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Recent progress in constructing fluorinated solid-electrolyte interphases for stable lithium metal anodes

International Journal of Minerals,Metallurgy and Materials 2025年第2期32卷 270-291页

作者： di zhang Pengfei Lv Wei Qin Xin He Yuanhua He Civil Aircraft Fire Science and Safety Engineering Key Laboratory of Sichuan Province College of Civil Aviation Safety EngineeringCivil Aviation Flight University of ChinaGuanghan 618307China School of Chemical Engineering Sichuan UniversityChengdu 610065China

Lithium metal batteries(LMBs)are emerging as a promising energy storage solution owing to their high energy density and specific ***,the non-uniform plating of lithium and the potential rupture of the solid-electrolyte interphase(SEI)during extended cycling use may result in dendrite growth,which can penetrate the separator and pose significant short-circuit *** a stable SEI is essential for the long-term operation of the ***-rich SEI has garnered significant attention for its ability to effectively passivate electrodes,regulate lithium deposition,and inhibit electrolyte *** the structural components and preparation methods of existing fluorinated SEI is crucial for optimizing lithium metal anode *** paper reviews the research on optimizing LiF passivation interfaces to protect lithium metal *** focuses on four types of compositions in fluorinated SEI that work synergistically to enhance SEI *** instance,combining compounds with LiF can further enhance the mechanical strength and ionic conductivity of the *** metals with LiF significantly improves electrochemical performance at the SEI/anode interface,with a necessary focus on reducing electron tunneling ***,incorporating polymers with LiF offers balanced improvements in interfacial toughness and ionic conductivity,though maintaining structural stability over long cycles remains a critical area for future *** alloys combined with LiF increase surface energy and lithium affinity,challenges such as dendrite growth and volume expansion *** summary,this paper emphasizes the crucial role of interfacial structures in LMBs and offers comprehensive guidance for future design and development efforts in battery technology.

关键词： LiF lithium metal anodes solid-electrolyte interphase interface cycling stability

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A mechanical reinforced and antifreezing polyacrylate hydrogel electrolyte for high-performance zinc-ion batteries

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Nano Research 2025年第1期18卷 341-350页

作者： Zili zhang Ruolin Wang Hongfei Lu di zhang Yu Zhao Jing Xu Bin Sun Zhi-Min Dang Yang Jin School of Electrical and Information Engineering Zheng Zhou UniversityZhengzhou 450001China State Key Lab of New Ceramics and Fine Processing School of Materials Science and EngineeringTsinghua UniversityBeijing 100084China

The operation of aqueous zinc-ion batteries in flexible energy storage field is plagued by the uncontrollable growth of Zn-dendrite and inevitable freeze of water below 0 ℃.Therefore,it is necessary to design a hydrogel electrolyte with good mechanical property and freezing resistance to uniform the Zn-deposition and resist flexibility loss at low *** find that the mechanical property(strength and toughness)of hydrogel electrolyte has a significant impact on the suppression of dendrite growth and the uniform deposition of zinc ***,a polyacrylate hydrogel is prepared in one step by ultraviolet(UV)curing method with Zn(CF_(3)SO_(3))_(2)salt and polyvinyl alcohol(PVA)addition to increase the antifreezing ability and mechanical *** adsorption of water molecules by 2-hydroxyethyl acrylate(HEA)and PVA reduces the freezing point of the hydrogel,which is beneficial for enhancing the electrochemical stability at low *** this basis,the Zn-symmetrical battery with hydrogel electrolyte has a long lifespan of 4710 h at 0.5 mA·cm^(-2)and 0.5 mAh·cm^(-2)at room ***,the hydrogel electrolyte exhibits an outstanding stability at low temperature of^(-2)0 ℃,the lifespan of symmetrical battery reaches to 4000 h at 0.5 mA·cm^(-2)and 0.5 mAh·cm^(-2).The assembled full cell with NaV3O8·1.5H_(2)O(NVO)cathode and hydrogel electrolyte possesses a high capacity retention ratio of 77%after 10,000 cycles at^(-2)0 ℃.The flexible cell can power light-emitting diode(LED)lamp under bending,warping and cutting without liquid leakage and an electronic watch at the operating temperature of^(-2)0 ℃.

关键词： zinc ion battery hydrogel electrolyte mechanical enhancement freezing resistance

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Research on the Performance of Supercritical CO_2 Dry Gas Seal with different Deep Spiral Groove

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Journal of Thermal Science 2019年第3期28卷 547-558页

作者： DU Qiuwan zhang di MOE Key Laboratory of Thermo-Fluid Science and Engineering Xi'an Jiaotong University

The performance of supercritical CO_2(SCO_2) dry gas seal(DGS) with different deep spiral groove is investigated with the thermal-fluid-solid coupling method. The performance parameters of DGSs with five different kinds of grooves are obtained. The influence of inlet temperature, inlet pressure, velocity and film thickness on performance is analyzed compared with air DGS. The average film pressure, open force and leakage decrease while the average face temperature and flow velocity increase as the spiral groove number increases. The average film pressure, average face temperature, open force and leakage of DGS with radial different deep groove are higher than those of DGS with circumferential different deep groove respectively under the same spiral groove number while the average flow velocity is the opposite. SCO_2 DGS can generate larger average film pressure, open force and leakage with lower average face temperature than air DGS. SCO_2 DGS could maintain better sealing performance despite larger leakage with the variations of inlet temperature, inlet pressure, velocity and film thickness. The variables hold a more remarkable influence on SCO_2 DGS compared with air DGS.

