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experimental validation of double-fed induction generator in oscillating water column using circulatory system-based optimization

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Clean energy 2024年第2期8卷 127-143页

作者： Basem e.elnaghi Ahmed M.Ismaiel Fathy el Sayed Abdel-Kader Reham h.Mohammed M.N.Abelwhab electrical Power and Machine Department Suez Canal UniversityIsmailiaEgypt electrical Power and Machine Department Menoufia UniversityMenoufiaEgypt Computer and Control Department Suez Canal UniversityIsmailiaEgypt

This paper validates the optimal operation for a grid-connected double-fed induction generator(DFIG)in an oscillating water column power plant(OWCPP).This study presents a novel optimization technique called the circulatory system-based optimization(CSBO)approach to develop six adaptive fuzzy logic controllers(AFLCs)with 30 parameters and compare them to chaotic-billiards optimization(C-BO)and genetic algorithm(GA).The proposed controller is also compared with a proportional-integral differential(PID)controller based on a self-adaptive global-best harmony search(SGhS).CSBO-based AFLCs are fully investigated under different scenarios and experimented with using a real-time interface *** results of using CSBO-AFLCs revealed a fast time response,fast convergence,less overshoot and minimal error compared with those achieved with C-BO-AFLC,SGhS-PID and GA-AFLC during different case *** CSBO-based AFLCs ensure maximum power from the DFIG in an OWCPP and enhance dynamic response with very low *** results show that the CSBO shows better power tracking by 25%as compared with C-BO,by 45%when compared with the GA and by 56%when compared with ***,the integral absolute errors of six controllers are investigated to demonstrate the feasibility of *** root mean square of the errors of six controllers using CSBO is improved by 68.27%when compared with GA,by 22.57%when compared with C-BO and by 38.42%when compared with *** indicators demonstrate the feasibility of CSBO when compared with other algorithms with the same OWCPP.

关键词： circulatory system-based optimization approach adaptive fuzzy logic controller grid-tied oscillating water column power plant maximum power point tracking

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Development of an active-site titrant for SARS-CoV-2 main protease as an indispensable tool for evaluating enzyme kinetics

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Acta Pharmaceutica Sinica B 2024年第5期14卷 2349-2357页

作者： Rabea Voget Julian Breidenbach Tobias Claff Alexandra hingst Katharina Sylvester Christian Steinebach Lan Phuong Vu Renato h.Weiße Ulrike Bartz Norbert Sträter Christa e.Müller Michael Gütschow Pharmaceutical Institute Pharmaceutical&Medicinal ChemistryUniversity of BonnBonn 53121Germany Institute of Bioanalytical Chemistry Center for Biotechnology and BiomedicineLeipzig UniversityLeipzig 04103Germany Department of Natural Sciences University of Applied Sciences Bonn-Rhein-SiegRheinbach 53359Germany

A titrant for the SARS-CoV-2 main protease(M^(pro))was developed that enables,for the first time,the exact determination of the concentration of the enzymatically active M^(pro) by active-site *** covalent binding mode of the tetrapeptidic titrant was elucidated by the determination of the crystal structure of the enzyme–titrant *** fluorogenic substrates of M^(pro),including a prototypical,internally quenched Dabcyl-eDANS peptide,were compared in terms of solubility under typical assay *** exploiting the new titrant,key kinetic parameters for the M^(pro)-catalyzed cleavage of these substrates were determined.

