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Magnesium isotopes of chlorite-rich hydrothermal sediments in the Okinawa Trough and indications for Mg cycle

Science China Earth Sciences 2023年第3期66卷 648-662页

作者： Hebin shao Shouye YANG Aiguo dong Zhongya HU Key Laboratory for Polar Science of the State Oceanic Administration Polar Research Institute of ChinaShanghai 200136China State Key Laboratory of Marine Geology Tongji UniversityShanghai 200092China Institute of Earth Sciences China University of Geosciences(Beijing)Beijing 100083China

Seafloor hydrothermal systems play a significant role in the oceanic Mg cycle due to ubiquitous deposits of secondary Mg-rich clays during the strong fluid-rock ***,the magnitude of net Mg enrichment and Mg isotopic fractionation,particularly within the medium-high temperature hydrothermal systems in felsic-hosted settings,are not well studied *** we report elemental and isotopic compositions of Mg in hydrothermal chlorite-rich sediments,volcanic materials,and terrigenous sediments collected during the IODP Expedition 331 drilled to the thick sediment-covered and felsic-hosted middle Okinawa Trough(Iheya North Knoll) in the West *** investigate the sources of Mg in chlorite and Mg isotopic behavior at medium-high temperature hydrothermal *** 1 mol/L HCl leaching,Mg isotopic compositions of chlorite-rich sediments present overall similar values in the residual fractions and bulk samples albeit with slightly higher values in the *** differentiation primarily determines the Mg isotopic compositions,showing that siliciclastic residues have slightly higher δ^(26) Mg values than the leachates dominated by carbonates and oxides/*** Mg isotopic fractionation happened in the medium-high temperature(~150°C to 260°C) felsic-hosted hydrothermal system,with Δ^(26)MgChl-SW ranging from 0.15‰ to 0.71‰ and yielding a negative correlation with *** observation suggests the preferential incorporation of heavy Mg isotopes by the secondary chlorite *** infer that the medium-high temperature hydrothermal systems can take up about 8–14% of riverine input of Mg in the arc and back-arc *** removal of aqueous Mg in porewater and vent fluids by the medium-high temperature hydrothermal alterations in the arc and back-arc basins provides constraints on the Mg budget and isotopic composition of seawater.

关键词： Hydrothermal alteration Chlorite Okinawa Trough Magnesium(Mg)isotopes Integrated Ocean Drilling Program

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Manufacture and characteristics of Al2O3 composite coating on steel substrate by SHS process

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Rare Metals 2019年第7期38卷 704-712页

作者： Hai-dong Gao Ze-Hua Wang Jia shao College of Mechanics and Materials Hohai University

Many steel components are needed to be reinforced on their surface to have a high abrasive resistance and corrosion resistance. Based on self-propagating hightemperature synthesis, a process to making Al2O3 composite coatings on mild steel substrate in atmospheric environment with the help of simple auxiliary facilities was developed successfully. A pre-coated bilayer coating was employed. The effects of Fe content in pre-coated transition layer on phase composition, porosity and interfacial bon ding were studied using scanning electron microscopy (SEM), energy-dispersive spectrum (EDS) and X-ray diffraction (XRD). The thermal shock resistance and abrasive resistance were investigated. When Fe content changes from 0 wt% to 50 wt%, the bond quality at first becomes better and then worse gradually. When Fe content is less 20 wt%, there is a small gap between the transition layer and the substrate;when Fe contents are 30 wt% and 40 wt%, working layer, the transition layer and the substrate bond together well. The working layer is mainly composed of Al2O3, Fe-Cr and Al(Cr)2O3 phases and has a dense structure with porosity of less than 1 %. The coating has a good thermal shock resistance and abrasive resistance. The abrasive resistance of the working layer is about ten times that of the substrate.

