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Acetylacetone-TiO_(2) Promoted Large Area Compatible Cascade Electron Transport Bilayer for Efficient Perovskite Solar Cells

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Energy & Environmental materials 2024年第2期7卷 221-228页

作者： Hyong Joon Lee Jin Kyoung Park Jin Hyuck Heo Sang Hyuk im Department of Chemical and Biological Engineering Korea University145 Anam-ro Seongbuk-guSeoul 17104Korea

In designing efficient perovskite solar cells(PSCs),the selection of suitable electron transport layers(ETLs)is critical to the final device performance as they determine the driving force for selective charge ***_(2)nanoparticles(NPs)based ETLs have been a popular choice for PSCs due to superior electron mobility,but their relatively deep-lying conduction band energy levels(ECB)result in substantial potential ***,TiO_(2)NPs establish favorable band alignment owing to shallower ECB,but their low intrinsic mobility and abundant surface trap sites impede the final *** this reason,constructing a cascaded bilayer ETL is highly desirable for efficient PSCs,as it can rearrange energy levels and exploit on advantages of an individual *** this study,we prepare SnO_(2)NPs and acetylacetone-modified TiO_(2)(Acac-TiO_(2))NPs and implement them as bilayer SnO_(2)/Acac-TiO_(2)(BST)ETL,to assemble cascaded energy band ***_(2)contributes to rapid charge carrier transport from high electron mobility while Acac-TiO_(2)minimizes band-offset and effectively suppresses interfacial ***,the optimized BST ETL generates synergistic influence and delivers power conversion efficiency(PCE)as high as 23.14%with open-circuit voltage(V_(oc))reaching 1.14 ***,the BST ETL is transferred to a large scale and the corresponding mini module demonstrates peak performance of 18.39%PCE from 25 cm^(2)aperture ***,the BST-based mini module exhibit excellent stability,maintaining 83.1%of its initial efficiency after 1000 h under simultaneous 1 Sun light-soaking and damp heat(85℃/RH 85%)environment.

关键词： acetylacetone large area perovskite solar cells TiO_(2)

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Solar Driven 15.7% Hydrogen Conversion by Harmony of Light Harvesting,Electron Transporting Bridge,and S-Defection in a Self-Assembled microscale CuS/rGO/CP Photoanode

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Energy & Environmental materials 2024年第3期7卷 190-201页

作者： Sujeong Kim Boseok Seo Hyerim Park Younghwan im Jeong Yeon Do Byung Sub Kwak Namgyu Son minkyu Kim misook Kang Department of Chemistry College of Natural SciencesYeungnam UniversityGyeongsan Gyeongbuk 38541Korea School of Chemical Engineering Yeungnam UniversityGyeongsan Gyeongbuk 38541Korea Department of Energy and Hydrocarbon Chemistry Graduate School of EngineeringKyoto UniversityKyoto 615-8510Japan Korea Evaluation Institute of Industrial Technology(Keit) Cheomdan-Ro 8-GilDong-GuDaegu 41069Korea Korea Electric Power Research Institute(KEPRI)105 munji-ro Yooseong-guDaejeon 34056Korea

CuS is an encouraging photoelectrode candidate that meets the essential requirements for efficient solar-to-hydrogen production,but it has not been thoroughly studied.A CuS light absorber layer is grown by the self-assembly of copper and sulfur precursors on a carbon paper(CP)***,rGO is introduced as a buffer layer to control the optical and electrical properties of the *** well-ordered microstructural arrangement suppresses the recombination loss of electrons and holes owing to enhanced charge-carrier generation,separation,and *** potential reaching 10 mA cm^(-2)in 1.0 m KOH solution is significantly lowered to 0.87 V,and the photocurrent density at 1.23 V is 94.7 mA cm^(-2).The computational result reveals that the potential-determining step is sensitive to O^(*)stability;the lower stability of O^(*)in the thin layer of CuS/rGO decreases the free-energy gap between the initial and final states of the potential-determining step,resulting in a lowering of the onset *** faradaic efficiency for the photoelectrochemical oxygen evolution reaction in the optimized 2CuS/1rGO/CP photoanode is 98.60%,and the applied bias photon-to-current and the solar-to-hydrogen efficiencies are 11.2%and 15.7%,respectively,and its ultra-high performance is maintained for 250 *** record-breaking achievement indices may be a trigger for establishing a green hydrogen economy.

