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Crystalline-amorphous M@MN_x(M=Co,Fe,Ni)encapsulated in nitrogen-doped carbon for enhanced efficient and durable hydrogen evolution reaction

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Rare Metals 2024年第4期43卷 1547-1556页

作者： Yang Yang Xiao-Chuan duan Shao-Hui Guo Xian-Ming Zhang College of Materials Science and Engineering College of ChemistryKey Laboratory of Interface Science and Engineering in Advanced MaterialsTaiyuan University of TechnologyYuci030600China

Developing earth-abundant electrocatalysts for hydrogen evolution reaction(HER)is important for the sustainable energy ***,efficient and stable heterocatalysts consisting of crystalline-amorphous M@MN_(x)(M=Co,Fe,Ni)encapsulated in N-doped carbon layers supported with N-doped graphene sheets(denoted as M@MN_(x)@NC-NG)are synthesized by facile hydrothermal reaction and nitridation *** the nitriding process,metal ions in M(tzbc)_2(H_(2)O)_4(tzbc=4-(1H-1,2,4-triazol-1-yl)benzoic acid)complexes are reduced to crystalline M cores,accompanied by the formation of amorphous MN_(x)shells;the tzbc ligands are insitu carbonized to form outermost N-doped carbon(NC)layers that connect with inner MN_(x)via M-N-C motifs inherited from the complex precursors and inhibit the transition of MN_(x)from amorphous to crystalline *** Co@CoN_(x)@NC-NG catalyst exhibits excellent HER activity with small overpotentials of 45 and 64 mV at a cathode current density of 10 mA·cm^(-2)and low Tafel slopes of 40 and 85 mV·dec^(-1)in 0.5 mol·L^(-1)H_(2)SO_4 and1.0 mol·L^(-1)KOH electrolytes,*** Co@CoN_(x)@NC-NG retains 97%of the initial overpotential after 100,000 s in both acidic and alkaline *** outstanding HER performance originates from the crystalline-amorphous Co@CoN_(x)that redistributes electrons around the heterointerfaces,facilitating the conversion process of H^(+)/H_(2)O to hydrogen and thereby promoting HER *** outermost NC layers serve as the armor of Co@CoN_(x),and graphene nanosheets act as carriers of egg-like Co@CoN_(x)@NC and conduction paths for electron shuttles,ensuring stable and continuous electrocatalytic hydrogen production.

关键词： Hydrogen evolution reaction Electrocatalysts Iron group metals Heterojunction Crystalline-amorphous structure

The Negative Thermal Expansion Property of NdMnO_(3) Based on Pores Effect and Phase Transition

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Journal of Wuhan University of Technology(Materials Science) 2024年第1期39卷 39-43页

作者：李玉成张扬 ZHANG Muqun duan Rong LIU Xiteng Department of Avionics Engineering Aviation Maintenance NCO Academy of Air Force Engineering UniversityXinyang 464000China

A novel negative thermal expansion(NTE) material NdMnO_(3) was synthesized by solid-state method at 1 523 K. The crystal structure, phase transition, pores effect and negative expansion properties of NdMnO_(3) were investigated by variable temperature X-ray diffraction(XRD), scanning electron microscope(SEM) and variable temperature Raman spectra. The compound exhibits NTE properties in the orderly O' phase crystal structure. When the temperature is from 293 to 759 K, the ceramic NdMnO_(3) shows negative thermal expansion of-4.7×10^(-6)/K. As temperature increases, the ceramic NdMnO_(3) presents NTE property range from 759 to 1 007 K. The average linear expansion coefficient is-18.88×10^(-6)/K. The physical mechanism of NTE is discussed and clarified through experiments.

关键词： negative thermal expansion NdMnO_(3) pores effect phase transition

OcBSA:An NGS-based bulk segregant analysis tool for outcross populations

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Molecular Plant 2024年第4期17卷 648-657页

作者： Lingkui Zhang Yanfeng duan Zewei Zhang Lei Zhang Shumin Chen Chengcheng Cai Shaoguang duan Kang Zhang Guangcun Li Feng Cheng State Key Laboratory of Vegetable Biobreeding Key Laboratory of Biology and Genetic Improvement of Horticultural Crops of the Ministry of Agriculture and Rural AffairsKey Laboratory of Biology and Genetic Improvement of Tuber and Root Crop of Ministry of Agriculture and Rural AffairsSino-Dutch Joint Laboratory of Horticultural GenomicsInstitute of Vegetables and FlowersChinese Academy of Agricultural SciencesBeijing 100081China

