检索结果-南通市图书馆

Advances in ice avalanches on the Tibetan Plateau

在线全文

学校读者我要写书评

暂无评论

Journal of Mountain Science 2024年第6期21卷 1814-1829页

作者： TANG Minggao li Guang ZHAO Huanle XU Qiang WU Guangjian yang Wei guo Daojing State Key Laboratory of Geohazard Prevention and Geoenvironment Protection Chengdu University of TechnologyChengdu 610059China College of Environment and Civil Engineering Chengdu University of TechnologyChengdu 610059China Institute of Tibetan Plateau Research Chinese Academy of SciencesBeijing 100101China

As some of the greatest natural disasters in the cryosphere,ice avalanches(IAs)seriously threaten lives and cause catastrophic damage to the resource environment,but a comprehensive overview of the state of knowledge on IAs remains *** summarized 63 IAs on the Tibetan Plateau(TP)since the 20th century,of which,over 20 IAs occurred after the 21st *** distributions of IAs are mainly concentrated in the southeastern and northwestern TP,and the occurrence time of IAs is mostly concentrated from July to *** highlight recent advances in mechanical properties and genetic mechanisms of IAs and emphasize that temperature,rainfall,and seismicity are the inducing *** failure modes of IAs are summarized into 6 categories by examples:slip pulling type,slip toppling type,slip breaking type,water level collapse type,cave roof collapse type,and wedge failure ***,we deliver recommendations concerning the risk assessment and prediction of *** results provide important scientific value for addressing climate change and resisting glacier-related hazards.

关键词： Ice avalanche Global warming Genetic mechanism Risk assessment Tibetan Plateau

Dual-additives enable stable electrode-electrolyte interfaces for long life li-SPAN batteries

在线全文

学校读者我要写书评

暂无评论

Chinese Chemical Letters 2024年第5期35卷 459-465页

作者： Zhenqiang guo Huicong yang Qian Wei Shengjun Xu Guangjian Hu Shuo Bai Feng li School of Materials Science and Engineering University of Science and Technology of ChinaShenyang 110016China Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016China Department of Biochemistry and Molecular Biology College of Life ScienceChina Medical UniversityShenyang 110122China Dalian National Laboratory for Clean Energy Dalian 116023China Shenyang King Power Technology Co. Ltd.Shenyang 110016China

Sulfurized polyacrylonitrile(SPAN)is proposed as a promising cathode material for lithium sulfur ***,the continuous side reactions at the electrolyte-electrode interfaces as well as the slow redox kinetics of SPAN cathode deteriorate the electrochemical *** this study,an electrolyte with dual-additives comprising 2-fluoropyridine(2-FP)and lithium difluorobis(oxalato)phosphate(liDFBOP)was used to improve the performance of li||SPAN cells.2-FP has a lower lowest occupied molecular orbital energy than that of the solvents in the electrolyte,leading to its prior reduction.A liF-rich film can be formed on the electrode,effectively improving the stability of the electrolyte-electrode interfaces and prolonging the ***,liDFBOP could form an electrolyte-electrode interface film containing a large amount of li_(x)PO_(y)F_(z) species,compensating for the kinetic deterioration caused by the lower ionic conductive of liF formed at the electrolyte-electrode ***,an electrode-interface film with good chemical stability and high li^(+) transport was established by liF and li_(x)PO_(y)F_(z)-rich *** li||SPAN cell with the electrolyte containing dual-additives demonstrates an excellent capacity retention of 97.5%after 200 cycles at 1.0 C,25℃,comparing to 56.2%capacity retention without ***,the rate capacities of cells with dual-additives can reach 1128.1 mAh/g at 5 C,comparing to only 813.5 mAh/g using electrolyte without *** results shown that the dual-additives in electrolyte provide a promising strategy for practical application of lithium sulfur batteries with SPAN cathodes.

关键词： Sulfurized polyacrylonitrile lithium metal Interface film 2-Fluoropyridine Difluorobis(oxalato)phosphate

Reconfigurable logic and in-sensor encryption operations in an asymmetrically tunable van der Waals heterostructure

在线全文

学校读者我要写书评

暂无评论

Nano Research 2024年第4期17卷 3113-3119页

作者： Fan Gong Wenjie Deng Yi Wu Fengming liu Yihao guo Zelin Che Jingjie li Jingzhen li yang Chai Yongzhe Zhang Key Laboratory of Optoelectronics Technology of Education Ministry of China Faculty of Information TechnologyBeijing University of TechnologyBeijing 100124China Key Laboratory of Advanced Functional Materials Ministry of EducationFaculty of Materials and ManufacturingBeijing University of TechnologyBeijing 100124China Department of Applied Physics Hong Kong Polytechnic UniversityKowloonHong KongChina