关键词： supercritical carbon dioxide different deep spiral groove dry gas seal thermal-fluid-solid coupling method

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Tail Bounds for the Supremums of Empirical Processes over Unbounded Classes of Functions

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Acta Mathematica Sinica,English Series 2006年第2期22卷 339-346页

作者： di Xin zhang Department of Finance Business SchoolNanjing University

So far the study of exponential bounds of an empirical process has been restricted to a bounded index class of functions. The case of an unbounded index class of functions is now studied on the basis of a new symmetrization idea and a new method of truncating the original probability space; the exponential bounds of the tail probabilities for the supremum of the empirical process over an unbounded class of functions are obtained. The exponential bounds can be used to establish laws of the logarithm for the empirical processes over unbounded classes of functions.

关键词： empirical process tail bound unbounded class of functions

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The blow-up of the conformal mean curvature flow

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Science China Mathematics 2020年第4期63卷 733-754页

作者： Xingxiao Li di zhang College of Mathematics and Information Sciences Henan Normal UniversityXinxiang 453007China

In this paper, we introduce and study the conformal mean curvature flow of submanifolds of higher codimension in the Euclidean space R^n. This kind of flow is a special case of a general modified mean curvature flow which is of various origination. As the main result, we prove a blow-up theorem concluding that, under the conformal mean curvature flow in R^n, the maximum of the square norm of the second fundamental form of any compact submanifold tends to infinity in finite time. Furthermore, we also prove that the external conformal forced mean curvature flow of a compact submanifold in R^n with the same pinched condition as Andrews-Baker's will be convergent to a round point in finite time.

关键词： conformal mean curvature flow conformal external force blow-up of the curvature round point

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Robust load-balanced backbone-based multicast routing in mobile opportunistic networks

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Frontiers of Computer Science 2023年第4期17卷 109-125页

作者： di zhang Dong ZHAO uadong MA Beijing Key Laboratory of Intelligent Telecommunications Software and Multimedia Beijing University of Posts and TelecommunicationsBeijing 100876China

Mobile opportunistic network(MON)is an efficient way of communication when there is no persistent connection between *** in MONs can be used to efficiently deliver messages to multiple destination ***,because multiple destination nodes are involved,multicast routing is more complex than unicast and brings a higher communication ***-based routing can effectively reduce the network overhead and the complexity of routing ***,the load of backbone nodes is larger than that of regular *** the backbone node’s buffer is exhausted,it will have a significant impact on the performance of the routing *** balancing can improve the ability of backbone to deal with the change of network load,and backbone maintenance algorithm can provide backbone *** this paper,we propose a robust load-balanced backbone-based multicast routing scheme in *** the backbone construction algorithm,we transform the problem of backbone construction into a multi-objective optimization problem,and propose a multi-objective evolutionary algorithmbased backbone construction algorithm,namely LBMBCMOEA *** addition,in order to increase the robustness of the backbone-based routing scheme,we propose a localized multicast backbone maintenance algorithm(MBMA)to deal with the buffer exhaustion of backbone *** a backbone node’s residual buffer is insufficient,MBMA algorithm selects other nodes to replace the backbone *** results on extensive simulations show that when considering the node buffer size constraints,compared with previous backbone-based multicast routing schemes,our proposed algorithm has better performance,and when the node’s residual buffer is insufficient,MBMA algorithm can significantly improve the performance of the backbone-based multicast routing scheme.

关键词： mobile opportunistic network multicast multiobjective optimization backbone construction backbone maintenance

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Post-Cloud Computing Paradigms： A Survey and Comparison

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Tsinghua Science and Technology 2017年第6期22卷 714-732页

作者： Yuezhi Zhou di zhang Naixue Xiong Department of Computer Science and Technology Tsinghua National Laboratory for Information Science and Technology Tsinghua University Beijing 100084 China Department Mathematics and Computer Science Northeastern State University Tahlequah OK 74464 USA.

