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MXene-based hybrid materials for electrochemical and photoelectrochemical H_(2) generation

Journal of Energy Chemistry 2024年第6期93卷 111-125,I0004页

作者： Jun Young Kim Seung Hun roh Chengkai Xia Uk Sim Jung Kyu Kim School of Material Science and Engineering North University of ChinaTaiyuan 030051China School of Chemical Engineering Sungkyunkwan University(SKKU)2066Seobu-roJangan-guSuwon 16419Republic of Korea Hydrogen Energy Technology Laboratory Korea Institute of Energy Technology(KENTECH)NajuJeollanamdo 58330Republic of Korea SKKU Advanced Institute of Nano Technology(SAINT) Sungkyunkwan University(SKKU)2066Seobu-roJangan-guSuwon 16419Republic of Korea

The conversion of solar energy to produce clean hydrogen fuel through water splitting is an emerging strategy for efficiently storing solar energy in the form of solar fuel.This aligns with the increasing global demand for the development of an ideal energy alternative to fossil fuels that does not emit greenhouse gases.Electrochemical(EC) and photoelectrochemical(PEC) water splitting technologies have garnered significant attention worldwide for advanced hydrogen solar fuel production in recent decades.To achieve sustainable green H_(2) production,it is essential to create efficient catalyst materials that are low-cost and can replace expensive noble metal-based catalysts.These characteristics make them an ideal catalyst material for the process.Two-dimensional MXenes with M_(n+1)X_(n) structure have been identified as a promising option for EC and PEC water splitting due to their superior hydrophilicity,metal-like conductivity,large surface area,and adjustable surface chemistry.Here,we present a summary of recent advancements in the synthesis and performance enhancement methods for MXene hybrid materials in hydrogen production through EC and PEC water splitting.Furthermore,we examine the challenges and insights associated with the rational design of MXene-based hybrid materials to facilitate efficient water splitting for sustainable solar fuel production.

关键词： MXene Hybrid materials EC PEC HER OER Water splitting

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East Asian VLBI Network observations of active galactic nuclei jets:imaging with KaVA+Tianma+Nanshan

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Research in Astronomy and Astrophysics 2021年第8期21卷 220-234页