关键词： 15.7%-solar to hydrogen density functional theory lower photopotential p-CuS/rGO/CP photoanode photoelectrochemical oxygen evolution

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Biomimetic Fe_(7)S_(8)/Carbon electrocatalyst from[FeFe]-Hydrogenase for improving pH-Universal electrocatalytic hydrogen production Special Collection:Aggregation-Induced Processes and Functions

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Aggregate 2024年第1期5卷 451-459页

作者： Dohun Kim Subramani Surendran Sejin im Jaehyoung Lim Kyoungsuk Jin Ki Tae Nam Uk Sim Department of Energy Science&Engineering Daegu Gyeongbuk Institute of Science&Technology(DGIST)DaeguRepublic of Korea Hydrogen Energy Technology Laboratory Korea Institute of Energy Technology(KENTECH)NajuRepublic of Korea Department of Chemistry Korea UniversitySeoulRepublic of Korea Department of materials Science and Engineering Seoul National UniversitySeoulRepublic of Korea

Efficient and cost-effective electrocatalysts that can operate across a wide range of pH conditions are essential for green hydrogen *** by biological systems,Fe_(7)S_(8)nanoparticles incorporated on polydopamine matrix electrocatalyst were synthesized by co-precipitation and annealing *** resulting Fe_(7)S_(8)/C electrocatalyst possesses a three-dimensional structure and exhibits enhanced electrocatalytic performance for hydrogen production across various pH ***,the Fe_(7)S_(8)/C electrocatalyst demonstrates exceptional activity,achieving low overpotentials of 90.6,45.9,and 107.4 mV in acidic,neutral,and alkaline environments,*** impedance spectroscopy reveals that Fe_(7)S_(8)/C exhibits the lowest charge transfer resistance under neutral conditions,indicating an improved proton-coupled electron transfer ***-wave electron paramagnetic resonance results confirm a change in the valence state of Fe from 3+to 1+during the hydrogen evolution reaction(HER).These findings closely resemble the behavior of natural[FeFe]-hydrogenase,known for its superior hydrogen production in neutral *** remarkable performance of our Fe_(7)S_(8)/C electrocatalyst opens up new possibilities for utilizing bioinspired materials as catalysts for the HER.

关键词： biomimetic electrocatalyst hydrogen production renewable energy

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Species Diversity,Distribution,and microhabitats of Anurans on ***-Kalo of the *** Range Natural Park,Bukidnon,Philippines

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Asian Herpetological Research 2021年第1期12卷 58-75页

作者： Von Carlo P.dela TORRE Olga m.NUNEZA Department of Biological Sciences and Environmental Studies University of the Philippines MindanaoMintal.Tugbok District.Davao City 8022Philippines Wildlife-Human Interaction Studies Ecological Researchand Biodiversity Conservation Laboraory.University of the PhilippinesMindanaoMintalTugbok DistrictDavao City 8022Philippines Department of Biological Sciences and Biodiversity Laboratory Premier Research lnstitute of Science and MathematicsMindanaoState University-lligan Institute of TechnologyA.Bonifacio Avelligan City 9200Philippines

Anurans are considered good indicators of habitat quality due to their bi-phasic life mode,limited dispersal abilities,and sensitivity to environmental changes brought about by habitat fragmentation,pollution,climate change,and emerging infectious *** study aimed to determine species diversity and local distribution of anurans in lower(1000–1400 masl)and upper(1400–1600 masl)montane forests on ***-Kalo of the *** Range Natural Park,Central mindanao,Southern Philippines by employing standard sampling techniques for *** recorded a total of 251 individual anurans,representing 12 species during a brief recent study ***-Kalo’s upper montane forest has a higher diversity index(H’=1.276)than the lower montane forest(H’=0.851).Despite the very low diversity indices,the level of endemism of anurans was 100%where ten of the recorded species are mindanao Faunal Region endemics and an additional two species are Philippine *** muelleri exhibited the highest local abundance and individuals of this species which constituted 73%of individual anurans *** of the species encountered prefer terrestrial and aquatic microhabitats,specifically on the rocks and bank substrates along the rivers and *** species of anurans(Philautus acutirostris,***,and Rhacophorus bimaculatus)were strictly found in arboreal *** magnus and *** have overlapping *** indicate that for such a short survey and modest sampling effort,the lower and upper montane forests of ***-Kalo support high endemism of anuran species suggesting that conservation efforts continue to be a priority in this unique protected area.

关键词： conservation endemic indicator species montane forest protected area

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Spatial analysis of vegetation cover response to climate trends in Khakassia(South Siberia)

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Journal of mountain Science 2023年第10期20卷 2869-2884页

作者： im Sergei Institute of Natural Sciences and mathematics Khakassian State University named after N.F.KatanovAbakan 655000Russia V.N.Sukachev Institute of Forest Krasnoyarsk Science Centre of the Siberian Branch of Russian Academy of ScienceKrasnoyarsk 660036Russia Institute of Ecology and Geography Siberian Federal UniversityKrasnoyarsk 660041Russia Institute of Space Research and High Technologies Reshetnev Siberian State University of Science and TechnologyKrasnoyarsk660014Russia

