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Layered double hydroxide(LDH)-based materials:A mini-review on strategies to improve the performance for photocatalytic water splitting

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Journal of Energy Chemistry 2022年第1期31卷 406-431,I0011页

作者： Hanane Boumeriame Eliana S.Da Silva Alexey S.Cherevan Tarik Chafik Joaquim L.Faria dominik eder Laboratory of Separation and Reaction Engineering-Laboratory of Catalysis and Materials(LSRE-LCM) Faculdade de EngenhariaUniversidade do PortoRua Dr Roberto Frias s/n4200-465 PortoPortugal Institute of Materials Chemistry Technische Universicat Wien(TU Wien)Getreidemarkt 9Vienna 1060Austria Laboratory of Chemical Engineering and Valorization of Resources(LGCVR-UAE/L01FST).Faculte des Sciences et Techniques Universite Abdelmalek EssaadiTangierMorocco

The high energy demand we currently face in society and the subsequent large consumption of fossil fuels cause its depletion and increase the pollution *** quest for the production of clean energy from renewable and sustainable sources remains *** conversion of solar energy into hydrogen via the water-splitting process,assisted by pho tores pons ive semiconductor catalysts,is one of the most promising *** progress has been made on water splitting in the past few years and a variety of photocatalysts active not only under ultra-violet(UV) light but especially with the visible part of the electromagnetic spectrum have been *** double hydroxides(LDH)-based materials have emerged as a promising class of nanomaterials for solar energy applications owing to their unique layered structure,compositional flexibility,tunable bandgaps,ease of synthesis and low manufacturing *** review covers the most recent research dedicated to LDH materials for photocatalytic water-splitting applications and encompasses a range of synthetic strategies and post-modifications used to enhance their ***,we provide a thorough discussion of the experimental conditions crucial to obtaining improved photoactivity and highlight the impact of some specific parameters,namely,catalysts loading,cocatalysts,sacrificial agents,and irradiation *** review provides the necessary tools to select the election technique for adequately enhancing the photoactivity of LDH and modified LDH-based materials and concludes with a critical summary that outlines further research directions.

关键词： Layered double hydroxides Water splitting Photocatalysis Hydrogen generation Oxygen evolution Nanomaterials

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