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Aggregate 2024年第1期5卷 95-114页

作者： Yaxuan Wang Ting xu Kun Liu Meng Zhang xu-Min Cai Chuanling Si State Key Laboratory of Biobased Fiber Manufacturing Technology Tianjin Key Laboratory of Pulp and PaperTianjin University of Science and TechnologyTianjinChina Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Chemical EngineeringNanjing Forestry UniversityNanjingChina

Supercapacitors exhibit considerable potential as energy storage devices due to their high power density,fast charging and discharging abilities,long cycle life,and *** the increasing environmental concerns associated with synthetic compounds,the use of environment friendly biopolymers to replace conventional petroleum-based materials has been widely ***-based materials are biodegradable,renewable,environment friendly and *** unique hierarchical nanostructure,excellent mechanical properties and hydrophilicity allow them to be used to create functional conductive materials with precisely controlled structures and different *** this review,the latest development of biomass-based supercapacitor materials is reviewed and *** paper describes the physical and chemical properties of various biopolymers and their impact on supercapacitors,as well as the classification and basic principles of ***,a comprehensive discussion is presented on the utilization of biomass-based materials in supercapacitors and their recent applications across a range of supercapacitor ***,an overview of the future prospects and challenges pertaining to the utilization of biomass-based materials in supercapacitors is provided.

关键词： biomass electrodes electrolyte energy storage supercapacitor

Effect of proppant sizes and injection modes on proppant transportation and distribution in the tortuous fracture model

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Particuology 2024年第1期84卷 261-280页

作者： Jun Li xu Han Siyuan He Mingyi Wu Xin Huang Nianyin Li State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500China Chongqing Industry Polytechnic college Chongqing401120China Sichuan Particles Energy and Technology Co. LtdChengdu611630China engineering Technology Research Institute of PetroChina Southwest Oil and Gas Field Company Chengdu610017China

Particle-fluid transport and placement mechanism in tortuous fracture played a crucial role in uncon-ventional ***,most studies focused on mono-size proppant with fluid transport pro-cesses in tortuous ***,the mixture-size proppant with fluid movement mechanism in tortuous fracture was still ***,this study designed and applied a series of experiments with a physical analog model of a tortuous fracture with 120°and 90°-angled bends and combined high-speed camera-based *** experimental system was used to track different-mixture-sized proppant particle motion trajectories for a series of proppant injection schemes;The following conclu-sions were drawn from this study:*** pile-up processes mechanism in all investigated schemes were similar and could be reduced to four main *** packing structure at both sides of the fracture wall had different variation rates,which were controlled by the mix ratio(change from 1∶1-1∶5)of proppant *** new packing patterns,such as Zebra Stripe,had occurred,controlled by the different proppant injection ***-sized mono-proppant(30/50 mesh)had the highest transport efficiency in the tortuous fracture,followed by the mixed-sized multi-proppant(10/20 mesh:30/50 mesh),large-sized proppant(10/20 mesh)was the *** optimized alternating in-jection mode was recommended as injecting small-sized proppant first(30/50 mesh)and followed by mixed-sized multi-proppant(10/20 mesh:30/50 mesh),which could contribute to obtaining the optimal both proppant packing height and travel distance in tortuous *** correlations were devel-oped for predicting the proppant packing height and transportation distance.

关键词： Tortuous fracture model Mixed-sized proppant Multi-sized proppant injection mode Proppant motion and distribution Packing mechanism

Ti_(3)C_(2)T_(x) MXene/carbon composites for advanced supercapacitors:Synthesis,progress,and perspectives

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Carbon Energy 2024年第2期6卷 113-142页

作者： Yanqing Cai Xinggang Chen Ying xu Yalin Zhang Huijun Liu Hongjuan Zhang Jing Tang college of Materials Science and engineering North China University of Science and TechnologyTangshanChina Hebei Iron and Steel Laboratory North China University of Science and TechnologyTangshanChina Songshan Lake Materials Laboratory DongguanChina Shanghai Key Laboratory of Green Chemistry and Chemical Processes School of Chemistry and Molecular EngineeringEast China Normal UniversityShanghaiChina State Key Laboratory of petroleum Molecular and Process engineering(SKLPMPE) Sinopec Research Institute of Petroleum Processing Co.Ltd.BeijingChina Institute of Eco-Chongming ShanghaiChina

