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Cu-substituted nickel hexacyanoferrate with tunable reaction potentials for superior ammonium ion storage

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Journal of Materials Science & Technology 2024年第2期169卷 19-27页

作者： Leiyu fan Guangchang shu Yiwen Liu Haoxiang Yu Lei Yan Liyuan Zhang Jie shu School of Materials Science and Chemical Engineering Ningbo UniversityNingbo 315211China

In this work,a variety of Cu_(x)Ni_(2-x)Fe(CN)_(6)(x=0,0.4,0.8,1.2,1.6,2)cathodes for ammonium ion batteries are prepared and their electrochemical performances are *** the introduction of copper in nickel hexacyanoferrate,the electrochemical performance varies without changing the structure of nickel *** increase of Cu content in nickel hexacyanoferrate leads to the enhancement of reaction potential and *** results suggest that the substitution of Cu for Ni has a positive effect on improving the cycling stability and rate capacity of nickel hexacyanoferrate when x in Cu_(x)Ni_(2-x)Fe(CN)_(6)is less than ***,Cu_(0.4)Ni_(1.6)Fe(CN)_(6)exhibits the best cycling per-formance(capacity retention of 97.54%at 0.3 C)and the highest rate capacity(41.4 mAh g^(-1)at 10 C)in Cu_(x)Ni_(2-x)Fe(CN)_(6).Additionally,the X-ray diffraction(XRD)and X-ray photoelectron spectroscopy(XPS)tests also reveal that the structural evolution of Cu_(0.4)Ni_(1.6)Fe(CN)_(6)is highly reversible upon NH_(4)^(+)***,this work proposes a candidate material for ammoniumion batteries and offers a novel avenue for adjusting the operating potential of the material.

关键词： Nickel hexacyanoferrate Copper hexacyanoferrate NH_(4)^(+)storage Ammonium ion batteries Aqueous batteries

Angular distribution of products in multinucleon transfer reactions

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Chinese Physics C 2024年第10期48卷 193-200页

作者： Xian-Kai Le Kuan fan Feng-Zhu xing shu-Qing Guo Nan Wang College of Physics and Optoelectronic Engineering Shenzhen UniversityShenzhen 518060China Shenzhen Key Laboratory of Nuclear and Radiation Safety Shenzhen 518060China

A method based on the dinuclear system(DNS)is proposed to describe the angular distribution of products in multinucleon transfer(MNT)*** considering fluctuation effects,the angular distributions of reactions involving^(136)Xe+^(208)Pb,^(136)Xe+^(209)Bi,^(86)Kr+^(166)Er,^(84)Kr+^(209)Bi,and^(84)Kr+^(208)Pb are examined,demonstrating good agreement with experimental ***,the double differential cross-sections(dσ^(2)/dl_(i)dΘand dσ^(2)/dZdΘ)of reactions^(136)Xe+^(208)Pb and^(136)Xe+^(209)Bi are analyzed to explore the mechanism of angular distribution in MNT ***,the optimal angles for detecting N=126 isotopes are determined via an analysis on the influence of proton and neutron numbers of the projectiles on the angular distribution of the N=126 isotopic *** results of this study can provide valuable insights for experimental detection.

关键词： angular distribution multinucleon transfer reaction dinuclear system model neutron-rich nuclei

Effect of low-speed waterjet pressure on the rock-breaking performance of unsubmerged cavitating abrasive waterjet

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Petroleum Science 2024年第4期21卷 2638-2649页

作者： Chen-xing fan Deng Li Yong Kang Hai-Tao Zhang Hubei Key Laboratory of Waterjet Theory and New Technology Wuhan University School of Power and Mechanical Engineering Wuhan University

Unsubmerged cavitating abrasive waterjet(UCAWJ) has been shown to artificially create a submerged environment that produces shear cavitation, which effectively enhances rock-breaking performance. The shear cavitation generation and collapse intensity depend on the pressure difference between the intermediate high-speed abrasive waterjet and the coaxial low-speed waterjet. However, the effect of the pressure of the coaxial low-speed waterjet is pending. For this purpose, the effect of low-speed waterjet pressure on rock-breaking performance at different standoff distances was experimentally investigated,and the effects of erosion time and ruby nozzle diameter on erosion performance were discussed. Finally,the micromorphology of the sandstone was observed at different locations. The results show that increased erosion time and ruby nozzle diameter can significantly improve the rock-breaking performance. At different standoff distances, the mass loss increases first and then decreases with the increase of low-speed waterjet pressure, the maximum mass loss is 10.4 g at a low-speed waterjet pressure of0.09 MPa. The surface morphology of cavitation erosion was measured using a 3D profiler, the increase in both erosion depth and surface roughness indicated a significant increase in the intensity of the shear cavitation collapse. At a low-speed waterjet pressure of 0.18 MPa, the cavitation erosion surface depth can reach 600 μm with a roughness of 127 μm.

