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Rapid lithium-ion insertion/extraction and migration behavior of Na_(2)WO_(4)-encapsulated lithium-rich layered oxide cathode

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Rare Metals 2024年第8期43卷 3647-3660页

作者： Yu-Shen Zhao fan-fan Wang Jian-Cang Wang Peng-Fei Wang Ting-Feng Yi Jun-Hong Zhang School of Materials Science and Engineering Northeastern UniversityShenyangShenyang 110819China Key Laboratory of Dielectric and Electrolyte Functional Material Hebei Province School of Resources and MaterialsNortheastern University at QinhuangdaoQinhuangdao 066004China Shandong Provincial Key Laboratory of Chemical Energy Storage and Novel Cell Technology College of Chemistry and Chemical EngineeringLiaocheng UniversityLiaocheng 252059China

Due to the low cost,high working voltage and high storage capacity,Li-rich Mn-based layered compounds show promise as the cathode materials for lithiumion batteries(LIBs).However,the side reactions at the solid-liquid interface of the cathode will lead to rapid capacity decay and inferior rate ***,this article proposes a liquid-phase dispersion strategy to introduce a Na_(2)WO_(4)layer on the Li_(1.2)Ni_(0.13)-Co_(0.13)Mn_(0.54)O_(2) cathode,which can reduce the side effects between raw materials and electrolyte and promote the insertion/extraction rate of Li^(+),thus enhancing the material stability and rate *** a result,the capacity retention rate is 96.9%after 200 cycles under ***,the capacities are 177.5,149.5,111.1 and58.3 mAh·g^(-1)at 1C,2C,5C and 10C,implying a superior fast charging *** exceptional performance can be ascribed to both the increased conductivity and enhanced structural stability of the cathode ***'s more,based on the investigation of ion insertion/extraction behavior in electrode materials and the ion migration kinetics in the electrolyte,this study suggests that coating Li-rich Mn-based materials with Na_(2)WO_(4)can be a promising strategy to improve their performance in LIBs.

关键词： Li-ion battery Coating Rate performance Li_(1.2)Ni_(0.13)Co_(0.13)Mn_(0.54)O_(2) Reaction kinetics

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Circulating tumor cells shielded with extracellular vesicle-derived CD45 evade T cell attack to enable metastasis

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Signal Transduction and Targeted Therapy 2024年第5期9卷 2114-2131页

作者： Chuan Yang Xueping Wang Kenneth K.W.To Caimei Cui Min Luo Shaocong Wu Lamei Huang Kai Fu Can Pan Zeyu Liu Teng fan Caibo Yang fang Wang Liwu Fu State Key Laboratory of Oncology in South China Guangdong Provincial Clinical Research Center for CancerSun Yat-sen University Cancer CenterGuangzhou 510060P.R.China School of Pharmacy Faculty of MedicineThe Chinese University of Hong KongHong KongChina LABVIV Technology(Shenzhen)Co. LtdShenzhen 518057China

Circulating tumor cells(CTCs)are precursors of distant metastasis in a subset of cancer patients.A better understanding of CTCs heterogeneity and how these CTCs survive during hematogenous dissemination could lay the foundation for therapeutic prevention of cancer *** remains elusive how CTCs evade immune surveillance and elimination by immune *** this study,we unequivocally identified a subpopulation of CTCs shielded with extracellular vesicle(EVs)-derived CD45(termed as CD45^(+)CTCs)that resisted T cell attack.A higher percentage of CD45^(+)CTCs was found to be closely correlated with higher incidence of metastasis and worse prognosis in cancer ***,CD45^(+)tumor cells orchestrated an immunosuppressive milieu and CD45^(+)CTCs exhibited remarkably stronger metastatic potential than CD45−CTCs in ***,CD45 expressing on tumor surfaces was shown to form intercellular CD45-CD45 homophilic interactions with CD45 on T cells,thereby preventing CD45 exclusion from TCR-pMHC synapse and leading to diminished TCR signaling transduction and suppressed immune ***,these results pointed to an underappreciated capability of EVs-derived CD45-dressed CTCs in immune evasion and metastasis,providing a rationale for targeting EVs-derived CD45 internalization by CTCs to prevent cancer metastasis.

关键词： CD45 metastasis prevention

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Semisymmetric Graphs of Order 2p^(3)with Valency p^(2)

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Algebra Colloquium 2024年第2期31卷 199-208页

作者： Li Wang Songtao Guo Genghua fan School of Mathematics and Information Science Henan Polytechnic University JiaozuoHenan 454000China School of Mathematics and Statistics Henan University of Science and Technology LuoyangHenan 471023China 不详

A simple undirected regular graph is said to be semisymmetric if it is edge-transitive but not *** a semisymmetric graphΓof order 2p^(3),p a prime,it is well known thatΓis bipartite with two biparts having equal *** complete classification of such graphs has been given for the full automorphism group Aut(Γ)acting unfaithfully on at least one bipart ofΓ,which shows that there is only one infinite family of such graphs with valency p^(2).The graphs of this kind have been determined when Aut(Γ)acts faithfully and primitively on at least one bipart ofΓ,and thus there is only one remaining case for classifying such graphs of valency p^(2),Aut(Γ)acting faithfully and imprimitively on both biparts ofΓ,which is dealt with in this *** a result,there is only one infinite family of semisymmetric graphs of order 2p^(3)with valency p^(2).

