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Boron Nitride-Integrated Lithium Batteries:Exploring Innovations in Longevity and Performance

Energy & Environmental Materials 2024年第6期7卷 13-40页

作者： Shayan Angizi Sayed Ali Ahmad Alem Mahdi Torabian Maryam Khalaj dmitri golberg Amir Pakdel Department of Chemical Engineering McMaster University1280 Main St WHamiltonONL8S 4L7 Canada Institute of Chemistry of Polymeric Materials Montanuniversität LeobenOtto-Glöckel-Strasse 2A-8700 LeobenAustria Department of Chemistry Materials and Chemical EngineeringPolitecnico di MilanoPiazza Leonardo da Vinci 3220133 MilanItaly Department of Materials Science and Engineering Northwestern UniversityEvanstonIL60208 USA Centre for Materials Science and School of Chemistry and Physics Queensland University of Technology(QUT)2 GeorgeBrisbaneQLD4000 Australia Research Centre for Materials Nanoarchitectonics(MANA) National Institute for Materials Science(NIMS)Namiki 1Ibaraki3050044 Japan Department of Mechanical Manufacturing and Biomedical EngineeringTrinity College DublinThe University of DublinDublinD02PN40 Ireland

The current global warming,coupled with the growing demand for energy in our daily lives,necessitates the development of more efficient and reliable energy storage *** batteries(LBs)are at the forefront of emerging power sources addressing these *** studies have shown that integrating hexagonal boron nitride(h-BN)nanomaterials into LBs enhances the safety,longevity,and electrochemical performance of all LB components,including electrodes,electrolytes,and separators,thereby suggesting their potential value in advancing eco-friendly energy *** review provides an overview of the most recent applications of h-BN nanomaterials in *** begins with an informative introduction to h-BN nanomaterials and their relevant properties in the context of LB ***,it addresses the challenges posed by h-BN and discusses existing strategies to overcome these limitations,offering valuable insights into the potential of BN *** review then proceeds to outline the functions of h-BN in LB components,emphasizing the molecular-level mechanisms responsible for performance ***,the review concludes by presenting the current challenges and prospects of integrating h-BN nanomaterials into battery research.

关键词： electrode electrolyte hexagonal boron nitride lithium battery separator

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Recent Progress in One-dimensional ZnS Nanostructures:Syntheses and Novel Properties

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Journal of Materials Science & Technology 2008年第4期24卷 512-519页

作者： Yoshio BANDO dmitri golberg Nanoscale World Premier International Center for Materials Nanoarchitectonics and Nanoscale Materials Center National Institute for Materials ScienceNamiki 1-1TsukbaIbaraki 305-0044Japan

In this review, the progress made during the last two years with respect to the syntheses and novel properties of one-dimensional （1D） ZnS nanostructures is presented. Primarily the research on 1D ZnS nanostructures has been of growing interest owing to their promising applications in nanoscale optoelectronic devices. Diverse 1D ZnS nanostructures with delicately-tuned morphologies, sizes, and microstructures have been synthesized through relatively simple and well-controlled techniques. Some novel properties of the nanomaterials have been explored and the relationships between their structural features and functions have been understood gradually.

关键词： Semiconductors ZnS Nanomaterlals Nanostructures Filed-emitters

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One-dimensional ZnS-based Hetero-,Core/shell and Hierarchical Nanostructures

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Journal of Materials Science & Technology 2008年第4期24卷 520-528页

作者： Ujjal K.Gautam Yoshio BANDO dmitri golberg Nanoscale World Premier International Center for Materials Nanoarchitectonics and Nanoscale Materials Center National Institute for Materials ScienceNamiki 1-1TsukbaIbaraki 305-0044Japan

A focus of the current nanotechnology has shifted from routine fabrication of nanostructures to designing functional electronic devices and realizing their immense potentials for applications. Due to infusion of multi-functionality into a single system, the utilization of hetero-, core/shell and hierarchical nanostructures has become the key issue for building such devices. ZnS, due to its direct wide bandgap, high index of refraction, high transparency in the visible range and intrinsic polarity, is one of the most useful semiconductors for a wide range of electronics applications. This article provides a dense review of the state-of-the-art research activities in one-dimensional （1D） ZnS-based hetero-, core/shell and hierarchical nanostructures. The particular emphasis is put on their syntheses and applications.

关键词： Heterostructures Core/shell Hierarchical structures ZnS Nanodevices

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One-Dimensional(1-D) Nanoscale Heterostructures

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Journal of Materials Science & Technology 2008年第4期24卷 541-549页

作者： Guozhen SHEN Di CHEN Yoshio BANDO dmitri golberg National Institute for Materials Science Tsukuba 305-0044 Ibaraki Japan Department of Electrical Engineering University of Southern California Los Angeles CA 90089 USA

One-dimensional （l-D） nanostructures have been attracted much attention as a result of their exceptional properties, which are different from bulk materials. Among 1-D nanostructures, 1-D heterostructures with modulated compositions and interfaces have recently become of particular interest with respect to potential applications in nanoscale building blocks of future optoelectronic devices and systems. Many kinds of methods have been developed for the synthesis of 1-D nanoscale heterostructures. This article reviews the most recent development, with an emphasize on our own recent efforts, on 1-D nanoscale heterostructures, especially those synthesized from the vapor deposition methods, in which all the reactive precursors are mixed together in the reaction chamber. Three types of 1-D nanoscale heterostructures, defined from their morphologies characteristics, are discussed in detail, which include 1-D co-axial core-shell heterostructures, 1-D segmented heterostructures and hierarchical heterostructures. This article begins with a brief survey of various methods that have been developed for synthesizing 1-D nanoscale heterostructures and then mainly focuses on the synthesis, structures and properties of the above three types of nanoscale heterostructures. Finally, this review concludes with personal views towards the topic of 1-D nanoscale heterostructures.