MXenes are a family of two-dimensional(2D)layered transition metal carbides/nitrides that show promising potential for energy storage applications due to their high-specific surface areas,excellent electron conductivity,good hydrophilicity,and tunable *** various types of MXenes,Ti_(3)C_(2)T_(x) is the most widely studied for use in capacitive energy storage applications,especially in supercapacitors(SCs).However,the stacking and oxidation of MXene sheets inevitably lead to a significant loss of electrochemically active *** overcome such challenges,carbon materials are frequently incorporated into MXenes to enhance their electrochemical *** review introduces the common strategies used for synthesizing Ti_(3)C_(2)T_(x),followed by a comprehensive overview of recent developments in Ti_(3)C_(2)T_(x)/carbon composites as electrode materials for ***_(3)C_(2)T_(x)/carbon composites are categorized based on the dimensions of carbons,including 0D carbon dots,1D carbon nanotubes and fibers,2D graphene,and 3D carbon materials(activated carbon,polymer-derived carbon,etc.).Finally,this review also provides a perspective on developing novel MXenes/carbon composites as electrodes for application in SCs.

关键词： electrochemical performance MXene/carbon composites supercapacitors

Study on metal recovery process and kinetics of oxidative leaching from spent LiFePO_(4)Li-batteries

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Chinese Journal of Chemical engineering 2024年第4期68卷 94-102页

作者： Xiaoming Zhang Wen Xie Xiaolei Zhou Wenjie Zhang Jiawei Wen Xin Wang Guoyong Huang Shengming xu college of New Energy and Materials China University of PetroleumBeijing 102249China State Key Laboratory of Heavy Oil Processing College of Chemical EngineeringChina University of PetroleumBeijing 102249China Beijing Spacecrafts Beijing 100094China Ganfeng Lithium Group Co. Ltd.Xinyu 338000China Institute of Nuclear and New Energy Technology Tsinghua UniversityBeijing 100084China Beijing Key Laboratory of Fine Ceramics Tsinghua UniversityBeijing 100084China

A green environmental protection and enhanced leaching process was proposed to recover all elements from spent lithium iron phosphate(LiFePO_(4)) lithium *** order to reduce the influence of Al impurity in the recovery process,NaOH was used to remove *** impurity removal,the spent LiFePO_(4) cathode material was used as raw material under the H_(2)SO_(4) system,and the pressure oxidation leaching process was adopted to achieve the preferential leaching of *** E-pH diagram of the Fe-P-Al-H_(2)O system can determine the stable region of each element in the recovery process of spent LiFePO_(4)*** the optimal conditions(500 r·min^(-1),15 h,363.15 K,0.4 MPa,the liquid-solid ratio was 4:1 ml·g^(-1)and the acid-material ratio was 0.29),the leaching rate of Li was 99.24%,Fe,Al,and Ti were 0.10%,2.07%,and 0.03%,*** Fe and P were precipitated and recovered as FePO_(4)·2H_(2)*** kinetic analysis shows that the process of high-pressure acid leaching of spent LiFePO_(4) materials depends on the surface chemical *** the life cycle assessment(LCA)of the spent LiFePO_(4) whole recovery process,eight midpoint impact categories were selected to assess the impact of recovery *** results can provide basic environmental information on production process for recycling industry.