关键词： COVID-19 SARS-CoV-2 Main protease Peptide nitriles Fluorogenic substrates Active-site titration X-ray crystallography Inner filter effect

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Prediction of chemical short-range order in high-/medium-entropy alloys

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Journal of Materials Science & Technology 2024年第2期169卷 115-123页

作者： Pei-Yu Cao Jing wang Ping Jiang Yun-Jiang wang Fu-Ping Yuan Xiao-Lei Wu State Key Laboratory of Nonlinear Mechanics Institute of MechanicsChinese Academy of ScienceBeijing 100190China School of engineering Science University of Chinese Academy of SciencesBeijing 100049China

Chemical short-range orders(CSROs),as the built-in sub-nanoscale entities in a high-/medium-entropy alloy(h/MeA),have aroused an ever-increasing *** multi-principal elements in an h/MeA to form a complex concentrated solution,a variety of sub-systems of species exist to induce the metastable ordered compounds as candidates for ultimate *** issues remain pending on the origin of CSROs as to how to judge if CSRO will form in an h/MeA and particularly,what kind of CSROs would be stably produced if there were multiple ***,the first-principles method,along with the proposed local formation energy calculation in allusion to the atomic-scale chemical heterogeneities,is used to predict the CSRO formation based on the mechanical stability,thermodynamic formation energy,and electronic *** simulations are detailed in an equiatomic ternary VCoNi MeA with three kinds of potential compounds,i.e.,L1_(1),L1_(2),and B2,in the face-centered cubic *** turns out that L1_(1)is stable but hard to grow up so as to become the final CSRO.L1_(1)is further predicted as CSROs in CrCoNi,but unable to form in FeCoNi and CrMnFeCoNi *** predictions are consistent with the experimental *** findings shed light on understanding the formation of *** method is applicable to other h/MeAs to design and tailor CSROs by tuning chemical species/contents and thermal processing for high performance.

关键词： Short-range order high-entropy alloy Microstructure First-principles calculation Gibbs free energy Local electronic density of states

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Lithium-ion and solvent co-intercalation enhancing the energy density of fluorinated graphene cathode

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Journal of energy Chemistry 2024年第2期89卷 208-215,I0006页

作者： hao wang Jie Jiang Pengyu Chen Zhenrui Wu Xiaobin Niu Chuying Ouyang Jian Liu Liping wang School of Materials and energy University of Electronic Science and Technology of ChinaChengdu 611731SichuanChina School of engineering Faculty of Applied ScienceThe University of British ColumbiaKelowna V1V 1V7Canada 21C Innovation Laboratory Contemporary Amperex Technology Ltd.(21C LAB)Ningde 352100FujianChina

Fluorinated carbons CF_xhold the highest theoretical energy density(e.g.,2180 W h kg^(-1)when x=1)among all cathode materials of lithium primary ***,the low conductivity and severe polarization limit it to achieve its *** this study,we design a new electrolyte,namely 1 M LiBF_(4)DMSO:DOL(1:9 vol.),achieving a high energy density in Li/CF_xprimary *** DMSO with a small molecular size and high donor number successfully solvates Li^(+)into a defined Li^(+)-solvation *** solvated Li^(+)can intercalate into the large-spacing carbon layers and achieve an improved ***,when discharged to 1.0 V,the CF_(1.12)cathode demonstrates a specific capacity of 1944 m A h g^(-1)with a specific energy density of 3793 W h kg^(-1).This strategy demonstrates that designing the electrolyte is powerful in improving the electrochemical performance of CF_(x) cathode.

关键词： Fluorinated carbon Conversion reaction high-energy-density primary battery Li^(+)-solvation structure Solvent co-intercalation

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Characteristics and stability of oxide+carbonitride in h13 steel at 1250℃

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Journal of Iron and Steel Research International 2024年第1期31卷 134-142页

作者： Xiao-lin Sun han-jie Guo Jing Guo Fei wang Dong Xu Gao-yang Song Shuai wang School of Materials Science and engineering Hebei University of EngineeringHandan056038HebeiChina School of Metallurgical and ecological engineering University of Science and Technology BeijingBeijing100083China high Temperature Materials Research Institute Central Iron and Steel Research Institute Co.Ltd.Beijing100081China Technology Innovation Center for high Quality Cold heading Steel of hebei Province Hebei University of EngineeringHandan056038HebeiChina