With the rapid development of pervasive intelligent devices and ubiquitous network technologies, new network applications are emerging, such as the Internet of Things, smart cities, smart grids, virtual/augmented reality, and unmanned vehicles. Cloud computing, which is characterized by centralized computation and storage,is having difficulty meeting the needs of these developing technologies and applications. In recent years, a variety of network computing paradigms, such as fog computing, mobile edge computing, and dew computing, have been proposed by the industrial and academic communities. Although they employ different terminologies, their basic concept is to extend cloud computing and move the computing infrastructure from remote data centers to edge routers, base stations, and local servers located closer to users, thereby overcoming the bottlenecks experienced by cloud computing and providing better performance and user experience. In this paper, we systematically summarize and analyze the post-cloud computing paradigms that have been proposed in recent years. First, we summarize the main bottlenecks of technology and application that cloud computing encounters. Next, we analyze and summarize several post-cloud computing paradigms, including fog computing, mobile edge computing, and dew ***, we discuss the development opportunities of post-cloud computing via several examples. Finally, we note the future development prospects of post-cloud computing.

关键词： cloud computing fog computing edge computing mobile edge computing dew computing

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Minimizing serrated flow in Al-Mg alloys by electroplasticity

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Journal of Materials Science & Technology 2019年第6期35卷 1108-1112页

作者： Hui Xu Xuebing Liu di zhang Xinfang zhang School of Metallurgical and Ecological Engineering University of Science and Technology Beijing Beijing 100083 China State Key Laboratory of Advanced Metals and Materials University of Science and Technology Beijing Beijing 100083 China

Serrated flow under the influence of electroplasticity in Al-Mg alloys is investigated within the dynamic strain aging interpretations of the Portevin-Le Chatelier effect. The stability of plastic region is extended by the pulsed electric current with the increase of critical strain and the extension of waiting ***, the dislocation density, affecting the plastic instabilities due to the interaction between solute atoms and mobile dislocations, is greatly reduced, which plays a dominant role in the suppression of serrated flow.

关键词： Portevin-Le Chatelier effect Dynamic strain aging dislocation Electroplastic effect Aluminum alloy

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Si-induced insertion of Li into SiC to form Li-rich SiC twin crystal

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Particuology 2023年第3期74卷 56-63页

作者： di zhang Chenxi zhang Feng Lu Hairong Jiang Fei Wei Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology Department of Chemical EngineeringTsinghua UniversityBeijing100084China

The energy density of Li-ion batteries is closely related to the capacity and average voltage of cathode ***,current cathode materials either have low capacity or voltage,which limits the development of high-energy-density Li-ion *** has given challenge to many attempts to develop new cathode materials with high capacity and *** this study,we find that Li easily inserts into the(111)plane of SiC in the presence of Si,and a well-organized Li-rich SiC twin crystal is ***-visible diffuse reflectance spectra and electrochemical test results suggest that this Li-rich SiC twin crystal possesses the band gap energy of 3.5 eV and charging capacity of 1979 mAh/g at the current density of 200 mA/g,making it a promising candidate for the cathode material in high-capacity Li-ion batteries.X-ray photoelectron spectroscopy and high-resolution transmission electron microscopy results reveal that Si-induced Li insertion contributes to the changes in the surface species and structure of pristine *** findings suggest that the Li-rich SiC twin crystal raises new possibilities for the development of high-capacity cathode materials and merits further investigation to expand its application scope.

关键词： Si Li insertion SiC Li-rich twin crystal CathodeLi-ion batteries

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Gibberellins,brassinolide,and ethylene signaling were involved in flower differentiation and development in Nelumbo nucifera

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Horticultural Plant Journal 2022年第2期8卷 243-250页

作者： Jiangyuan Sheng Xin Li di zhang Department of Landscape Science and Engineering School of DesignShanghai Jiao Tong UniversityShanghai 200240China Administrative Station of Suzhou Wetland Protection SuzhouJiangsu 215008China

Hormones play important roles in vegetative and reproductive processes;however,the regulatory roles of hormones in Nelumbo nucifera(Lotus)growth and development are *** this study,nine types of endogenous hormones,including gibberellins(GA_1,GA_3,and GA_4),indole-3-acetic acid(IAA),brassinolide(BR),ethylene(ETH),jasmonic acid(JA),abscisic acid(ABA),and zeatin(ZT)were detected in dormant shoot tips,vegetative shoot tips,developing leaf buds,and developing flower buds of *** results indicated that GA,ETH,and BR signaling can promote vegetative and reproductive development of *** signaling regulates plant height and stimulates flower bud *** levels were the highest in the flower buds;exogenous GA3+4 increased plant height by approximately 90%,increased flower quantity by nearly 40%,and advanced flowering by 4 *** GA biosynthesis using paclobutrazol decreased plant height and flower quantity by 38%and 87.1%,respectively,and delayed flowering by 15.6 *** signaling has positive regulatory effects on vegetative growth and flower *** ETH concentration in the developing leaf buds was at least 50%higher than that in other *** spraying led to remarkable increases in plant height and leaf thickness and extended the flowering *** signaling acts as a growth promoter during vegetative and reproductive development in *** highest BR levels were detected in the vegetative shoot *** application of28-epihomobrassinolide resulted in growth-promoting phenotypes including longer scapes,thicker leaves,and prolonged flowering.

关键词： Nelumbo nucifera Gibberellin Brassinolide Ethylene Flowering

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