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利用XRD、XRF、FT-IR和Rs分析浙江缙云恐龙化石及围岩

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信阳师范学院学报（自然科学版） 2014年第3期27卷 332-336页

作者：刘东亮邓建国彭光照金幸生四川理工学院材料腐蚀与防护四川省重点实验室四川自贡643000 自贡恐龙博物馆四川自贡643013 浙江自然博物馆浙江杭州310014

通过XRF、XRD、FT-IR和RS对产自浙江缙云恐龙骨骼化石和围岩的元素组成、矿物结构和基团特征进行了分析.结果表明:化石中主要元素为钙、磷,钙磷质量比为12.7,围岩中硅、铁、钙、钾和铝含量较高;化石中钙含量是围岩的15倍,磷量为31.9倍,... 详细信息

通过XRF、XRD、FT-IR和RS对产自浙江缙云恐龙骨骼化石和围岩的元素组成、矿物结构和基团特征进行了分析.结果表明:化石中主要元素为钙、磷,钙磷质量比为12.7,围岩中硅、铁、钙、钾和铝含量较高;化石中钙含量是围岩的15倍,磷量为31.9倍,围岩中铁量是化石的8.5倍,硅含量是化石的11.25倍,钾含量是化石的45.6倍,铝含量是化石的7.36倍;恐龙化石的主要成分为羟基碳氟磷酸钙与碳酸钙,分别占63.9%和36.1%,围岩主要成分二氧化硅约为36.9%,其余为碳酸钙和硅酸盐的混合物.红外与拉曼峰表明,化石中存在羟基碳氟磷酸钙、方解石及少量有机物;有机物的存在表明,化石未被完全石化,且恐龙死亡后初始阶段埋藏在缺氧环境中;而围岩中则为石英、方解石和有机物.

关键词：恐龙骨骼化石围岩光谱分析矿物成分

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Multi boron-doping effects in hard carbon toward enhanced sodium ion storage

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Journal of Energy Chemistry 2025年第1期100卷 730-738页

作者： peng Zheng Wang Zhou Ying Mo Biao Zheng Miaomiao Han Qin Zhong Wenwen Yang peng Gao Lezhi Yang Jilei Liu College of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology for Clean Energy Hunan Province Key Laboratory for Advanced Carbon Materials and Applied Technology Hunan University Greater Bay Area Institute for Innovation Hunan University Changsha Research Institute of Mining & Metallurgy Co. LTD.

Hard carbon （HC） has been considered as promising anode material for sodium-ion batteries （SIBs）.The optimization of hard carbon’s microstructure and solid electrolyte interface （SEI） property are demonstrated effective in enhancing the Na+storage capability,however,a one-step regulation strategy to achieve simultaneous multi-scale structures optimization is highly ***,we have systematically investigated the effects of boron doping on hard carbon’s microstructure and interface chemistry.A variety of structure characterizations show that appropriate amount of boron doping can increase the size of closed pores via rearrangement of carbon layers with improved graphitization degree,which provides more Na+storage ***-situ Fourier transform infrared spectroscopy/electrochemical impedance spectroscopy （FTIR/EIS） and X-ray photoelectron spectroscopy （XPS） analysis demonstrate the presence of more BC3and less B–C–O structures that result in enhanced ion diffusion kinetics and the formation of inorganic rich and robust SEI,which leads to facilitated charge transfer and excellent rate *** a result,the hard carbon anode with optimized boron doping content exhibits enhanced rate and cycling *** general,this work unravels the critical role of boron doping in optimizing the pore structure,interface chemistry and diffusion kinetics of hard carbon,which enables rational design of sodium-ion battery anode with enhanced Na+storage performance.