Constructing inbred lines for self-incompatible species and species with long generation times is challenging,making the use of F1 outcross/segregating populations the main strategy for genetic studies of such ***,there is a lack of dedicated algorithms/tools for rapid quantitative trait locus(QTL)mapping using the F1 *** this end,we have designed and developed an algorithm/tool called OcBSA specifically for QTL mapping of F1 *** transforms the four-haplotype inheritance problem from the two heterozygous diploid parents of the F1 population into the two-haplotype inheritance problem common in current genetic studies by removing the two haplotypes from the heterozygous parent that do not contribute to phenotype segregation in the F1 *** of OcBSA on 1800 simulated F1 populations demonstrated its advantages over other currently available tools in terms of sensitivity and *** addition,the broad applicability of OcBSA was validated by QTL mapping using seven reported F1 populations of apple,pear,peach,citrus,grape,tea,and *** also used OcBSA to map the QTL for flower color in a newly constructed F1 population of potato generated in this *** OcBSA mapping result was verified by the insertion or deletion markers to be consistent with a previously reported locus harboring the ANTHOCYANIN 2 gene,which regulates potato flower *** together,these results highlight the power and broad utility of OcBSA for QTL mapping using F1 populations and thus a great potential for functional gene mining in outcrossing *** ease of use,we have developed both Windows and Linux versions of OcBSA,which are freely available at:https://***/Bioinformaticslab/OcBSA.

关键词： outcross BSA self-incompatible F1 population QTL mapping potato

CNN demodulation model with cascade parallel crossing for CPM signals

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The Journal of China Universities of Posts and Telecommunications 2024年第3期31卷 30-42页

作者： Yang Jiachen duan Ruifeng Li Chengju School of Information Science and Technology Beijing Forestry UniversityBeijing 100083China Engineering Research Center for Forestry-Oriented Intelligent Information Processing of National Forestry and Grassland Administration Beijing 100083China

The continuous phase modulation(CPM)technique is widely used in range telemetry due to its high spectral efficiency and power ***,the demodulation performance of the traditional maximum likelihood sequence detection(MLSD)algorithm significantly deteriorates in non-ideal synchronization or fading *** address this issue,this work proposes a convolutional neural network(CNN)called the cascade parallel crossing network(CPCNet)to enhance the robustness of CPM signals *** CPCNet model employs a multiple parallel structure and feature fusion to extract richer features from CPM *** approach constructs feature maps at different levels,resulting in a more comprehensive training of the model and improved demodulation *** results show that under Gaussian channel,the proposed CPCNet achieves the same bit error rate(BER)performance as MLSD method when there is no timing error,but with 1/4 symbol period timing error,the proposed method has 2 dB demodulation gain compared with CNN and convolutional long short-term memory deep neural network(CLDNN).In addition,under Rayleigh channel,the BER of the proposed method is reduced by 5%-87%compared to that of MLSD in the wide signal-to-noise ratio(SNR)region.

关键词： continuous phase modulation(CPM) convolutional neural network(CNN) maximum likelihood sequence detection(MLSD) Rayleigh fading timing error

Energy conversion due to non-ideal electric field in separatrix region of magnetotail reconnection

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Earth and Planetary Physics 2024年第5期8卷 787-796页

作者： YiNan Liu Keizo Fujimoto JianQiang Wang XiaoChuan duan School of Space and Environment Beihang University Key Laboratory of Space Environment Monitoring and Information Processing Ministry of Industry and Information Technology School of Automation Science and Electrical Engineering Beihang University

A recent satellite observation has revealed the presence of energy conversion in the separatrix region(SR) of magnetotail reconnection, driven by perpendicular components. We investigated this phenomenon by means of particle-in-cell simulations in twodimensional(2D) and three-dimensional(3D) systems. Our result indicates that in the 2D simulation, energy conversion in the SR is dominated by parallel components, with the main influencing factor being the parallel electric field, which is not consistent with the observation. However, a case that is similar to the observation is found in the 3D simulation, suggesting that the observation result may be attributed to the 3D characteristics. Our findings provide a potential explanation for the satellite observation.

关键词： magnetic reconnection energy conversion PIC simulation separatrix region

The Role of Consumer Privacy Concerns in Shaping Platform Strategy for Online Markets

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Journal of the Operations Research Society of China 2024年第2期12卷 363-386页

作者： Jin-Kun Yang Yong-Rui duan Jia-Zhen Huo School Economics and Management Tongji UniversityShanghai 200092China

We investigate the effects of consumer privacy concerns on the pricing and personal data collection strategy of an online *** online platform derives revenues from disclosing consumer information to *** compete for the information in order to enable them to price discriminate and thus derive revenues from consumer purchases.A novel aspect of our research is that we allow the online platform to sell only a subset of consumer *** develop analytical models where consumers can/cannot protect their *** analysis yields three main ***,in the monopoly case,we find that when the consumer privacy disclosure aversion cost is relatively low,it is optimal for the platform to sell all consumer information to the ***,in the duopoly case,we illustrate that when the consumer privacy disclosure aversion cost is relatively low,the platform will sell all consumer information to only one firm;when the cost is moderate,the platform will choose to sell the information of only some consumers and to only one firm;when the cost is relatively high,the platform will select only some of the consumers and sell their information to both ***,it will be better for the platform to provide the information protection service for free when the privacy cost is low.