Reconfigurable devices can be used to achieve multiple logic operation and intelligent optical sensing with low power consumption,which is promising candidates for new generation electronic and optoelectronic integrated ***,the versatility is still limited and need to be extended by the device architectures ***,we report an asymmetrically gate two-dimensional(2D)van der Waals heterostructure with hybrid dielectric layer SiO_(2)/hexagonal boron nitride(h-BN),which enable rich function including reconfigurable logic operation and in-sensor information encryption enabled by both volatile and non-volatile optoelectrical *** the partial gate is grounded,the non-volatile light assisted electrostatic doping endowed partially reconfigurable doping between n-type and p-type,which allow the switching of logic XOR and not implication(NIMP).When the global gate is grounded,additionally taking the optical signal as another input signal,logic AND and OR is realized by combined regulation of the light and localized gate *** on the high on/off current ratio approaching 105 and reliable&switchable logic gate,in-sensor information encryption and decryption is demonstrated by manipulating the logic ***,these results provide strong extension for current reconfigurable electronic and optoelectronic devices.

关键词： in-sensor encryption reconfigurable logic van der Waals heterostructure asymmetrical tunable architecture

In situ Preparation and Visible-light-driven Photocatalytic Degradation Performance of Nano 3C-SiC@Multilayer Graphene Oxide Heterostructure

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chemical Research in Chinese Universities 2024年第3期40卷 536-547页

作者： yang Xiaodan guo Ziqi XU Yichen li Ziliang ZHOU yangtao yang Zhenming ZHOU Zishuai GAO Yong ZHANG Jinsong Shenyang National Laboratory for Materials Science Institute of Metal ResearchChinese Academy of SciencesShenyang 110016P.R.China Nano Science and Technology Institute University of Science and Technology of ChinaSuzhou 215123P.R.China Shenyang SCIENCREAT Chemicals Co. Ltd.Shenyang 110144P.R.China School of Materials Science and Engineering Northeastern UniversityShenyang 110819P.R.China

Nano 3C-SiC@multilayer graphene oxide(NS@MGO)heterostructure was in situ prepared by carbothermal reduction of pyrolyzed precursor composed of highly dispersed cured phenolic resin and silicon dioxide derived from tetraethyl *** heterojunction interface,number of layers of MGO,and defect content in graphene are the three most important factors for promoting photocatalytic *** contact between 3C-SiC nanograins and MGO layers facilitates the photogenerated electrons to migrate across the heterojunction interface and avoid the formation of SiO_(2) nanolayers on the surface of SiC *** number of MGO layers is supposed to be less than ten instead of over-thick *** concentrations of oxygenated components,considered the defect contents,decrease with the increase of sintering temperature for NS@MGO 0.175-T-150,and relative carbon content in the multilayer graphene *** to the heterostructures,properties,and photocatalytic reaction performance of the NS@MGO materials,the highest photocatalytic kinetic rate constant of 0.00891/min for NS@MGO 0.175-1500-150 shows that the significant enhancement in photocatalytic degradation activity under visible light(>420 nm)irradiation is ascribed to the advantageous synergistic effects between the nano 3C-SiC particles and the direct contact multilayer graphene oxide with appropriate layers and sufficient oxygen content of 3.51%(atomic fraction)in MGO.

关键词： Photocatalysis Multilayer graphene oxide Nano 3C-SiC Visiblelight degradation

Isomeric fluorescence sensors for wide range detection of ionizing radiations

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Defence Technology（防务技术） 2024年第4期34卷 247-257页

作者： Jimin Han Tianyu yang li yang Yuanjian li State Key Laboratory of Explosion Science and Technology of China Beijing Institute of TechnologyBeijing 100081China Chongqing Innovation Center Beijing Institute of TechnologyChongqing 401120China

In order to achieve a wider range of ionizing radiations detection,novel fluorescence sensing materials have been developed that utilize the fluorescence enhancement phenomenon caused by the intramolecular photoinduced electron transfer(PET)*** perylene diimide isomers PDI-P and PDI-B were designed and synthesized,and their molecular structures were characterized by high-resolution Fourier transform mass spectrometry(HRMS),nuclear magnetic resonance hydrogen and carbon spectroscopy(~1H and~(13)C NMR).The interaction between ionizing radiation and fluorescent molecules was simulated by HCl *** results show that combining PDIs and HCl can improve fluorescence through the retro-PET *** the similarities in chemical structures,the fluorescent enhancement multiple of PDI-B with aromatic amine as electron donor is much higher than that of PDI-P with alkyl *** the direct irradiation experiments of ionizing radiation,the emission enhancement multiples of PDI-P and PDI-B are 2.01 and 45.4,***,density functional theory(DFT)and time-dependent density functional theory(TDDFT)calculations indicate that the HOMO and HOMO-1 energy ranges of PDI-P and PDI-B are 0.54 e V and 1.13 e V,respectively.A wider energy range has a stronger driving force on electrons,which is conducive to fluorescence *** femtosecond transient absorption spectroscopy(fs-TAS)and transient fluorescence spectroscopy(TFS)tests show that PDI-B has shorter charge separation lifetime and higher electron transfer rate *** both isomers can significantly reduce LOD during PET process,PDI-B with aromatic amine has a wider detection range of 0.118—240 Gy due to its larger emission enhancement,which is a leap of three orders of *** breaks through the detection range of gamma radiation reported in existing studies,and provides theoretical support for the further study of sensitive and effective new materials for ionizing radiation dete