关键词： X ray photoelectron spectroscopy

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四川西昌盆地白垩纪恐龙足迹群的新发现

地质通报 2018年第10期37卷 1771-1776页

作者：童馗邢立达姜巽彭光照叶勇江山丑春永李轲李智武成都理工大学油气藏地质及开发工程国家重点实验室四川成都610059 中国地质大学(北京)地球科学与资源学院北京100083 中国地质大学(北京)生物地质与环境地质国家重点实验室北京100083 中国科学院南京地质古生物研究所/现代古生物学和地层学国家重点实验室江苏南京210008 自贡恐龙博物馆四川自贡643013

四川西昌盆地白垩系小坝组尚未发现骨骼化石记录,其白垩系恐龙动物群的信息全赖于足迹化石。2017年,在喜德县洛甘发现小坝组迄今最大型的恐龙足迹群。该足迹点保存了大量的兽脚类足迹。足迹保存条件较差,但具备了基本的形态学特征。总... 详细信息

四川西昌盆地白垩系小坝组尚未发现骨骼化石记录,其白垩系恐龙动物群的信息全赖于足迹化石。2017年,在喜德县洛甘发现小坝组迄今最大型的恐龙足迹群。该足迹点保存了大量的兽脚类足迹。足迹保存条件较差,但具备了基本的形态学特征。总体来看,兽脚类足迹具有尺寸较小(8~13cm),中等中趾前凹(0.5~0.6)和第Ⅱ趾和第Ⅳ趾间较宽趾间角(70°~100°)的特征;少量足迹保存了跖骨垫。初步分析认为,洛甘兽脚类足迹与四川盆地夹关组的兽脚类足迹Eubrontes和Grallator形态类型相似,为两地在白垩纪中期具有类似的恐龙动物群的观点提供了新的证据。该发现对于西昌盆地的古气候、古地理和地层对比都具有重要的意义,足迹详细分类还有待进一步研究。

关键词：恐龙足迹兽脚类小坝组白垩系西昌盆地

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中国西南攀西地区下侏罗统益门组蜥脚类足迹:分类学与潜在的造迹者（英文）

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地质通报 2016年第6期35卷 851-855页

作者：邢立达 Lockley Martin G 尤海鲁彭光照唐翔冉浩王涛胡健 Persons Ⅳ W Scott 中国地质大学(北京)生物地质与环境地质国家重点实验室北京100083 中国地质大学(北京)地球科学与资源学院北京100083 中国科学院古脊椎动物与古人类研究所北京100044 美国科罗拉多大学丹佛分校恐龙追踪者团队美国丹佛80217 自贡恐龙博物馆四川自贡643013 会理县文物管理所四川会理615100 广西师范大学珍稀濒危动植物生态与环境保护省部共建教育部重点实验室广西桂林541004 禄丰县国土资源局云南禄丰651200 四川省地矿局物探队资源与环境研究所四川成都610072 阿尔伯塔大学生物科学系加拿大埃德蒙顿T6G 2E9

恐龙足迹和骨骼的记录往往出现在不同的地区。然而,一些地层显示了关系紧密的骨骼和足迹,它们都指向同一个来源。报道了来自四川省攀西地区会理县通安镇通保村下侏罗统益门组中上部的蜥脚类足迹(雷龙足迹Brontopodus),其地理和地层归属... 详细信息

恐龙足迹和骨骼的记录往往出现在不同的地区。然而,一些地层显示了关系紧密的骨骼和足迹,它们都指向同一个来源。报道了来自四川省攀西地区会理县通安镇通保村下侏罗统益门组中上部的蜥脚类足迹(雷龙足迹Brontopodus),其地理和地层归属均与真蜥脚类的何氏通安龙极为接近。通保足迹与造迹者的关联是可能的,但目前还需要更多的证据。通保的雷龙足迹是攀西地区首次发现侏罗纪的蜥脚类足迹,这也表明,在早侏罗世,原始蜥脚类和基干蜥脚型类共存于中国西南地区。

关键词：恐龙足迹蜥脚类益门组下侏罗统通安

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Recent advances in exploring new blood-based biomarkers for the early diagnosis of gastric cancer

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Science China Chemistry 2025年第1期 35-45页

作者： Xinyu peng Qian Ma Da Han School of Life Science Shanghai University Institute of Molecular Medicine Shanghai Key Laboratory for Nucleic Acid Chemistry and Nanomedicine State Key Laboratory of Oncogenes and Related Genes Renji Hospital School of Medicine Shanghai Jiao Tong University Department of Research and Development Intellinosis Biotechnologies Co.Ltd.