关键词： Price discrimination User privacy Consumer information Two-sided market Privacy disclosure aversion cost

A novel pathogen Fusarium cuneirostrum causing common bean(Phaseolus vulgaris)root rot in China

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Journal of Integrative Agriculture 2024年第1期23卷 166-176页

作者： Dong Deng Wenqi Wu Canxing duan Suli Sun Zhendong Zhu Institute of Crop Sciences Chinese Academy of Agricultural SciencesBeijing 100081China

Several fungal pathogens cause root rot of common bean,among which Fusarium *** the most common pathogens causing Fusarium root rot(FRR)*** has been becoming an increasingly severe disease of common bean in China,but the species of Fusarium *** remained ***,this study was performed to identify the pathogen causing common bean root rot in Liangcheng County,Inner Mongolia,*** Fusarium-like isolates were obtained after pathogen isolation and *** pathogenicity test indicated that eight isolates caused severe disease symptoms on common bean,while 11 other isolates were not *** eight pathogenic isolates,FCL1–FCL8,were identified as Fusarium cuneirostrum by morphological characterization and phylogenetic analysis using partial sequences of EF-1α,ITS,28S,and IGS *** range test showed that the representative *** isolate FCL3 was also pathogenic to mung bean,while not pathogenic to adzuki bean,chickpea,cowpea,faba bean,pea,and ***,50 common bean and 50 mung bean cultivars were screened for resistance to FRR,and seven highly resistant or resistant cultivars of common bean were identified,while no resistant cultivars of mung bean were *** study revealed that *** was one of common bean FRR pathogens in Inner Mongolia and it could induce mung bean root rot as *** our knowledge,this is the first report of *** causing FRR of common bean in China.

关键词： Fusarium cuneirostrum fusarium root rot pathogenicity molecular phylogenetic analysis Phaseolus vulgaris

A TRUST-REGION METHOD FOR SOLVING TRUNCATED COMPLEX SINGULAR VALUE DECOMPOSITION

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Journal of Computational Mathematics 2024年第4期42卷 999-1031页

作者： Jiaofen Li Lingchang Kong Xuefeng duan Xuelin Zhou Qilun Luo School of Mathematics and Computing Science Guangxi Colleges and Universities Key Laboratory of Data Analysis and ComputationGuangxi Key Laboratory of Automatic Detecting Technology and InstrumentsGuilin University of Electronic TechnologyCenter for Applied Mathematics of Guangxi(GUET)Guilin 541004China School of Mathematical Sciences South China Normal UniversityGuangzhou 510000China School of Mathematics and Computing Science Guilin University of Electronic TechnologyGuilin 541004China School of Mathematics and Computing Science Guangxi Colleges and Universities Key Laboratory of Data Analysis and ComputationGuilin University of Electronic TechnologyCenter for Applied Mathematics of Guangxi(GUET)Guilin 541004China School of Mathematics and Statistics Yunan UniversityKunming 650000China

The truncated singular value decomposition has been widely used in many areas of science including engineering,and statistics,*** this paper,the original truncated complex singular value decomposition problem is formulated as a Riemannian optimiza-tion problem on a product of two complex Stiefel manifolds,a practical algorithm based on the generic Riemannian trust-region method of Absil et *** presented to solve the underlying problem,which enjoys the global convergence and local superlinear conver-gence *** experiments are provided to illustrate the efficiency of the proposed *** with some classical Riemannian gradient-type methods,the existing Riemannian version of limited-memory BFGS algorithms in the MATLAB toolbox Manopt and the Riemannian manifold optimization library ROPTLIB,and some latest infeasible methods for solving manifold optimization problems,are also provided to show the merits of the proposed approach.

关键词： Truncated singular value decomposition Riemannian optimization Trust-region method

Blockchain-Enabled Privacy Protection and Access Control Scheme Towards Sensitive Digital Assets Management

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China Communications 2024年第7期21卷 224-236页

作者： duan Pengfei Ma Zhaofeng Zhang Yuqing Wang Jingyu Luo Shoushan School of Cyberspace Security Beijing University of Posts and TelecommunicationsBeijing 100876China

With the growth of requirements for data sharing,a novel business model of digital assets trading has emerged that allows data owners to sell their data for monetary *** the distributed ledger of blockchain,however,the privacy of stakeholder's identity and the confidentiality of data content are ***,we proposed a blockchainenabled privacy-preserving and access control scheme to address the above ***,the multi-channel mechanism is introduced to provide the privacy protection of distributed ledger inside the channel and achieve coarse-grained access control to digital ***,we use multi-authority attribute-based encryption(MAABE)algorithm to build a fine-grained access control model for data trading in a single channel and describe its instantiation in *** analysis shows that the scheme has IND-CPA secure and can provide privacy protection and collusion *** with other schemes,our solution has better performance in privacy protection and access *** evaluation results demonstrate its effectiveness and practicability.

关键词： access control data trading MAABE multi-channel privacy preserving