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Green Energy & Environment 2024年第3期9卷 544-555页

作者： Hengyuan Liu Xingjiang Wu Yuhao geng Xin Li Jianhong Xu The State Key Laboratory of Chemical Engineering Department of Chemical EngineeringTsinghua UniversityBeijing100084China

Electrocatalytic nitrogen reduction reaction(NRR)is considered as a promising candidate to achieve ammonia synthesis because of clean electric energy,moderate reaction condition,safe operating process and harmless ***,the chemical inertness of nitrogen and poor activated capacity on catalyst surface usually produce low ammonia yield and faradic ***,the microfluidic technology is proposed to efficiently fabricate enriched iridium nanodots/carbon *** to in-situ co-precipitation reaction and microfluidic manipulation,the iridium nanodots/carbon nanomaterials possess small average size,uniform dispersion,high conductivity and abundant active sites,producing good proton activation and rapid electrons transmission and moderate adsorption/desorption *** a result,the as-prepared iridium nanodots/carbon nanomaterials realize large ammonia yield of 28.73 μg h^(-1. cm^(-2) and faradic efficiency of 9.1.%in KOH ***,the high ammonia yield of 1..21.μg h^(-1. cm^(-2) and faradic efficiency of 24.30%are also achieved in H_(2)SO_(4) *** microfluidic method provides a reference for large-scale fabrication of nano-sized catalyst materials,which may accelerate the progress of electrocatalytic NRR in industrialization field.

关键词： Iridium nanodots Carbon Microfluidic technology Efficient synthesis Electrocatalytic nitrogen fixation

Recyclable hydrolyzed polymers of intrinsic microporosity-1.Fe_(3)O_(4) magnetic composites as adsorbents for selective cationic dye adsorption

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Frontiers of Chemical Science and Engineering 2024年第2期18卷 113-125页

作者： Feng Zhang Shuainan Xu Xiumei geng Meixia Shan Yatao Zhang School of Chemical Engineering Zhengzhou UniversityZhengzhou 450001China

Polymers of intrinsic microporosity shows great potential for dye adsorption and magnetic Fe_(3)O_(4) are easy to be *** this work,hydrolyzed polymers of intrinsic microporosity-1.Fe_(3)O_(4) composite adsorbents were prepared by phase inversion and hydrolysis process for cationic dye *** chemical structure and morphology of the composite adsorbents were systematically characterized by several characterization *** methylene blue as the target dye,the influences of solution pH,contact time,initial dye concentration,and system temperature on the methylene blue adsorption process were *** incorporation of Fe_(3)O_(4) particle into hydrolyzed polymers of intrinsic microporosity-1.endow the adsorbent with high magnetic saturation(20.7 emu·g^(–1.)which allows the rapid separation of the ***,the adsorption process was simulated by adsorption kinetics,isotherms and thermodynamics to gain insight onto the intrinsic adsorption *** addition,the composite adsorbents are able to selectively adsorb cationic dyes from mixed dyes *** polymers of intrinsic microporosity/Fe_(3)O_(4) shows only a slight decrease for methylene blue adsorption after 1. adsorption/regeneration cycles,demonstrating the outstanding regeneration *** high adsorption capacity,outstanding regeneration ability,together with simple preparation method,endow the composite adsorbents great potential for selective removal of cationic dyes in wastewater system.

关键词： polymers of intrinsic microporosity magnetic adsorbent cationic dye adsorption

Command filtered integrated estimation guidance and control for strapdown missiles with circular field of view

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Defence Technology（防务技术） 2024年第5期35卷 211-221页

作者： Wei Wang Jiaqi Liu Shiyao Lin Baokui geng Zhongjiao Shi School of Aerospace Engineering Beijing Institute of TechnologyBeijing 10081China China Research and Development Academy of Machinery Equipment Beijing 100089China Northwest Industries Group CO. Ltd.Xi'an 710043China

