检索结果-南通市图书馆

Chinese Journal of Polymer Science 2024年第10期42卷 1425-1434,I0007页

作者： Xiao-Ming An Yi-ping Wang tang-Song Zhu Chong Xing Xu-Dong Jia Qiu-Hong Zhang Key Laboratory of High Performance Polymer Material and Technology of MOE Department of Polymer Science and EngineeringSchool of Chemistry and Chemical EngineeringNanjing UniversityNanjing210093China State Key Laboratory of Coordination Chemistry Nanjing UniversityNanjing210093China

Elastomers with high mechanical toughness can guarantee their durability during service ***-healing ability,as well as recyclability,can also extend the life of materials and save the consuming cost of the *** efforts have been dedicated to promoting the mechanical toughness as well as the self-healing capability of elastomers at the same time,while it remains a challenge to balance the trade-off between the above properties in one *** we proposed a molecular design driven by dual interactions of acylsemicarbazide hydrogen bonding and Cu^(2+)-neocuproine coordination *** introducing the reversible multiple hydrogen bonds and strong coordination bonds,we successfully fabricated an extremely tough and self-healing *** elastomer can achieve an impressive top-notch toughness of 491 MJ/m^(3).Furthermore,it boasted rapid elastic restorability within 10 min and outstanding crack tolerance with high fracture energy(152.6kJ/m^(2)).Benefiting from the combination of dynamic interactions,the material was able to self-repair under 80℃conveniently and could be reprocessed to restore the exceptional mechanical properties.

关键词： Metal-ligand coordination Hydrogen bond Ultra-tough elastomer Self-healing

2.5 μm-Thick Ultrastrong Asymmetric Separator for Stable Lithium Metal Batteries

在线全文

学校读者我要写书评

暂无评论

ENERGY & ENVIRONMENTAL MATERIALS 2024年第6期7卷 106-117页

作者： Xie, Donghao Wang, Zekun Ma, Xin Feng, Yuchen tang, Xiaomin Gu, Qiao Deng, Yonghong Gao, ping Hong Kong Univ Sci & Technol Adv Mat Thrust Interdisciplinary Off Clear Water Bay Hong Kong 999077 Peoples R China Hong Kong Univ Sci & Technol Guangzhou Adv Mat Thrust Funct Hub Guangzhou 511453 Peoples R China Hong Kong Univ Sci & Technol Dept Chem & Biol Engn Clear Water Bay Hong Kong 999077 Peoples R China Southern Univ Sci & Technol Dept Mat Sci & Engn Shenzhen 518055 Peoples R China

Lithium metal batteries (LMBs) are considered the ideal choice for high volumetric energy density lithium-ion batteries, but uncontrolled lithium deposition poses a significant challenge to the stability of such devices. In this paper, we introduce a 2.5 mu m-thick asymmetric and ultrastrong separator, which can induce tissue-like lithium deposits. The asymmetric separator, denoted by utPE@Cu2O, was prepared by selective synthesis of Cu2O nanoparticles on one of the outer surfaces of a nanofibrous (diameter similar to 10 nm) ultrastrong ultrahigh molecular weight polyethylene (UHMWPE) membrane. Microscopic analysis shows that the lithium deposits have tissue-like morphology, resulting in the symmetric lithium cells assembled using utPE@Cu2O with symmetric Cu2O coating exhibiting stable performance for over 2000 h of cycling. This work demonstrates the feasibility of a facile approach ultrathin separators for the deployment of lithium metal batteries, providing a pathway towards enhanced battery performance and safety.

关键词： in situ SEI lithium deposition regulation separator ultrastrong ultrathin DEAD LITHIUM GROWTH MECHANISMS ELECTRODEPOSITION DISSOLUTION MICROSCOPY DEPENDENCE MORPHOLOGY BEHAVIOR CELL

Simulating a Chern Insulator with𝐶C=±2 on Synthetic Floquet Lattice

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Chinese Physics Letters 2024年第9期41卷 1-8页

作者： Ling-Xiao Lei Wei-Chen Wang Guang-Yao Huang Shun Hu Xi Cao Xin-fang Zhang Ming-tang Deng ping-Xing Chen Institute for Quantum Science and Technology College of ScienceNational University of Defense TechnologyChangsha 410073China Institute for Quantum Information&State Key Laboratory of High Performance Computing College of Computer Science and TechnologyNational University of Defense TechnologyChangsha 410073China Greatwall Quantum Laboratory Changsha 410006China Hefei National Laboratory Hefei 230088China