作者：崔玉竹 Kazuhiro Hada Motoki Kino Bong-Won Sohn Jongho Park Hyun-Wook Ro Satoko Sawada-Satoh Wu Jiang Lang Cui Mareki Honma 沈志强 Fumie Tazaki 安涛 Ilje Cho Guang-Yao Zhao Xiao-Peng Cheng Kotaro Niinuma Kiyoaki Wajima Ying-Kang Zhang Noriyuki Kawaguchi Juan-Carlos Algaba Shoko Koyama Tomoya Hirota Yoshinori Yonekura Nobuyuki Sakai Bo Xia Yong-Bin Jiang Lin-Feng Yu Wei Gou Ju-Yeon Hwang Yong-Chen Jiang Yun-Xia Sun Dong-Kyu Jung Hyo-Ryoung Kim Jeong-Sook Kim Hideyuki Kobayashi Jee-Won Lee Jeong-Ae Lee Hua Zhang Guang-Hui Li Zhi-Qiang Xu Peng Li Jung-Hwan Oh Se-Jin Oh Chung-Sik Oh Tomoaki Oyama duk-gyoo roh Katsunori-M.Shibata 郭文 Rong-Bing Zhao Wei-Ye Zhong Jin-Qing Wang Wen-Jun Yang 闫浩 Jae-Hwan Yeom Bin Li 李笑飞 Jian-Ping Yuan Jian Dong Zhong Chen Kazunori Akiyama Keiichi Asada Do-Young Byun Yoshiaki Hagiwara Jeffrey Hodgson Tae-Hyun Jung Kee-Tae Kim Sang-Sung Lee Kunwoo Yi Qing-Hui Liu Xiang Liu Ru-Sen Lu Masanori Nakamura Sascha Trippe Na Wang Xue-Zheng Wang 张波 Department of Astronomical Science The Graduate University for Advanced StudiesSOKENDAI2-21-1 OsawaMitakaTokyo 181-8588Japan Mizusawa VLBI Observatory National Astronomical Observatory of Japan2-12 HoshigaokaMizusawaOshuIwate 023-0861Japan Kogakuin University of Technology and Engineering Academic Support Center2665-1 NakanoHachiojiTokyo 192-0015Japan Korea Astronomy and Space Science Institute Yuseong-guDaejeon 34055Korea Department of Astronomy Yonsei University50 Yonsei-roSeodaemun-guSeoul 03722Korea Department of Astronomy and Space Science University of Science and Technology217 Gajeong-roDaejeonKorea Institute of Astronomy and Astrophysics Academia Sinica645 N Aohoku PIHiloHI 96720USA Graduate School of Sciences and Technology for Innovation Yamaguchi UniversityYoshida 1677-1YamaguchiYamaguchi 753-8512Japan Shanghai Astronomical Observatory Chinese Academy of SciencesShanghai 200030China Xinjiang Astronomical Observatory Chinese Academy of SciencesUrumqi 830011China Key Laboratory of Radio Astronomy Chinese Academy of SciencesNanjing 210008China Institute of Astronomy The University of Tokyo2-21-1 OsawaMitakaTokyo 181-0015Japan Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomia s/nGranada E-18008Spain Department of Physics Faculty of ScienceUniversity of MalayaKuala Lumpur 50603Malaysia Center for Astronomy Ibaraki University2-1-1 BunkyoMitoIbaraki 310-8512Japan Space Light Laboratory 77Yangjaedae-ro 86 roadGangdong-guSeoulKorea Massachusetts Institute of Technology Haystack Observatory 99 Millstone RoadWestfordMA 01886USA National Radio Astronomy Observatory 520 Edgemont RdCharlottesvilleVA 22903USA Toyo University 5-28-20 HakusanBunkyo-kuTokyo 112-8606Japan Department of Physics and Astronomy Seoul National UniversityGwanak-guSeoul 08826Korea Max Planck Institute for Radio Astronomy Auf dem hiigel 69Bonn 53121Germany SNU Astronomy Research Center Seoul National UniversityGwanak-guSeoul 08826Korea

The East Asian Very Long Baseline Interferometry(VLBI) Network(EAVN) is a rapidly evolving international VLBI array that is currently promoted under joint efforts among China,Japan and Korea.EAVN aims at forming a joint VLBI Network by combining a large number of radio telescopes distributed over East Asian regions.After the combination of the Korean VLBI Network(KVN) and the VLBI Exploration of Radio Astrometry(VERA) into Ka VA,further expansion with the joint array in East Asia is actively promoted.Here we report the first imaging results(at 22 and 43 GHz) of bright radio sources obtained with Ka VA connected to Tianma 65-m and Nanshan 26-m Radio Telescopes in China.To test the EAVN imaging performance for different sources,we observed four active galactic nuclei(AGN) having different brightness and morphology.As a result,we confirmed that the Tianma 65-m Radio Telescope(TMRT) significantly enhances the overall array sensitivity,a factor of 4 improvement in baseline sensitivity and 2 in image dynamic range compared to the case of Ka VA only.The addition of the Nanshan 26-m Radio Telescope(NSRT) further doubled the east-west angular resolution.With the resulting high-dynamic-range,high-resolution images with EAVN(Ka VA+TMRT+NSRT),various fine-scale structures in our targets,such as the counter-jet in M87,a kink-like morphology of the 3 C 273 jet and the weak emission in other sources are successfully detected.This demonstrates the powerful capability of EAVN to study AGN jets and to achieve other science goals in general.Ongoing expansion of EAVN will further enhance the angular resolution,detection sensitivity and frequency coverage of the network.