In this paper,an integrated estimation guidance and control(IEGC)system is designed based on the command filtered backstepping approach for circular field-of-view(FOV)strapdown *** threedimensional integrated estimation guidance and control nonlinear model with limited actuator deflection angle is established considering the seeker's FOV *** boundary time-varying integral barrier Lyapunov function(IBLF)is employed in backstepping design to constrain the body line-of-sight(BLOS)in IEGC system to fit a circular ***,the nonlinear adaptive controller is designed to estimate the changing aerodynamic *** generalized extended state observer(GESO)is designed to estimate the acceleration of the maneuvering targets and the unmatched time-varying disturbances for improving tracking ***,the command filters are used to solve the"differential expansion"problem during the backstepping *** Lyapunov theory is used to prove the stability of the overall closed-loop IEGC ***,the simulation results validate the integrated system's effectiveness,achieving high accuracy strikes against maneuvering targets.

关键词： Integrated estimation guidance and control Circular field-of-view Time-varying integral barrier Lyapunov function Command filtered backstepping control Nonlinear adaptive control Extended state observer

Polymer: Non-fullerene acceptor heterojunction-based phototransistor for short-wave infrared photodetection

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Nano Research 2024年第4期17卷 3087-3095页

作者： Jing Li Weigang Zhu Yang Han Yanhou geng Wenping Hu Key Laboratory of Organic Integrated Circuits of Ministry of Education&Key Laboratory of Molecular Optoelectronic Sciences School of Science&Collaborative Innovation Center of Chemical Science and Engineering(Tianjin)Tianjin UniversityTianjin 300072China Key Laboratory of Organic Integrated Circuits of Ministry of Education&Key Laboratory of Molecular Optoelectronic Sciences School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

It remains full of challenge for extending short-wave infrared(SWIR)spectral response and weak-light detection in the context of broad spectral responses for *** this work,a novel poly(2,5-bis(4-hexyldodecyl)-2,5-dihydro-3,6-di-2-thienyl-pyrrolo[3,4-c]pyrrole-1.4-dione-alt-thiophene)(PDPPT3-HDO):COTIC-4F organic bulk-heterojunction is prepared as active layer for bulk heterojunction ***3-HDO serves as a hole transport material,while COTIC-4F enhances the absorption of SWIR light to 1.20 *** a result,smooth and connected PDPPT3-HDO film is fabricated by blade coating method and exhibits high hole mobility up to 2.34 cm^(2)·V^(-1.·s^(-1. with a current on/off ratio of 4.72×1.^(5) in organic thin film ***3-HDO:COTIC-4F heterojunction phototransistors exhibit high responsivity of 2680 A·W^(-1. to 900 nm and 81. A·W^(-1. to 1.20 nm,with fast response time(rise time~20 ms and fall time~1.0 ms).The photosensitivity of the heterojunction phototransistor improves as the mass ratio of non-fullerene acceptors increases,resulting in an approximately two orders of magnitude enhancement compared to the bare polymer ***,the phototransistor exhibits decent responsivity even under ultra-weak light power of 43μW·cm^(-2) to 1.20 *** work represents a highly effective and general strategy for fabricating efficient and sensitive SWIR light photodetectors.

关键词： photodetection phototransistor organic semiconductor heterojunction non-fullerene acceptor

Experimental investigation on fluid-induced slip behavior of fault filled with fault gouge

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Journal of Rock Mechanics and Geotechnical Engineering 2024年第9期16卷 3661-3672页

作者： Yongshui Kang Zhi geng Bin Liu Youqi Huang State Key Laboratory of Geomechanics and Geotechnical Engineering Institute of Rock and Soil MechanicsChinese Academy of SciencesWuhan430071China University of Chinese Academy of Sciences Beijing100049China

