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Is atmospheric oxidation capacity better in indicating tropospheric O_(3) formation?

Frontiers of Environmental Science & Engineering 2022年第5期16卷 127-133页

作者： Peng Wang Shengqiang Zhu Mihalis Vrekoussis guy pbrasseur Shuxiao Wang Hongliang Zhang Department of Atmospheric and Oceanic Sciences Fudan UniversityShanghai 200438China IRDR ICoE on Risk Interconnectivity and Governance on Weather/Climate Extremes Impact and Public Health Fudan UniversityShanghai 200438China Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention Department of Environmental Science&EngineeringFudan UniversityShanghai 200438China Institute of Environmental Physics University of BremenBremen D-28359Germany Climate and Atmosphere Research Center(CARE-C) the Cyprus InstituteNicosia 27456Cyprus Max Planck Institute for Meteorology Hamburg 20146Germany National Center for Atmospheric Research BoulderCO 80307USA State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex Beijing 100084China Institute of Eco-Chongming(IEC) Shanghai 202162China

Tropospheric ozone(O_(3))concentration is increasing in China along with dramatic changes in precursor emissions and meteorological conditions,adversely affecting human health and ecosystems.O_(3) is formed from the complex nonlinear photochemical reactions from nitrogen oxides(NOx=NO+NO_(2))and volatile organic compounds(VOCs).Although the mechanism of O_(3) formation is rather clear,describing and analyzing its changes and formation potential at fine spatial and temporal resolution is still a challenge *** this study,we briefly summarized and evaluated different approaches that indicate O_(3) formation *** identify that atmospheric oxidation capacity(AOC)is a better indicator of photochemical reactions leading to the formation of O_(3) and other secondary *** show that AOC has a prominent positive relationship to O_(3) in the major city clusters in China,with a goodness of fit(R^(2))up to *** outcome provides a novel perspective in characterizing O_(3) formation and has significant implications for formulating control strategies of secondary pollutants.

关键词： O_(3) AOC O_(3) formation regime

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