关键词： galaxies:active galaxies:jets instrumentation:interferometers radio continuum:galaxies

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Stable operation of highly loaded pure Si-Fe anode under ambient pressure via carboxy silane-directed robust solid electrolyte interphase

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Journal of Energy Chemistry 2024年第7期94卷 568-576页

作者： Guntae Lim Dong Guk Kang Hyeon Gyu Lee Yen Hai Thi Tran Kihun An Junghyun Choi Kwang Chul roh Do Youb Kim Seung-Wan Song Department of Chemical Engineering&Applied Chemistry Chungnam National University Daejeon 34134Republic of Korea Energy Storage Materials Center Korea Institute of Ceramic Engineering&TechnologyJinju 52851Republic of Korea Advanced Energy Materials Research Center Korea Research Institute of Chemical TechnologyDaejeon 34114Republic of Korea

Incorporation of higher content Si anode material beyond 5 wt%to Li-ion batteries(LIBs)is challenging,owing to large volume change,swelling,and solid electrolyte interphase(SEl)instability issues.Herein,a strategy of diacetoxydimethylsilane(DAMS)additive-directed SEI stabilization is proposed for a stable operation of Si-0.33FeSi_(2)(named as Si-Fe)anode without graphite,which provides siloxane inorganics and organics enrichment that compensate insufficient passivation of fluoroethylene carbonate(FEC)additive and reduce a dependence on FEC.Unprecedented stable cycling performance of highly loaded(3.5 mA h cm^(-2))pure Si-Fe anode is achieved with 2 wt%DAMS combined with 9 wt%FEC additives under ambient pressure,yielding high capacity 1270 mA h g^(-1)at 0.5 C and significantly improved capacity retention of 81%after 100 cycles,whereas short circuit and rapid capacity fade occur with FEC only addi-tive.DAMS-directed robust SEI layer dramatically suppresses swelling and particles crossover through separator,and therefore prevents short circuit,demonstrating a possible operation of pure Si or Si-dominant anodes in the next-generation high-energy-density and safe LIBs.

关键词： High-energy Li-ion battery Pure Si-Fe anode without graphite Silane additive SEI layer Suppressed swelling

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Parasitic leiomyoma in the trocar site after laparoscopic myomectomy:A case report

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World Journal of Clinical Cases 2022年第9期10卷 2895-2900页

作者： Chul Kyu roh Hyuk-Jae Kwon Min Jung Jung Department of Surgery National Police HospitalSeoul 05715South Korea Department of Surgery Ajou University School of MedicineSuwon 16499South Korea Department of Pathology College of MedicineThe Catholic University of KoreaSeoul 06591South Korea

BACKGROUND Laparoscopic myomectomy is increasingly used for resecting gynecological tumors.Leiomyomas require morcellation for retrieval from the peritoneal cavity.However,morcellated fragments may implant on the peritoneal cavity during retrieval.These fragments may receive a new blood supply from an adjacent structure and develop into parasitic leiomyomas.Parasitic leiomyomas can occur spontaneously or iatrogenically;however,trocar-site implantation is an iatrogenic complication of laparoscopic uterine surgery.We describe a parasitic leiomyoma in the trocar-site after laparoscopic myomectomy with power morcellation.CASE SUMMARY A 50-year-old woman presented with a palpable abdominal mass without significant medical history.The patient had no related symptoms,such as abdominal pain.Computed tomography findings revealed a well-defined contrast-enhancing mass measuring 2.2 cm,and located on the trocar site of the left abdominal wall.She had undergone laparoscopic removal of uterine fibroids with power morcellation six years ago.The differential diagnosis included endometriosis and neurogenic tumors,such as neurofibroma.The radiologic diagnosis was a desmoid tumor,and surgical excision of the mass on the abdominal wall was successfully performed.The patient recovered from the surgery without complications.Histopathological examination revealed that the specimen resected from the trocar site was a uterine leiomyoma.CONCLUSION Clinicians should consider the risks and benefits of laparoscopic vs laparotomic myomectomy for gynecological tumors.Considerable caution must be exercised for morcellation to avoid excessive tissue fragmentation.