关键词： semisymmetric graph semitransitive graph bi-coset graph

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Construction of conjugated scaffolds driven by mechanochemistry towards energy storage applications

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Green Chemical Engineering 2024年第2期5卷 155-172页

作者： Juntian fan Zhenzhen Yang Sheng Dai Department of Chemistry Institute for Advanced Materials and ManufacturingUniversity of TennesseeKnoxvilleTN37996USA Chemical Sciences Division Oak Ridge National LaboratoryOak RidgeTN37831USA

Mechanochemistry has been recognized as an efficient and sustainable methodology to provide a unique driven force and reaction environments under ambient and neat conditions for the construction of functionalized materials possessing promising *** them,highly porous conjugated scaffolds with attractive electronic conductivities and high surface areas are one of the representative categories exhibiting diverse taskspecific applications,especially in electrochemical energy *** recent years,the mechanochemistry-driven procedures have been deployed to construct conjugated scaffolds with engineered structures and properties leveraging the tunability in chemical structures of building blocks and polymerization capability of diverse ***,a thorough review of related works is required to gain an in-depth understanding of the mechanochemical synthesis procedure and property-performance relationship of the as-produced conjugated ***,the mechanochemistry-driven construction of conjugated porous networks(CPNs),the carbon-based materials(e.g.,graphite and graphyne),and carbon supported single atom catalysts(CS-SACs)are discussed and *** electrochemical performance of the afforded conductive scaffolds as electrode materials in supercapacitors and alkali-ion batteries is ***,the challenges and potential opportunities related to the construction of conjugated scaffolds driven by mechanochemistry are also discussed and concluded.

关键词： Mechanochemistry Conjugated scaffolds Porous organic networks Alkali-ion battery Supercapacitor

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Risk factors for early death in severe non-brain- injured trauma patients

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World Journal of Emergency Medicine 2024年第5期15卷 404-406页

作者： Hui Feng Ronghai Shao Zihao fan Limei Ma Jiake Gao Lijun Liu Lichao fang Jianjun Zhu Department of Emergency and Critical Care Medicine the Second Affi liated Hospital of Soochow UniversitySuzhou 215004China Department of Emergency the First People's Hospital of Taicang(Taicang Affi liated Hospital of Soochow University)Suzhou 215400China Center for Emergency and Critical Care Medicine Beijing Friendship HospitalCapital Medical UniversityBeijing 100050China Department of Emergency and Intensive Care Unit Suzhou Xiangcheng People’s HospitalSuzhou 215131China

Severe trauma is one of the main causes of premature death,posing a significant challenge to public health systems.[1]At present,there is a lack of universally accepted guidelines for rapid detection of life-threatening severe trauma,[2]and the accuracy of existing prognostic models in predicting early death is limited.[3,4]Severe non-brain-injured trauma(SNT)patients account for approximately 70%of all trauma-related ***,there is a lack of studies on early death in SNT patients.[5]This study aims to identify risk factors associated with early death(≤72 h post-admission)in SNT patients.

关键词： death patients trauma

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TSCND:Temporal Subsequence-Based Convolutional Network with Difference for Time Series Forecasting

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Computers, Materials & Continua 2024年第3期78卷 3665-3681页

作者： Haoran Huang Weiting Chen Zheming fan MOE Research Center of Software/Hardware Co-Design Engineering East China Normal UniversityShanghai200062China

Time series forecasting plays an important role in various fields, such as energy, finance, transport, and weather. Temporal convolutional networks (TCNs) based on dilated causal convolution have been widely used in time series forecasting. However, two problems weaken the performance of TCNs. One is that in dilated casual convolution, causal convolution leads to the receptive fields of outputs being concentrated in the earlier part of the input sequence, whereas the recent input information will be severely lost. The other is that the distribution shift problem in time series has not been adequately solved. To address the first problem, we propose a subsequence-based dilated convolution method (SDC). By using multiple convolutional filters to convolve elements of neighboring subsequences, the method extracts temporal features from a growing receptive field via a growing subsequence rather than a single element. Ultimately, the receptive field of each output element can cover the whole input sequence. To address the second problem, we propose a difference and compensation method (DCM). The method reduces the discrepancies between and within the input sequences by difference operations and then compensates the outputs for the information lost due to difference operations. Based on SDC and DCM, we further construct a temporal subsequence-based convolutional network with difference (TSCND) for time series forecasting. The experimental results show that TSCND can reduce prediction mean squared error by 7.3% and save runtime, compared with state-of-the-art models and vanilla TCN.