关键词： Al2O3 composite coating Self-propagating high-temperature synthesis Interfacial bonding Thermal shock resistance Abrasive resistance

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Nickel-catalyzed kinetic resolution to achieve P-chiral phosphine oxides and sec-phosphine oxides

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Science China Chemistry 2023年第9期66卷 2569-2575页

作者： Xi Zhang shao-Qiu Wang Shang-dong Yang State Key Laboratory of Applied Organic Chemistry College of Chemistry and Chemical EngineeringLanzhou UniversityLanzhou 730000China School of Pharmaceutical Science Hangzhou Medical CollegeHangzhou 310012China State Key Laboratory for Oxo Synthesis and Selective Oxidation Lanzhou Institute of Chemical PhysicsChinese Academy of SciencesLanzhou 730000China

P-Chiral phosphines and sec-phosphine oxides(SPO) are found in a diverse range of compounds that play crucial roles in various fields, including asymmetric catalysis, materials, agrochemistry, and pharmaceutical chemistry. Herein, we describe an enantioselective Ni-catalyzed kinetic resolution of racemic sec-phosphine oxides to obtain the corresponding optically pure Pchiral phosphine oxides and sec-phosphine oxides, respectively. These products are versatile chiral phosphine building blocks that can be used to construct an extensive range of P-chiral phosphines.

关键词： P-chiral phosphine oxide kinetic resolution Ni catalysis

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CONVERGENCE ANALYSIS FOR A NONCONFORMING MEMBRANE ELEMENT ON ANISOTROPIC MESHES

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Journal of Computational Mathematics 2005年第4期23卷 373-382页

作者： dong-yang Shi shao-chun Chen Ichiro Hagiwara Department of Mathematics Zhengzhou University Zhengzhou 450052 China Tokyo Institute of Technology 2-12-1 Ohokayama Megro Tokyo 152-8552 Japan

Regular assumption of finite element meshes is a basic condition of most analysis of finite element approximations both for conventional conforming elements and nonconforming elements. The aim of this paper is to present a novel approach of dealing with the approximation of a four-degree nonconforming finite element for the second order elliptic problems on the anisotropic meshes. The optimal error estimates of energy norm and L^2-norm without the regular assumption or quasi-uniform assumption are obtained based on some new special features of this element discovered herein. Numerical results are given to demonstrate validity of our theoretical analysis.

关键词： Anisotropic mesh Nonconforming finite element Optimal estimate

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AZD1775 synergizes with SLC7A11 inhibition to promote ferroptosis

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Science China Life Sciences 2025年第1期 204-218页

作者： Chen Xiong Hong Ling Yingdan Huang Hanzhi dong Bangxiang Xie Qian Hao Xiang Zhou Fudan University Shanghai Cancer Center and Institutes of Biomedical Sciences Fudan University Department of Oncology Shanghai Medical CollegeFudan University Department of Breast Surgery Fudan University Shanghai Cancer CenterFudan University Department of Oncology First Affiliated Hospital of Nanchang University Beijing Institute of Hepatology Beijing Youan HospitalCapital Medical University Beijing Engineering Research Center for Precision Medicine and Transformation of Hepatitis and Liver Cancer Key Laboratory of Breast Cancer in Shanghai Fudan University Shanghai Cancer CenterFudan University Shanghai Key Laboratory of Medical Epigenetics International Co-laboratory of Medical Epigenetics and Metabolism (Ministry of Science and Technology)Institutes of Biomedical SciencesFudan University