An analysis of the changes in vegetation cover on the territory of the Republic of Khakassia in 2000–2021 due to climatic trends was carried out based on the mODIS *** changes in vegetation cover were estimated based on trends in Normalized Difference Vegetation Index(NDVI)and Enhanced Vegetation Index(EVI).In general,in the 21st century,an increase in the biomass of vegetation cover is *** trends were observed in 16%–22%of the territory,and negative only in 1%–3%.For about 20%of the analyzed territory,a significant influence of climate on the changes in vegetation cover was *** most pronounced negative impact on vegetation cover was caused by summer air and soil temperatures,spring temperature,and summer winds,and the positive impact was caused by summer precipitation and soil *** response of the vegetation cover to climate was non-uniform concerning the ***,a significant correlation with the amount of precipitation was observed for~20%–35%of vegetation growing below 600 m above sea level and for less than 5%above this *** negative effect of summer temperatures on plants prevailed mainly at an elevation below~1400 m above sea *** climate change is likely to lead to significant degradation of vegetation in the steppe and foreststeppe in Khakassia in the coming decades.

关键词： Khakassia South Siberia Vegetation cover Climate trends Remote sensing mODIS NDVI EVI Relief

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Phenology-based delineation of irrigated and rain-fed paddy fields with Sentinel-2 imagery in Google Earth Engine

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Geo-Spatial Information Science 2021年第4期24卷 695-710页

作者： Daniel marc G.dela Torre Jay Gao Cate macinnis-Ng Yan Shi School of Environment University of AucklandAucklandNew Zealand School of Biological Sciences University of AucklandAucklandNew Zealand

Paddy rice agriculture is practiced in both rain-fed and irrigated ecosystems in the ***,small farms are prevalent in the region,and current satellite-based mapping techniques do not distinguish between the two ecosystems at farm *** study developed an approach to rapidly map irrigated and rain-fed paddy rice in Iloilo,Philippines at 10 m resolutions using Google Earth *** approach used an ensemble of classifiers based on time-series vegetation indices to produce dry and wet seasonal maps for the entire *** showed a predominance of rain-fed rice areas in both seasons,with irrigated rice making up only onefourth of the total rice *** overall accuracy was achieved at 68%for the dry season and 75%for the wet season based on ground-acquired points and very high-resolution *** two types of paddies were classified at accuracies up to 87%.Furthermore,the land cover maps showed a strong agreement with the municipal *** resultant maps complement current official statistics and demonstrate the prowess of phenology-based mapping to create paddy inventories in a timely manner to inform food security and agricultural policies.

关键词： Phenology-based mapping paddy type Google Earth Engine Sentinel-2 rice mapping

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Outcome of gastric antral vascular ectasia and related anemia after orthotopic liver transplantation

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World Journal of Hepatology 2020年第11期12卷 1067-1075页

作者： Saad Emhmed Ali Karim m Benrajab Anna Christina dela Cruz Division of Hospital medicine Department of Internal MedicineUniversity of Kentucky College of MedicineLexingtonKY 40536United States Division of Digestive Diseases and Nutrition Department of Internal MedicineUniversity of Kentucky College of MedicineLexingtonKY 40536United States

BACKGROUND Gastric antral vascular ectasia(GAVE)is a significant complication of *** medical,surgical,and endoscopic treatment modalities have been proposed with varied satisfactory *** a few small studies,GAVE and associated anemia have resolved after orthotopic liver transplantation(OLT).Aim To assess the impact of OLT on the resolution of GAVE and related *** We retrospectively reviewed clinical records of adult patients with GAVE who underwent OLT between September 2012 and September *** and other relevant clinical findings were collected,including hemoglobin levels and upper endoscopy findings before and after *** primary outcome was the resolution of GAVE and its related anemia after *** Sixteen patients were *** pre-OLT Hgb was 7.7 g/dL and mean 12 mo post-OLT Hgb was 11.9 g/dL,(P=0.001).Anemia improved(defined as Hgb increased by 2g)in 87.5%of patients within 6 to 12 mo after OLT and resolved completely in half of the ***-OLT esophagogastroduodenoscopy was performed in 10 patients,and GAVE was found to have resolved entirely in 6 of those patients(60%).Although GAVE and associated anemia completely resolved in the majority of our patients after OLT,GAVE persisted in a few patients after *** studies in a large group of patients are necessary to understand the causality of disease and to better understand the factors associated with the persistence of GAVE post-transplant.