关键词： Perylene imide Intramolecular PET Ionizing radiation detection Fluorescence sensor Isomers

Machine Learning-Based Temperature and Wind Forecasts in the Zhangjiakou Competition Zone during the Beijing 2022 Winter Olympic Games

在线全文

学校读者我要写书评

暂无评论

Journal of Meteorological Research 2024年第4期38卷 664-679页

作者： Zhuo SUN Jiangbo li Ruiqiang guo Yiran ZHANG Gang ZHU Xiaoliang yang China Meteorological Administration Xiong'an Atmospheric Boundary Layer Key Laboratory Xiong'an New Area 071800 Hebei Key Laboratory of Meteorology and Ecological Environment Shijiazhuang 050021 Hebei Meteorological Observatory Shijiazhuang 050021 College of Computer and Cyber Security Hebei Normal UniversityShijiazhuang 050024

Weather forecasting for the Zhangjiakou competition zone of the Beijing 2022 Winter Olympic Games is a challenging task due to its complex *** weather prediction models generally perform poorly for cold air pools and winds over complex terrains,due to their low spatiotemporal resolution and limitations in the description of dynamics,thermodynamics,and microphysics in mountainous *** study proposes an ensemble-learning model,named ENSL,for surface temperature and wind forecasts at the venues of the Zhangjiakou competition zone,by integrating five individual models—linear regression,random forest,gradient boosting decision tree,support vector machine,and artificial neural network(ANN),with a ridge regression as meta *** ENSL employs predictors from the high-resolution ECMWF model forecast(ECMWF-HRES) data and topography data,and targets from automatic weather station *** categories of predictors(synoptic-pattern related fields,surface element fields,terrain,and temporal features) are fed into *** results demonstrate that ENSL achieves better performance and generalization than individual *** root-mean-square error(RMSE) for the temperature and wind speed predictions is reduced by 48.2% and 28.5%,respectively,relative to *** the gust speed,the performance of ENSL is consistent with ANN(best individual model) in the whole dataset,whereas ENSL outperforms on extreme gust samples(42.7% compared with 38.7% obtained by ECMWF-HRES in terms of RMSE reduction).Sensitivity analysis of predictors in the four categories shows that ENSL fits their feature importance rankings and physical explanations effectively.

关键词： machine learning ensemble learning post-processing cold air pools mountain Beijing 2022 Winter Olympic Games

Framework and Key Technologies of Human-machine Hybrid-augmented Intelligence System for Large-scale Power Grid Dispatching and Control

在线全文

学校读者我要写书评

暂无评论

CSEE Journal of Power and Energy Systems 2024年第1期10卷 1-12页

作者： Shixiong Fan Jianbo guo Shicong Ma lixin li guozheng Wang Haotian Xu Jin yang Zening Zhao China Electric Power Research Institute Beijing 100192China the Beijing Huairou Laboratory Beijing 101400China School of Engineering the University of GlasgowGlasgow G128QQUK

With integration of large-scale renewable energy,new controllable devices,and required reinforcement of power grids,modern power systems have typical characteristics such as uncertainty,vulnerability and openness,which makes operation and control of power grids face severe security *** of artificial intelligence(AI)technologies represented by machine learning in power grid regulation is limited by reliability,interpretability and generalization ability of complex *** of hybrid-augmented intelligence(HAI)based on human-machine collaboration(HMC)is a pivotal direction for future development of AI technology in this *** on characteristics of applications in power grid regulation,this paper discusses system architecture and key technologies of human-machine hybrid-augmented intelligence(HHI)system for large-scale power grid dispatching and control(PGDC).First,theory and application scenarios of HHI are introduced and analyzed;then physical and functional architectures of HHI system and human-machine collaborative regulation process are *** technologies are discussed to achieve a thorough integration of human/machine ***,state-of-theart and future development of HHI in power grid regulation are summarized,aiming to efficiently improve the intelligent level of power grid regulation in a human-machine interactive and collaborative way.

