B cells Th1 Th17 Tregs CD8 Microbial metabolites

River Morphology and River Channel changes

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Transactions of Tianjin University 2008年第4期14卷 254-262页

作者： chang howard h Civil and Environmental Engineering San Diego State University

River morphology has been a subject of great challenge to scientists and engineers who recognize that any effort with regard to river engineering must be based on a proper understanding of the morphological features involved and the responses to the imposed changes. In this paper, an overview of river morphology is presented from the geomorphic viewpoint. Included in the scope are the regime concept, river channel classification, thresholds in river morphology, and geomorphic analysis of river responses. Analytical approach to river morphology based on the physical principles for the hydraulics of flow and sediment transport processes is also presented. The application of analytical river morphology is demonstrated by an example. Modeling is the modern technique to determine both short-term and long-term river channel responses to any change in the environment. The physical foundation of fluvial process-response must be applied in formatting a mathematical model. A brief introduction of the mathematical model FLUVIAL-12 is described.

关键词： river morphology sediment transport river types mathematical model

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FLOW　INJECTION　SPECTROPhOTOMETRIC　DETERMINATION　OF　VITAMIN　B_1　AND　VITAMIN　B_2　IN　MULTIVITAMIN

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Chinese Chemical Letters 1995年第8期6卷 705-706页

作者： chang, h Yang, JN Fushun Petr Inst Petrochem Dept Fushun 113001 Peoples R China Liaoning Univ Dept Chem Shenyang 110036 Peoples R China

Vitamin B1 reacts with diazo-aminobenzene sulfonic acid to form a red complex in a basic mcdium and there is absorption of vitamin B2 at 440 nm. A flow injection lspectrophotometric determination of the two medicaments is described based on these *** method was simple and a high selecuivity and sampling rate of 60 *** dynamic linear ranges were 0-100 μg ml-1 of vitamin B1 and 0-80 μ g ml-1 of vitamin B2,*** relative standard deviation was 0.2881%(n=10)for vitamin B1.

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Endoscopic foregut surgery and interventions:The future is *** state-of-the-art and my personal journey

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World Journal of Gastroenterology 2019年第1期25卷 1-41页

作者： kenneth J chang h.h.Chao Comprehensive Digestive Disease Center University of CaliforniaIrvine Medical CenterOrangeCA 92868United States

In this paper, I reviewed the emerging field of endoscopic surgery and present data supporting the contention that endoscopy can now be used to treat many foregut diseases that have been traditionally treated surgically. Within each topic,the content will progress as follows: "lessons learned", "technical considerations"and "future opportunities". Lessons learned will provide a brief background and update on the most current literature. Technical considerations will include my personal experience, including tips and tricks that I have learned over the ***, future opportunities will address current unmet needs and potential new areas of development. The foregut is defined as "the upper part of the embryonic alimentary canal from which the pharynx, esophagus, lung, stomach, liver,pancreas, and part of the duodenum develop". Foregut surgery is well established in treating conditions such as gastroesophageal reflux disease(GERD), achalasia, esophageal diverticula, Barrett's esophagus(BE) and esophageal cancer, stomach cancer, gastric-outlet obstruction, and obesity. Over the past decade, remarkable progress in interventional endoscopy has culminated in the conceptualization and practice of endoscopic foregut surgery for various clinical conditions summarized in this paper. Regarding GERD, there are now several technologies available to effectively treat it and potentially eliminate symptoms, and the need for long-term treatment with proton pump *** the first time, fundoplication can be performed without the need for open or laparoscopic surgery. Long-term data going out 5-10 years are now emerging showing extended durability. In respect to achalasia, per-oral endoscopic myotomy(POEM) which was developed in Japan, has become an alternative to the traditional heller's myotomy. Recent meta-analysis show that POEM may have better results than heller, but the issue of post-POEM GERD still needs to be addressed. There is now a resurgence of endoscopic tre

关键词： Endoscopy Foregut diseases Gastroesophageal reflux disease Endoscopic sleeve gastroplasty Endoscopic submucosal dissection Per-oral endoscopic myotomy Endo-hepatology