关键词： Laparoscopic myomectomy Parasitic leiomyoma Trocar site Implantation Morcellation Case report

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An Intelligent Admission Control Scheme for Dynamic Slice Handover Policy in 5G Network Slicing

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Computers, Materials & Continua 2023年第5期75卷 4611-4631页

作者： Ratih Hikmah Puspita Jehad Ali Byeong-hee roh Department of AI Convergence Network Ajou UniversitySuwon16499Korea Department of Computer Engineering and Department of AI Convergence NetworkAjou UniversitySuwon16499Korea

5G use cases,for example enhanced mobile broadband(eMBB),massive machine-type communications(mMTC),and an ultra-reliable low latency communication(URLLC),need a network architecture capable of sustaining stringent latency and bandwidth requirements;thus,it should be extremely flexible and dynamic.Slicing enables service providers to develop various network slice architectures.As users travel from one coverage region to another area,the callmust be routed to a slice thatmeets the same or different expectations.This research aims to develop and evaluate an algorithm to make handover decisions appearing in 5G sliced networks.Rules of thumb which indicates the accuracy regarding the training data classification schemes within machine learning should be considered for validation and selection of the appropriate machine learning strategies.Therefore,this study discusses the network model’s design and implementation of self-optimization Fuzzy Qlearning of the decision-making algorithm for slice handover.The algorithm’s performance is assessed by means of connection-level metrics considering the Quality of Service(QoS),specifically the probability of the new call to be blocked and the probability of a handoff call being dropped.Hence,within the network model,the call admission control(AC)method is modeled by leveraging supervised learning algorithm as prior knowledge of additional capacity.Moreover,to mitigate high complexity,the integration of fuzzy logic as well as Fuzzy Q-Learning is used to discretize state and the corresponding action spaces.The results generated from our proposal surpass the traditional methods without the use of supervised learning and fuzzy-Q learning.

关键词： 5g network slice fuzzy q-Learning slice handover

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Deep Learning-based Wireless Signal Classification in the IoT Environment

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Computers, Materials & Continua 2022年第6期71卷 5717-5732页

作者： Hyeji roh Sheungmin Oh Hajun Song Jinseo Han Sangsoon Lim Department of Computer Engineering Sungkyul UniversityAnyang430742Korea

With the development of the Internet of Things(IoT),diverse wireless devices are increasing rapidly.Those devices have different wireless interfaces that generate incompatible wireless signals.Each signal has its own physical characteristics with signal modulation and demodulation scheme.When there exist different wireless devices,they can suffer from severe Cross-Technology Interferences(CTI).To reduce the communication overhead due to the CTI in the real IoT environment,a central coordinator can be able to detect and identify wireless signals existing in the same communication areas.This paper investigates how to classify various radio signals using Convolutional Neural Networks(CNN),Long Short-TermMemory(LSTM)and attention mechanism.CNN can reduce the amount of computation by reducing weights by using convolution,and LSTM belonging to RNNmodels can alleviate the long-term dependence problem.Furthermore,attention mechanism can reduce the short-term memory problem of RNNs by reexamining the data output from the decoder and the entire data entered into the encoder at every point in time.To accurately classify radio signals according to their weights,we design a model based on CNN,LSTM,and attention mechanism.As a result,we propose a model CLARINet that can classify original data by minimizing the loss and detects changes in sequences.In a case of the real IoT environment with Wi-Fi,Bluetooth and ZigBee devices,we can normally obtain wireless signals from 10 to 20 dB.The accuracy of CLARINet’s radio signal classification with CNN-LSTM and attention mechanism can be seen that signal-to-noise ratio(SNR)exhibits high accuracy at 16 dB to about 92.03%.