关键词： Difference data prediction time series temporal convolutional network dilated convolution

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Interface engineering via molecules/ions/groups for electrocatalytic water splitting

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Nano Research 2024年第9期17卷 7864-7879页

作者： Defang Ding Youwen Liu fan Xia Engineering Research Center of Nano-Geomaterials of Ministry of Education Faculty of Materials Science and ChemistryChina University of GeosciencesWuhan 430074China State Key Laboratory of Materials Processing and Die&Mould Technology and School of Materials Science and Engineering Huazhong University of Science and Technology WuhanHubei 430074China

The electrochemical water splitting to produce hydrogen converts electric energy into clean hydrogen energy,which is a groundbreaking concept of energy *** achieve high efficiency,numerous strategies have been developed to enhance the performance of *** these,interface engineering with molecules/ions/groups,serves as a versatile approach for optimizing the performance of electrocatalysts in water *** the basis of numerous achievements in high-performance electrocatalysts engineered through molecules/ions/groups at interface,a comprehensive understanding of these advancements is crucial for guiding future ***,after providing a concise overview of the background,the interface engineering via molecules/ions/groups for electrocatalytic water splitting is demonstrated from three ***,the engineering of electronic state of electrocatalysts by molecules/ions/groups at interface to reduce the Gibbs free energy of the corresponding ***,the modification of local microenvironment surrounding electrocatalysts via molecules/ions/groups at interface to enhance the transfer of reactants and ***,the protection of electrocatalysts with molecule/ion/group fences improves their durability,including protecting active sites from leaching and defending them against harmful *** fundamental principles of these three aspects are outlined for each,along with pertinent ***,several research directions and challenges are proposed.

关键词： electrocatalyst water splitting interface engineering molecules/ions/groups

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Some Simple Groups Which are Determined by Their Orders and Degree-Patterns

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Algebra Colloquium 2024年第2期31卷 341-346页

作者： Qinghong Guo Weijun Liu Genghua fan School of Mathematics and Statistics HNP-LAMACentral South University Changsha 410083China College of General Education Guangdong University of Science and Technology DongguanGuangdong 523083China 不详

Let G be a finite group and Irr(G)the set of all irreducible complex characters of *** cd(G)be the set of all irreducible complex character degrees of G and denote byρ(G)the set of all primes which divide some character degree of *** character-prime graphΓ(G)associated to G is a simple undirected graph whose vertex set isρ(G)and there is an edge between two distinct primes p and q if and only if the product p q divides some character degree of *** show that the finite nonabelian simple groups A_(7),J_(1),J_(3),J_(4),L_(3)(3)and U_(3)(4)are uniquely determined by their degree-patterns and orders.

关键词： irreducible complex character character-prime graph finite nonabelian simple group

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A Systematic Review and Performance Evaluation of Open-Source Tools for Smart Contract Vulnerability Detection

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Computers, Materials & Continua 2024年第7期80卷 995-1032页

作者： Yaqiong He Jinlin fan Huaiguang Wu School of Computer Science and Technology Zhengzhou University of Light IndustryZhengzhou450001China

With the rise of blockchain technology,the security issues of smart contracts have become increasingly *** the availability of numerous smart contract vulnerability detection tools,many face challenges such as slow updates,usability issues,and limited installation *** challenges hinder the adoption and practicality of these *** paper examines smart contract vulnerability detection tools from 2016 to 2023,sourced from the Web of Science(WOS)and Google *** systematically collecting,screening,and synthesizing relevant research,38 open-source tools that provide installation methods were selected for further *** a developer’s perspective,this paper offers a comprehensive survey of these 38 open-source tools,discussing their operating principles,installation methods,environmental dependencies,update frequencies,and installation *** on this,we propose an Ethereum smart contract vulnerability detection *** framework enables developers to easily utilize various detection tools and accurately analyze contract security *** validate the framework’s stability,over 1700 h of testing were ***,a comprehensive performance test was performed on the mainstream detection tools integrated within the framework,assessing their hardware requirements and vulnerability detection *** results indicate that the Slither tool demonstrates satisfactory performance in terms of system resource consumption and vulnerability detection *** study represents the first performance evaluation of testing tools in this domain,providing significant reference value.

关键词： Blockchain security ethereum smart contracts detection tools evaluation

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Normalized and self-normalized Cramér-type moderate deviations for the Euler-Maruyama scheme for the SDE

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Science China Mathematics 2024年第8期67卷 1865-1880页

作者： Xiequan fan Haijuan Hu Lihu Xu Center for Applied Mathematics Tianjin UniversityTianjin 300072China School of Mathematics and Statistics Northeastern University at QinhuangdaoQinhuangdao 066004China Department of Mathematics Faculty of Science and TechnologyUniversity of MacaoMacaoChina

In this paper,we establish normalized and self-normalized Cramér-type moderate deviations for the Euler-Maruyama scheme for *** to our results,Berry-Esseen's bounds and moderate deviation principles are also *** norm... 详细信息

关键词： Euler-Maruyama scheme Cramer-type moderate deviations self-normalized sequences Berry-Esseen’s bounds

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