Gastric cancer(GC) is a prevalent and lethal malignancy worldwide, and the 5-year survival rate is less than 30%. The absence of distinctive symptoms often leads to late-stage diagnosis, contributing to a grim prognosis. Early detection is pivotal for improving the survival rates and outcomes of GC patients. Traditional diagnostic methods, including gastroscopy and histopathological examination, are restricted in the early diagnosis of GC. Conventional protein biomarkers, such as carcinoembryonic antigen(CEA), carbohydrate antigen 19-9(CA19-9), and carbohydrate antigen 72-4(CA72-4), exhibit insufficient sensitivity and specificity for GC screening, which diminishes their clinical value. Recently, novel circulating biomarkers, such as circulating tumor cells(CTCs), circulating tumor cell DNA(ct DNA), and circulating free RNA(cf RNA), have emerged as promising candidates in the burgeoning field of liquid biopsy due to their superior sensitivity and specificity. This review focuses on the latest research on blood-based biomarkers for GC diagnosis and examines the clinical potentials and challenges associated with these emerging biomarkers.

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Advances in genotypic antimicrobialresistance testing: a comprehensive review

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Science China Life Sciences 2025年第01期 130-143页

作者： Boheng Duan Xianjun Zeng Junping peng Huan Kui College of Nanchang University Department of Imaging The Second Affiliated Hospital of Nanchang University NHC Key Laboratory of Systems Biology of Pathogens National Institute of Pathogen BiologyChinese Academy of Medical Sciences & Peking Union Medical College Key Laboratory of Respiratory Disease Pathogenomics Chinese Academy of Medical Sciences & Peking Union Medical College Key Laboratory of Pathogen Infection Prevention and Control (Ministry of Education) State Key Laboratory of Respiratory Health and MultimorbidityNational Institute of Pathogen BiologyChinese Academy of Medical Sciences & Peking Union Medical College

Antimicrobial resistance(AMR) represents a substantial threat to global public health, complicating the treatment of common infections and leading to prolonged illness and escalated healthcare expenses. To effectively combat AMR, timely and accurate detection is crucial for AMR surveillance and individual-based therapy. Phenotypic antibiotic resistance testing(AST) has long been considered the gold standard in clinical applications, serving as the foundation for clinical AMR diagnosis and optimized therapy. It has significantly contributed to ensuring patients′ health and the development of novel antimicrobials. Despite advancements in automated culture-based AST technologies,inherent limitations impede the widespread use of phenotypic AST in AMR surveillance. Genotypic AST technologies offer a promising alternative option, exhibiting advantages of rapidity, high sensitivity, and specificity. With the continuous advancement and expanding applications of genotypic AST technologies, such as microfluidics, mass spectrometry, and high-resolution melting curve analysis, new vigor has been injected into the development and clinical implementation of genotypic AST technologies. In this narrative review, we discuss the principles, applications, and advancements of emerging genotypic AST methods in clinical settings. The comprehensive review aims to highlight the significant scientific potential of emerging genotypic AST technologies in clinical AMR diagnosis, providing insights to enhance existing methods and explore novel approaches.

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Boosting bidirectional sulfur conversion enabled by introducing boron-doped atoms and phosphorus vacancies in Ni2P for lithium-sulfur batteries

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Journal of Energy Chemistry 2025年第1期100卷 760-769页

作者： Lin peng Yu Bai Hang Li Meixiu Qu Zhenhua Wang Kening Sun Advanced Research Institute of Multidisciplinary Science Beijing Institute of Technology Beijing Key Laboratory of Chemical Power Source and Green Catalysis School of Chemistry and Chemical Engineering Beijing Institute of Technology

Lithium-sulfur （Li-S） batteries have gained great attention due to the high theoretical energy density and low cost,yet their further commercialization has been obstructed by the notorious shuttle effect and sluggish redox ***,we supply a strategy to optimize the electron structure of Ni2P by concurrently introducing B-doped atoms and P vacancies in Ni2P （Vp-B-Ni2P）,thereby enhancing the bidirectional sulfur *** study indicates that the simultaneous introduction of B-doped atoms and P vacancies in Ni2P causes the redistribution of electron around Ni atoms,bringing about the upward shift of d-band center of Ni atoms and effective d-p orbital hybridization between Ni atoms and sulfur species,thus strengthening the chemical anchoring for lithium polysulfides （LiPSs） as well as expediting the bidirectional conversion kinetics of sulfur ***,theoretical calculations reveal that the incorporation of B-doped atoms and P vacancies in Ni2P selectively promotes Li2S dissolution and nucleation ***,the Li-S batteries with Vp-B-Ni2P-separators present outstanding rate ability of 777 m A h g-1at 5 C and high areal capacity of 8.03 mA h cm-2under E/S of 5μL mg-1and sulfur loading of 7.20 mg *** work elucidates that introducing heteroatom and vacancy in metal phosphide collaboratively regulates the electron structure to accelerate bidirectional sulfur conversion.