Tumor suppressor p53-mediated cell cycle arrest and DNA damage repair may exert cytoprotective effects against cancer therapies, including WEE1 inhibition. Considering that p53 activation can also lead to multiple types of cell death, the role of this tumor suppressor in WEE1 inhibitor-based therapies remains disputed. In this study, we reported that nucleolar stress-mediated p53 activation enhanced the WEE1 inhibitor AZD1775-induced ferroptosis to suppress lung cancer growth. Our findings showed that AZD1775 promoted ferroptosis by blocking cystine uptake, an action similar to that of Erastin. Meanwhile, inhibition of WEE1 by the WEE1 inhibitors or si RNAs induced compensatory upregulation of SLC7A11, which conferred resistance to ferroptosis. Mechanistically, AZD1775 prevented the enrichment of H3K9me3, a histone marker of transcriptional repression, on the SLC7A11 promoter by repressing the expression of the histone methyltransferase SETDB1, thereby enhancing NRF2-mediated SLC7A11 transcription. This finding was also validated using the H3K9me3 inhibitor BRD4770. Remarkably, we found that the nucleolar stress-inducing agent Actinomycin D(Act. D) inhibited SLC7A11 expression by activating p53, thus augmenting AZD1775-induced ferroptosis. Moreover, the combination of AZD1775 and Act. D synergistically suppressed wild-type p53-harboring lung cancer cell growth both in vitro and in vivo. Altogether, our study demonstrates that AZD1775 promotes ferroptosis by targeting cystine uptake but also mediates the adaptive activation of SLC7A11 through the WEE1-SETDB1 cascade and NRF2-induced transcription, and inhibition of SLC7A11 by Act. D boosts the anti-tumor efficacy of AZD1775 by enhancing ferroptosis in cancers with wild-type p53.

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TRAPEZOIDAL PLATE BENDING ELEMENT WITH DOUBLE SET PARAMETERS

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Journal of Computational Mathematics 2003年第4期21卷 513-518页

作者： shao-chunChen dong-yangShi IchiroHagiwara DepartmentofMathematics ZhengzhouUniversityZhengzhou450052China TokyoInstituteofTechnology 2-12-10hokayamaMegroTokyo152-8552Japan

Using double set parameter method, a 12-parameter trapezoidal plate bending element is presented. The first set of degrees of freedom, which make the element convergent, are the values at the four vertices and the middle points of the four sides together with the mean values of the outer normal derivatives along four sides. The second set of degree of freedom, which make the number of unknowns in the resulting discrete system small and computation convenient are values and the first derivatives at the four vertices of the element. The convergence of the element is proved.

关键词： Plate bending problem Nonconforming finite element Double set parameter method.

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论“慎捕”的法规范控制体系及实践问题破解

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武汉大学学报（哲学社会科学版） 2025年第1期78卷 172-184页

作者：董坤中国社会科学院法学研究所中国社会科学院大学北京100720

历次修法中涉及逮捕的制度机制的演进轨迹和条文变化的内在逻辑表明,为实现“慎捕”目标,《中华人民共和国刑事诉讼法》(以下简称《刑事诉讼法》)已初步构筑起一套结构严谨、衔接有序、层次分明的关于逮捕权的法规范控制体系。该体系在... 详细信息

历次修法中涉及逮捕的制度机制的演进轨迹和条文变化的内在逻辑表明,为实现“慎捕”目标,《中华人民共和国刑事诉讼法》(以下简称《刑事诉讼法》)已初步构筑起一套结构严谨、衔接有序、层次分明的关于逮捕权的法规范控制体系。该体系在事前的权力配置阶段“两次分离”逮捕权,以具体社会危险性评估为重心改造逮捕要件;在事中的权力行使阶段以“兼听则明”为原则设计了充分听取控辩双方意见的审查逮捕机制;在事后的权力制约阶段要求检察院、法院及时纠正撤销错捕决定,释放犯罪嫌疑人。从司法办案的角度来看,现有的法规范控制体系在规则制定和程序执行时仍有不足和缺漏,如逮捕权分离不彻底,控辩意见“兼听”机制保障不充分,径行逮捕条件设计机械、不周延,当事人对错捕的救济途径缺失等。本轮《刑事诉讼法》修改应坚持“实践—规范”的互动逻辑,关注司法实践,将解决和弥补逮捕中的权力运行失范和权利保障不足等现实问题作为修法方向,破难题、开新局,不断推动中国刑事诉讼法治现代化进程。