The morphology,size,quantity,and composition of complex oxide+carbonitride in h13 steel held at 1250℃for 5,10,and 15 h were *** results show that the ratio and number of complex carbonitrides with cores in h13 steel are gradually increased when holding at 1250℃compared with those in the original h13 steel,and the core size *** are one or more oxide cores in(Ti_(x),V_(1-x))(Cy,N_(1-y)),including xCaO·zAl_(2)O_(3),xCaO·yMgO·zAl_(2)O_(3),and CaO after holding at 1250℃,in addition to MgO·Al_(2)O_(3)and Al_(2)O_(3)in the original *** equilibrium temperature for(Ti_(x),V_(1-x))(Cy,N_(1-y))precipitation at the solidification front and decomposition in the solid state was theoretically analyzed,which was affected by the x value and the product of Ti and N contents in h13 ***,the composition of(Ti_(x),V_(1-x))(Cy,N_(1-y))is influenced by the oxide *** is convinced that(Ti_(x),V_(1-x))(Cy,N_(1-y))with oxide cores has a higher stability,especially for oxides with a high Al_(2)O_(3)*** treatment at high temperature facilitates a more reasonable analysis of oxide+carbonitride,and the generation mechanism of oxide+carbonitride was discussed.

关键词： Complex carbonitride Decomposition Oxide core Characteristic Stability

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Prediction of subsurface settlement induced by shield tunnelling in sandy cobble stratum

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Journal of Rock Mechanics and Geotechnical engineering 2024年第1期16卷 192-212页

作者： Fan wang Xiuli Du Pengfei Li Key Laboratory of Urban Security and Disaster engineering Ministry of EducationBeijing University of TechnologyBeijing100124China

This study focuses on the analytical prediction of subsurface settlement induced by shield tunnelling in sandy cobble stratum considering the volumetric deformation modes of the soil above the tunnel crown.A series of numerical analyses is performed to examine the effects of cover depth ratio(C/D),tunnel volume loss rate(h t)and volumetric block proportion(VBP)on the characteristics of subsurface settle-ment trough and soil volume *** the ground loss variation with depth,three modes are deduced from the volumetric deformation responses of the soil above the tunnel ***,analytical solutions to predict subsurface settlement for each mode are presented using stochastic medium *** influences of C/D,h t and VBP on the key parameters(i.e.B and N)in the analytical expressions are discussed to determine the fitting formulae of B and ***,the proposed analytical solutions are validated by the comparisons with the results of model test and numerical *** show that the fitting formulae provide a convenient and reliable way to evaluate the key ***,the analytical solutions are reasonable and available in predicting the subsurface settlement induced by shield tunnelling in sandy cobble stratum.

关键词： Shield tunnelling Sandy cobble stratum Subsurface settlement Volumetric deformation mode Stochastic medium theory

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Soil properties and not plant factors affect both abundant and rare microbial taxa after thinning in a mixed stand of Cunninghamia lanceolata and Sassafras tzumu

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Journal of Forestry Research 2024年第2期35卷 81-94页

作者： Wanxia Peng Tongqing Song hu Du Feng wang Fuping Zeng Yang wang Shulin Chen Yinzhu Chen Key Laboratory of Agro‑ecological Processes in Subtropical Region Institute of Subtropical AgricultureChinese Academy of SciencesChangsha 410125People’s Republic of China Guangxi Industrial Technology Research Institute for Karst Desertification Control Nanning 530001People’s Republic of China huanjiang Observation and Research Station for Karst ecosystems Institute of Subtropical AgricultureChinese Academy of SciencesChangsha 410125People’s Republic of China hubei ecology Polytechnic College Wuhan 430200People’s Republic of China hubei Tongshan Damushan State Forest Farm Tongshan 437652People’s Republic of China