关键词： Artificial intelligence human-machine collaborative control human-machine hy brid intelligence optimization and evolution power grid dispatching and control

Enhanced population of excited single state strategy:Irradiation and ultrasound dual-response and host tumor-driven nanosensitizers construction in triple synergistic therapy

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第6期17卷 5501-5511页

作者： Yaning li Mengyan Tian Tianyue yang Jiayu Cao Hongli Chen Jun guo Pai liu Yi liu State Key Laboratory of Separation Membranes and Membrane Processes School of Materials Science and EngineeringTiangong UniversityTianjin 300387China State Key Laboratory of Separation Membranes and Membrane Processes School of ChemistryTiangong UniversityTianjin 300387China State Key Laboratory of Separation Membranes and Membrane Processes School of Life ScienceTiangong UniversityTianjin 300387China State Key Laboratory of Separation Membrane and Membrane Process&Tianjin Key Laboratory of Green Chemical Technology and Process Engineering School of ChemistryTiangong UniversityTianjin 300387China School of Chemical and Environmental Engineering Wuhan Polytechnic UniversityWuhan 430023China Cangzhou Institute of Tiangong University Cangzhou 061000China

Phototheranostics is an emerging field in synergistic antitumor therapy in which irradiation and sensitizers are combined to produce reactive oxygen species(ROS),bio-images,and high *** of these are arrived from the energy of sensitizers,which located in excited single state(S_(1)).Undeniably,the decentralization of the S_(1)population indirectly decreases the effect of each individual *** this study,a strategy was proposed for enhancing the S_(1)population,and a sensitizer with mitochondrial targeting property,1,4-indolyl iodinated pyrrolo[3,2-b]pyrrole derivative(2I-TPIS),was assembled into adenosine triphosphate(ATP)-responsive nanoparticles(DPA-2I NPs)to achieve dual responses to irradiation and ultrasonication(US)for application to photo-sonodynamic therapy(PSDT).Compared with monotherapies,2I-TPIS generated more ROS in PSDT,inducing mitochondrial autophagy and apoptosis,which in turn triggered immunogenic cell death(ICD).Subsequently,DPA-2I NPs were constructed and self-assembled with the chemotherapeutic agents DPA-Cd and 2I-TPIS to achieve a triple synergistic strategy involving chemotherapy(CT)and ***-2I NPs exhibited absolute sensitization,intra-tumoral overexpression of ATP,and ***,the biosafety and potent antitumor efficiency of the DPA-2I NP-based“PSDT+CT”therapy were revealed using a 4T1 tumor *** study results provide insights into the design of sensitizers possessing a sufficient S_(1)population and a highly efficient tumor ablation capacity derived from molecular structural modulation,further enabling triple synergistic antitumor therapies,and expanding the clinical application of sensitizers.

关键词： triphosphate(ATP)-activated nano-sensitizers photo-sonodynamic therapy aggregation-induced emission enhanced excited state population

Two imprinted genes primed by DEMETER in the central cell and activated by WRKY10 in the endosperm

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Genetics and Genomics 2024年第8期51卷 855-865页

作者： Ke yang Yuling Tang Yue li Wenbin guo Zhengdao Hu Xuanpeng Wang Frédéric Berger Jing li College of life Science and Technology Huazhong Agricultural UniversityWuhanHubei 430070China Sanya Institute of Breeding and Multiplication Hainan UniversitySanyaHainan 572025China School of Tropical Agriculture and Forestry Hainan UniversityHaikouHainan 570228China Hainan Yazhou Bay Seed Laboratory SanyaHainan 572025China Gregor Mendel Institute Austrian Academy of SciencesVienna BioCenter1030 ViennaAustria

The early development of the endosperm is crucial for balancing the allocation of maternal nutrients to *** process is believed to be evolutionarily associated with genomic imprinting,resulting in parentally biased allelic gene *** Fertilization Independent Seed(FIS)genes,the number of imprinted genes involved in early endosperm development and seed size determination remains *** study introduces early endosperm-expressed HAIKU(IKU)downstream Candidate F-box 1(ICF1)and ICF2 as maternally expressed imprinted genes(MEGs)in Arabidopsis *** these genes are also demethylated by DEMETER(DME)in the central cell,their activation differs from the direct DME-mediated activation seen in classical MEGs such as the FIS ***,ICF maternal alleles carry pre-established hypomethylation in their promoters,priming them for activation by the WRKY10 transcription factor in the *** the contrary,paternal alleles are predominantly suppressed by CG ***,we find that ICF genes partially contribute to the small seed size observed in iku *** discovery reveals a two-step regulatory mechanism that highlights the important role of conventional transcription factors in the activation of imprinted genes,which was previously not fully ***,the mechanism provides a new dimension to understand the transcriptional regulation of imprinting in plant reproduction and development.

关键词： Imprinting Epigenetics DNAmethylation Seedsize Endosperm