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Magnetic activated carbon for the removal of methyl orange from water via adsorption and Fenton-like degradation

Particuology 2024年第11期94卷 314-326页

作者： Qianyu Wang Yuming Zhang Yuhua Zheng emmanuel oluwaseyi fagbohun Yanbin Cui State Key Laboratory of Heavy Oil Processing China University of Petroleum(Beijing)Beijing102249China State Key Laboratory of Mesoscience and Engineering Institute of Process EngineeringChinese Academy of SciencesBeijing100190China Laboratory for Nanomaterials and Molecular Plasmonics Department of Chemistry and BiologyToronto Metropolitan University350 Victoria StTorontoONM5B2K3Canada

Water pollution caused by organic dyes is a critical environmental *** activated carbon(AC)is commonly used for dye adsorption,its effectiveness is limited by challenges in separation and *** address these limitations,a convenient recyclable magnetic activated carbon(MAC)was fabricated via co-precipitation and calcination method,serving as adsorbent and catalyst for methyl orange(MO)removal through a Fenton-like degradation *** techniques,including XRD,FTIR,SEM and TEM,confirmed that Fe_(3)O_(4) nanoparticles(10–20 nm)were uniformly dispersed on AC *** MAC maintaining a high surface area(997 m^(2)/g)and pore volume(0.795 cm^(3)/g)and exhibited superparamagnetic properties with a saturated magnetization of 5.52 emu/g,enabling effective separation from aqueous solutions by *** adsorption studies revealed that MO adsorption onto MAC followed pseudo-second-order kinetic and Freundlich isotherm model,with a maximum adsorption capacity of 205 mg/g at 25℃.Thermodynamic analysis showed that the adsorption process was spontaneous and *** degradation of MO and in-situ regeneration of MAC were achieved via Fenton-like reaction using sodium persulfate(PS).Under a PS concentration of 9 mmol/L,the MO removal efficiency near 95%after 60 min,with a total organic carbon(TOC)reduction of 83.1%.The reaction of Fe_(3)O_(4) and oxygen functional groups on AC surface with PS facilitated the generation of SO_(4)^(·-),thereby enhancing catalytic degradation of *** degradation efficiency improved as the temperature increased from 25℃ to 45℃.Cycle tests demonstrated that the MO removal efficiency of MAC remained above 90%after 5 cycles of ***,this study highlights the potential of MAC for efficient removal of organic dyes from water through the coupling of adsorption and Fenton-like degradation,providing a promising solution for addressing water pollution challenges.

关键词： Magnetic activated carbon Methyl orange Adsorption Sodium persulfate Fenton-like degradation

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Synthesis ofγ-MnS/nanoporous carbon/reduced graphene oxide composites for high-performance supercapacitor

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Carbon Resources Conversion 2022年第3期5卷 222-230页

作者： Abiola Ganiyat Olatoye Jie Zhang Qianyu Wang Erping Cao Wenli Li emmanuel oluwaseyi fagbohun Yanbin Cui State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China Center of Materials Science and Optoelectronics Engineering University of Chinese Academy of SciencesBeijing 100049China

In the present work,nanoporous carbon(NPC)was prepared from a metal-organic framework(zeolite imidazolate framework 8,ZIF-8).Different concentrations of graphene oxide(GO)were used to make NPC/reduced graphene oxide(NPC/rGO-x,x=0.5,1.0,1.5,and 2.0)composites,and thenγ-MnS/NPC/rGO-1 composite was synthesized via a simple hydrothermal *** electrochemical characteristics of porous carbon composites(NPC/rGO-x)andγ-MnS/NPC/rGO-1 electrodes were investigated by galvanostatic charge and discharge,cyclic voltammetry,and electrochemical impedance ***/rGO-1 showed the highest specific capacitance of 207 F/g at 0.5 A/***,theγ-MnS/NPC/rGO-1 electrode demonstrates exceptional electrochemical performance with a high specific capacitance of 300 F/g at 0.5 A/g and impressive cyclic stability of 70%capacitance retention after 10,000 cycles at 1 A/*** a result,this study demonstrates thatγ-MnS/NPC/rGO-1 electrode can be considered a promising candidate for high-performance supercapacitors.

关键词： Metal-organic framework Nanoporous carbon Reduced graphene oxide γ-MnS Supercapacitor

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Improved thermal conductivity of styrene acrylic resin with carbon nanotubes, graphene and boron nitride hybrid fillers

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Carbon Resources Conversion 2021年第1期4卷 190-196页

作者： Fuhua Jia emmanuel oluwaseyi fagbohun Qianyu Wang Duoyin Zhu Jianling Zhang Bin Gong Yanbin Cui State Key Laboratory of Multiphase Complex Systems Institute of Process EngineeringChinese Academy of SciencesBeijing 100190China College of Mechanical and Power Engineering Shenyang University of Chemical TechnologyShenyang 110142China University of Chinese Academy of Sciences Beijing 100049 China

In the process of printing and copying,the volatilization of toner produces tiny particles and harmful gases that are detrimental to the human ***-temperature printing and copying can reduce harmful gas *** acrylic resin is the main component of toner and the thermal conductivity of toner can be improved by increasing the thermal conductivity of styrene acrylic *** this paper,hexagonal boron nitride(h-BN),carboxyl modified multi-walled carbon nanotubes(MWCNTs-COOH)and graphene hybrid fillers were added into styrene acrylic resin to improve the thermal conductivity of resin composite by forming a connected thermal conductivity network in *** experimental result shows that the thermal conductivity of the h-BN/styrene acrylic resin composite increases with the increase in h-BN filler content(0-20wt%).When 20.0 wt%h-BN is added into styrene acrylic resin,the thermal conductivity is increased by 83.63%.Hybrid fillers(MWCNTs-COOH/graphene and 3.0 wt%h-BN)were added in styrene acrylic resin and the thermal conductivity of the composite is almost the same or higher than that of 20.0 wt%h-BN/styrene acrylic resin *** thermal conductivity of styrene acrylic resin composites improved by 69.57%and 87.14%via adding 1.5wt%CNTs-3 wt%h-BN and 1.0wt%graphene-3 wt%***-COOH or graphene can bridge isolated h-BN aggregates to form a thermally conductive network in styrene acrylic resin,while the addition of graphene improves the thermal conductivity of resin composite higher than that of MWCNTs-COOH.

关键词： Styrene acrylic resin Boron nitride Carbon nanotubes Graphene Thermal conductivity

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