Fault zones are usually filled with fault gouge and accompanied by fault *** coupled effect of fault gouge and water significantly impacts the slip behavior of the fault,which may weaken the fault structure and further induce rupture propagation and *** this study,we carried out a laboratory experiment to investigate the fluid-induced slip behavior of fault filled with *** friction evolution characteristic associated with fluid pressure and effective stress was investigated during the slip *** addition,the role transformation process of the gouge on the slip behavior of fault was *** experimental result indicates that the friction on the filled fault surface is significantly affected by fault *** rupture of the gouge promotes fault slip and the fluid pressure plays a vital role in the initiation of fault *** fault gouge enhances the shearing strength of the fault and acts as a barrier before the initial slip under fluid ***,the fault gouge would accelerate the fault slip and transform into lubricant after the initial slip.

关键词： Fault gouge Fluid Slip behavior Friction Shear strength

Representation learning: serial-autoencoder for personalized recommendation

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Frontiers of Computer Science 2024年第4期18卷 61-72页

作者： Yi ZHU Yishuai geng Yun LI Jipeng QIANG Xindong WU School of Information Engineering Yangzhou UniversityYangzhou 225127China Key Laboratory of Knowledge Engineering with Big Data(Ministry of Education of the People’s Republic of China) Hefei University of TechnologyHefei 230009China School of Computer Science and Information Engineering Hefei University of TechnologyHefei 230009China

Nowadays,the personalized recommendation has become a research hotspot for addressing information *** this,generating effective recommendations from sparse data remains a ***,auxiliary information has been widely used to address data sparsity,but most models using auxiliary information are linear and have limited *** to the advantages of feature extraction and no-label requirements,autoencoder-based methods have become quite ***,most existing autoencoder-based methods discard the reconstruction of auxiliary information,which poses huge challenges for better representation learning and model *** address these problems,we propose Serial-Autoencoder for Personalized Recommendation(SAPR),which aims to reduce the loss of critical information and enhance the learning of feature ***,we first combine the original rating matrix and item attribute features and feed them into the first autoencoder for generating a higher-level representation of the ***,we use a second autoencoder to enhance the reconstruction of the data representation of the prediciton rating *** output rating information is used for recommendation *** experiments on the MovieTweetings and MovieLens datasets have verified the effectiveness of SAPR compared to state-of-the-art models.

关键词： personalized recommendation autoencoder representation learning collaborative filtering

Biosensor-assisted CRISPRi high-throughput screening to identify genetic targets in Zymomonas mobilis for high d-lactate production

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Synthetic and Systems Biotechnology 2024年第2期9卷 242-249页

作者： Qiqun Peng Weiwei Bao Binan geng Shihui Yang State Key Laboratory of Biocatalysis and Enzyme Engineering and School of Life SciencesHubei UniversityWuhan430062China

Lactate is an important monomer for the synthesis of poly-lactate(PLA),which is a substitute for the petrochemical *** achieve the goal of high lactate titer,rate,and yield for commercial production,efficient lactate production pathway is needed as well as genetic targets that affect high lactate production and *** this study,an LldR-based d-lactate biosensor with a broad dynamic range was first applied into Zymomonas mobilis to select mutant strains with strong GFP fluorescence,which could be the mutant strains with increased d-lactate ***,LldR-based d-lactate biosensor was combined with a genome-wide CRISPR interference(CRISPRi)library targeting the entire genome to generate thousands of mutants with gRNA targeting different genetic targets across the whole ***,two mutant libraries were selected containing 1.5 and 1.4 mutants with different interference sites from two rounds of fluorescence-activated cell sorting(FACS),*** genetic targets of ZMO1.23 and ZMO1.30 were characterized and confirmed to be associated with the increased d-lactate production,further knockout of ZMO1.23 and ZMO1.30 resulted in a 1.%and 21.increase of d-lactate production,*** work thus not only established a high-throughput approach that combines genome-scale CRISPRi and biosensor-assisted screening to identify genetic targets associated with d-lactate production in ***,but also provided a feasible high-throughput screening approach for rapid identification of genetic targets associated with strain performance for other industrial microorganisms.