Thinning is an effective management step for sustainable forest development,yet less attention is paid to the restoration of soil microbiota after *** this study,both abundant and rare soil microbial communities(i.e.,bacterial,fungal),were evaluated under various thinning treatments in a mixed stand of Cunninghamia lanceolata and Sassafras tzumu using Mi Seq *** did not significantly change either abundant or rare bacterial and fungal community composition,but affected their alpha *** Shannon–Wiener indexes of rare fungal taxa under medium thinning were significantly lower than in the light thinning(Pevel).Xanthobacteraceae dominated the abundant bacterial taxa,and Saitozyma and Mortierlla the abundant fungal *** most common rare bacterial taxa varied;there was no prevalent rare fungal taxa under different *** addition,soil available nitrogen,total phosphorus,and p h had significant effects on rare bacterial ***,especially available phosphorus,but not nitrogen,affected abundant and rare soil *** results indicate that soil properties rather than plant factors affect abundant and rare microbial communities in soils of mixed ***,through mediating soil properties,influences both abundant and rare bacterial and fungal communities in the mixed *** and *** stand.

关键词： Diversity Abundant taxa Rare taxa Thinning Mixed stand

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In situ regulating intimately connected heterostructure by decomposition of solid solution oxides toward high-efficient water oxidation

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Rare Metals 2024年第4期43卷 1557-1569页

作者： Shao-Fei Zhang Xiao-Lu Yin Jin wang Jian-Li Kang Tian-Tian Li Jin-Feng Sun Yong-Qiang Meng Jian-Jiang wang Dian-Long wang Kai-Qiang Qin hebei Key Laboratory of Flexible Functional Materials/hebei Key Laboratory of Material Near-Net Forming Technology School of Materials Science and EngineeringHebei University of Science and TechnologyShijiazhuang050018China Key Laboratory of Advanced Ceramics and Machining Technology/Ministry of education School of Materials Science and EngineeringTianjin UniversityTianjin300072China electrochemical engine Center Department of Mechanical EngineeringPennsylvania State UniversityUniversity ParkPA16802USA

heterogeneous interfaces produced by interdomain interactions on a nanoscale performs a crucial role in boosting the properties of an electrocatalyst toward oxygen evolution reaction(OeR)***,a series of dual-phase electrodes with intimately connected heterointerfaces are prepared by in situ decomposing solid solution oxide of Ni_(x)Co_(y)Fe_(100-x-y)O,which grew on Ni foam massively via an ultrafast combustion ***,with high-reaction kinetics caused by the reduction treatment at 450℃,the less electronegative Fe and Co are more oxyphilic than Ni,which facilitated their co-exsolution and formation of CoFe_2O_4/NiO oxide with enriched oxygen *** from the nanoporous framework,heterojunction structure,and oxygen defects,the self-supporting electrodes present rapid charge/mass transmission and provide abundant active sites for *** optimized sample(R-SNCF4.5)shows low overpotentials of 226 and 324 mV at 10 and100 mA·cm^(-2),a small Tafel slope(46.7 mV·dec^(-1)),and excellent *** assembled R-SNCF4.5//Pt/C/NF electrolyzer demonstrates continuous electrolysis over 50 h at a current density of 10 mA·cm^(-2),under 1.51 *** functional theory(DFT)calculations verify that the strong electronic modulation plays a critical part in the CoFe_2O_4/NiO hybrid by lowering the energy barriers for the ratedetermining steps,and Fe sites are the most active OeR sites.

关键词： Rapid combustion Decomposition of solid solution oxide Dual-phase heterostructure Oxygen evolution reaction Theoretical calculation

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Viability of all-solid-state lithium metal battery coupled with oxide solid-state electrolyte and high-capacity cathode

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Journal of energy Chemistry 2024年第4期91卷 122-131页

作者： Xingxing Jiao Xieyu Xu Yongjing wang Xuyang wang Yaqi Chen Shizhao Xiong Weiqing Yang Zhongxiao Song Yangyang Liu Research Institute of Frontier Science Southwest Jiaotong UniversityChengdu 610031SichuanChina State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong UniversityXi'an 710049ShaanxiChina Department of Physics Chalmers University of TechnologyGöteborgSE 41296Sweden