关键词： Nanostructures Heterostructures One-dlmenslonal Chemical vapor deposition

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Stabilising Cobalt Sulphide Nanocapsules with Nitrogen-Doped Carbon for High-Performance Sodium-Ion Storage

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Nano-Micro Letters 2020年第4期12卷 29-40页

作者： Yilan Wu Rohit RGaddam Chao Zhang Hao Lu Chao Wang dmitri golberg Xiu Song Zhao School of Chemical Engineering The University of QueenslandSt LuciaBrisbaneQLD 4072Australia School of Chemistry Physics and Mechanical EngineeringScience and Engineering FacultyQueensland University of TechnologyBrisbaneQLD 4001Australia Institute of Materials for Energy and Environment College of Materials Science and EngineeringQingdao University308 Ningxia RoadQingdao 266071People’s Republic of China

Conversion-type anode materials with a high charge storage capability generally su er from large volume expansion, poor electron conductivity, and sluggish metal ion transport kinetics. The electrode material described in this paper, namely cobalt sulphide nanoparticles encapsulated in carbon cages(Co9S8@NC), can circumvent these problems. This electrode material exhibited a reversible sodium-ion storage capacity of 705 mAh g^-1 at 100 mA g^-1 with an extraordinary rate capability and good cycling stability. Mechanistic study using the in situ transmission electron microscope technique revealed that the volumetric expansion of the Co9S8 nanoparticles is bu ered by the carbon cages, enabling a stable electrode–electrolyte interface. In addition, the carbon shell with high-content doped nitrogen significantly enhances the electron conductivity of the Co9S8@NC electrode material and provides doping-induced active sites to accommodate sodium ions. By integrating the Co9S8@NC as negative electrode with a cellulose-derived porous hard carbon/graphene oxide composite as positive electrode and 1 M NaPF6 in diglyme as the electrolyte, the sodium-ion capacitor full cell can achieve energy densities of 101.4 and 45.8 Wh kg^-1 at power densities of 200 and 10,000 W kg^-1, respectively.

关键词： Cobalt sulphide Nitrogen-doped carbon Core–shell structure Sodium-ion capacitors

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Recent Progress on Fabrications and Applications of Boron Nitride Nanomaterials:A Review

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Journal of Materials Science & Technology 2015年第6期31卷 589-598页

作者： Xiang-Fen Jiang Qunhong Weng Xue-Bin Wang Xia Li Jun Zhang dmitri golberg Yoshio Bando World Premier International Center for Materials Nanoarchitectonics(WPI-MANA) National Institute for Materials Science(NIMS)Namiki 1-1TsukubaIbaraki 3050044Japan International Center for Young Scientists(ICYS) NIMSNamiki 1-1TsukubaIbaraki 3050044Japan College of Engineering and Applied Sciences Nanjing University School of Materials Science and Engineering Hebei University of Technology

Boron nitride(BN) nanostructures with complementary functions to their carbon counterparts are one of the most intriguing *** we devote a compact review on the syntheses of BN nanomaterials:typical zero-dimensional(OD) fullerenes and nanoparticles,one-dimensional(1D) nanotubes and nanoribbons,two-dimensional(2D) nanosheets as well as three-dimensional(3D) nanoporous *** low-dimensional quantum confinement and surface effects with unique physical and chemical properties of BN,*** electric insulation,wide band gap,and high chemical and thermal stability,BN nanomaterials have drawn particular attention in a variety of potential applications,***,functional composites,hydrogen accumulators,and advanced insulators,which are also reviewed.

关键词： Boron nitride Nanoparticle Nanotube Nanosheet Poro

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Nanotubes in a Gradient Electric Field as Revealed by STM TEM Technique

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Nano Research 2008年第2期1卷 166-175页

作者： dmitri golberg Pedro M.F.J.Costa Masanori Mitome Yoshio Bando Nanoscale Materials Center Namiki 1-1TsukubaIbaraki 305-0044Japan International Center for Materials Nanoarchitectonics(MANA) National Institute for Materials ScienceNamiki 1-1TsukubaIbaraki 305-0044Japan Center for Research in Ceramics and Composite Materials University of Aveiro3810-193 AveiroPortugal

We have investigated the behavior of two nanotube systems,carbon and boron nitride,under controlled applied voltages in a high-resolution transmission electron microscope(TEM)equipped with a scanning tunneling microscope(STM)*** nanotubes(or thin bundles)were positioned between a piezo-movable gold electrode and a biased(up to±140 V)STM tip inside the pole-piece of the *** structures studied include double-and multi-walled carbon nanotubes(the latter having diverse morphologies due to the various synthetic procedures utilized),few-layered boron nitride nanotube bundles and multi-walled boron nitride nanotubes(with or without functionalized surfaces).The electrical breakdown,physical failure,and electrostatic interactions are documented for each system.