关键词： D-lactate Biosensor LldR Genome-wide CRISPRi FACS Zymomonas mobilis

Intelligent Small Sample Defect Detection of Concrete Surface Using Novel Deep Learning Integrating Improved YOLOv5

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IEEE/CAA Journal of Automatica Sinica 2024年第2期11卷 545-547页

作者： Yongming Han Lei Wang Youqing Wang Zhiqiang geng IEEE College of Information Science and Technology Beijing University of Chemical TechnologyBeijing 100029 Engineering Research Center of Intelligent PSE Ministry of Education in ChinaBeijing 100029China

Dear Editor,This letter presents an intelligent small sample defect detection of concrete surface using novel deep learning integrating the improved YOLOv5 based on the Wasserstein GAN(WGAN)enhancement *** proposed method is capable of producing top-notch data sets to address the issues of insufficient samples and substandard quality.

关键词： concrete integrating algorithm

Study on moisture absorption characteristics of glass fibrereinforced epoxy resin material for composite insulators based on the 3D-Fick model

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High Voltage 2024年第4期9卷 888-901页

作者： Yuming Zhang Yunpeng Liu Sizu Hou Jianghai geng Ping Wang Hebei Provincial Key Laboratory of Power Transmission Equipment Security Defense North China Electric Power UniversityBaodingChina Hebei Key Laboratory of Power Internet of Things Technology BaodingChina

Long-term exposure to moisture leads to a gradual deterioration of performance and reduced service life of glass fibre-reinforced epoxy resin(GFRP)material in composite ***,it is necessary to analyse the moisture absorption characteristics of GFRP material and the evolution of damage to their internal interface *** absorption tests on GFRP rod material used in composite insulators to obtain their three-dimensional diffusion coefficients are *** force microscopy was then employed to obtain the composite material system's fibre/matrix interfacial phase ***,a finite element model incorporating representative volume elements with interfacial phases and a mesoscale transient moisture absorption finite element model for the composite material was ***,the moisture absorption characteristics of GFRP material and the evolution of damage to the interfacial phase under thermal-humidity cycling conditions were *** results showed that the diffusion coefficient along the fibre direction in GFRP material was higher than that in the perpendicular *** moisture diffusion finite element model,incorporating an anisotropic interfacial phase,fitted the anisotropic diffusion coefficients of GFRP material more *** moisture invaded the GFRP material,the mismatch stresses continuously increased during the moisture ***,the non-uniform arrangement of fibres resulted in uneven distribution of moistureinduced stresses inside the material,leading to higher mismatch stresses in areas with dense fibre arrangements in the *** high and low humidity cycles led to the development of micro-cracks,micro-porosity,and interface debonding along the fibre direction at the GFRP material interfaces,thereby affecting the anisotropic moisture absorption characteristics of the *** findings of this study provide valuable insights into the mechanisms underlying the

关键词： composite fibre moisture

Locally and globally uniform approximations for ruin probabilities of a nonstandard bidimensional risk model with subexponential claims

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Applied Mathematics(A Journal of Chinese Universities) 2024年第1期39卷 98-113页

作者： LIU Zai-ming geng Bing-zhen WANG Shi-jie School of Mathematics and Statistics Central South UniversityChangsha 410083China School of Big Data and Statistics Anhui UniversityHefei 230601China

Consider a nonstandard continuous-time bidimensional risk model with constant force of interest,in which the two classes of claims with subexponential distributions satisfy a general dependence structure and each pair of the claim-inter-arrival times is arbitrarily *** some mild conditions,we achieve a locally uniform approximation of the finite-time ruin probability for all time horizon within a finite *** we further assume that each pair of the claim-inter-arrival times is negative quadrant dependent and the two classes of claims are consistently-varying-tailed,it shows that the above obtained approximation is also globally uniform for all time horizon within an infinite interval.

关键词： bidimensional risk model asymptotic formula subexponential distribution consistently varying tail ruin probability