关键词： Attention mechanism wireless signal CNN-LSTM classification deep-learning

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Brassinosteroids enhance salicylic acid-mediated immune responses by inhibiting BIN2 phosphorylation of clade I TGA transcription factors in Arabidopsis

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Molecular Plant 2022年第6期15卷 991-1007页

作者： Yeong-Woo Kim Ji-Hyun Youn Jeehee roh Jeong-Mok Kim Seong-Ki Kim Tae-Wuk Kim Department of Life Science Hanyang UniversitySeoul 04763Republic of Korea Department of Life Science Chung-Ang UniversitySeoul 06973Republic of Korea Research Institute for Convergence of Basic Science Hanyang UniversitySeoul 04763Republic of Korea Hanyang Institute of Bioscience and Biotechnology Hanyang UniversitySeoul 04763Republic of Korea

Salicylic acid (SA) plays an important role in plant immune response, including resistance to pathogens and systemic acquired resistance. Two major components, NONEXPRESSOR OF PATHOGENESIS-RELATED GENES (NPRs) and TGACG motif-binding transcription factors (TGAs), are known to mediate SA signaling, which might also be orchestrated by other hormonal and environmental changes. Nevertheless, the molecular and functional interactions between SA signaling components and other cellular signaling pathways remain poorly understood. Here we showed that the steroid plant hormone brassinosteroid (BR) promotes SA responses by inactivating BR-INSENSITIVE 2 (BIN2), which inhibits the redox-sensitive clade I TGAs in Arabidopsis. We found that both BR and the BIN2 inhibitor bikinin synergistically increase SA-mediated physiological responses, such as resistance to Pst DC3000. Our genetic and biochemical analyses indicated that BIN2 functionally interacts with TGA1 and TGA4, but not with other TGAs. We further demonstrated that BIN2 phosphorylates Ser-202 of TGA4, resulting in the suppression of the redox-dependent interaction between TGA4 and NPR1 as well as destabilization of TGA4. Consistently, transgenic Arabidopsis overexpressing TGA4-YFP with a S202A mutation displayed enhanced SA responses compared to the wild-type TGA4-YFP plants. Taken together, these results suggest a novel crosstalk mechanism by which BR signaling coordinates the SA responses mediated by redox-sensitive clade I TGAs.

关键词： brassinosteroid salicylic acid immune responses BIN2 clade I TGA

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Fabrication of High-Density Out-of-Plane Microneedle Arrays with Various Heights and Diverse Cross-Sectional Shapes

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Nano-Micro Letters 2022年第2期14卷 60-78页

作者： Hyeonhee roh Young Jun Yoon Jin Soo Park Dong-Hyun Kang Seung Min Kwak Byung Chul Lee Maesoon Im Brain Science Institute Korea Institute of Science and Technology(KIST)Seoul 02792South Korea Division of Electrical Engineering College of EngineeringKorea UniversitySeoul 02841South Korea Micro/Nano Fabrication Center KISTSeoul 02792South Korea Division of Bio‑Medical Science&Technology KIST SchoolUniversity of Science&Technology(UST)Seoul 02792South Korea

Out-of-plane microneedle structures are widely used in various applications such as transcutaneous drug delivery and neural signal recording for brain machine interface.This work presents a novel but simple method to fabricate high-density silicon(Si)microneedle arrays with various heights and diverse cross-sectional shapes depending on photomask pattern designs.The proposed fabrication method is composed of a single photolithography and two subsequent deep reactive ion etching(DRIE)steps.First,a photoresist layer was patterned on a Si substrate to define areas to be etched,which will eventually determine the final location and shape of each individual microneedle.Then,the 1st DRIE step created deep trenches with a highly anisotropic etching of the Si substrate.Subsequently,the photoresist was removed for more isotropic etching;the 2nd DRIE isolated and sharpened microneedles from the predefined trench structures.Depending on diverse photomask designs,the 2nd DRIE formed arrays of microneedles that have various height distributions,as well as diverse cross-sectional shapes across the substrate.With these simple steps,high-aspect ratio microneedles were created in the high density of up to 625 microneedles mm^(-2)on a Si wafer.Insertion tests showed a small force as low as~172μN/microneedle is required for microneedle arrays to penetrate the dura mater of a mouse brain.To demonstrate a feasibility of drug delivery application,we also implemented silk microneedle arrays using molding processes.The fabrication method of the present study is expected to be broadly applicable to create microneedle structures for drug delivery,neuroprosthetic devices,and so on.