关键词： Carbon nanotubes boron nitride nanotubes transmission electron microscope scanning tunneling microscope

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Boron nitride nanotube growth via boron oxide assisted chemical vapor transport-deposition process using LiNO3 as a promoter

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Nano Research 2015年第6期8卷 2063-2072页

作者： Andrei T. Matveev Konstantin L. Firestein Alexander E. Steinman Andrey M. Kovalskii Oleg I. Lebedev Dmitry V. Shtansky dmitri golberg National University of Science and Technology 'MISIS' Leninskiy prospect 4 Moscow 119049 Russia CRISMAT UMR 6508 CNRS-ENSICAEN 6BdMarechalJuin Caen 14050 France Institute for Materials Science (NIMS) Namiki 1 Ibaraki Tsukuba 3050044 Japan

High-purity straight and discrete multiwalled boron nitride nanotubes （BNNTs） were grown via a boron oxide vapor reaction with ammonia using LiNO3 as a promoter. Only a trace amount of boron oxide was detected as an impurity in the BNNTs by energy-dispersive X-ray （EDX） and Raman spectroscopies. Boron oxide vapor was generated from a mixture of B, FeO, and MgO powders heated to 1,150 ℃, and it was transported to the reaction zone by flowing ammonia. Lithium nitrate was applied to the upper side of a BN bar from a water solution. The bar was placed along a temperature gradient zone in a horizontal tubular furnace. BNNTs with average diameters of 30-50 nm were mostly observed in a temperature range of 1,280-1,320 ℃. At higher temperatures, curled polycrystalline BN fibers appeared. Above 1,320 ℃, the number of BNNTs drastically decreased, whereas the quantity and diameter of the fibers increased. The mechanism of BNNT and fiber growth is proposed and discussed.

关键词： boron nit-ride nanotubes CVD lithium nitrate lithium borate BNNT growth mechanism

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Nacre-bionic nanocomposite membrane for efficient in-plane dissipation heat harvest under high temperature

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Journal of Materiomics 2021年第2期7卷 219-225页

作者： Jiemin Wang Dan Liu Quanxiang Li Cheng Chen Zhiqiang Chen Minoo Naebe Pingan Song David Portehault Christopher J.Garvey dmitri golberg Weiwei Lei Institute for Frontier Materials Deakin UniversityWaurn Ponds CampusLocked Bag 20000Victoria3220Australia Center for Future Materials University of Southern QueenslandToowoomba4350Australia Sorbonne Universite CNRSLaboratoire de Chimie de La Matiere Condensee de Paris(CMCP)4 Place JussieuF-75005ParisFrance Australia Nuclear Science and Technology Organization(ANSTO) SydneyNew South Wales2232Australia Centre for Materials Science and School of Chemistry and Physics Queensland University of Technology(QUT)BrisbaneQLD4001Australia

Waste heat management holds great promise to create a sustainable and energy-efficient society as well as contributes to the alleviation of global *** and converting this waste heat in order to improve the efficiency is a major *** we report biomimetic nacre-like hydroxyl-functionalized boron nitride(BN)-polyimide(PI)nanocomposite membranes as efficient 2D in-plane heat conductor to dissipate and convert waste heat at high *** hierarchically layered nanostructured membrane with oriented BN nanosheets gives rise to a very large anisotropy in heat transport properties,with a high in-plane thermal conductivity(TC)of 51 Wm^(-1) K^(-1) at a temperature of~300 C,7314%higher than that of the pure *** membrane also exhibits superior thermal stability and fire resistance,enabling its workability in a hot *** addition to cooling conventional exothermic electronics,the large TC enables the membrane as a thin and 2D anisotropic heat sink to generate a large temperature gradient in a thermoelectric module(△T=23 ℃)through effective heat diffusion on the cold side under 220 C *** waste heat under high temperature is therefore efficiently harvested and converted to power electronics,thus saving more thermal energy by largely decreasing consumption.

关键词： Boron nitride nanosheets Nanocomposite membrane Nacre-biomimetic High temperature heat spreader In-plane dissipation heat

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二维材料中的几何位点在储能中的作用

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科学新闻 2019年第2期 149-149页

作者： Yijun Yang Xizheng Liu Zhian Zhu Yeteng Zhong Yoshio Bando dmitri golberg 姚建年王熙中国科学院化学研究所北京交通大学

文章简介二维纳米材料被广泛地用作锂/钠离子电池的电极材料,以提高电池的能量和功率密度以及循环稳定性,并满足电动车辆和发电站不断增长的需求。本综述利用"几何驱动"这个概念来阐明二维材料中的几何位点与电化学性能的相互作用

关键词：二维材料

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