The synthetic Floquet lattice,generated by multiple strong drives with mutually incommensurate frequencies,provides a powerful platform for quantum simulation of topological *** this study,we propose a 4-band tight-binding model of the Chern insulator with a Chern number𝐶=±2 by coupling two layers of the half Bernevig–Hughes–Zhang lattice and subsequently mapping it onto the Floquet lattice to simulate its topological *** determine the Chern number of our Floquet-version model,we extend the energy pumping method proposed by Martin et al.[2017 ***.X 7041008]and the topological oscillation method introduced by Boyers et al.[2020 ***.125160505],followed by numerical simulations for both *** simulation results demonstrate the successful extraction of the Chern number using either of these methods,providing an excellent prediction of the phase diagram that closely aligns with the theoretical one derived from the original bilayer half Bernevig–Hughes–Zhang ***,we briefly discuss a potential experimental implementation for our *** work demonstrates significant potential for simulating complex topological matter using quantum computing platforms,thereby paving the way for constructing a more universal simulator for non-interacting topological quantum states and advancing our understanding of these intriguing phenomena.

关键词： properties. topological quantum

Effect of Humidity on Formaldehyde Oxidation over Ce_(0.8)Zr_(0.2)O_(y)Catalyst

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Wuhan University of Technology(Materials Science) 2024年第5期39卷 1108-1115页

作者： tang Ruijiu YANG Zonglin LIU Xiang JIA Lijuan WANG fang DUAN Kaijiao LIU Tiancheng College of Chemistry and Environment Yunnan Minzu UniversityTechnology Innovation Team of Green Purification Technology for Industrial Waste GasEducation Department of YunnanKey Laboratory of Environmental Functional Materials of Yunnan Province Education DepartmentKunming 650504China

In the preparation of a series of Ce_(0.8)Zr_(0.2)O_(y)catalysts catalyzing the removal of formaldehyde,BET,H2-TPR,IR,SEM,XPS,and XRD were used to characterize the catalyst,and the influence of humidity on the catalyst activity was studied by adjusting the humidity during the *** experimental results showed that the formaldehyde removal rate increased with the increase of *** the humidity was higher than 50%,the formaldehyde removal rate decreased by 3%over that when the humidity was 50%.The characterization results showed that humidity facilitated the activation of oxygen and the formation of hydroxyl groups,which both promoted the formation and oxidative decomposition of intermediates and prevented the deposition of intermediates that clogged the pores,allowing more formaldehyde to be adsorbed and oxidized,which increased the activity of the *** provides new mechanistic evidence for the oxidation of formaldehyde and helps in the development of relatively low-cost materials for formaldehyde purification.

关键词： formaldehyde humidity Ce_(0.8)Zr_(0.2)O_(y) catalytic oxidation

Photocatalytic oxidation of methane to methanol over zinc titanate supported silver catalysts

在线全文

学校读者我要写书评

暂无评论

Journal of Rare Earths 2024年第5期42卷 899-906,I0004页

作者： Yuyan Gan Jinbi Huang Qian Lv Yanru Li Lizhi Wu YU tang Yuanxing fang Pengfei Zhu Li Tan Institute of Molecule Catalysis and In-Situ/Operando Studies State Key Laboratory of Photocatalysis on Energy and EnvironmentCollege of ChemistryFuzhou UniversityFuzhou350108China School of Environmental Science and Engineering Shaanxi University of Science and TechnologyXi'an 70021China

The direct activation of methane under mild condition to achieve highly selective of oxygenates is a challenging *** this study,a well dispersed silver supported ZnTiO_(3) catalyst was prepared to achieve selective preparation of methanol from methane and water under mild condition.X-ray diffraction,transmission electron microscopy and X-ray photoelectron spectroscopy characterizations demonstrate that silver species are uniformly dispersed on ZnTiO_(3) surface in the form of metallic silver *** photoelectric characterizations reveal that the addition of silver species enhances light absorption and promotes charge separation of the *** the reaction conditions of 50℃and 3 MPa,the methanol is obtained as the only liquid product over the designed Ag/ZnTiO_(3) catalyst under light *** this photocatalytic process,the holes generated by ZnTiO_(3) activate water to produce intermediate·OH,which further reacts with methane to synthesize *** silver species as co-catalysts extend the light absorption range of ZnTiO_(3) as well as promote charge separation.

关键词： Photocatalytic Methane oxidation Zinc titanate Silver Methanol

Evaluation of the binding affinity and antioxidant activity of phlorizin to pepsin and trypsin

在线全文

学校读者我要写书评

暂无评论

Food Science and Human Wellness 2024年第1期13卷 392-400页

作者： Jing Zhang Lan tang Xia Hu Zhen Zeng Wen Wu fang Geng Hui Li Di Wu Meat Processing Key Laboratory of Sichuan Province School of Food and Biological EngineeringChengdu UniversityChengdu 610106China School of Chemical Engineering Sichuan UniversityChengdu 610065China