关键词： Liver cirrhosis Iron deficiency anemia End-stage liver disease Gastroscopy Gastrointestinal hemorrhage Liver transplantation

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Epidemiological Aspects of Obesity, Overweight and Cardiovascular Risk Factors at Associes in Semi-Urban Areas (Case of Sébikotane)

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Food and Nutrition Sciences 2024年第5期15卷 390-400页

作者： Djiby Sow Nafy Ndiaye mouhamed Yakham Leye maty Diagne Camara michel Assane Ndour mouhamed Dieng Houleye Saou Ndiouga Fall Boundia Djiba Demba Diédhiou im Diallo Anna Sarr mbaye maimouna Ndour Abdoulaye Leye Clinique mé dicale II Centre Hospitalier Abass Ndao Universit&#233 Cheikh Anta Diop de Dakar Dakar Senegal Pikine Department of Internal medicine and Endocrinology Cheikh Anta Diop University Dakar Senegal Department of Public Health Cheikh Anta Diop University Dakar Senegal

Introduction: Obesity and overweight are a public health problem. The general objective was to determine the epidemiological aspects of obesity, overweight and associated risk factors in a semi-urban environment. Patients and methods: This was a cross-sectional, descriptive study conducted on November 28 and 29, 2023 in Sébikotane. It focused on volunteers for screening for chronic non-communicable diseases. Epidemiological and clinical data were evaluated. Results: One hundred and twenty-nine cases of obesity were recorded (28%). Two hundred and eighty-two cases were overweight or obese (61.3%). The mean age was 49.55 years, with a standard deviation of 12.41 years. The age group [40 - 49 years] was the most representative, with 85 cases (30.1%), and the majority were female, with 264 cases (93.6%). Primary education was the most common, with 75 cases (46.3%). Grade 1 obesity concerned ninety-seven cases (75.2%), and diabetes was present in thirty cases (23%). Hypertension was present in ninety-five cases (33.7%). Obesity was more marked in the age group [40 - 49 years] with 45 cases (36%). Conclusion: Obesity and overweight are a major cause of morbidity and mortality. The development and implementation of a prevention and management program is essential.

关键词： Obesity Overweight Risk Factors Sébikotane Senegal

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Bringing gut microbiota into the spotlight of clinical research and medical practice

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World Journal of Clinical Cases 2024年第14期12卷 2293-2300页

作者： Efstathia Davoutis Zoi Gkiafi Panagis m Lykoudis School of medicine National and Kapodistrian University of AthensAthens 11527Greece Division of Surgery and Interventional Science University College LondonLondon WC1E 6BTUnited Kingdom

Despite the increasing scientific interest and expanding role of gut microbiota(Gm)in human health,it is rarely reported in case reports and deployed in cli-nical *** and metabolites produced by microbiota contribute to im-mune system development,energy homeostasis and ***-and endoge-nous factors can alter its *** of microbiota,also known as dysbiosis,is associated with various pathological *** bacterial taxa and related metabolites are involved in disease pathogenesis and therefore can serve as a diagnostic *** could also be a useful prognostic factor by predicting future disease onset and preventing hospital-associated ***-ditionally,it can influence response to treatments,including those for cancers,by altering drug bioavailability.A thorough understanding of its function has per-mitted significant development in therapeutics,such as probiotics and fecal ***,Gm should be considered as a ground-breaking biological parameter,and it is advisable to be investigated and reported in literature in a more consistent and systematic way.

关键词： Gut microbiota Biomarker Fecal microbiota transplantation Dysbiosis Prebiotics

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Deciphering the controlling factors for phase transitions in zeolitic imidazolate frameworks

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National Science Review 2024年第4期11卷 151-163页

作者： Tao Du Shanwu Li Sudheer Ganisetti mathieu Bauchy Yuanzheng Yue morten m.Smedskjaer Department of Chemistry and Bioscience Aalborg University Department of mechanical Engineering-Engineering mechanics Michigan Technological University Physics of Amo Rphous and Inorganic Solids Laboratory(PARISlab) Department of Civil and Environmental EngineeringUniversity of CaliforniaLos Angeles

Zeolitic imidazolate frameworks（ZIFs） feature complex phase transitions, including polymorphism,melting, vitrification, and polyamorphism. Experimentally probing their structural evolution during transitions involving amorphous phases is a significant challenge, especially at the medium-range length scale. To overcome this challenge, here we first train a deep learning-based force field to identify the structural characteristics of both crystalline and non-crystalline ZIF phases. This allows us to reproduce the structural evolution trend during the melting of crystals and formation of ZIF glasses at various length scales with an accuracy comparable to that of ab initio molecular dynamics, yet at a much lower computational cost. Based on this approach, we propose a new structural descriptor, namely, the ring orientation index, to capture the propensity for crystallization of ZIF-4(Zn（im）2, im = C3H3N2-) glasses, as well as for the formation of ZIF-zni(Zn（im）2) out of the high-density amorphous phase. This crystal formation process is a result of the reorientation of imidazole rings by sacrificing the order of the structure around the zinc-centered tetrahedra. The outcomes of this work are useful for studying phase transitions in other metal-organic frameworks（mOFs） and may thus guide the development of mOF glasses.

关键词： metal-organic frameworks phase transitions melting glass formation transferable deep learning force field ring orientation

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