关键词：慎捕法规范控制体系径行逮捕权利保障《刑事诉讼法》修改

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Magnetron sputtered nickel oxide with suppressed interfacial defect states for efficient inverted perovskite solar cells

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Journal of Energy Chemistry 2025年第1期100卷 348-355页

作者： Guoqiang Ma Qin Tan Zhaoning Li Jingwei Xiu Jiafeng Wang Tianle Cheng dong He Qiang Sun Xuhang Ma Francesco Lamberti Zhubing He Department of Materials Science and Engineering Institute of Innovative Materials (I2M) Shenzhen Key Laboratory of Full Spectral Solar Electricity Generation (FSSEG)Southern University of Science and Technology (SUSTech) Core Research Facilities Southern University of Science and Technology Department of Chemical Sciences Department of Industrial Engineering University of Padova

Widely used spin-coated nickle oxide （NiOx） based perovskite solar cells often suffer from severe interfacial reactions between the NiOxand adjacent perovskite layers due to surface defect states,which inherently impair device performance in a long-term view,even with surface molecule *** this study,we developed high-quality magnetron-sputtered NiOxthin films through detailed process optimization,and compared systematically sputtered and spin-coated NiOxthin film surfaces from materials to *** sputtered NiOxfilms exhibit improved crystallinity,smoother surfaces,and significantly reduced Ni3+or Ni vacancies compared to their spin-coated ***,the interface between the perovskite and sputtered NiOxfilm shows a substantially reduced density of defect *** solar cells （PSCs） fabricated with our optimally sputtered NiOxfilms achieved a high power conversion efficiency （PCE） of up to 19.93%and demonstrated enhanced stability,maintaining 86.2% efficiency during 500 h of maximum power point tracking under one standard sun ***,with the surface modification using (4-(2,7-dibromo-9,9-dimethylacridin-10（9H）-yl)butyl)p hosphonic acid （DMAcPA）,the device PCE was further promoted to 23.07%,which is the highest value reported for sputtered NiOxbased PSCs so far.

关键词： Nickle oxide Magnetron sputter Defect Stability Perovskite solar cell

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A New Approach for Controlling Chaos Based on Direct Optimizing Predictive Control

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Communications in Theoretical Physics 2006年第3期45卷 473-476页

作者： LI dong-Mei YANG shao-Zhen School of Economy and Management Hebei University of Science and Technology Shijiazhuang 050018 China

We introduce the predictive control theory into predictive control algorithm based on a neural network model the study of chaos control and propose a direct optimizing The proposed control system stabilizes the chaotic motion in an unknown chaotic system onto the desired target trajectory. Compared with the existing similar algorithms, the proposed control system has faster response, so it requires much shorter time for the stabilization of the chaotic systems. The proposed approach can control hyperchaos and the algorithm is simple. The convergence of the control algorithm and the stability of the control system can be guaranteed. The theoretic analysis and simulations demonstrate the effectiveness of the algorithm.

关键词： vchaos control predictive control chaotic system neural networks

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Optimal Output Power Control of Switched Reluctance Generator at a Constant Speed

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Journal of Beijing Institute of Technology 2020年第4期29卷 435-444页

作者： Liwei shao Lei dong Lulu Ling School of Automation Beijing Institute of TechnologyBeijing 100081China Zhongshan Research Institute Beijing Institute of TechnologyZhongshan 528437GuangdongChina

In order to control the output power of a switched reluctance generator(SRG)at a constant speed,the output power of SRG is theoretically analyzed by using freewheeling ***,through a theoretical analysis,a finite element simulation and an experiment,it was verified that the output power of SRG cannot be improved by using freewheeling control with a single pulse control method(SPCM).Then,the maximum output power can be obtained by optimizing the turn off angles of SPCM at a constant speed,and at the same time,the formula of the optimal turn-off angle was presented,which meets the criterion for the output power ***,numerical simulation and experimental results demonstrated the validity of the theoretical analysis.

关键词： freewheeling technique output power maximization single pulse control switched reluctance generator(SRG)

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