关键词： Lithium sulfur batteries

Increase in the variability of terrestrial carbon uptake in response to enhanced future ENSO modulation

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Atmospheric and Oceanic Science Letters 2025年第1期18卷 32-38页

作者： Younong Li Li Dan Jing peng Qidong Yang Fuqiang Yang Key Laboratory of Regional Climate-Environment for Temperate East Asia Institute of Atmospheric PhysicsChinese Academy of SciencesBeijingChina Key Laboratory of Atmospheric Environment and Processes in the Boundary Layer over the Low-Latitude Plateau Region Department of Atmospheric ScienceYunnan UniversityKunmingChina

El Niño-Southern Oscillation(ENSO)is a major driver of climate change in middle and low latitudes and thus strongly influences the terrestrial carbon cycle through land-air *** the ENSO modulation and carbon flux variability are projected to increase in the future,but their connection still needs further *** investigate the impact of future ENSO modulation on carbon flux variability,this study used 10 CMIP6 earth system models to analyze ENSO modulation and carbon flux variability in middle and low latitudes,and their relationship,under different scenarios simulated by CMIP6 *** results show a high consistency in the simulations,with both ENSO modulation and carbon flux variability showing an increasing trend in the *** higher the emissions scenario,especially SSP5-8.5 compared to SSP2-4.5,the greater the increase in *** flux variability in the middle and low latitudes under SSP2-4.5 increases by 30.9%compared to historical levels during 1951-2000,while under SSP5-8.5 it increases by 58.2%.Further analysis suggests that ENSO influences mid-and low-latitude carbon flux variability primarily through *** occurrence may potentially be attributed to the increased responsiveness of gross primary productivity towards regional temperature fluctuations,combined with the intensified influence of ENSO on land surface temperatures.

关键词： Carbon variability ENSO modulation CMIP6 models

Synergistic effect of bonding heterogeneity and phonon localization in introducing excellent thermoelectric properties in layered heteroanionic NdZnSbO material

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Journal of Energy Chemistry 2025年第1期100卷 259-272页

作者： Da Wan Shuwei Tang Shulin Bai Xiaodong Li peng Ai Wanrong Guo Tuo Zheng College of Materials Science and Engineering Liaoning Technical University Faculty of Chemistry Northeast Normal University

Layered rare-earth metal oxides, harnessing the dual properties of oxides and two-dimensional layered materials, exhibit remarkable thermal stability and quantum confinement effects. Therefore, this work adopts the first-principles calculation combined with the Boltzmann transport theory to predict the thermoelectric properties of NdZnSbO compound. The coexistence of weak interlayer van der Waals interactions, robust intralayer ionic bonding, and partial covalent bonding leads to remarkable bonding heterogeneity, which engenders pronounced phonon scattering and imposes constraints on thermal transport along the out-of-plane direction. The weakened chemical bonds induced by the antibonding states, together with the rattling-like behavior of the Zn atom, culminate in the profound anharmonicity in the layered NdZnSbO compound. The weakening bond and heavy element contribute to the softness of phonon modes, which significantly diminishes the phonon group velocity. The redistribution-dominated four-phonon scattering process spans a large optical gap, which effectively reduces the lattice thermal conductivity. The NdZnSbO compound exhibits direct semiconductor characteristic with a bandgap of 0.73 e V by adopting the Heyd-Scuseria-Ernzerhof(HSE06) functional in combination with spin–orbit coupling(SOC) effect. The multi-valley feature of NdZnSbO compound augur favorably for band degeneracy, thus amplifying the power factor. Consequently, an optimal figure-of-merit(ZT) of 3.40 at 900 K is achieved for the n-type NdZnSbO compound. The present study delves deeply insights into the origins for the low thermal conductivity of NdZnSbO compound and proposes an optimization scheme to enhance overall thermoelectric performance.

关键词： Bond strength (chemical)