Owing to the utilization of lithium metal as anode with the ultrahigh theoretical capacity density of 3860 mA h g^(-1)and oxide-based ceramic solid-state electrolytes(Se),e.g.,garnet-type Li7La_(3)Zr_(2)O_(12)(LLZO),all-state-state lithium metal batteries(ASLMBs)have been widely accepted as the promising alternatives for providing the satisfactory energy density and ***,its applications are still challenged by plenty of technical and scientific *** this contribution,the co-sintering temperature at 500℃is proved as a compromise method to fabricate the composite cathode with structural integrity and declined capacity fading of LiNi_(0.5)Co_(0.2)Mn_(0.3)O_(2)(NCM).On the other hand,it tends to form weaker grain boundary(GB)inside polycrystalline LLZO at inadequate sintering temperature for LLZO,which can induce the intergranular failure of Se during the growth of Li filament inside the unavoidable defect on the interface of ***,increasing the strength of GB,refining the grain to 0.4μm,and precluding the interfacial defect are suggested to postpone the electro-chemo-mechanical failure of Se with weak ***,the advanced sintering techniques to lower the co-sintering temperature for both NCM-LLZO composite cathode and LLZO Se can be posted out to realize the viability of state-of-the-art ASLMBs with higher energy density as well as the guaranteed safety.

关键词： All-solid-state lithium metal battery LiNi_(0.5C)o_(0.2)Mn_(0.3)O_(2)-Li7La_(3)Zr_(2)O_(12)composite cathode Co-sintering Lithium metal anode electro-chemo-mechanical failure

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Suspect and non-targeted screening of chemical pollutants in Botswana's aquatic environments

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emerging Contaminants 2024年第3期10卷 363-373页

作者： Kgato P.Selwe Charlotte R.head Gothatamang N.Phokedi Jens e.T.Andersen J.Brett Sallach Caroline e.h.Dessent Department of Chemistry University of YorkHeslingtonYorkUnited Kingdom Department of environment and Geography University of YorkHeslingtonYorkUnited Kingdom Department of Biology University of YorkHeslingtonYorkUnited Kingdom Department of Chemical and Forensic Sciences Botswana International University of Science and TechnologyBotswana

Chemical pollution in the aquatic systems of Botswana has been sparsely studied despite its potential ecological ***,we perform a study of water samples collected from 13 locations distributed across Botswana to obtain the first overview of the nature and distribution of chemical contaminants across the country's aquatic *** resolution mass spectrometry was applied using nontargeted and suspect screening methods to qualitatively analyse samples.A total of 114 contaminants of emerging concern(CeCs)were identified including 68(59.6%)pharmaceuticals and pharmaceutical metabolites;16(14.2%)pesticides;13(11.4%)psychoactive compounds and metabolites;11(9.7%)industrial chemicals and intermediates and lastly,5(4.4%)personal care ***,3,4-dimethylmethcathinone,and diazolidinyl urea represented the most commonly detected pharmaceutical,psychoactive drug and personal care product,*** pesticide dodemorph and three industrial chemicals(stearamide,pthalic acid and bis(2-ethylhexyl)phthalate)were detected in all samples obtained.90 CeCs were detected in receiving water(from 7 sample locations),75 in wastewater(from 3 sample locations)and 60 in surface water(from 9 sample locations).Of the compounds detected,only 8 had been identified in environmental samples acquired in Botswana *** discuss the variations in the nature and frequency of chemical pollutants detected in this work in a geographical *** results indicate that Botswana's aquatic systems are subject to pollution,despite wastewater treatment and that in order to mitigate potentially harmful effects on both human and aquatic ecosystems,more investigations are required to correctly identify,track and tackle the sources of pollution.

关键词： emerging contaminants Chemical pollution Water analysis Pharmaceuticals LC-hRMS/MS

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