Phlorizin(PHL)is a natural compound with strong antioxidant properties mainly found in *** this paper,the interaction mechanism of PHL with pepsin and trypsin was comparatively evaluated by computer simulation,fluorescence spectra,circular dichroism(CD),and Fourier transform infrared(FT-IR)spectra at a molecular *** spectra showed that PHL quenches the pepsin/trypsin by static *** parameters indicated that PHL binds to pepsin mainly through hydrogen bonds and van der Waals forces,and that of trypsin was electrostatic *** ground state complexes PHL and protease have a moderate affinity of 105 L/mol PHL binds more strongly to trypsin than to *** and FT-IR spectra results showed that pepsin/trypsin decreased theβ-sheet content and slightly changed its secondary structure upon *** experimental results are mutually verified with the predicted computer-aid simulation *** PHL and trypsin binding,the antioxidant capacity of PHL was ***,the antioxidant capacity of PHL was decreased after binding to *** work elucidates the binding of PHL binding mechanisms to pepsin/trypsin and provides useful information for the digestion of PHL to improve the application of PHL in food processing.

关键词： Interaction Phlorizin Pepsin Trypsin Antioxidation

Safety and efficacy comparison of remimazolam and propofol for intravenous anesthesia during gastroenteroscopic surgery of older patients:A meta-analysis

在线全文

学校读者我要写书评

暂无评论

World Journal of Clinical Cases 2024年第7期12卷 1272-1283页

作者： fang-Zhuo Li Cheng Zhao Yi-Xun tang Ji-Tong Liu Department of Anesthesiology The First Affiliated Hospital of Hunan Normal University(Hunan Provincial People’s Hospital)Changsha 410005Hunan ProvinceChina Department of Anesthesiology Zhangjiajie People's HospitalZhangjiajie 427000Hunan ProvinceChina

BACKGROUND Remimazolam is characterized by rapid action and inactive *** is used as the general anesthetic for many clinical *** this study,we performed a meta-analysis to evaluate whether remimazolam is superior to propofol for gastroenteroscopy in older *** To compare the adverse events and efficacy of remimazolam and propofol during gastroenteroscopy in older *** The PubMed,Web of Science,the Cochrane Library databases were queried for the relevant key words"remimazolam,""and propofol,""and gastrointestinal endoscopy or gastroscopy."The search scope was"Title and Abstract,"and the search was limited to human studies and publications in *** studies wherein remimazolam and propofol were compared were included for the *** We selected seven randomized controlled trials involving 1445 cases for the *** reduced the hypotension(relative risk,RR=0.44,95%CI:0.29-0.66,P=0.000),respiratory depression(RR=0.46,95%CI:0.30-0.70,P=0.000),injection pain(RR=0.12,95%CI:0.05-0.25,P=0.000),bradycardia(RR=0.37,95%CI:0.24-0.58,P=0.000),and time to discharge[weighted mean difference(WMD)=-0.58,95%CI:-0.97 to-0.18,P=0.005],compared to those after propofol *** obvious differences were observed for postoperative nausea and vomiting(RR=1.09,95%CI:0.97-1.24,P=0.151),dizziness(RR=0.77,95%CI:0.43-1.36,P=0.361),successful sedation rate(RR=0.96,95%CI:0.93-1.00,P=0.083),or the time to become fully alert(WMD=0.00,95%CI:-1.08-1.08,P=0.998).CONCLUSION Remimazolam appears to be safer than propofol for gastroenteroscopy in older ***,further studies are required to confirm these findings.

关键词： Remimazolam Propofol Gastroenteroscopy Anesthesia Older adults Sedation Adverse events

Liquid-metals-induced formation of MXene/polyacrylamide composite organohydrogels for wearable flexible electronics

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Nano Research 2024年第3期17卷 1913-1922页

作者： Minying Wu Bin Chen Xueliang Fan Tong Ye Yuanyuan fang Qian Zhang fangzhou Zhou Yajun Wang Yi tang Department of Chemistry Fudan UniversityShanghai 200433China College of Chemistry&Materials Engineering Wenzhou UniversityWenzhou 325027China

Organohydrogels have demonstrated superior environmental adaptability and frost resistance compared to conventional hydrogels,thereby prompting considerable interests in the development and design of innovative ***,we report an effective one-pot method for fabricating MXene/polyacrylamide(MXene/PAM)composite organohydrogel(MAOH)by employing Ga liquid metals(Ga LMs)as a highly reactive component in the induced free radical polymerization reaction,without the need for additional heating or cross-linking *** synthetic protocol addresses the time-consuming and organic solvent waste concerns associated with traditional solvent displacement methods for organohydrogel *** incorporation of MXene not only highly enhances the conductivity but also confers improved mechanical properties of *** MAOH exhibits excellent environmental adaptability(>7 d),sustained moisture retention,remarkable self-healing capabilities,and outstanding mechanical properties under low temperatures(-20℃).It demonstrates exceptional performance in micro-motion monitoring,rapid response time(125 ms),superior stretchability,and a broad range of strains(0.3%–600%).Therefore,the designed MAOH has great potential for applications in diverse fields such as prosthetics,electronic skin,human–machine interaction,and smart terminals.