关键词： Microneedle Various heights Cross-sectional shapes Isotropic etch Deep reactive ion etching

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Novel Architecture of OneM2M-Based Convergence Platform for Mixed Reality and IoT

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Computers, Materials & Continua 2022年第4期71卷 51-69页

作者： Seungwoon Lee Woogeun Kil Byeong-hee roh SJ Kim Jin-suk Kang Department of Computer Engineering and Department of AI Convergence Network Ajou UniversitySuwon16499Korea Howard R.Hughes College of Engineering University of NevadaLas VegasNV89154USA AST Co.Ltd. Suwon16681Korea

There have been numerous works proposed to merge augmented reality/mixed reality(AR/MR)and Internet of Things(IoT)in various ways.However,they have focused on their specific target applications and have limitations on interoperability or reusability when utilizing them to different domains or adding other devices to the system.This paper proposes a novel architecture of a convergence platform for AR/MR and IoT systems and services.The proposed architecture adopts the oneM2M IoT standard as the basic framework that converges AR/MR and IoT systems and enables the development of application services used in general-purpose environments without being subordinate to specific systems,domains,and device manufacturers.We implement the proposed architecture utilizing the open-source oneM2M-based IoT server and device platforms released by the open alliance for IoT standards(OCEAN)and Microsoft HoloLens as an MR device platform.We also suggest and demonstrate the practical use cases and discuss the advantages of the proposed architecture.

关键词： Internet of things(IoT) augmented realty(AR) mixed reality(MR) microsoft HoloLens oneM2M convergence platform

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Separator Dependency on Cycling Stability of Lithium Metal Batteries Under Practical Conditions

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Energy & Environmental Materials 2023年第5期6卷 307-316页

作者： Hyeongguk An Youngjoon roh Youngseong Jo Hyuntae Lee Minhong Lim Mingyu Lee Yong Min Lee Hongkyung Lee Department of Energy Science and Engineering Daegu Gyeongbuk Institute of Science and Technology DGIST333 Techno Jungang-daeroDaegu 42988Korea Energy Science and Engineering Research Center Daegu Gyeongbuk Institute of Science and Technology(DGIST)333 Techno Jungang-daeroDaegu 42988Korea

Development of practical lithium(Li)metal batteries(LMBs)remains challenging despite promises of Li metal anodes(LMAs),owing to Li dendrite formation and highly reactive surface nature.Polyolefin separators used in LMBs may undergo severe mechanical and chemical deterioration when contacting with LMAs.To identify the best polyolefin separator for LMBs,this study investigated the separator-deterministic cycling stability of LMBs under practical conditions,and redefined the key influencing factors,including pore structure,mechanical stability,and chemical affinity,using 12 different commercial separators,including polyethylene(PE),polypropylene(PP),and coated separators.At extreme compression triggered by LMA swelling,isotropic stress release by balancing the machine direction and transverse direction tensile strengths was found to be crucial for mitigating cell short-circuiting.Instead of PP separators,a PE separator that possesses a high elastic modulus and a highly connected pore structure can uniformly regulate LMA swelling.The ceramic coating reinforced short-circuiting resistance,while the cycling efficiency degraded rapidly owing to the detrimental interactions between ceramics and LMAs.This study identified the design principle of separators for practical LMBs with respect to mechanical stability and chemical affinity toward LMAs by elucidating the impacts of separator modification on the cycling performance.

关键词： chemical inertness lithium metal batteries mechanical strength polyolefin separators short-circuiting

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