关键词： Rock-breaking Coaxial low-speed waterjet pressure Abrasive waterjet Cavitation Unsubmerged environment

A hybrid WUDT-NAFnet for simultaneous source data deblending

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Petroleum Science 2024年第3期21卷 1649-1659页

作者： Chao-fan Ke Shao-Huan Zu Jun-xing Cao Xu-Dong Jiang Chao Li xing-Ye Liu Key Laboratory of Earth Exploration and Information Technology of Ministry of Education Chengdu University of Technology State Key Laboratory of Oil and Gas Reservoir Geology and Exploitation Chengdu University of Technology College of Geophysics Chengdu University of Technology

Simultaneous source technology,which reduces seismic survey time and improves the quality of seismic data by firing more than one source with a narrow time interval,is compromised by the massive blended ***,deblending algorithms have been developed to separate this ***,deep learning(DL)has been proved its great potential in suppressing the *** most popular DL method employs neural network as a filter to attenuate the blended noise in an iterative estimation and subtraction framework(IESF).However,there are still amplitude distortion and blended noise residual problems,especially when dealing with weak signal submerged in strong *** address these problems,we propose a hybrid WUDT-NAFnet,which contains two *** first network is a wavelet based U-shape deblending transformer network(WUDTnet),incorporated into IESF as a robust regularization term to iteratively separate the blended *** second network is a nonlinear activate free network(NAFnet)designed to recover the event amplitude and further suppress the weak noise residual in *** the hybrid network,the blended noise can be separated purposefully and *** using synthetic and field seismic data demonstrate that the WUDTNAFnet outperforms traditional curvelet transform(CT)based method and the deblending transformer(DT)model in terms of ***,for field applications,the data augmentation method of bicubic interpolation is applied to mitigate the feature difference between synthetic and field ***,the trained network exhibits strong signal preservation ability in numerical field example without requiring additional training.

关键词： Simultaneous-source Deblending Deep learning Transformer

A daptive Normal Image Coding Scheme Basedon DCT Spectrum Distribution and H-Order

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The Journal of China Universities of Posts and Telecommunications 1999年第2期6卷 22-27页

作者： fan shu-xing LIU Chun-yang(1.Vocational and Technical Teacher’s College, Beijing United University, Beijing, 100011, P.R. China, 2. CSSAR Centre for Space Scienceand Applied Research, Chinese Academy of Sciences as Post-doctor, Beijing 100011, PR. China) Vocational and Technical Teacher's College Beijing United University Beijing 100011 P.R. China CSSAR Centre for Space Science and Applied Research Chinese Academy of Sciences as Post-doctor Beijing 100011 PR. China

In this paper according to the results of DCT spectrum disfribution analysis. we propose an adaptivenormal image coding scheme and image pre treatment, which use multi-scale adaptive sub-blocks in h-order anddecompose direct current component Dc into both components. Redundancy in one of both components can beremoved by multi-direction in h-order, the other component can be quantified finitely in loss. with less influence onthe quality of the reconstructed image. A new method combining quart-tree and template matching is used to extractnon-zero data from the coefficient matrix,the ideal result has been achieved from the coding scheme. The newscheme is called ANQS (adaptive normal quantification scheme ). Experiments prove that ANQS is much betterthan JPEG in the same image. With ANQS excellent quality of reconstruction is obtained at data rate as low as 0.0625 bpp and their PSNR as high as 30.31 dB, respectively but JPEG method is only obtained at data rate: 0.180 bppand PSNR: 32. 19 dB.

关键词： inage coding DCT DCT spectrum disgtribution Hilbert order

The CBL-interacting protein kinase OsCIPK1 phosphorylated by SAPK10 positively regulates responses to ABA and osmotic stress in rice

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The Crop Journal 2024年第2期12卷 364-374页

作者： Caihua Qin xing fan Qianqian fang Lan Ni Mingyi Jiang College of Life Sciences State Key Laboratory of Crop Genetics&Germplasm Enhancement and UtilizationKey Laboratory of Crop Physiology Ecology and Production ManagementMinistry of AgricultureNanjing Agricultural UniversityNanjing 210095JiangsuChina

SubclassⅢsucrose nonfermenting1-related protein kinase 2s(SnRK2s)function in ABA and abiotic stress responses by unknown *** found that osmotic stress/ABA-activated protein kinase 10(SAPK10),a member of rice SnRK2s,physically interacted with CBL-interacting protein kinase 1(OsCIPK1).OsCIPK1 expression was up-regulated by ABA and PEG treatment,and overexpression increased the ABA sensitivity of seed germination and root growth and plant osmotic stress *** stress or ABA-induced activation of OsCIPK1 is dependent on ***10 phosphorylates Thr-24 of OsCIPK1 in vitro,and this phosphorylation increases the activity of OsCIPK1 and positively regulates the function of OsCIPK1 in ABA responses and plant osmotic stress *** study suggests that OsCIPK1 is a direct phosphorylated substrate of SAPK10,and SAPK10-mediated phosphorylation of OsCIPK1 functions in ABA signaling and increases rice osmotic stress tolerance.