关键词： organohydrogels MXene conductivity mechanical properties environmental adaptability

Insight into the Permeability and Microstructure Evolution Mechanism of the Sliding Zone Soil: A Case Study from the Huangtupo Landslide, Three Gorges Reservoir, China

在线全文

维普期刊数据库

学校读者我要写书评

暂无评论

Journal of Earth Science 2024年第3期35卷 941-954页

作者： Qianyun Wang Huiming tang Pengju An Kun fang Junrong Zhang Minghao Miao Qingwen Tan Lei Huang Shengming Hu Badong National Observation and Research Station of Geohazards China University of GeosciencesWuhan 430074China Faculty of Engineering China University of GeosciencesWuhan 430074China Institute of Rock Mechanics Ningbo UniversityNingbo 315211China National and Provincial Joint Engineering Laboratory for the Hydraulic Engineering Safety and Efficient Utilization of Water Resources of Poyang Lake Basin Nanchang Institute of TechnologyNanchang 330099China

A large number of laboratory investigations related to the permeability have been conducted on the sliding *** little attention has been paid to the particular sliding zones of the slideprone Badong ***,we experimentally investigate the permeability nature and the mechanism of seepage in the viscous sliding zone of the Huangtupo *** seepage tests have been performed first with consideration of six dry densities and thirteen hydraulic gradients,in conjunction with the mercury intrusion porosimetry test and scanning electron microscopy test for the microstructure analysis after *** results show that seepage in the sliding zone soil does not follow Darcy’s Law,since there is a threshold hydraulic gradient(i0)below which no flow is observed and a critical hydraulic gradient(icr)over which the hydraulic conductivity(K)tends to be *** percentage of bound water could be responsible for the occurrence of i0 and ***,pore size distributions(PSD)less than 0.6µm and between 10 and 90µm exhibit positive and negative correlations with the i0,respectively,indicating that the i0 is related to the *** mechanism accounting for this result is that pore water pressure forces fine clay particles into the surrounding large pores and converts arranged particles to discretely distributed ones,thereby weakening the connectivity of *** seepages in the sliding zones behave differently from that in the sliding mass and sliding bed in response to the permeability.

关键词： reservoir landslides sliding zone soil permeability microstructure seepage.

Antibacterial properties of cerium oxide nanoparticles: Recent progresses and future challenges

在线全文

学校读者我要写书评

暂无评论

PARTICUOLOGY 2024年第10期93卷 264-283页

作者： Zheng, Heishu tang, Jiajing Wei, Yanhua Deng, Xi Zhang, Yingjuan Ma, Xiangyu Jiang, Xudong Xu, Zhi ping Liao, Hongbing Guangxi Med Univ Coll & Hosp Stomatol Nanning 530021 Peoples R China Guangxi Med Univ Guangxi Key Lab Oral & Maxillofacial Rehabil & Rec Nanning 530021 Peoples R China Guangxi Med Univ Affiliated Hosp 1 Nanning 530021 Peoples R China Guangxi Univ Sci & Technol Sch Med Liuzhou 545005 Peoples R China Shenzhen Bay Lab Inst Biomed Hlth Technol & Engn Shenzhen 518107 Peoples R China Shenzhen Bay Lab Inst Syst & Phys Biol Shenzhen 518107 Peoples R China Univ Queensland Australian Inst Bioengn & Nanotechnol Bld 75 St Lucia Qld 4074 Australia

Use of cerium oxide nanoparticles (CeO2 2 NPs) to optimize management of resistant microorganisms has received increasing attention due to non-specific activity of inorganic antibacterial agents. Understanding the mechanism of action is essential to elucidating the antibacterial activity of CeO2 2 NPs against bacteria. Therefore, this review aims to summarize the antibacterial mechanisms of CeO2 2 NPs and correlate the structural and physicochemical properties of CeO2 2 NPs to their antibacterial activity. We further summarize the strategies for the improvement of the antibacterial performance of CeO2 2 NPs and provide our opinions for future challenges as a conclusion. (c) 2024 Published by Elsevier B.V. on behalf of Chinese Society of Particuology and Institute of Process Engineering, Chinese Academy of Sciences.

关键词： Nanoparticles Cerium oxide Antibacterial activity Nanozyme Fenton reaction CEO2 NANOPARTICLES GREEN SYNTHESIS BIOFILM FORMATION ESCHERICHIA-COLI OXIDATIVE STRESS LEAF EXTRACT GROWTH TOXICITY MECHANISMS NANOMATERIALS