关键词： Spent LiFePO_(4)Li-batteries Oxidative leaching Kinetic study Life cycle assessment

Sn-decorated CeO_(2) with different morphologies for direct dehydrogenation of ethylbenzene

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Journal of Rare Earths 2024年第1期42卷 102-109,I0004页

作者： Kai Zhang Guoju Cui Mengzhen Yuan Huiwen Huang Ning Li Jiale xu Guowei Wang Chunyi Li State Key Laboratory of Heavy Oil Processing China University of Petroleum(East China)Qingdao266580China Petrochemical Plant of Sinopec Shengli Oilfield Company Dongying257237China college of Chemical and Biological engineering Shandong University of Science and TechnologyQingdao266590China

Three Sn-decorated ceria catalysts with various morphologies(rods,particles,and cubes)were prepared and applied to the direct dehydrogenation of ***-technology characterizations,including X-ray photoelectro n spectroscopy(XPS),H_(2)-tempe rature programmed reduction(H_(2)-TPR),and Raman spectroscopy,prove that the oxygen vacancies are the active sites for ethylbenzene dehydrogenation,which can be regulated by engineering CeO_(2) morphology and enhanced via introducing metal *** the results of activity test,the catalytic activities for ethylbenzene dehydrogenation over different samples are closely dependent on the amount of oxygen *** reduced Sn-decorated CeO_(2) catalyst with nanoparticles morphology exhibits better dehydrogenation performance than the other two studied catalysts at 600℃.This work provides an effective approach to regulate the active oxygen vacancies and further enhance the dehydrogenation activities through engineering the surface morphology of the catalyst and introducing suitable additives.

关键词： Ethylbenzene dehydrogenation CeO_(2) Sn Morphology Oxygen vacancy Rare earths

Analysis of Maximum Liquid Carrying Capacity Based on Conventional Tubing Plunger Gas Lift

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Energy engineering 2024年第6期121卷 1521-1533页

作者： Yanqun Yu Wenhao xu Yahui Huangfu Jinhai Liu Bensheng Wang Kai Liu college of Mechanical and Electronic engineering China University of Petroleum(East China)Qingdao266580China Energy Technology&Services Oil Production Services Company CNOOCTianjin300450China

China’s unconventional gas fields have a large number of low-productivity and low-efficiency wells, many of whichare located in remote and environmentally harsh mountainous areas. To address the long-term stable productionof these gas wells, plunger-lift technology plays an important role. In order to fully understand and accurately graspthe drainage and gas production mechanisms of plunger-lift, a mechanical model of plunger-liquid column uplift inthe plunger-lift process was established, focusing on conventional plunger-lift systems and representative wellboreconfigurations in the Linxing region. The operating casing pressure of the plunger-lift process and the calculationmethod for the maximum daily fluid production rate based on the work regime with the highest fluid recovery ratewere determined. For the first time, the critical flow rate method was proposed as a constraint for the maximumliquid-carrying capacity of the plunger-lift, and liquid-carrying capacity charts for conventional plunger-lift withdifferent casing sizes were developed. The results showed that for 23/8 casing plunger-lift, with a well depth ofshallower than 808 m, the maximum drainage rate was 33 m3/d;for 27/8 casing plunger-lift, with a well depth ofshallower than 742 m, the maximum drainage rate was 50.15 m3/d;for 31/2 casing plunger-lift, with a well depthof shallower than 560 m, the maximum drainage rate was 75.14 m3/d. This research provides a foundation for thescientific selection of plunger-lift technology and serves as a decision-making reference for developing reasonableplunger-lift work regimes.

关键词： Unconventional well conventional tubing string plunger gas lift critical flow rate liquid carry-over chart version

Fracture sealing performance of granular lost circulation materials at elevated temperature:A theoretical and coupled CFD-DEM simulation study

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petroleum Science 2024年第1期21卷 567-581页

作者： Chong Lin Qi-Cong xu Lie-Xiang Han Gao Li Hai He Hong-Ling Zhou Ji-Ping She CCDC Drilling&Production Technology Research Institute Guanghan618300SichuanChina State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Southwest Petroleum UniversityChengdu610500SichuanChina college of Materials Science and engineering Chongqing UniversityChongqing400044China State Key Lab of Oil and Gas Reservoir Geology and Exploitation(Chengdu University of Technology) Chengdu610059SichuanChina college of Energy Chengdu University of TechnologyChengdu610059SichuanChina