关键词： Rice ABA Osmotic stress OsCIPK1 SAPK10

Enhanced activation of peroxymonosulfate on layered molybdenum disulfide loaded with Co-La bimetallic oxide for efficient degradation of chloramphenicol

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Rare Metals 2024年第9期43卷 4628-4635页

作者： Yu-Ning fan Yun-Qiu Zhang San-shuang Gao Zeng-Hui Bi Yin Wang shu-xing Zhou Qian Liu Tian-Ping Lv Guang-Zhi Hu Institute for Ecological Research and Pollution Control of Plateau Lakes School of Ecology and Environmental ScienceYunnan UniversityKunming 650504China Hubei Key Laboratory of Low Dimensional Optoelectronic Materials and Devices Hubei University of Arts and ScienceXiangyang 441053China Institute for Advanced Study Chengdu UniversityChengdu 610106China

The use of transition metal-activated peroxymonosulfate(PMS)as an advanced oxidation technology has gained *** study developed a catalyst using cobaltDlanthanum bimetallic oxide supported on layered molybdenum disulfide(Mo S_(2))as a *** CoDLa/Mo S_(2)catalyst was synthesised through coprecipitation,followed by calcination with an optimised metal ratio of Co:La=2:1 to activate PMS and degrade trace chloramphenicol(CAP)in *** chemical composition of the catalyst was confirmed using X-ray diffraction(XRD)and X-ray photoelectron spectroscopy(XPS).At catalyst and PMS dosages of 0.1 and 0.5 g·L^(-1),respectively,the degradation rate of CAP was 95%with in 30 *** catalyst exhibitedstrong resistance to most interfering anions and maintained a high degradation rate at p H *** chromatographyDmass spectrometry analysis revealed the potential degradation pathways of CAP in the CoDLa/Mo S_(2)(2:1)/PMS *** other pollutants,such as oxytetracycline,complete degradation was achieved within 20 min,demonstrating the broad applicability of the CoDLa/Mo S_(2)(2:1)/PMS system for the degradation and removal of antibiotic organic contaminants.

关键词： catalyst molybdenum disulfide

Transition from grain boundary migration to grain boundary sliding in magnesium bicrystals

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Acta Mechanica Sinica 2024年第8期40卷 17-31页

作者： Zheyuan xing Haidong fan Chuanlong Xu Guozheng Kang School of Mechanics and Aerospace Engineering Southwest Jiaotong UniversityChengdu610031China Department of Mechanics Sichuan UniversityChengdu610065China

In polycrystalline magnesium(Mg)and Mg alloys,as the grain size decreases,the grain boundary(GB)mediated plasticity including GB sliding and GB migration becomes the dominant deformation *** this study,the motion of[1100]symmetric tilt GBs in Mg bicrystals is investigated using molecular dynamics(MD)*** effects of GB misorientation angle and temperature are *** low/room temperatures and varied GB misorientation angles in the range ofθ≥58.36°,the GB migration occurs via the shear coupling with the invariant plane of{0001};At 35.80°<θ<58.36°,both the GB migration and GB sliding happen and the invariant plane changes from{0001}plane to[1122]plane;At 26.54°≤θ≤35.80°,the GB migrates with the invariant plane of[1122];Finally,atθ<26.54°,the GB sliding becomes the main deformation *** 700 K,the GB sliding occurs at the misorientation angles in the range ofθ<58.36θ;while the GB migration occurs at the misorientation angles ofθ≥58.36°.By comparing the energy barriers of GB migration and GB sliding,it yields that the deformation mode with a low energy barrier always happens,which leads to the transition of deformation modes and agrees well with the MD simulation results.

关键词： Molecular dynamics simulations Magnesium Grain boundary migration Grain boundary sliding Temperature

Photocatalytic applications and modification methods of two-dimensional nanomaterials:a review

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Tungsten 2024年第1期6卷 77-113页

作者： fan Yang Ping Hu fan Yang xing-Jiang Hua Bo Chen Lili Gao Kuai-She Wang School of Metallurgy Engineering Xi’an University of Architecture and TechnologyXi’an 710055China National and Local Joint Engineering Research Center for Functional Materials Processing Xi’an University of Architecture and TechnologyXi’an 710055China

Due to its unique electronic structure and special size effect,two-dimensional(2D)nanomaterials have shown great potential far beyond bulk materials in the field of *** to deeply explore the photocatalytic mechanism of 2D nanomaterials and design more efficient 2D semiconductor photocatalysts are research *** review provides a comprehensive introduction to typical 2D nanomaterials and discusses their current application status in the field of *** effects of material properties such as band structure,morphology,crystal face structure,crystal structure and surface defects on the photocatalytic process are *** main modification methods are highlighted,including doping,noble metal deposition,heterojunction,thickness adjustment,defect engineering,and dye sensitization in 2D material ***,the future development of 2D nanomaterials is *** is hoped that this paper can provide systematic and useful information for researchers engaged in the field of photocatalysis.

关键词： Photocatalysis Two-dimensional Nanomaterials Bandgap Modification strategy