Lost circulation is a common downhole problem of drilling in geothermal and high-temperature,high-pressure(HTHP)*** circulation material(LCM)is a regular preventive and remedial measure for lost ***,conventional LCMs seem ineffective in high-temperature *** may be due to the changes in the mechanical properties of LCMs and their sealing performance under high-temperature *** understand how high temperature affects the fracture sealing performance of LCMs,we developed a coupled computational fluid dynamics-discrete element method(CFD-DEM)model to simulate the behavior of granular LCMs in *** summarized the literature on the effects of high temperature on the mechanical properties of LCMs and the rheological properties of drilling *** conducted sensitivity analyses to investigate how changing LCM slurry properties affected the fracture sealing efficiency at increasing *** results show that high temperature reduces the size,strength,and friction coefficient of LCMs as well as the drilling fluid ***,softer,and less frictional LCM particles have lower bridging probability and slower bridging *** particles tend to form dual-particle bridges rather than single-particle *** result in a deeper,tighter,but unstable sealing *** drilling fluid viscosity leads to faster and shallower sealing zones.

关键词： Geothermal well drilling HTHP formationLost circulation material CFD-DEM Fracture sealing

Research on multi-parametric sensors based on multi-mode microfiber

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Optoelectronics Letters 2024年第1期20卷 18-22页

作者： DONG Taiji LIU xu WANG Yunkai GAO Bingkun JIANG Chunlei WANG Xiufang college of Electrical and Information engineering Northeast Petroleum UniversityDaqing 163318China

A multi-parametric sensor based on multi-mode microfiber(MMF)is proposed,utilizing the modal interference between HE11mode and HE12mode in the elongated multi-mode fiber to achieve the temperature and pressure *** this paper,the simulation model of modal interference based on MMF is established and the mechanism of modal interference is *** the different mechanisms of modal response in the fiber at different wavelengths,the temperature was inverted using the offset of wavelengths in the spectrum,and the pressure was measured using the change of light *** independent measurement of temperature and pressure was *** experimental results show that the sensor has a temperature sensitivity of 1.305 nm/℃.In the case of pressure sensing,the sensor shows a sensitivity of-0.163 d Bm/g.

关键词： measurement mode modal

One-pot Synthesis of MoO_(3)/PI Composite with Enhanced Photocatalytic Performance for Oxidative Coupling of Amines to Imines

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China petroleum Processing & Petrochemical Technology 2024年第2期26卷 57-71页

作者： Zhao Wenjie Du Chengxin Song Yu Zhou Yafen Wang Qing Zhou Limei xu Bin Chemical Synthesis and Pollution Control Key Laboratory of Sichuan Province College of Chemistry and Chemical EngineeringChina West Normal UniversityNanchongChina Key Laboratory of Green Chemistry of Sichuan Institutes of Higher Education Sichuan University of Science&EngineeringZigongChina

Organic-inorganic MoO_(3)/PI(MoPI)composites were prepared using a simple one-pot thermal copolymerization *** resulting composites exhibited enhanced photocatalytic activity for the selective oxidation of benzylamine to N-benzylidene benzylamine(N-BDBA)in ambient air under simulated solar light irradiation compared to pristine MoO_(3) or polyimide(PI).In particular,the MoPI composite with a 0.3:1 molar ratio of Mo to melamine,referred to as MoPI-0.3,demonstrated the best performance in the photo-oxidation of benzylamine,achieving a benzylamine conversion of 95%with a N-BDBA selectivity exceeding 99%after 3 h *** enhanced photocatalytic activity of the MoPI-0.3 catalyst was attributed to the formation of a direct Z-scheme heterojunction between MoO_(3) and PI,facilitating more efficient separation of the photoinduced electrons and ***,the MoPI-0.3 composite maintained considerably high activity over four consecutive cycles,highlighting its good stability and ***,the MoPI-0.3 composite could photo-oxidize benzylamine derivatives and heterocyclic amines to their corresponding imines,demonstrating the universal applicability of this composite catalyst.

关键词： MoO3/PI composite photocatalysis amine oxidation imine